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Preferential Formation of Ethylene via Electrocatalytic CO_(2) Reduction on Mesoporous Cu_(2)O Nanoparticles:Synergistic Effects of Pore Structure Confinement and Surface Amine

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Chinese Journal of Chemistry 2024年第16期42卷 1846-1852页

作者： Haifeng Zhang Dun Li Zhifang Chen Yingying Wang Haoyu Sun Feng Liu Maochang Liu Yiqun Zheng Hongwen Huang School of Chemistry Chemical Engineering and MaterialsJining UniversityQufuShandong 273155China college of Materials Science and Engineering Hunan UniversityChangshaHunan 410082China Health Management Department Shandong Vocational College of Light IndustryZiboShandong 255300China international Research Center for Renewable Energy National Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiotong UniversityXi'anShaanxi 710049China

We present a facile synthetic strategy to create mesoporous Cu_(2)O nanocrystals with tunable pore structures and surface functional groups of amine derivatives for efficient and preferable electrochemical conversion of CO_(2) into *** structural characteristics of theseCu_(2)O nanocrystals can be manipulated using a set of amine derivatives,such as pyridine,4,4'-bipyridine,and hexamethylenetetramine,during the oxidative etching process of Cu nanocrystals by bubbling gaseous oxygen in N,N-dimethylformamide *** amine derivatives not only serve as surface functional groups but also significantly affect the resulting pore *** synergistic effect of pore structure confinement and surface amine functionalization leads to the superb Faradaic efficiency(FE)of 51.9% for C_(2)H_(4),respectively,together with the C_(2)H_(4) partial current density of -209.4 mA·cm^(-2) at -0.8 V *** hydrogen electrode(RHE).The relatively high selectivity towards C_(2)H_(4) was investigated using DFT simulations,where 4,4'-bipyridine functionalized Cu_(2)O seemed to favor the C_(2)H_(4) formation with the low free energy of the *** study provides a feasible strategy to manipulate the pore structure and surface functionalization of mesoporous Cu_(2)O nanocrystals by regulating the oxidative etching process,which sheds light on the rational preparation of high-performance CO_(2)RR electrocatalysts.

关键词： Amines Ethylene Cuprous oxide CO_(2)reduction Mesoporous materials

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Why can some countries perform better in resolving some social problems:A comparative study

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Economic and Political Studies 2024年第3期12卷 250-266页

作者： Wilson X.B.Li Tina T.He Faculty of business and Management BNU-HKBU United International CollegeZhuhaiChina

This study explores the rationale why some countries fare better in resolving social problems such as poverty and the COVID-19 *** simple model introduces the term of resident viability and points out that the solution to a social problem with a large ratio of nonviable to viable residents requires the mobilisation of more societal resources,and the affordable price ratio of societal to individual resources is determined by country characteristics such as the cultural background,political regime,ideology towards the free-market mechanism,government efficiency and social *** study also makes between-country comparisons and conducts preliminary regression analyses with cross-country data,and all the results are consistent with the model predictions on the relationship between country characteristics and country performances in fighting poverty and handling the COVID-19 pandemic.

关键词： Social problems COVID-19 poverty eradication viability between-country comparison

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Optimization design and experiment of the variable differential gear train planting mechanism

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international Journal of Agricultural and Biological Engineering 2024年第2期17卷 85-93页

作者： Xiong Zhao Ziwei Liu Yuanwu Jia Xingxiao Ma Pengfei Zhang Jianneng Chen School of Mechanical Engineering Zhejiang Sci-Tech UniversityHangzhou 310018China Xi’an international University Engineering college Xi’an 710077China Hangzhou vocational&Technical college Hangzhou 310018China

In order to improve the adaptability of the planting mechanism for different plant spacings,a variable differential gear train planting mechanism based on precise pose and trajectory control was proposed by combining the open chain 2R rod group and the variable differential gear *** to the pose requirements of receiving seedling point,transporting seedling point and planting point,three precise pose points of constrained planting trajectory were *** the three-position motion generation structural synthesis method,combined with computer-aided optimization design software,a set of mechanism parameters that meet the planting requirements were *** on the optimized mechanism parameters,by only changing the coordinates of two trajectory shape control points,three planting trajectories with key point position information adapted to 300 mm,400 mm and 500 mm plant spacing were obtained by interpolation,and three pairs of total transmission ratio of three groups of variable differential gear trains were *** distributing the total transmission ratio of the mechanism,the fixed axis gear train and the differential gear train are *** fixed axis gear train included a pair of non-circular gear pairs and a pair of positive gear pairs,which were convenient for disassembly and *** former drives the sun gear at variable speed,and the latter drives the planet carrier at uniform *** on this structure,the transmission ratio of the positive gear pair is-1,and the transmission ratio of the differential gear train is *** sub-transmission ratio of the single-stage non-circular gear pair was calculated and the pitch curves of three pairs of noncircular gears were *** pairs of non-circular gear pairs with different transmission ratios were replaced in turn and three sets of planting mechanisms were modeled in three *** virtual prototype motion simulation was completed by ADAMS software,and the p

关键词： plant spacing planting mechanism variable differential gear train precise pose trajectory control parameter optimization

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Investigating the interaction between umami peptides and umami receptor T1R1/T1R3-VFT: a computational approach

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Food Science and Human Wellness 2024年

作者： Hengli Meng Zhiyong Cui Yingqiu Li Yanyang Yu Shui Jiang Yuan Liu Department of Food Science & Technology， School of Agriculture and Biology， Shanghai Shanghai Jiao Tong University Secondary college of Cereals and Tourism， Guangxi vocational college of Technology and business

The study of ligand-receptor interactions is of great significance in food flavor perception. In this study， a computer simulation method was used to investigate the mechanism of interaction between umami peptides and T1R1/T1R3-VFT receptor. The binding site， conformational changes， and binding free energy between umami peptides and T1R1/T1R3-VFT were analyzed through molecular modeling， molecular docking， and molecular dynamics simulations. The receptor model constructed using AlphaFold2 has the best rationality. The molecular docking results showed that umami peptides primarily bound to T1R1-VFT through hydrogen bonding， with key binding residues such as 149THR， 151ARG， and 108ASP. The binding of umami peptides led to a more stable complex system， and the positively charged amino acids contributed positively to the overall binding free energy. This study provides theoretical support for the development of a better understanding of the interaction between umami substances and the umami receptor.

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The spillover effect of customers’ESG performance on suppliers’green innovation quality

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China Journal of Accounting Research 2024年第3期17卷 198-225页

作者： Yani Sun Yuezhe Shen Qingmei Tan The international business School Hainan UniversityHaikouHainanChina college of Management and Economics Tianjin UniversityTianjinChina

This study investigates whether and how customer firms’environmental,social and governance(ESG)performance impacts suppliers’green innovation quality using a sample of Chinese A-share listed companies from 2009 to *** find that customers’ESG performance facilitates suppliers’green innovation quality through green learning and corporate *** tests indicate that customers with stickier customer-supplier relationships and a more central position in the supply chain network than peers enhance suppliers’green innovation *** categorizing whether customers engage in greenwashing,we determine that those adherence to green principles,genuinely promote suppliers’green innovation ***,we find the above effect ultimately enhances suppliers’environmental *** study provides valuable insights for supply chain companies into collaboratively achieving sustainable development.

关键词： ESG performance Spillover effect Green innovation quality Supply chain

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Reducing carbon emissions with Geoscience solutions:A look at the contributions of nuclear energy,technology,and green finance

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Geoscience Frontiers 2024年第4期15卷 411-426页

作者： Aifeng Liu Muhammad Imran Abdelmohsen A.Nassani Rima H.Binsaeed Khalid Zaman international business School Shaanxi Normal UniversityXi’anChina Department of Economics The University of HaripurHaripur Khyber Pakhtunkhwa 22620Pakistan Department of Management College of Business AdministrationKing Saud UniversityP.O.Box 71115Riyadh 11587Saudi Arabia

Standards for Low-Carbon Energy Portfolios(LC-EPS)mandate that a certain percentage of a region's electricity generation originate from zero-or low-emissions *** 1995Q1 through 2020Q4,the study used the ARDL-Bounds testing technique to estimate coefficient parameters,Granger causality to draw causal inferences,and variance decomposition analysis to anticipate the factors that will have the greatest impact on carbon emissions in the US *** power significantly impacts carbon emissions,as seen by an inverted U-shaped environmental Kuznets curve,whereas long-term impact of innovation leads to lower *** the other hand,exports of sophisticated technology reduce carbon *** growth has a discernible effect on carbon emissions,nuclear power,innovation,and environmentally friendly ***-tech exports will likely impact carbon emissions most,followed by a demand for nuclear power,innovation,economic expansion,and sustainable finance for the next ten *** results give policymakers helpful insight into how the US economy may reduce carbon emissions and fight climate change via renewable energy and green finance.

关键词： Nuclear energy demand High technology exports Innovation Economic growth Green finance USA

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Infiltration,runoff,and slope stability behaviors of infinite slope with macropores based on an improved Green–Ampt model

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Journal of Mountain Science 2024年第7期21卷 2220-2235页

作者： LI Shanghui WU Guoxiong QUE Yun JIANG Zhenliang CHENG Gaoyun college of Intelligent Construction Fuzhou University of International Studies and TradeFuzhou 350202China college of Civil Engineering Chongqing Jiao Tong UniversityChongqing 400074China Chongqing vocational college of Architectural Engineering Chongqing 400072China college of Civil Engineering Fuzhou UniversityFuzhou 350000China Department of Civil and Environmental Engineering Hong Kong University of Science and TechnologyHong Kong 999077China T.Y.Lin international Engineering Consulting(China)Co.Ltd Chongqing 401120China

Infiltration–runoff–slope instability mechanism of macropore slope under heavy rainfall is *** paper studied its instability mechanism with an improved Green–Ampt(GA)model considering the dual-porosity(i.e.,matrix and macropore)and ponding condition,and proposed the infiltration equations,infiltration–runoff coupled model,and safety factor calculation *** show that the infiltration processes of macropore slope can be divided into three stages,and the proposed model is rational by a comparative *** wetting front depth of the traditional unsaturated slope is 17.2%larger than that of the macropore slope in the early rainfall stage and 27%smaller than that of the macropore slope in the late rainfall ***,macropores benefit the slope stability in the early rainfall but not in the *** flow does not occur initially but becomes pronounced with increasing rainfall *** equal depth of the wetting front in the two domains is regarded as the onset criteria of macropore *** analysis shows that macropore flow is delayed by increasing proportion of macropore domain(ω_(f)),whereas promoted by increasing ratio of saturated permeability coefficients between the two domains(μ).The increasing trend of ponding depth is sharp at first and then grows ***,when rainfall duration is less than 3 h,ωf andμhave no significant effect on the safety factor,whereas it decreases with increasingωf and increases with increasingμunder longer duration(≥3 h).With the increase ofω_(f),the slope maximum instability time advances by 10.5 h,and with the increase ofμ,the slope maximum instability time delays by 3.1 h.

关键词： Macropore slope Green–Ampt infiltration model Equivalent wetting front Ponding response time Slope stability

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Visibility restoration for real-world hazy images via improved physical model and Gaussian total variation

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Frontiers of Computer Science 2024年第1期18卷 267-269页

作者： Chuan LI Enping HU Xinyu ZHANG Hao ZHOU Hailing XIONG Yun LIU college of Computer and Information Science Southwest UniversityChongqing 400715China School of Big Data and Intelligent Engineering Chongqing College of International Business and EconomicsChongqing 401520China college of Artificial Intelligence Southwest UniversityChongqing 400715China college of Electronic and Information Engineering Southwest UniversityChongqing 400715China

1 Introduction Under real-world haze conditions,the existence of haze particles in the atmosphere reduces the visibility of captured ***,the noise is inevitably introduced into the degraded image,which further deteriorates the visual quality of the *** enhance the visibility and quality of outdoor real-world hazy images,numerous algorithms have been proposed to remove haze from a single input *** existing methods are broadly lumped into two categories:prior-based methods[1,2]and learning-based methods[3–6].Unfortunately,the widely used atmospheric scattering model and the corresponding haze removal methods fail to take the noise interference into account,which may result in poor visibility restoration performance.

关键词： visibility remove noise

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Heterosis Analysis in Endogenous Substances in Root Bleeding Sap of Sorghum

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Phyton-international Journal of Experimental Botany 2024年第8期93卷 1963-1980页

作者： Renjie Zhao Yueqiao Li Chen Xu Zhian Zhang Ziyang Zhou Yihan Zhou Zexin Qi college of Agriculture Jilin Agricultural UniversityChangchun130118China Jilin Academy of Agricultural Sciences Changchun130033China Jilin Engineering vocational college Siping136001China

Despite hybrid dominance contributing to the genetic improvement of crops,little is known about heterosis and inheritance patterns of endogenous substances in sorghum(Sorghum bicolor(L.)Moench)root bleeding *** this study,six sterile and six restorer lines of sorghum and 36 hybrid sorghum combinations formulated as incomplete double-row crosses were selected as test materials,and heterosis,combining ability,heritability,and their interrelationships of root bleeding sap endogenous substances in different hybrid sorghum combinations and their parents were *** results showed that the root bleeding sap of the F1 generation of hybrid sorghum had a high heterosis in both soluble sugar content and amino acid content at the flowering stage,and the average high-parent heterosis was 129.34%and 74.57%,***-3-acetic acid(IAA),cytokinins(CTK),gibberellic acid(GA_(3)),abscisic acid(ABA),soluble sugar,amino acid,and root bleeding intensity were mainly affected by non-additive genetic effects of the *** protein was affected by additive genetic effects of the genes and had a high narrow heritability(75.50%),which could be selected at low generations in *** combining ability analyses showed that the sterile lines 521A and 170A,and the restorer lines Ji318R and 0–30 were promising parents with high general combining *** analysis showed that all endogenous substances of root bleeding sap were positively correlated with the sum of parental general combining ability(GCA)at highly significant levels,and IAA,CTK,GA_(3),ABA,soluble sugar,amino acid,and root bleeding intensity were positively correlated with male GCA at significant or highly significant ***,the GCA of the restorer lines root bleeding sap endogenous material or the sum of both parents’GCA can be used to predict the performance of wounding endogenous material in the F1 generation of hybrid ***,this study results can help elucidate hetero

关键词： Sorghum heterosis root bleeding sap combining ability heritability

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An Underwater Biomimetic Robot that can Swim,Bipedal Walk and Grasp

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Journal of Bionic Engineering 2024年第3期21卷 1223-1237页

作者： Qiuxuan Wu Liwei Pan FuLin Du ZhaoSheng Wu XiaoNi Chi FaRong Gao Jian Wang Anton A.Zhilenkov School of Automation Hangzhou Dianzi UniversityHangzhou310018China international Joint Research Laboratory for Autonomous Robotic Systems Hangzhou310018China GEELY Automotive Institute Hangzhou Vocational and Technical CollegeHangzhou310018China Institute of Hydrodynamics and Control Processes Sankt-Petersburg Saint Petersburg State Marine Technical UniversitySankt-PetersburgRussia

In developing and exploring extreme and harsh underwater environments,underwater robots can effectively replace humans to complete *** meet the requirements of underwater flexible motion and comprehensive subsea operation,a novel octopus-inspired robot with eight soft limbs was designed and *** robot possesses the capabilities of underwater bipedal walking,multi-arm swimming,and grasping *** closely interact with the underwater seabed environment and minimize disturbance,the robot employs a cable-driven flexible arm for its walking in underwater floor through a bipedal walking *** multi-arm swimming offers a means of three-dimensional spatial movement,allowing the robot to swiftly explore and navigate over large areas,thereby enhancing its ***,the robot’s walking arm enables it to grasp and transport objects underwater,thereby enhancing its practicality in underwater environments.A simplified motion models and gait generation strategies were proposed for two modes of robot locomotion:swimming and walking,inspired by the movement characteristics of octopus-inspired multi-arm swimming and bipedal *** experimental verification,the robot’s average speed of underwater bipedal walking reaches 7.26 cm/s,while the horizontal movement speed for multi-arm swimming is 8.6 cm/s.

关键词： Underwater soft robots Underwater bipedal walking Multi-arm swimming Cable drive

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