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Bimetal MOF-derived NiFe-P nanocomposites coupled with Cu_(3)P nanoparticles to construct tandem electron transfer channels for photocatalytic hydrogen evolution

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Journal of Environmental Sciences 2024年第3期137卷 333-346页

作者： Haiyan Zhang Shitao Yang Peng Zhu Senpei Tang Ming Li College of Chemistry and Chemical Engineering Jishou UniversityJishou 416000China School of Account Hunan University of Technology and BusinessChangsha 410205China

Finely modulated light-induced charge separation and transfer is a central challenge to achieve efficient *** progress has been made in this field,most of the previous research works focused on the separation or migration of photogenerated carriers but did not build a bridge between the *** to realize the strong driving and precise migration of carriers has become the focus of our *** report an ingeniously designed ternary *** NiFe-MOF as the“parent material”,the FeP_(4)/Ni_(x)P_(y)heterojunction is derived in situ while maintaining the frame structure through gas-solid reaction,and finally the Z-type electron transfer is *** Cu_(3)P anchoring spindle matrix,an electron transport tunnel is opened up in Cu_(3)P/FeP_(4)/Ni_(x)P_(y)ternary heterojunction under the action of p-n heterojunction built-in electric field driving and accurate energy band *** strong driving force of the built-in electric field provides an inexhaustible power for the transmission of electrons,and the fine series of electron transmission channels realizes the precise transmission of *** above fine design makes the perfect fit between the built-in electric field and the electron transfer channel,which not only effectively improves the embarrassing situation of insufficient electron driving force of hydrogen evolution reaction in the previous research,but also makes up for the weakening of semi-conductor reduction ability caused by the construction of traditional p-n *** research work provides a new idea for the construction of multiple heterostructures and the design of fine interface engineering in the future.

关键词： Cu_(3)P/FeP_(4)/Ni_(x)P Built-in electric field Electron transfer channels Photocatalysis

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Research of caged dynamics of clusters center atoms in Pd_(82)Si_(18) amorphous alloy

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Chinese Physics B 2024年第4期33卷 623-629页

作者：邓永和陈贝祁清华李兵兵高明文大东王小云彭平 School of Computational Science and Electronics Hunan Institute of EngineeringXiangtan 411104China School of Physics and Mechanical&Electrical Engineering Jishou UniversityJishou 416000China School of Materials Science and Engineering Hunan UniversityChangsha 410082China

To date,there is still a lack of a comprehensive explanation for caged dynamics which is regarded as one of the intricate dynamic behaviors in amorphous *** study focuses on Pd_(82)Si_(18)as the research object to further elucidate the underlying mechanism of caged dynamics from multiple perspectives,including the cage's lifetime,atomic local environment,and atomic potential *** results reveal that Si atoms exhibit a pronounced cage effect due to the hindrance of Pd atoms,resulting in an anomalous peak in the non-Gaussian *** in-depth investigation was conducted on the caged dynamics differences between fast and slow Si *** comparison to fast Si atoms,slow Si atoms were surrounded by more Pd atoms and occupied lower potential energy states,resulting in smaller diffusion displacements for the slow Si ***,slow Si atoms tend to be in the centers of smaller clusters with coordination numbers of 9 and *** the isothermal relaxation process,clusters with coordination numbers 9 and 10 have longer lifetimes,suggesting that the escape of slow Si atoms from their cages is more *** findings mentioned above hold significant implications for understanding the caged dynamics.

关键词： caged dynamics Pd_(82)Si_(18) amorphous alloy fast and slow atoms clusters lifetime

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Interacting topological magnons in a checkerboard ferromagnet

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Chinese Physics B 2024年第3期33卷 596-601页

作者：朱恒施洪潮唐政国唐炳 Department of Physics Jishou UniversityJishou 416000China

This work is devoted to studying the magnon-magnon interaction effect in a two-dimensional checkerboard ferromagnet with the Dzyaloshinskii-Moriya *** a first-order Green function method,we analyze the influence of magnon-magnon interaction on the magnon band *** find that Chern numbers of two renormalized magnon bands are different above and below the critical temperature,which means that the magnon band gap-closing phenomenon is an indicator for one topological phase transition of the checkerboard *** results show that the checkerboard ferromagnet possesses two topological phases,and its topological phase can be controlled either via the temperature or the applied magnetic field due to magnon-magnon ***,it is found that the topological phase transition can occur twice with the increase in the temperature,which is different from the results of the honeycomb ferromagnet.

关键词： topological magnons magnon-magnon interactions topological phase transitions checkerboard ferromagnets

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Double Moving Extremes Ranked Set Sampling Design

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Acta Mathematicae Applicatae Sinica 2024年第1期40卷 75-90页

作者： Meng Chen Wang-xue Chen Rui Yang Department of Mathematics and Statistics Jishou UniversityJishou416000China

The traditional simple random sampling(SRS)design method is inefficient in many *** proposed some new designs to increase *** this paper,as a variation of moving extremes ranked set sampling(MERSS),double MERSS(DMERSS)is proposed and its properties for estimating the population mean are *** turns out that,when the underlying distribution is symmetric,DMERSS gives unbiased estimators of the population ***,it is found that DMERSS is more efficient than the SRS and MERSS methods for usual symmetric distributions(normal and uniform).For asymmetric distributions considered in this study,the DMERSS has a small bias and it is more efficient than SRS for usual asymmetric distribution(exponential)for small sample sizes.

关键词： double moving extremes ranked set sampling symmetric distribution efficiency

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Anodic Electrosynthesis of Amide from Alcohol and Ammonia

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CCS Chemistry 2024年第1期6卷 125-136页

作者： Yuxuan Lu Yingying Li Bo Zhou Jingcheng Wu Ling Zhou Yuping Pan Zhongcheng Xia Ming Yang Yandong Wu Zhenran Yuan Rixin Peng Zhijie Kong Shuangyin Wang Yuqin Zou State Key Laboratory of Chemo/Biosensing and Chemometrics College of Chemistry and Chemical EngineeringAdvanced Catalytic Engineering Research Center of the Ministry of EducationHunan UniversityChangsha 410082 Shenzhen Institute of hunan university Shenzhen 518057 School of Chemistry and Chemical Engineering Jishou UniversityJishouHunan 416000

Amide is essential in biologically active compounds,synthetic materials,and building ***,conventional amide production relies on energyintensive consumption and activating agents that modulate processes to construct the C–N ***,for the first time,we have successfully realized the formation of amides at industrial current density via the anodic coelectrolysis of alcohol and ammonia under ambient *** have proved thatmodulation of the interface microenvironment concentration of nucleophile by electrolyte engineering can regulate the reaction pathways of amides rather than acetic *** C-N coupling strategy can be further extended to the electrosynthesis of the long-chain and aryl-ring amide with high selectivity by replacing ammonia with *** work opens up a vast store of information on the utilization of biomass alcohol for high-value N-containing chemicals via an electrocatalytic C-N coupling reaction.

关键词： electrocatalysis electrocatalysts biomass upgrading elctrochemical oxidation coupling amide production

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Double integral-enhanced Zeroing neural network with linear noise rejection for time-varying matrix inverse

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CAAI Transactions on Intelligence Technology 2024年第1期9卷 197-210页

作者： Bolin Liao Luyang Han Xinwei Cao Shuai Li Jianfeng Li College of Computer Science and Engineering Jishou UniversityJishouChina School of Management Shanghai UniversityShanghaiChina School of Engineering Swansea UniversitySwanseaUK

In engineering fields,time-varying matrix inversion(TVMI)issue is often *** neural network(ZNN)has been extensively employed to resolve the TVMI ***,the original ZNN(OZNN)and the integral-enhanced ZNN(IEZNN)usually fail to deal with the TVMI problem under unbounded noises,such as linear ***,a neural network model that can handle the TVMI under linear noise interference is urgently *** paper develops a double integral-enhanced ZNN(DIEZNN)model based on a novel integral-type design formula with inherent linear-noise ***,its convergence and robustness are verified by deriva-tion *** comparison and verification,the OZNN and the IEZNN models are adopted to resolve the TVMI under multiple identical noise *** experi-ments proved that the DIEZNN model has excellent advantages in solving TVMI problems under linear *** general,the DIEZNN model is an innovative work and is proposed for the first ***,the errors of DIEZNN are always less than 1�10−3 under linear noises,whereas the error norms of OZNN and IEZNN models are not convergent to *** addition,these models are applied to the control of the controllable permanent magnet synchronous motor chaotic system to indicate the superiority of the DIEZNN.

关键词： neural network real-time systems

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Uniformity of Asymmetric Augmented Designs

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Acta Mathematicae Applicatae Sinica 2024年第4期40卷 1025-1044页

作者： Zhi-qing WANG Xiang-yu FANG Zu-jun OU College of Mathematics and Statistics Jishou UniversityJishou 416000China

Follow-up experimental designs are widely applied to explore the relationship between factors and responses step by step in various fields such as science and *** some additional resources or information become available after the initial design of experiment is carried out,some additional runs and/or factors may be added in the follow-up *** this paper,the issue of the uniform row augmented designs and column augmented designs with mixed two-,three-and four-level is *** uniformity of augmented designs is discussed under the wrap-around L_(2)-*** lower bounds of wrap-around L_(2)-discrepancy for the augmented designs are obtained,which can be used to assess uniformity of augmented *** results show that augmented designs have high efficiency,which have low discrepancy and close to the proposed lower bounds.

关键词： augmented design follow-up design uniform design wrap-around L_(2)-discrepancy

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Electrospinning-hot pressing technique for the fabrication of thermal and electrical storage membranes and its applications

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International Journal of Minerals,Metallurgy and Materials 2024年第9期31卷 1945-1964页

作者： Panpan Che Baoshan Xie Penghui Cao Youfu Lv Daifei Liu Huali Zhu Xianwen Wu Zhangxing He Jian Chen Chuanchang Li Key Laboratory of Renewable Energy Electric-Technology of hunan Province School of Energy and Power EngineeringChangsha University of Science and TechnologyChangsha 410114China State Key Laboratory of Disaster Prevention&Reduction for Power Grid Changsha University of Science and TechnologyChangsha 410114China School of Chemistry and Chemical Engineering Jishou UniversityJishou 416000China School of Chemical Engineering North China University of Science and TechnologyTangshan 063009China

The combination of electrospinning and hot pressing,namely the electrospinning-hot pressing technique(EHPT),is an efficient and convenient method for preparing nanofibrous composite materials with good energy storage *** emerging composite membrane prepared by EHPT,which exhibits the advantages of large surface area,controllable morphology,and compact structure,has attracted immense *** this paper,the conduction mechanism of composite membranes in thermal and electrical energy storage and the performance enhancement method based on the fabrication process of EHPT are systematically ***,the state-of-the-art applications of composite membranes in these two fields are *** particular,in the field of thermal energy storage,EHPT-prepared membranes have longitudinal and transverse nanofibers,which generate unique thermal conductivity pathways;also,these nanofibers offer enough space for the filling of functional ***,EHPT-prepared membranes are beneficial in thermal management systems,building energy conservation,and electrical energy storage,e.g.,improving the electrochemical properties of the separators as well as their mechanical and thermal *** application of electrospinning-hot pressing membranes on capacitors,lithium-ion batteries(LIBs),fuel cells,sodium-ion batteries(SIBs),and hydrogen bromine flow batteries(HBFBs)still requires *** the future,EHPT is expected to make the field more exciting through its own technological breakthroughs or be combined with other technologies to produce intelligent materials.

关键词： electrospinning-hot pressing technique thermal storage electrical storage composite membranes nanofiber

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Exponential-Poisson Parameters Estimation in Moving Extremes Ranked Set Sampling Design

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Acta Mathematicae Applicatae Sinica 2024年

作者： Meng CHEN Wang-xue CHEN Rui YANG Ya-wen ZHOU Department of Mathematics and Statistics Jishou University

In this article, the maximum likelihood estimators (MLEs) of the scale and shape parameters βandλfrom the Exponential-Poisson distribution will be considered in moving extremes ranked set sampling(MERSS). These MLEs will be compared in terms of asymptotic efficiencies. The numerical results show that these MLEs in MERSS can be real competitors against those in simple random sampling.

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Separator functionalization enables high-performance zinc anode via ion-migration regulation and interfacial engineering

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Chinese Chemical Letters 2024年第9期35卷 496-500页

作者： Ningning Zhao Yuyan Liang Wenjie Huo Xinyan Zhu Zhangxing He Zekun Zhang Youtuo Zhang Xianwen Wu Lei Dai Jing Zhu Ling Wang Qiaobao Zhang School of Chemical Engineering North China University of Science and TechnologyTangshan 063009China School of Chemistry and Chemical Engineering Jishou UniversityJishou 416000China Department of Materials Science and Engineering College of MaterialsXiamen UniversityXiamen 361005China

Aqueous zinc ion batteries(AZIBs)are promising energy storage ***,the formation of dendrites,hydrogen evolution,and corrosion reaction seriously affect their electrochemical ***,the synergistic effect of ion-migration regulation and interfacial engineering has been confirmed as the potential strategy by kaolin functionalized glass fiber separator(KL-GF)to alleviate these *** rapid and orderly Zn^(2+)migration was achieved to improve the transfer kinetics and induced uniform zinc deposition by more zinc-philic sites of *** on the interfacial engineering,the side reactions were effectively mitigated and crystal planes were regulated through *** hydrophilicity of KL alleviated the corrosion and hydrogen ***,a preferential orientation of Zn(002)crystal plane by KL-GF was induced to further realize dendrite-free deposition by density functional theory(DFT)and X-ray diffraction(XRD)***,the Zn|KL-GF|MnO_(2)cell maintained a high discharge capacity of 96.8 mAh/g at 2 A/g after 1000 *** work can provide guidance enabling high-performance zinc anode for AZIBs.

关键词： Energy storage Aqueous zinc ion batteries Separators Ion-migration regulation Interfacial engineering

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