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Stress corrosion cracking failure of X80 carbon steel U-b end cause d by Desulfovibrio vulgaris biocorrosion

Journal of Materials Science & technology 2024年第7期174卷 95-105页

作者： Zhong Li Jike Yang Shihang Lu Wenwen Dou Tingyue Gu corrosion&Protection Center University of Science&Technology BeijingBeijing 100083China institute of Marine Science and technology Shandong UniversityQingdao 266237China Department of Chemical and Biomolecular Engineering Institute for Corrosion and Multiphase TechnologyOhio UniversityAthensOH 45701USA

Sulfate reducing bacteria(SRB)are widely present in oil and gas industry,causing pitting corrosion on pipeline *** corrosion cracking(SCC)often occurs in the presence of mechanical stress before pit-ting perforation failure,leading to economic losses and even catastrophic *** this study,stress distribution simulation using the finite element method(FEM),corrosion analysis techniques and elec-trochemical corrosion measurements were employed to investigate the SCC mechanism of X80 pipeline steel caused by Desulfovibrio vulgaris,which is a common SRB strain used in microbiologically influenced corrosion(MIC)*** was found that *** MIC caused sharp microcracks on an X80 U-bend coupon after only 2 weeks of immersion at 37℃in the deoxygenated ATCC 1249 culture medium inocu-lated with *** X80 U-bend coupon’s weight loss-based uniform corrosion rate for the 12 cm^(2)surface was 60%of that for the unstressed flat square coupon(2.3 mg cm^(−2)vs.3.8 mg cm^(−2)).This was likely because the square coupon had wide MIC pits,providing a larger effective surface area for more sessile cells(4.2×10^(8)cells cm^(−2)on square coupon vs.2.4×10^(8)cells cm^(−2)on U-bend coupon)to attach and harvest more *** SCC failure occurred on an X80 U-bend pre-cracked at the outer bottom after a 6-week immersion in the *** *** from MIC damage,this could also be because *** metabolism increased the availability hydrogen atoms on the steel surface,and promoted the diffusion of hydrogen atoms into the metal lattice,thus increasing the brittleness of the steel.

关键词： Stress corrosion cracking Microbiologically influenced corrosion Sulfate reducing bacteria X80 U-bend steel Tensile stress

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“corrosion-resistant”chromium steels for oil and gas pipelines can suffer from very severe pitting corrosion by a sulfate-reducing bacterium

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Journal of Materials Science & technology 2024年第7期174卷 23-29页

作者： Lingjun Xu Pruch Kijkla Sith Kumseranee Suchada Punpruk Tingyue Gu Department of Chemical&Biomolecular Engineering Institute for Corrosion and Multiphase TechnologyOhio UniversityAthens 45701USA PTT Exploration and Production Bangkok 10900Thailand

*** CO_(2)corrosion of pipelines is one of the major threats in the oil and gas industry[1].Chromium steels(CrSs)and more expen-sive stainless steels(SSs)can mitigate CO_(2)corrosion[2,3].A higher content of Cr results in greater uniform corrosion resistance to CO_(2),which is generally attributed to the enrichment of Cr in the corro-sion product film[4,5].The film,which mainly consists of FeCO_(3),Fe(OH)_(3),Cr(OH)_(3),and Cr_(2)O_(3),forms a passive layer on the metal surface,and the enrichment of Cr in this layer helps block corro-sive anions from contacting with the steel surface[6-8].

关键词： corrosion pitting steel

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Effect of exogenous flavins on the microbial corrosion by Geobacter sulfurreducens via iron-to-microbe electron transfer

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Journal of Materials Science & technology 2024年第4期171卷 129-138页

作者： Yuting Jin Jiaqi Li Mingxing Zhang Borui Zheng Dake Xu Tingyue Gu Fuhui Wang Shenyang National Laboratory for Materials Science Northeastern UniversityShenyang 110819China Key Laboratory for Anisotropy and Texture of Materials(Ministry of Education) Northeastern UniversityShenyang 110819China Department of Chemical and Biomolecular Engineering Institute for Corrosion and Multiphase TechnologyOhio UniversityAthens OH 45701USA

Microbes can cause or accelerate metal corrosion,leading to huge losses in corrosion damages each *** sulfurreducens is a representative electroactive bacterium in many soils,sediments,and wastew-ater *** has been confirmed to directly extract electrons from elemental ***,little is known about the effect of electron shuttles in *** corrosion on stainless *** this study,we report that exogenous flavins promote iron-to-microbe electron transfer,accelerating micro-bial *** caused 1.3 times deeper pits and increased electron uptake(with 2 times increase of i_(corr))from stainless steel when riboflavin was added to the culture ***-deficient mutant data suggest that *** utilizes riboflavin as a bound-cofactor in outer membrane c-type *** finding that,in the presence of microbes,riboflavin can substantially accelerate corrosion highlights the role of flavin redox cycling for enhanced iron-to-microbe electron transfer by *** and provides new insights in microbial corrosion.

关键词： Extracellular electron transfer Microbiological corrosion Geobacter sulfurreducens Outer membrane c-type cytochromes Exogenous flavins

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Electrically conductive nanowires controlled one pivotal route in energy harvest and microbial corrosion via direct metal-microbe electron transfer

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Journal of Materials Science & technology 2024年第7期174卷 226-233页

作者： Yuting Jin Jiaqi Li Toshiyuki Ueki Borui Zheng Yongqiang Fan Chuntian Yang Zhong Li Di Wang Dake Xu Tingyue Gu Fuhui Wang Shenyang National Laboratory for Materials Science Northeastern UniversityShenyang 110819China Key Laboratory for Anisotropy and Texture of Materials(Ministry of Education) Northeastern UniversityShenyang 110819China Department of Chemical and Biomolecular Engineering Institute for Corrosion and Multiphase TechnologyOhio UniversityAthensOH 45701USA

Extracellular electron transfer(EET)plays a critical role in bioelectrochemical processes,allowing cou-pling between microorganisms and extracellular solid-state electrodes,metals,or other cells in energy *** studies have suggested a role for outer-surface c-type cytochromes in direct metal-to-microbe electron transfer by Geobacter sulfurreducens,a model electroactive ***,we ex-amined the possibility of other microbially produced electrical contacts by deleting the gene for PilA,the protein monomer that *** assembles into electrically conductive protein nanowires(e-pili).Deleting pilA gene inhibited electron extraction from pure iron and 316L stainless steel up to 31%and 81%,respectively more than deleting the gene for the outer-surface cytochrome *** PilA-deficient phenotype,and the observation that relatively thick biofilms(21.7μm)grew on the metal surfaces at multi-cell distances from the metal surfaces suggest that e-pili contributed significantly to microbial cor-rosion via direct metal-to-microbe electron *** results have implications for the fundamental understanding of electron harvest via e-pili by electroactive microbes,their uses in bioenergy production,as well as in monitoring and mitigation of metal biocorrosion.

关键词： Electrically conductive protein nanowires Direct metal-to-microbe electron transfer Geobacter sulfurreducens Outer-surface c-type cytochromes Biofilm

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Carbon steel anticorrosion performance and mechanism of sodium lignosulfonate

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Rare Metals 2024年第1期43卷 356-365页

作者： Bo-Kai Liao Rui-Xuan Quan Ping-Xian Feng Huan Wang Wei Wang Li Niu School of Chemistry and Chemical Engineering Guangzhou Key Laboratory of Sensing Materials and DevicesJoint Institute of Guangzhou University and Institute of Corrosion Science and TechnologyGuangzhou UniversityGuangzhou 510006China

Lignin is a typical biological macromolecule with a three-dimensional network structure and abundant functional groups. It has excellent ionic complexation ability and amphiphilic molecular structure *** this study, the carbon steel anticorrosion performance of sodium lignosulfonate(SLS) in an acid solution was evaluated using the weight loss method, electrochemical measurements, scanning vibration electrode technique(SVET), and surface characterization methods. SLS exhibited excellent corrosion inhibition efficiency for Q235carbon steel in 1 mol·L^(-1) HCl, reaching a maximum value of 98%. A low SLS concentration of 20 mg·L^(-1) resulted in the maximum corrosion inhibition efficiency, which remained nearly constant at higher SLS *** SVET test demonstrated that the formation of an SLS adsorption film can impede corrosion. This study confirms the significance of the application of green biomass resources in the field of metal corrosion protection and green functional materials.

关键词： Lignin Sodium lignosulfonate corrosion inhibitor Carbon Steel

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Heat Transfer Characteristics of a Microchannel Heat Sink with Highly-Dense Micro-Jet Arrays

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Journal of Thermal Science 2024年第3期33卷 1148-1160页

作者： ZHANG Yu CHEN Xiaoyan MIAO Lin CHEN Liang HOU Yu State Key Laboratory of multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an710049China Beijing Aerospace technology institute Beijing100083China

This paper proposed a new structure of highly-dense micro-jet arrays for hybrid jet-impingement/microchannel heat sinks(~120 jet per cm^(2) with jet width of 0.35 mm).Parametric study is performed to investigate the influence of structure and flow parameters on the convective heat transfer of water jet cooling in confined *** simulation results show that the optimal jet width,jet spacing and impingement distance are around 0.2 mm,0.2 mm and 0.3 mm,respectively,which can achieve a low thermal resistance as well as a relatively low pressure *** analysis of the heat transfer pathways shows that the micro-fin jet structures can extend the impinging heat transfer area and conduct a considerable proportion of heat,which can reach up to 38.9%with the Reynolds number ranging from 797.1 to *** heat transfer characteristics in the heat sink will shift from impingement dominated heat transfer to the channel-convection dominated heat transfer as the jet impingement distance increases.A correlation is proposed to predict the average Nusselt number on the stagnation area for the heat sink with different structure parameters,and the deviations of predictions from the numerical results are less than 10%.

关键词： hybrid heat sink impingement microchannel thermal management high heat flux

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Effect of bipolar-plates design on corrosion,mass and heat transfer in proton-exchange membrane fuel cells and water electrolyzers:A review

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International Journal of Minerals,Metallurgy and Materials 2024年第7期31卷 1599-1616页

作者： Jiuhong Zhang Xiejing Luo Yingyu Ding Luqi Chang Chaofang Dong Key Laboratory for corrosion and Protection(MOE) Institute for Advanced Materials and TechnologyUniversity of Science and Technology BeijingBeijing 100083China Beijing Advanced Innovation Center for Materials Genome Engineering Beijing 100083China

Attaining a decarbonized and sustainable energy system,which is the core solution to global energy issues,is accessible through the development of hydrogen ***-exchange membrane water electrolyzers(PEMWEs)are promising devices for hydrogen production,given their high efficiency,rapid responsiveness,and *** plates account for a relatively high percentage of the total cost and weight compared with other components of ***,optimization of their design may accelerate the promotion of *** paper reviews the advances in materials and flow-field design for bipolar ***,the working conditions of proton-exchange membrane fuel cells(PEMFCs)and PEMWEs are compared,including reaction direction,operating temperature,pressure,input/output,and ***,the current research status of bipolar-plate substrates and surface coatings is summarized,and some typical channel-rib flow fields and porous flow fields are ***,the effects of materials on mass and heat transfer and the possibility of reducing corrosion by improving the flow field structure are ***,this review discusses the potential directions of the development of bipolar-plate design,including material fabrication,flow-field geometry optimization using threedimensional printing,and surface-coating composition optimization based on computational materials science.

关键词： bipolar-plates flow design mass and heat transfer corrosion water electrolyzers fuel cells

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Developing an atmospheric aging evaluation model of acrylic coatings:A semi-supervised machine learning algorithm

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International Journal of Minerals,Metallurgy and Materials 2024年第7期31卷 1617-1627页

作者： Yiran Li Zhongheng Fu Xiangyang Yu Zhihui Jin Haiyan Gong Lingwei Ma Xiaogang Li Dawei Zhang Beijing Advanced Innovation Center for Materials Genome Engineering Institute for Advanced Materials and TechnologyUniversity of Science and Technology BeijingBeijing 100083China National Materials corrosion and Protection Data Center University of Science and Technology BeijingBeijing 100083China BRI Southeast Asia Network for corrosion and Protection(MOE) Shunde Innovation School of University of Science and Technology BeijingFoshan 528399China

To study the atmospheric aging of acrylic coatings,a two-year aging exposure experiment was conducted in 13 representative climatic environments in *** atmospheric aging evaluation model of acrylic coatings was developed based on aging data including11 environmental factors from 567 cities.A hybrid method of random forest and Spearman correlation analysis was used to reduce the redundancy and multicollinearity of the data set by dimensionality reduction.A semi-supervised collaborative trained regression model was developed with the environmental factors as input and the low-frequency impedance modulus values of the electrochemical impedance spectra of acrylic coatings in 3.5wt%NaCl solution as *** model improves accuracy compared to supervised learning algorithms model(support vector machines model).The model provides a new method for the rapid evaluation of the aging performance of acrylic coatings,and may also serve as a reference to evaluate the aging performance of other organic coatings.

关键词： acrylic coatings coatings aging atmospheric environment machine learning

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Stress-assisted corrosion mechanism of 3Ni steel by using gradient boosting decision tree machining learning method

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International Journal of Minerals,Metallurgy and Materials 2024年第6期31卷 1311-1321页

作者： Xiaojia Yang Jinghuan Jia Qing Li Renzheng Zhu Jike Yang Zhiyong Liu Xuequn Cheng Xiaogang Li institute of Advanced Materials and technology University of Science and Technology BeijingBeijing 100083China AECC Key Laboratory of Advanced corrosion and Protection of Aeronautical Materials AECC Beijing Institute of Aeronautical MaterialsBeijing 100095China Shunde Innovation School University of Science and Technology BeijingFoshan 528399China

Traditional 3Ni weathering steel cannot completely meet the requirements for offshore engineering development,resulting in the design of novel 3Ni steel with the addition of microalloy elements such as Mn or Nb for strength enhancement becoming a *** stress-assisted corrosion behavior of a novel designed high-strength 3Ni steel was investigated in the current study using the corrosion big data *** information on the corrosion process was recorded using the galvanic corrosion current monitoring *** gradi-ent boosting decision tree(GBDT)machine learning method was used to mine the corrosion mechanism,and the importance of the struc-ture factor was *** exposure tests were conducted to verify the calculated results using the GBDT *** indic-ated that the GBDT method can be effectively used to study the influence of structural factors on the corrosion process of 3Ni ***-ferent mechanisms for the addition of Mn and Cu to the stress-assisted corrosion of 3Ni steel suggested that Mn and Cu have no obvious effect on the corrosion rate of non-stressed 3Ni steel during the early stage of *** the corrosion reached a stable state,the in-crease in Mn element content increased the corrosion rate of 3Ni steel,while Cu reduced this *** the presence of stress,the increase in Mn element content and Cu addition can inhibit the corrosion *** corrosion law of outdoor-exposed 3Ni steel is consistent with the law based on corrosion big data technology,verifying the reliability of the big data evaluation method and data prediction model selection.

关键词： weathering steel stress-assisted corrosion gradient boosting decision tree machining learning

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Influence of Micro/Nano-Ti Particles on the corrosion Behavior of AZ31-Ti Composites

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Acta Metallurgica Sinica(English Letters) 2024年第3期37卷 484-498页

作者： Jinchao Jiao Jin Zhang Yong Lian Shengli Han Kaihong Zheng Fusheng Pan institute for Advanced Materials and technology University of Science and Technology BeijingBeijing 10083China Beijing Key Laboratory for corrosion Erosion and Surface technology Beijing 100083China institute of New Materials Guangdong Academy of SciencesGuangzhou 510650China National Engineering Research Center for Magnesium Alloys Chongqing UniversityChongqing 404100China

Adding Ti particles to magnesium alloy simultaneously enhances its strength and ***,how these particles influence on Mg alloy’s corrosion performance is seldom *** corrosion behavior of AZ31-Ti composites containing titanium nanoparticles(1.5 and 5 wt%)and micron particles(10 wt%)prepared by powder metallurgical in 3.5 wt%NaCl solution was *** results indicate that Ti particles serve as the primary location for the cathodic hydrogen reduction reaction,resulting in intense galvanic corrosion between the Ti and Mg *** nanoparticles distributed at the interface of the original AZ31 powder were in a discontinuous mesh structure,thus failing to act as a barrier against *** corrosion products with the existence of numerous cracks gradually peel off during the corrosion process and cannot protect the *** average corrosion rate P_(w) of AZ31,AZ31-1.5%Ti,AZ31-5%Ti,and AZ31-10%Ti after 7 days of immersion is 27.55,105.65,283.67,and 99.35 mm/y,***,AZ31-Ti composites can be considered as potential candidates for degradable fracturing ***,it is recommended to improve their corrosion resistance through surface treatment.

关键词： AZ31-Ti composite Nano-Ti Micro-Ti corrosion behavior Scanning Kelvin probe force microscopy(SKPFM)

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