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Measurement of yields and angular distributions ofγ-quanta from the interaction of 14.1 MeV neutrons with oxygen,phosphorus,and sulfur

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Chinese Physics C 2024年第3期48卷 79-92页

作者： D.N.Grozdanov N.A.Fedorov S.B.Dabylova Yu.N.Kopatch I.N.Ruskov V.R.Skoy T.Yu.Tretyakova C.Hramco P.I.Kharlamov G.V.Pampushik P.G.Filonchik A.V.Andreev Joint Institute for nuclear Research(JINR) DubnaRussia Institute for nuclear Research and nuclear energy Bulgarian Academy of SciencesSofiaBulgaria Faculty of Physics Lomonosov Moscow State UniversityMoscowRussia L.N.Gumilyov Eurasian National University AstanaKazakhstan Skobeltsyn Institute of nuclear Physics Moscow State UniversityMoscowRussia Institute of Chemistry of Moldova ChisinauRepublic of Moldova Moscow Institute of Physics and technology MoscowRussia

A study of the inelastic scattering of neutrons with an energy of 14.1 MeV on the nuclei of oxygen,phosphorus,and sulfur was performed at the TANGRA facility at JINR(Dubna).The experiment aimed to refine existing data and obtain new data on the yields and angular distributions ofγ-quanta emitted by the studied nuclei due to neutron-induced nuclear reactions using the tagged neutron *** types of detector systems were used to registerγ-***γ-ray yields were measured using a high-purity germanium(HPGe)*** angular distributions ofγ-rays were obtained using a system of 18 scintillation detectors based on bismuth germanite Bi_(4)Ge_(3)O_(12)(BGO)located around the *** performed experiments measured the yields of two transitions for the reaction of tagged neutrons with 16O,nine transitions for the reaction with ^(31)P,and nine transitions for the reaction with ^(32)S for the first *** angular anisotropy of theγ-radiation accompanying the inelastic scattering of neutrons with an energy of 14.1 MeV on ^(31)P nuclei was also measured for the first time.

关键词： tagged neutron method yields of gamma-quanta high-resolution gamma-spectrometry neutron-nuclear reactions neutron scattering

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Systematic study of cluster radioactivity in trans-lead nuclei with various versions of proximity potential formalisms

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Chinese Physics C 2024年第5期48卷 209-225页

作者：刘潇蒋杰栋吴喜军李小华 School of nuclear Science and technology University of South ChinaHengyang 421001China School of Math and Physics University of South ChinaHengyang 421001China National Exemplary Base for International Sci&Tech.Collaboration of nuclear energy and nuclear Safety University of South ChinaHengyang 421001China Cooperative Innovation Center for nuclear Fuel Cycle technology&Equipment University of South ChinaHengyang 421001China Key Laboratory of Low Dimensional Quantum Structures and Quantum Control Hunan Normal UniversityChangsha 410081China

In this study,based on the framework of the Coulomb and proximity potential model(CPPM),we systematically investigate the cluster radioactivity half-lives of 26 trans-lead nuclei by considering the cluster preformation probability,which possesses a simple mass dependence on the emitted cluster according to *** and ***[***.61,1930(1988)].Moreover,we investigate 28 different versions of the proximity potential formalisms,which are the most complete known proximity potential formalisms proposed to describe proton radioactivity,two-proton radioactivity,αdecay,heavy-ion radioactivity,quasi-elastic scattering,fusion reactions,and other *** calculated results show that the modified forms of proximity potential 1977,denoted as Prox.77-12,and proximity potential 1981,denoted as Prox.81,are the most appropriate proximity potential formalisms for the study of cluster radioactivity,as the root-mean-square deviation between experimental data and relevant theoretical results obtained is the least;both values are *** comparison,the universal decay law(UDL)proposed by Qi et al.[***.C 80,044326(2009)],unified formula of half-lives forαdecay and cluster radioactivity proposed by Ni et al.[***.C 78,044310(2008)],and scaling law(SL)in cluster radioactivity proposed by Horoi et al.[***.G 30,945(2004)]are also *** addition,utilizing CPPM with Prox.77-12,Prox.77-1,Prox.77-2,and Prox.81,we predict the half-lives of 51 potential cluster radioactive candidates whose cluster radioactivity is energetically allowed or observed but not yet quantified in *** predicted results are in the same order of magnitude as those obtained using the compared semi-empirical and/or empirical *** the same time,the competition betweenαdecay and cluster radioactivity of these predicted nuclei is *** comparing the half-lives,this study reveals thatαdecay predominates.

关键词： cluster radioactivity half-lives Coulomb and proximity potential model

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Description of moment of inertia and the interplay between anti-pairing and pairing correlations in^(244)Pu and^(248)Cm

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Chinese Physics C 2024年第10期48卷 176-184页

作者： Anshul Dadwal Xiao-Tao He Department of nuclear Science and technology College of Materials Science and TechnologyNanjing University of Aeronautics and AstronauticsNanjing 210016China

A variable moment of inertia(VMI)inspired interacting boson model(IBM),which includes many-body interactions and a perturbation possessing(5)(or(5))symmetry,is used to investigate the rotational bands of the mass region.A novel modification is introduced,extending the Arima coefficient to the third *** study is dedicated to the quantitative analysis of evolving trends in intrabandγ-transition energy as well as the kinematic and dynamic moments of inertia(MoIs)within the rotational bands of^(244)Pu and^(248)*** computed outcomes exhibit an exceptional degree of agreement with experimental observations across various *** significance of including a higher-order Arima coefficient is further examined by contrasting it with the previously proposed *** calculated results demonstrate the significance of both the anti-pairing and pairing effects in the evolution of the dynamic ***,these insights reveal the importance of a newly introduced parameter in accurately depicting complex nuclear behaviors,such as back-bending,up-bending,and downturn in the MoI.

关键词： rotational bands nuclear structure back-bending up-bending 250 mass region

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Non-contact gaseous microplasma electrode as anode for electrodeposition of metal and metal alloy in molten salt

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Chinese Chemical Letters 2024年第4期35卷 166-169页

作者： Junhan Luo Qi Qing Liqin Huang Zhe Wang Shuang Liu Jing Chen Yuexiang Lu Institute of nuclear and New energy technology Tsinghua UniversityBeijing 100084China The MOE Key Laboratory of Resources and Environmental System Optimization College of Environmental Science and EngineeringNorth China Electric Power UniversityBeijing 102206China nuclear Research Institute for Future technology and Policy Seoul National UniversitySeoul 08826Republic of Korea

Microplasma based on glow discharge could act as a non-contact gaseous electrode and has attracted much attention in both fundamental research and application. Herein, with microplasma as the anode,the electrodeposition process of a series of metal and metal alloys in molten salt has been systemically studied. Four metal cations with different valence states, silver(Ag~+), nickel(Ni^(2+)), copper(Cu^(2+)), and iron(Fe^(3+)), could all be reduced on the solid cathode with high current efficiency and the corresponding metal products were of high purity. The electrodeposition of aluminum-lanthanum(Al-Ln) alloy on the aluminum cathode was also successfully carried out with microplasma as the anode, and the same alloy was obtained by using the conventional anode electrode. These results indicated that microplasma anode based on non-contact direct-current(DC) glow discharge is a promising electrode to be applied in molten salt electrolysis.

关键词： Microplasma Anode Molten salt Electrodeposition Al-Ln alloy

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A simple model for two-proton radioactivity

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Chinese Physics C 2024年第10期48卷 247-255页

作者： Jie-Dong Jiang Xiao Liu Dong-Meng Zhang Ming Li Xi-Jun Wu Xiao-Hua Li School of nuclear Science and technology University of South ChinaHengyang 421001China School of Math and Physics University of South ChinaHengyang 421001China National Exemplary Base for International Sci&Tech.Collaboration of nuclear energy and nuclear Safety University of South ChinaHengyang 421001China Cooperative Innovation Center for nuclear Fuel Cycle technology&Equipment University of South ChinaHengyang 421001China Key Laboratory of Low Dimensional Quantum Structures and Quantum Control Hunan Normal UniversityChangsha 410081China

In this work,considering the preformation factor of the emitted two protons in parent nucleus S_(2p) and the effect of the parent nucleus deformation,based on the Wentzel-Kramers-Brillouin approximation and Bohr-Sommerfeld quantization condition,we improve a simple phenomenological model proposed by Bayrak[***.G:47,025102(2020)]to systematically study 2p radioactivity *** model contains two adjustable parameters V_(0) and a_(β),which are related to the depth of nuclear potential and effect of *** calculated results show that this model can effectively reproduce the experimental data with a corresponding root-mean-square(RMS)standard deviation of σ=*** comparison,we include the Gamow-like model(GLM)proposed by Liu et al.[***.C 45,044110(2021)],generalized liquid drop model(GLDM)proposed by Cui et al.[***.C 101,014301(2020)],effective liquid drop model(ELDM)proposed by *** et al.[***.B 774,14(2017)],two-potential approach with Skyrme-Hartree-Fock(TPASHF)proposed by Pan et al.[***.C 45,124104(2021)],phenomenological model with a screened electrostatic barrier(SEB)propoesed by Zou et al.[***.C 45,104101(2021)],unified fission model(UFM)proposed by Xing et al.[***.C 45,124105(2021)],Coulomb and proximity potential model for deformed nuclei(CPPMDN)proposed by Santhosh[***.C 104,064613(2021)],two-parameter empirical formula proposed by Liu et al.[***.C 45,024108(2021)],and four-parameter empirical formula proposed by Sreeja et al.[***.J.A 55,33(2019)].In addition,we use this model to 2p predict the radioactive half-lives of some possible potential nuclei whose 2p radioactivity are energetically allowed or observed but not yet quantified in NUBASE2020.

关键词： two-proton radioactivity half-lives Wentzel-Kramers-Brillouin approximation

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Theoretical calculations of proton emission half-lives based on a deformed Gamow-like model

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Chinese Physics C 2024年第4期48卷 107-114页

作者：张冬萌胡笑源亓林静刘宏铭李明李小华 School of nuclear Science and technology University of South ChinaHengyang 421001China Institute of Modern Physics Fudan UniversityShanghai 200433China National Exemplary Base for International Sci&Tech.Collaboration of nuclear energy and nuclear Safety University of South ChinaHengyang 421001China Cooperative Innovation Center for nuclear Fuel Cycle technology&Equipment University of South ChinaHengyang 421001China Key Laboratory of Low Dimensional Quantum Structures and Quantum Control Hunan Normal UniversityChangsha 410081China

In this study,proton emission half-lives were investigated for deformed proton emitters with 53≤Z≤83based on the presented deformed Gamow-like model,where the deformation effect was included in the Coulomb *** experimental half-lives of proton emitters can be reproduced within a factor of *** comparison,the results from the universal decay law and the new Geiger-Nuttall law are also ***,the relevance of the half-lives to the angular momentum l for ^(117)La,^(121)Pr,^(135)Tb,and ^(141)Ho were analyzed,and the corresponding possible values of l were proposed:l=3,3,4,4.

关键词： proton emission half-lives deformed nuclei Gamow-like model

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FPGA-based position reconstruction method for neutron beam flux spatial distribution measurement in BNCT

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nuclear Science and Techniques 2024年第3期35卷 96-108页

作者： Wei Jiang Ping Cao Yi-Ming Wu Xian-Ke Liu Zhu-Jun Fang Zhi-Yong Zhang Bin Shi Jun Chen State Key Laboratory of Particle Detection and Electronics University of Science and Technology of ChinaHefei 230026China Department of Modern Physics University of Science and Technology of ChinaHefei 230026China School of nuclear Science and technology University of Science and Technology of ChinaHefei 230026China National Key Laboratory for Metrology and Calibration Techniques China Institute of Atomic EnergyBeijing 102413China

A new measurement method for the spatial distribution of neutron beam flux in boron neutron capture therapy(BNCT)is being developed based on the two-dimensional Micromegas *** address the issue of long processing times in traditional offline position reconstruction methods,this paper proposes a field programmable gate array based online position reconstruction method utilizing the micro-time projection chamber *** method encapsulates key technical aspects:a self-adaptive serial link technique built upon the dynamical adjustment of the delay chain length,fast sorting,a coordinate-matching technique based on the mapping between signal timestamps and random access memory(RAM)addresses,and a precise start point-merging technique utilizing a circular combined *** performance test of the selfadaptive serial link shows that the bit error rate of the link is better than 10-12 at a confidence level of 99%,ensuring reliable data *** experiment utilizing the readout electronics and Micromegas detector shows a spatial resolution of approximately 1.4 mm,surpassing the current method’s resolution level of 5 *** beam experiment confirms that the readout electronics system can obtain the flux spatial distribution of neutron beams online,thus validating the feasibility of the position reconstruction *** online position reconstruction method avoids traditional methods,such as bubble sorting and traversal searching,simplifies the design of the logic firmware,and reduces the time complexity from O(n2)to O(n).This study contributes to the advancement in measuring neutron beam flux for BNCT.

关键词： Position reconstruction FPGA Readout electronics Neutron flux spatial distribution

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α-particle preformation factors in heavy and superheavy nuclei

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Chinese Physics C 2024年第4期48卷 146-158页

作者：骆松张冬萌亓林静陈勋初鹏程李小华 School of nuclear Science and technology University of South ChinaHengyang 421001China School of Mathematics and Physics Qingdao University of Science and TechnologyQingdao 266033China National Exemplary Base for International Sci&Tech.Collaboration of energy and nuclear Safety University of South ChinaHengyang 421001China Cooperative Innovation Center for nuclear Fuel Cycle technology&Equipment University of South ChinaHengyang 421001China Key Laboratory of Low Dimensional Quantum Structures and Quantum Control Hunan Normal UniversityChangsha 410081China

In this study,α-particle preformation factors in heavy and superheavy nuclei from ^(220)Th to ^(294)Og are *** combing experimental α decay energies and half-lives,the α-particle preformation factors P_(α) are extracted from the ratios between theoretical α decay half-lives calculated using the Two-Potential Approach (TPA)and experimental *** find that the α-particle preformation factors exhibit a noticeable odd-even staggering behavior,and unpaired nucleons inhibit α-particle ***,we find that both the α decay energy and mass number of parent nucleus exhibit considerable regularity with the extracted experimental α-particle preformation *** considering the major physical factors,we propose a local phenomenological formula with only five valid parameters for α-particle preformation factors P_(α).This analytic expression has a clear physical meaning as well as good *** an application,this analytic formula is extended to estimate the α-particle preformation factors and further predict the α decay half-lives for unknown even-even nuclei with Z=118 and 120.

关键词： αdecay half-lives preformation factors heavy and superheavy nuclei

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In situ luminescence measurements of GaN/Al_(2)O_(3) film under different energy proton irradiations

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Chinese Physics B 2024年第5期33卷 704-710页

作者：蒋文丽欧阳潇仇猛淋英敏菊陈琳庞盼张春雷张耀锋廖斌 Key Laboratory of Beam technology of Ministry of Education College of Nuclear Science and TechnologyBeijing Normal UniversityBeijing 100875China Institute of Radiation technology Beijing Academy of Science and TechnologyBeijing 100875China

Ion beam-induced luminescence(IBIL) experiments were performed to investigate the in situ luminescence of GaN/Al_(2)O_(3) at varying ion energies,which allowed for the measurement of defects at different depths within the *** energies of H^(+)were set to 500 keV,640 keV and 2 MeV,the Bragg peaks of which correspond to the GaN film,GaN/Al_(2)O_(3) heterojunction and Al_(2)O_(3) substrate,respectively.A photoluminescence measurement at 250 K was also performed for comparison,during which only near band edge(NBE) and yellow band luminescence in the GaN film were *** evolution of the luminescence of the NBE and yellow band in the GaN film was discussed,and both exhibited a decrease with the fluence of H^(+).Additionally,the luminescence of F centers,induced by oxygen vacancies,and Cr^(3+),resulting from the ^(2)E →^(4)A_(2) radiative transition in Al_(2)O_(3),were measured using 2 MeV H^(+).The luminescence intensity of F centers increases gradually with the fluence of H^(+).The luminescence evolution of Cr^(3+)is consistent with a yellow band center,attributed to its weak intensity,and it is situated within the emission band of the yellow band in the GaN *** results show that IBIL measurement can effectively detect the luminescence behavior of multilayer films by adjusting the ion *** measurement can be excited by various techniques,but IBIL can satisfy in situ luminescence measurement,and multilayer structural materials of tens of micrometers can be measured through IBIL by adjusting the energy of the inducing *** evolution of defects at different layers with ion fluence can be obtained.

关键词： ion beam-induced luminescence(IBIL) GaN/Al_(2)O_(3) ion beam

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Synthesis of carbon nitride in potassium hydroxide molten salt for efficient uranium extraction from radioactive wastewater

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Frontiers of Environmental Science & Engineering 2024年第8期18卷 89-99页

作者： Shuang Liu Junhan Luo Daniel-James Maguire Liyuan Zheng Zhe Wang Yuexiang Lu Institute of nuclear and New energy technology Tsinghua UniversityBeijing 100084China nuclear Research Institute for Future technology and Policy Seoul National UniversitySeoul 08826Republic of Korea Department of Earth Sciences University of CambridgeCambridge CB23EQUK The MOE Key Laboratory of Resources and Environmental System Optimization College of Environmental Science and EngineeringNorth China Electric Power UniversityBeijing 102206China

Photocatalysis-assisted removal of uranium has been proven as an effective method for the elimination of radioactive pollution from *** this work,carbon nitride materials were synthesized in potassium hydroxide(KOH)molten salt and applied to photocatalytic uranyl *** materials were confirmed to possess the triazine-s-heptazine structure by NMR,XPS and UV-Vis characterization,and exhibited a wider visible light absorption than graphitic carbon nitride(g-C_(3)N_(4)).The photocatalytic activity of the carbon nitride materials was tailored by varying the precursor mass *** carbon nitride obtained at 80%melamine as precursor(K-CN-80)exhibited the highest photocatalytic extraction ability and its photocatalytic reaction rate is 6.6 times faster than that of g-C_(3)N_(4).The influence of sacrificial agents was studied and the results showed that triethanolamine inhibited U(Ⅵ)photoreduction,but methanol can accelerate U(Ⅵ)photoreduction by consuming photogenerated *** unary KOH molten salt synthesis method has exceptional potential applications in the preparation of carbon nitrides,and the obtained products showed potential in extracting U(Ⅵ)from aqueous solutions for use in nuclear fuel industry and for U(Ⅵ)environmental pollution cleanup.

关键词： Uranium Carbon nitride Molten salt Photocatalysis Radioactive wastewater

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