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Research in Astronomy and Astrophysics 2024年第8期24卷 42-51页

作者： Jin-Hui Rao Shu-Xu Yi Lian Tao Qing-Wen Tang Department of Physics School of Physics and Materials ScienceNanchang UniversityNanchang 330031China institute of high Energy Physics Chinese Academy of SciencesBeijing 100049China

Theories of modified gravity suggest that the propagation speed of gravitational waves(GW)v_gmay deviate from the speed of light c.A constraint can be placed on the difference between c and v_gwith a simple method that uses the arrival time delay between GW and electromagnetic wave simultaneously emitted from a burst *** simulated the joint observation of GW and short gamma-ray burst signals from binary neutron star merger events in different observation campaigns,involving advanced LIGO(aLIGO)in design sensitivity and Einstein Telescope(ET)joint-detected with Fermi/*** a result,the relative precision of constraint on v_gcan reach~10~(-17)(aLIGO)and~10^(-18)(ET),which are one and two orders of magnitude better than that from GW170817,*** continue to obtain the bound of graviton mass m_g≤7.1(3.2)×10~(-20)eV with aLIGO(ET).Applying the Standard-Model Extension test framework,the constraint on v_gallows us to study the Lorentz violation in the nondispersive,nonbirefringent limit of the gravitational *** obtain the constraints of the dimensionless isotropic coefficients S_(00)^(4)at mass dimension d=4,which are-1×10^(-15)

关键词： gravitational waves-(stars)gamma-ray burst general-stars neutron

The chance of sodium titanate anode for the practical sodium-ion batteries

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Chinese Journal of Chemical Engineering 2024年第8期72卷 226-244页

作者： Feng Chen Haoyu Li Xianyan Qiao Ruoyang Wang Changyan Hu Ting Chen Yifan Niu Benhe Zhong Zhenguo Wu Xiaodong Guo School of Chemical Engineering Sichuan UniversityChengdu 610065China institute for Advanced Study Chengdu UniversityChengdu 610106China Chengdu No.7 high School Chengdu 6100412China

Supporting sustainable green energy systems,there is a big demand gap for grid energy *** storage,especially sodium-ion batteries(SIBs),have advanced significantly and are now emerging as a feasible alternative to the lithium-ion batteries equivalent in large-scale energy storage due to their natural abundance and prospective inexpensive *** various anode materials of SIBs,beneficial properties,such as outstanding stability,great abundance,and environmental friendliness,make sodium titanates(NTOs),one of the most promising anode materials for the rechargeable ***,there are still enormous challenges in application of NTO,owing to its low intrinsic electronic conductivity and collapse of *** research on NTOs is still in its infancy;there are few conclusive reviews about the specific function of various modification ***,we summarize the typical strategies of optimization and analysis the fine structures and fabrication methods of NTO anodes combined with the application of in situ characterization *** work provides effective guidance for promoting the continuous development,equipping NTOs in safety-critical systems,and lays a foundation for the development of NTO-anode materials in SIBs.

关键词： Sodium titanates Sodium-ion batteries Modification methods Electronic materials Electrochemistry Synthesis

Reversible aqueous aluminum metal batteries enabled by a water-in-salt electrolyte

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Green Energy & Environment 2024年第7期9卷 1183-1191页

作者： Wenjing Tang Lijun Deng Longyuan Guo Shoubin Zhou Qinhai Jiang Jiayan Luo Shanghai Key Lab of Advanced high-Temperature Materials and Precision Forming State School of Materials Science and Engineering Shanghai Jiao Tong University School of Science Harbin Institute of Technology Key Laboratory for Green Chemical Technology of Ministry of Education School of Chemical Engineering and Technology Tianjin University HuaFu high Technology Energy Storage CO. LTD Shanghai Jiao Tong University Shaoxing Research institute of Renewable Energy and Molecular Engineering

Aluminum（Al）, the most abundant metallic element on the earth crust, has been reckoned as a promising battery material for its the highest theoretical volume capacity(8046 mAh cm-3). Being rechargeable in ionic liquid electrolytes, however, the Al anode and battery case suffer from corrosion. On the other hand, Al is irreversible in aqueous electrolyte with severe hydrogen evolution reaction. Here, we demonstrate a water-in-salt aluminum ion electrolyte（WISE） based on Al and lithium salts to tackle the above challenges. In the WISE system, water molecules can be confined within the Li+solvation structures. This diminished Al3+-H2O interaction essentially eliminates the hydrolysis effect, effectively protecting Al anode from corrosion. Therefore, long-term Al plating/stripping can be realized. Furthermore, two types of high-performance full batteries have been demonstrated using copper hexacyanoferrate（CuHCF, a Prussian Blue Analogues） and LiNi0.8Co0.1Mn0.1O2（NCM） as cathodes. The reversibility of Al anode laid the foundation for low cost rechargeable batteries suffering for large-scale energy *** context: Al batteries are expected to become a safe and sustainable alternative to lithium batteries. For decades, chase for a feasible Al secondary battery has not been successful. The key challenge is to find suitable cathode and electrolyte materials, together with which Al anode battery can function reversibly. Currently, fatal drawbacks have impeded the practical application of Al metal batteries（AMBs）, such as sustained corrosion of Al anode and battery case in ionic liquid electrolytes, irreversibility issues as well as severe hydrogen evolution reaction during cycling in aqueous electrolyte. Therefore, electrolyte and their electrochemical kinetics play a vital role in the performance and environmental operating limitations of high-energy Al metal batteries. In this work, we demonstrate a nearly neutral Al ion water-in-salt electrolyte（WISE） to tackle th

关键词： Water-in-salt electrolyte Rechargeable aluminum anode Solvation sheath Hybrid battery Abundance

Enhanced quality of Al2O3/SiC gate stack via microwave plasma annealing

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Rare Metals 2024年第10期43卷 5362-5371页

作者： Nan-Nan You Xin-Yu Liu Qian Zhang Zhen Wang Jia-Yi Wang Yang Xu Xiu-Yan Li Yu-Zheng Guo Sheng-Kai Wang high-Frequency high-Voltage Device and Integrated Circuits R&D Center Institute of Microelectronics of the Chinese Academy of Sciences School of Integrated Circuits University of Chinese Academy of Sciences School of Electrical Engineering and Automation Wuhan University Department of Micro/Nano Electronics School of Electronic Information and Electrical EngineeringShanghai Jiao Tong University

The high-quality gate dielectric on silicon carbide （SiC） surface is critical to fabricate high-performance SiC metal-oxide-semiconductor field-effect transistors（MOSFETs）.This research employs microwave plasma annealing （MPA） to obtain high-quality Al2O3/SiC gate *** designing MPA atmosphere and optimizing the plasma power,the SiC MOS capacitor with a Al2O3dielectric film shows the enhanced *** interface state density is reduced by 1 order of magnitude to 6×1011cm-2·eV-1,the breakdown electric field is increased,and the voltage shift is effectively suppressed Besides,the mechanism of MPA process is discussed in terms of the thermal effect and reactant species.X-ray photoelectron spectroscopy （XPS） results unveil oxygen plasma plays the main *** plasma power during the MPA process results in defect repairs of the firstneighbor Al-O bonding and partial removal of Al-O-H bond from the interface *** study demonstrates that MPA process is an effective option to realize highquality dielectric and interface on SiC.

关键词： Al2O3 Defect repairs Metal–oxide–semiconductor Microwave plasma annealing Silicon carbide X-ray photoelectron spectroscopy

Review of 2D Bi_(2)X_(3)(X=S,Se,Te):from preparation to photodetector

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Rare Metals 2024年第6期43卷 2349-2370页

作者： Zhi Zeng Dong-Bo Wang Xuan Fang Jia-Mu Cao Bing-Ke Zhang Jing-Wen Pan Dong-Hao Liu Si-Hang Liu Shu-Jie Jiao Tian-Yuan Chen Gang Liu Lian-Cheng Zhao Jin-Zhong Wang Department of Optoelectronic Information Science School of Materials Science and EngineeringHarbin Institute of TechnologyHarbin 150001China Changchun University Science and Technology School of PhysicsThe State Key Laboratory of High Power Semiconductor LasersChangchun 130022China School of Astronautics Harbin Institute of TechnologyHarbin 150001China Center for high Pressure Science and Technology Advanced Research Shanghai 201203China

Detector has become an indispensable part of human *** increasing demand for photodetectors with high performance has promoted the research of novel *** the same time,with the development of rising material system,two-dimensional(2D)materials attract a lot of attention,while the suitable option for fabricating photodetector is still *** prospering of bismuth chalcogenides injected new vitality for material field,thereinto,the unique topological insulator characteristics make the research on bismuth selenide(Bi_(2)X_(3))and bismuth telluride(Bi_(2)X_(3)) intriguing.2D Bi_(2)X_(3) also exhibits unique features among various 2D materials,of which,the adjustable narrow energy band gap and polarization-sensitive photocurrent contribute to the promising application of high performance and broadband *** this review,from a bottom-up perspective,we summarize fundamental properties,synthesis method,photodetector performance of 2D Bi_(2)X_(3) based on the previous study,which provide an overall perspective of 2D Bi_(2)X_(3).Wherein,the section of the photodetector is specifically discu ssed with regard to pure Bi_(2)X_(3) photodetector and heterojunction photodetector.A brief summary and outlook were also explored in the end.

关键词： Bi_(2)X_(3) Preparation 2D Photodetector

Two-dimensional precise figuring of 500 mm-long X-ray mirror using one-dimensional ion beam system

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Advances in Manufacturing 2024年第1期12卷 177-184页

作者： Qiu-Shi Huang Han-Dan Huang Qiao-Yu Wu Jun Yu Zhong Zhang Zhan-Shan Wang MOE Key Laboratory of Advanced Micro-Structured Materials Institute of Precision Optical Engineering(IPOE)School of Physics Science and EngineeringTongji UniversityShanghai200092People’s Republic of China Shanghai Professional Technical Service Platform for Full-Spectrum and high-performance Optical Thin Film Devices and Applications Tongji UniversityShanghai200092People’s Republic of China Shanghai Frontiers Science Center of Digital Optics Tongji UniversityShanghai200092People’s Republic of China

In this study,a new method was developed to realize two-dimensional(2D)figure correction of grazing-incidence X-ray mirrors using a one-dimensional(1D)ion-beam figuring system.A mask of holes was specifically designed to generate removal functions at different widths and extend the figuring capability over a wide ***,a long mirror could be *** this method,the surface height root-mean-square(RMS)error of the center area of 484 mm×16 mm was reduced from 11.49 nm to 2.01 nm,and the 1D meridional RMS error reached 1.0 *** proposed method exhibits high precision and cost effectiveness for production of long X-ray mirrors.

关键词： Long-size mirrors Ion beam figuring Two-dimensional figure correction Mask

Unlocking efficient energy storage via regulating ion and electron-active subunits:an(SbS)_(1.15)TiS_(2)superlattice for large and fast Na^(+)storage

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Science China Chemistry 2024年第1期67卷 336-342页

作者： Baixin Peng Tianxun Cai Shaoning Zhang Yuqiang Fang Zhuoran Lv Yusha Gao Fuqiang Huang State Key Laboratory of high performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China School of Physical Science and Technology ShanghaiTech UniversityShanghai 200031China Beijing National Laboratory for Molecular Sciences State Key Laboratory of Rare Earth Materials Chemistry and ApplicationsCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China

Alloying-type metal sulfides with high sodiation activity and theoretical capacity are promising anode materials for high energy density sodium ion ***,the large volume change and the migratory and aggregation behavior of metal atoms will cause severe capacity decay during the charge/discharge ***,a robust and conductive TiS_(2)framework is integrated with a high-capacity SbS layer to construct a single phase(SbS)_(1.15)TiS_(2)superlattice for both high-capacity and fast Na^(+)*** metallic TiS_(2)sublayer with high electron activity acts as a robust and conductive skeleton to buffer the volume expansion caused by conversion and alloying reaction between Na+and SbS ***,high capacity and high rate capability can be synergistically realized in a single phase(SbS)_(1.15)TiS_(2)*** novel(SbS)_(1.15)TiS_(2)anode has a high charge capacity of 618 mAh g^(-1)at 0.2 C and superior rate performance and cycling stability(205 mAh g^(-1)at 35 C after 2,000 cycles).Furthermore,in situ and ex situ characterizations are applied to get an insight into the multi-step reaction *** integrity of robust Na-Ti-S skeleton during(dis)charge process can be *** superlattice construction idea to integrate the Na^(+)-active unit and electron-active unit would provide a new avenue for exploring high-performance anode materials for advanced sodium-ion batteries.

关键词： (SbS)_(1.15)TiS_(2) sulfides sodium ion battery superlattice fast-charging

Recess-free enhancement-mode AlGaN/GaN RF HEMTs on Si substrate

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Journal of Semiconductors 2024年第6期45卷 81-86页

作者： Tiantian Luan Sen Huang Guanjun Jing Jie Fan Haibo Yin Xinguo Gao Sheng Zhang Ke Wei Yankui Li Qimeng Jiang Xinhua Wang Bin Hou Ling Yang Xiaohua Ma Xinyu Liu high-Frequency high-Voltage Device and Integrated Circuits R&D Center Institute of Microelectronics of Chinese Academy of SciencesBe i-jing 100029China School of integrated Circuits University of Chinese Academy of SciencesBeijing 100049China Faculty of integrated Circuits Xidian UniversityXi’an 710071China

Enhancement-mode(E-mode)GaN-on-Si radio-frequency(RF)high-electron-mobility transistors(HEMTs)were fabri-cated on an ultrathin-barrier(UTB)AlGaN(<6 nm)/GaN heterostructure featuring a naturally depleted 2-D electron g... 详细信息

Enhancement-mode(E-mode)GaN-on-Si radio-frequency(RF)high-electron-mobility transistors(HEMTs)were fabri-cated on an ultrathin-barrier(UTB)AlGaN(high threshold voltage(VTH)of+1.1 V with good uniformity.A maxi-mum current/power gain cut-off frequency(fT/fMAX)of 31.3/99.6 GHz with a power added efficiency(PAE)of 52.47%and an out-put power density(Pout)of 1.0 W/mm at 3.5 GHz were achieved on the fabricated E-mode HEMTs with 1-μm gate and Au-free ohmic contact.

关键词： AlGaN/GaN heterostructure ultrathin-barrier enhancement-mode radio-frequency power added efficiency silicon substrate

不同应力水平对2195-T34 Al-Li合金时效行为的影响机制研究

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Journal of Central South University 2024年第1期31卷 11-24页

作者：陈非湛利华徐永谦刘春辉马博林曾泉清胡正根朱文俐鄢东洋 Light Alloy Research institute of Central South University Changsha 410083China School of Mechanical and Electrical Engineering Central South UniversityChangsha 410083China State Key Laboratory of high-performance Complex Manufacturing Central South UniversityChangsha 410083China Beijing institute of Astronautical Systems Engineering Beijing 100176China

研究了不同应力水平下2195-T34 Al-Li合金的时效特性变化。当应力低于材料的高温屈服强度(YS)时,低应力时效(LSA)和无应力时效(SFA)试样的屈服强度和延伸率(EL)相近。当应力超过材料的高温屈服强度时,试样的极限拉伸强度(UTS)和伸长率... 详细信息

研究了不同应力水平下2195-T34 Al-Li合金的时效特性变化。当应力低于材料的高温屈服强度(YS)时,低应力时效(LSA)和无应力时效(SFA)试样的屈服强度和延伸率(EL)相近。当应力超过材料的高温屈服强度时,试样的极限拉伸强度(UTS)和伸长率显著下降,表明应力的增加降低了材料的抗破坏性。透射电子显微镜(TEM)和扫描电子显微镜(SEM)的观察结果表明:应力对材料时效性能的影响归因于内部析出物特征和晶界富铜析出物的共同作用。应力的增加促使铜原子在晶界发生偏析形成富铜析出物,同时促进了晶界无沉淀区(PFZ)的形成,而富铜析出物是脆性相,可作为损伤的起始位置,容易导致裂纹萌生和发展,降低材料的延展性。

关键词：铝锂合金应力水平时效力学性能

Optimizing high-coordination shell of Co-based single-atom catalysts for efficient ORR and zinc-air batteries

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Journal of Energy Chemistry 2024年第8期95卷 306-314,I0007页

作者： Yugang Qi Qing Liang Kexin Song Xinyan Zhou Meiqi Liu Wenwen Li Fuxi Liu Zhou Jiang Xu Zou Zhongjun Chen Wei Zhang Weitao Zheng Key Laboratory of Automobile Materials MOE School of Materials Science&Engineering Electron Microscopy Centerand International Center of Future ScienceJilin Provincial International Cooperation Key Laboratory of High-Efficiency Clean Energy MaterialsJilin UniversityChangchun 130012JilinChina institute of high Energy Physics Chinese Academy of SciencesBeijing 100049China

Atom-level modulation of the coordination environment for single-atom catalysts(SACs)is considered as an effective strategy for elevating the catalytic *** the MNxsite,breaking the symmetrical geometry and charge distribution by introducing relatively weak electronegative atoms into the first/second shell is an efficient way,but it remains challenging for elucidating the underlying mechanism of ***,a practical strategy was reported to rationally design single cobalt atoms coordinated with both phosphorus and nitrogen atoms in a hierarchically porous carbon derived from metal-organic frameworks.X-ray absorption spectrum reveals that atomically dispersed Co sites are coordinated with four N atoms in the first shell and varying numbers of P atoms in the second shell(denoted as Co-N/P-C).The prepared catalyst exhibits excellent oxygen reduction reaction(ORR)activity as well as zinc-air battery *** introduction of P atoms in the Co-SACs weakens the interaction between Co and N,significantly promoting the adsorption process of ^(*)OOH,resulting in the acceleration of reaction kinetics and reduction of thermodynamic barrier,responsible for the increased intrinsic *** discovery provides insights into an ultimate design of single-atom catalysts with adjustable electrocatalytic activities for efficient electrochemical energy conversion.

关键词： Electrocatalytic Oxygen reduction reaction Single atom catalyst Shell coordination optimization