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Hexamerin and allergen are required for female reproduction in the American cockroach,Periplaneta americana

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Insect Science 2024年第1期31卷 186-200页

作者： Shiming Zhu Xiaoyi Chen Sishi Xia Qin Li Ziqi Ye Shaoting Zhao Kexin Liu Fangfang Liu Guangdong Provincial Key laboratory of Insect developmental Biology and Applied Technology Institute of Insect Science and TechnologyInstitute of Insect Science and Technology&School of Life SciencesSouth China Normal UniversityGuangzhouChina Guangmeiyuan r&d Center Guangdong Provincial Key Laboratory of Insect Developmental Biology and Applied TechnologySouth China Normal UniversityMeizhouGuangdong ProvinceChina Guangdong laboratory for Lingnan Modern Agriculture South China Agricultural UniversityGuangzhouChina

reproduction is of great importance for the continuation of the *** insects,the fat body is the major tissue for nutrient storage and involved in vitellogenesis,which is essential for female ***,2 proteins,hexamerin and allergen,were separated from the fat bodies of adult female American cockroaches(Periplaneta americana)and identified as storage proteins,encoding for 733 amino acids with molecular weight of 87.88 kda and 686 amino acids with molecular weight of 82.18 kda,*** encoding genes of these 2 storage proteins are mainly expressed in the fat *** interference-mediated knockdown of Hexamerin and Allergen in the early stage of the first reproductive cycle in females suppressed vitellogenesis and ovarian maturation,indicating that these storage proteins are involved in controlling ***,the expression of Hexamerin and Allergen was repressed by knockdown of the juvenile hormone(JH)receptor gene Met and the primary response gene Kr-h1,and was induced by methoprene,a JH analog,in both in vivo and in vitro ***,we have determined that hexamerin and allergen are identified as storage proteins and play an important role in promoting female reproduction in the American *** expression of their encoding genes is induced by JH *** data reveal a novel mechanism by which hexamerin and allergen are necessary for JH-stimulated female reproduction.

关键词： fat body juvenile hormone ovary reproduction storage protein vitellogenesis

Constructing high-toughness polyimide binder with robust polarity and ion-conductive mechanisms ensuring long-term operational stability of silicon-based anodes

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Journal of Energy Chemistry 2024年第6期93卷 580-591,I0014页

作者： Yongjun Kang Nanxi dong Fangzhou Liu daolei Lin Bingxue Liu Guofeng Tian Shengli Qi dezhen Wu State Key laboratory of Chemical resource Engineering Beijing University of Chemical TechnologyBeijing 100029China ENFI r&d Institute China ENFI Engineering CorporationBeijing 100038China China Automotive Battery research Institute Co. Ltd.Beijing 101407China Changzhou Institute of Advanced Materials Beijing University of Chemical TechnologyChangzhou 213164JiangsuChina

Silicon-based materials have demonstrated remarkable potential in high-energy-density batteries owing to their high theoretical ***,the significant volume expansion of silicon seriously hinders its utilization as a lithium-ion ***,a functionalized high-toughness polyimide(PdMI) is synthesized by copolymerizing the 4,4'-Oxydiphthalic anhydride(OdPA) with 4,4'-oxydianiline(OdA),2,3-diaminobenzoic acid(dABA),and 1,3-bis(3-aminopropyl)-tetramethyl disiloxane(dMS).The combination of rigid benzene rings and flexible oxygen groups(-O-) in the PdMI molecular chain via a rigidness/softness coupling mechanism contributes to high *** plentiful polar carboxyl(-COOH) groups establish robust bonding *** ionic transport is achieved by incorporating the flexible siloxane segment(Si-O-Si),which imparts high molecular chain motility and augments free volume holes to facilitate lithium-ion transport(9.8 × 10^(-10) cm^(2) s^(-1) vs.16 × 10^(-10) cm^(2) s~(-1)).As expected,the SiO_x@PdMI-1.5 electrode delivers brilliant long-term cycle performance with a remarkable capacity retention of 85% over 500 cycles at 1.3 A g^(-1).The well-designed functionalized polyimide also significantly enhances the electrochemical properties of Si nanoparticles ***,the assembled SiO_x@PdMI-1.5/NCM811 full cell delivers a high retention of 80% after 100 *** perspective of the binder design strategy based on polyimide modification delivers a novel path toward high-capacity electrodes for high-energy-density batteries.

关键词： Polyimide binder High toughness robust ionic transport Silicon-based anodes Lithium-ion batteries

Fluorophosphates and fluorosulfates cathode materials: Progress towards high energy density sodium-ion battery

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Nano research 2024年第3期17卷 1427-1440页

作者： Mohammed Hadouchi Jingrong Hou Toshinari Koketsu Abdelilah Lahmar Jiwei Ma Laboratoire de Chimie Appliquée des Matériaux Centre des Sciences des MatériauxFaculty of ScienceMohammed V University in RabatAvenue Ibn BattoutaBP 1014RabatMorocco Shanghai Key laboratory for r&d and Application of Metallic Functional Materials Institute of New Energy for VehiclesSchool of Materials Science and EngineeringTongji UniversityShanghai 201804China Battery Materials development Section Business Creation Sector R&D CenterMitsui Mining&Smelting Co.Ltd.362-0021 SaitamaJapan Laboratoiry of Condensed Matter Physics University of Picardie Jules Verne33 Rue Saint-Leu 80039AmiensFrance

The rapid diffusion of renewable energy boosts the wide deployment of large-scale energy storage *** the low cost and high crustal abundance,sodium-ion battery(SIB)technology is expected to become a dominant technology in that area in the *** the practical application,novel cathode materials are urged to develop that show high energy density without sacrificing their cost and benignity to the *** the years of many studies,this still remains a huge challenge to battery *** this review,we discuss recent breakthroughs in SIB cathode materials with high energy density,namely fluorphosphates and *** design of materials,the crystal structure,the electrochemical performance,and the underlaying intercalation mechanism are systematically *** strategies and research directions are also provided to advance future high-energy,low-cost,and ecofriendly cathode materials for next generation SIB.

关键词： fluorophosphates fluorosulfates crystal structure intercalation mechanism high energy density sodium-ion battery

A vision system based on CNN-LSTM for robotic citrus sorting Author links open overlay panel

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Information Processing in Agriculture 2024年第1期11卷 14-25页

作者： Yonghua Yu Xiaosong An Jiahao Lin Shanjun Li Yaohui Chen College of Engineering Huazhong Agricultural UniversityWuhan 430070China Key laboratory of Agricultural Equipment in Mid-Lower Yangtze river Ministry of Agriculture and Rural AffairsWuhan 430070China National r&d Center for Citrus Preservation Wuhan 430070China Citrus Mechanization research Base Ministry of Agriculture and Rural AffairsWuhan 430070China

Compared with manual sorting of citrus fruit,vision-based sorting solutions can help achieve higher accuracy and *** this study,we present a vision system based on CNN-LSTM,which can cooperate with robotic grippers for real-time sorting and is readily applicable to various citrus processing plants.A CNN-based detector was adopted to detect the defective oranges in view and temporarily classify them into corresponding types,and an LSTM-based predictor was used to predict the position of the oranges in a future frame based on image sequential *** fusion of CNN and LSTM networks enabled the system to track defective ones during rotation and identify their true types,and their future path was also predicted which is vital for predictive control of visually guided robotic *** detection accuracy of 94.1%was obtained based on experimental results,and the error for path prediction was within 4.33 pixels 40 frames *** average time to process a frame was between 28 and 62 frames per second,which also satisfied real-time *** results proved the potential of the proposed system for automated citrus sorting with good precision and efficiency,and it can be readily extended to other fruit crops featuring high versatility.

关键词： deep learning Long short-term memory Vision system Online citrus sorting Path prediction

mtdNA-triggered pH response signal-amplified fluorescent probe for multiple cell discrimination

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Chinese Chemical Letters 2024年第3期35卷 363-368页

作者： Tianping Xia Yanxian Hou Zhuoran Xia Gengwen Chen Peichen Tang Jiangli Fan Xiaojun Peng State Key laboratory of Fine Chemicals Frontiers Science Center for Smart Materials Oriented Chemical EngineeringDalian University of TechnologyDalian 116024China Hematology reagent r&d department Mindray Bio-medical Electronics Co.Ltd.Shenzhen 518132China research Institute of dalian University of Technology in Shenzhen Shenzhen 518057China

developing fluorescence probes with multiple responses has vital significance but remains ***,for the first time,we present a mitochondrial dNA(mtdNA)-triggered pH response signalamplified fluorescent probe(QCY-dBT)for multiple cell *** probe exhibited a large stokes shift(229 nm),excellent dNA selectivity over rNA,and ultrasensitivity of detection limit(dL;74.0 ng/mL).Thus,QCY-dBT was successfully applied to analyze multiple human peripheral blood cells and visualize mtdNA in healthy and apoptotic *** the tumor acidic environment(pH 6.0–7.0),the absorbance of QCY-dBT at 436 nm increased,and the fluorescence signal(665 nm)was amplified by mtdNA,which enabled the direct observation of tumor *** study provides help in designing smart probes with multiple responses for efficient abnormal cell detection.

关键词： Fluorescence probe Mitochondrial dNA pH response Peripheral blood cells Multiple cell detection

Knowledge Graph Completion Method of Combining Structural Information with Semantic Information

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Chinese Journal of Electronics 2024年

作者： Binhao HU Jianpeng ZHANG Hongchang CHEN School of Cyber Science and Engineering Zhengzhou University National digital Switching System Engineering & Technological r&d Center (NdSC)

With the development of knowledge graphs, a series of applications based on knowledge graphs have emerged. The incompleteness of knowledge graphs makes the effect of the downstream applications and affected by the quality of the knowledge graphs. To improve the quality of knowledge graphs, translation-based graph embeddings, such as TransE, learn structural information by rep-resenting triples as low-dimensional dense vectors. However, is difficult to generalize to unseen entities, Entities that are not observed during training but appear during testing. The other methods use the powerful representational ability of pre-trained language models to learn entity descriptions and contextual representation of triples. Although they are robust to incompleteness, but they need to calculate the score of all candidate entities for each triple during inference. We consider combining two models to enhance the robustness of unseen entities by semantic information, and prevent combined explosion by reducing inference overhead through structured information. We use a pre-training language model to code triples and learn the semantic information within them, and then use a hyperbolic space-based distance model to learn structural information and integrate the two types of information together. We evaluate our model by performing link prediction experi-ments in standard datasets. In experiments, our model achieves better performances than state-of-the-art methods on two standard datasets.

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Biomass valorization via electrocatalytic carbon–carbon bond cleavage

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Journal of Energy Chemistry 2024年第4期91卷 542-578页

作者： Keping Wang Zhenyan Guo Min Zhou Ying Yang Lanyun Li Hu Li rafael Luque Shunmugavel Saravanamurugan National Key laboratory of Green Pesticide Key Laboratory of Green Pesticide&Agricultural BioengineeringMinistry of EducationState-Local Joint Laboratory for Comprehensive Utilization of BiomassCenter for R&D of Fine ChemicalsGuizhou UniversityGuiyang 550025GuizhouChina departamento de Quimica Organica Universidad de CordobaCampus de RabanalesEdificio Marie Curie(C-3)Ctra Nnal IVKm.396E-14014 CordobaSpain laboratory of Bioproduct Chemistry Centre of Innovative and Applied Bioprocessing(CIAB)Mohali 140306PunjabIndia

renewable electrocatalytic upgrading of biomass feedstocks into valuable chemicals is one of the promising strategies to relieve the pressure of traditional energy-based *** electrocatalytic carbon–carbon bond cleavage of high selectivity,various functionalized molecules,such as organic acids,amides,esters,and nitriles,have great potential to be accessed from ***,it has merely received finite concerns and interests in the *** review first showcases the research progress on the electrocatalytic conversion of lipid/sugar-and lignin-derived molecules(e.g.,glycerol,mesoerythritol,xylose,glucose,1-phenylethanol,and cyclohexanol)into organic acids via specific carbon–carbon bond scission processes,with focus on disclosing reaction mechanisms,recognizing actual active species,and collecting feasible modification *** the guidance of further extensive studies on biomass valorization,organic transformations via a variety of reactions,including decarboxylation,ring-opening,rearrangement,reductive hydrogenation,and carboxylation,are also disclosed for the construction of similar carbon skeletons/*** remaining challenges,prospective applications,and future objectives in terms of biomass conversion are also *** review is expected to provide references to develop renewed electrocatalytic carbon–carbon bond cleavage transformation paths/strategies for biomass upgrading.

关键词： Electrocatalysis Biomass conversion Carbon-carbon bond cleavage Organic acids

The AaBBX21–AaHY5 module mediates light-regulated artemisinin biosynthesis in Artemisia annua L.

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Journal of Integrative Plant Biology 2024年第8期66卷 1735-1751页

作者： Weizhi He Hang Liu Zhangkuanyu Wu Qing Miao Xinyi Hu Xin Yan Hangyu Wen Yaojie Zhang Xueqing Fu Li ren Kexuan Tang Ling Li Frontiers Science Center for Transformative Molecules Joint International ResearchLaboratory of Metabolic and Developmental SciencesKey Laboratory of Urban Agriculture(South)Ministry of AgriculturePlant Biotechnology Research CenterFudan-SJTU-Nottingham Plant Biotechnology R&D CenterSchool of Agriculture and BiologyShanghai Jiao Tong UniversityShanghai 200240China Institute for Agri-Food Standards and Testing Technology Shanghai Academy of Agricultural SciencesShanghai 201403China

The sesquiterpene lactone artemisinin is an important anti-malarial component produced by the glandular secretory trichomes of sweet wormwood(Artemisia annua L.).Light was previously shown to promote artemisinin production,but the underlying regulatory mechanism remains *** this study,we demonstrate that ELONGATEd HYPOCOTYL5(HY5),a central transcription factor in the light signaling pathway,cannot promote artemisinin biosynthesis on its own,as the binding of AaHY5 to the promoters of artemisinin biosynthetic genes failed to activate their *** analysis and yeast two-hybrid screening revealed the B-box transcription factor AaBBX21 as a potential interactor with ***21 showed a trichome-specific expression ***,the AaBBX21–AaHY5 complex cooperatively activated transcription from the promoters of the downstream genes AaGSW1,AaMYB108,and AaOrA,encoding positive regulators of artemisinin ***,AaHY5 and AaBBX21 physically interacted with the *** E3 ubiquitin ligase CONSTITUTIVELY PHOTOMOrPHOGENIC 1(COP1).In the dark,AaCOP1 decreased the accumulation of AaHY5 and AaBBX21 and repressed the activation of genes downstream of the AaHY5–AaBBX21 complex,explaining the enhanced production of artemisinin upon light *** study provides insights into the central regulatory mechanism by which light governs terpenoid biosynthesis in the plant kingdom.

关键词： AaBBX21 AaHY5 AaCOP1 Artemisia annua L. artemisinin biosynthesis light

Modified electronic structure and enhanced hydroxyl adsorption make quaternary Pt-based nanosheets efficient anode electrocatalysts for formic acid-/alcohol-air fuel cells

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Journal of Energy Chemistry 2024年第5期92卷 142-150页

作者： Fengling Zhao Qiang Yuan Siyang Nie Liang Wu Xun Wang State-Local Joint laboratory for Comprehensive Utilization of Biomass Center for R&D of Fine ChemicalsCollege of Chemistry and Chemical EngineeringGuizhou UniversityGuiyang 550025GuizhouChina Key Lab of Organic Optoelectronics&Molecular Engineering Tsinghua UniversityBeijing 100084China School of Chemistry and Chemical Engineering Shanghai Jiao Tong UniversityShanghai 200240China

Surface/interface engineering of a multimetallic nanostructure with diverse electrocatalytic properties for direct liquid fuel cells is desirable yet ***,using visible light,a class of quaternary Pt_(1)Ag_(0.1)Bi_(0.16)Te_(0.29)ultrathin nanosheets is fabricated and used as high-performance anode electrocatalysts for formic acid-/alcohol-air fuel *** modified electronic structure of Pt,enhanced hydroxyl adsorption,and abundant exterior defects afford Pt_(1)Ag_(0.1)Bi_(0.16)Te_(0.29)/C high intrinsic anodic electrocatalytic activity to boost the power densities of direct formic acid-/methanol-/ethanol-/ethylene glycol-/glycerol-air fuel cells,and the corresponding peak power density of Pt_(1)Ag_(0.1)Bi_(0.16)Te_(0.29)/C is respectively 129.7,142.3,105.4,124.3,and 128.0 mW cm^(-2),considerably outperforming Pt/*** in situ Fourier transform infrared reflection spectroscopy reveals that formic acid oxidation on Pt_(1)Ag_(0.1)Bi_(0.16)Te_(0.29)/C occurs via a CO_(2)-free direct *** functional theory calculations show that the presence of Ag,Bi,and Te in Pt_(1)Ag_(0.1)Bi_(0.16)Te_(0.29)suppresses CO^(*)formation while optimizing dehydrogenation steps and synergistic effect and modified Pt effectively enhance H_(2)O dissociation to improve electrocatalytic *** synthesis strategy can be extended to 43 other types of ultrathin multimetallic nanosheets(from ternary to octonary nanosheets),and efficiently capture precious metals(i.e.,Pd,Pt,rh,ru,Au,and Ag)from different water sources.

关键词： Pt-based nanosheets Modifiedelectronic structure Enhanced hydroxyl adsorption Formicacidand alcohol oxidation direct liquid fuel cells