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Late Jurassic oceanic plateau subduction in the Bangong-Nujiang Tethyan Ocean of northern Tibet

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Geoscience Frontiers 2024年第4期15卷 274-289页

作者： Hao Wu Haiyong Liu Yu Wang Xijun Liu Qinggao Zeng Panxi Wang Guangxi Key Laboratory of Hidden Metallic Ore Deposits Exploration&collaborative innovation Center for Exploration of Nonferrous Metal Deposits and Efficient utilization of Resources on Guangxi Guilin University of TechnologyGuilin 541006China Tibet Geological Survey Lhasa 850000China Tibet Bureau of Geological and Mineral Exploration and Development Lhasa 850000China

Oceanic plateau accretion and subsequent flat-slab subduction in modern convergent settings have profoundly influenced the nature of subduction and mantle ***,evaluating similar impacts in ancient convergent settings,where oceanic plateaus have been subducted but geological records are limited,remains *** this study,we present geochronological and geochemical data for a suite of ore-associated plutonic rocks from the Gaobaoyue area of northern *** rocks have zircon U-Pb ages of 152-146 Ma,with high Sr contents and Sr/Y and La/Yb ratios,low MgO,Yb,and Y contents,and depleted Sr-Nd-Hf isotopic compositions,consistent with an adakitic affinity that was generated by the partial melting of subducting oceanic *** compare the Late Jurassic adakitic magmatism with the spatiotemporal evolution of magmatism in northern Tibet to infer oceanic plateau subduction and subsequent flat-slab subduction in the Bangong-Nujiang Tethyan *** tectonic model explains(ⅰ)slab-derived adakitic magmatism,(ⅱ)the observed lull in magmatic activity,(ⅲ)intraplate compression and uplift,and(ⅳ)subduction jump and *** also propose that the subduction of heterogeneous oceanic crust(i.e.,buoyant oceanic plateau subduction)provided favorable conditions for tectonic exhumation,vertical slab tearing,and the formation of Cu-Au *** findings not only have implications for establishing the fundamental process of oceanic plateau accretion in ancient subduction zones but also provide an alternative explanation for Late Jurassic complex tectonomagmatic activity in north-ern Tibet.

关键词： Northern Tibet Adakitic magma Oceanic plateau Flat-slab subduction Vertical slab tearing

Structural engineering of hard carbon through spark plasma sintering for enhanced sodium-ion storage

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Rare Metals 2024年第9期43卷 4274-4285页

作者： Hao-Ming Xiao Heng Zheng Ping Yuan Jun-Hui Luo Lin-Lin Shen Jie-Feng Tan Xian-You Luo De Li Yong Chen Guangdong Key Laboratory for Hydrogen energy Technologies School of Materials Science and Hydrogen EnergyFoshan UniversityFoshan 528000China State Key Laboratory of Marine Resource utilization in South China Sea Hainan Provincial Key Laboratory of Research on Utilization of Si-Zr-Ti ResourcesHainan UniversityHaikou 570228China

Hard carbon(HC)has emerged as one of the superior anode materials for sodium-ion batteries(SIBs),with its electrochemical performance significantly influenced by the presence of oxygen functional groups and its closed pore ***,current research on the structural adjustment of these oxygen functional groups and the closed pore architecture within HC remains ***,energy-efficient and contamination-free spark plasma sintering technology was employed to tune the structure of coconut-shell HC,resulting in significant adjustments to the content of carboxyl(decreasing from 5.71 at%to 2.12 at%)and hydroxyl groups(decreasing from 7.73 at%to 6.26 at%).Crucially,these modifications reduced the irreversible reaction of oxygen functional groups with Na^(+).Simultaneously,a substantial number of closed pores with an average diameter of 1.22 nm were generated within the HC,offering an ideal environment for efficient Na^(+)*** structural changes resulted in a remarkable improvement in the electrochemical performance of the modified *** reversible specific capacity of the modified HC surged from 73.89 mAh·g^(-1)to an impressive 251.97 m Ah·g^(-1)at a current density of 50 mA·g^(-1).Even at 400 mA·g^(-1),the reversible specific capacity increased significantly from 14.55 to 85.44 mAh·g^(-1).Hence,this study provides a novel perspective for designing tailored HC materials with the potential to develop high-performance SIBs.

关键词： Hard carbon Spark plasma sintering Sodiumion batteries Closed pores Oxygen functional groups

Regulating Effect of Substrate Temperature on Sputteringgrown Ge/Si QDs under Low Ge Deposition

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Journal of Wuhan University of Technology(Materials Science) 2024年第4期39卷 888-894页

作者：舒启江 YANG Linjing LIU Hongxing 黄鹏儒 Institute of Information Yunnan University of Chinese MedicineKunming 650500China Guangxi Key Laboratory of Information Materials and Guangxi collaborative innovation Center of Structure and Property for New energy and Materials School of Material Science&EngineeringGuilin University of Electronic TechnologyGuilin 541004China

The effect of deposition temperature on the morphology and optoelectronic performance of Ge/Si QDs grown by magnetron sputtering under low Ge deposition(~4 nm)was investigated by atomic force microscopy,Raman spectroscopy,and photoluminescence(PL)*** experimental results indicate that temperatures higher than 750℃effectively increase the crystallization rate and surface smoothness of the Si buffer layer,and temperatures higher than 600℃significantly enhance the migration ability of Ge atoms,thus increasing the probability of Ge atoms meeting and nucleating to form QDs on Si buffer layer,but an excessively high temperature will cause the QDs to undergo an Ostwald ripening process and thus develop into super large *** addition,some PL peaks were observed in samples containing small-sized,high-density Ge QDs,the photoelectric properties reflected by these peaks were in good agreement with the corresponding structural characteristics of the grown *** results demonstrate the viability of preparing high-quality QDs by magnetron sputtering at high deposition rate,and the temperature effect is expected to work in conjunction with other controllable factors to further regulate QD growth,which paves an effective way for the industrial production of QDs that can be used in future devices.

关键词： Ge/Si QDs deposition temperatures evolution law photoelectric performance

Mechanism of high Li-ion conductivity in poly(vinylene carbonate)-poly(ethylene oxide)cross-linked network based electrolyte revealed by solid-state NMR

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Journal of energy Chemistry 2024年第6期93卷 377-383,I0010页

作者： Fan Li Tiantian Dong Yi Ji Lixin Liang Kuizhi Chen Huanrui Zhang Guanglei Cui Guangjin Hou State Key Laboratory of Catalysis Dalian National Laboratory for Clean EnergyCollaborative Innovation Center of Chemistry for Energy MaterialsDalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023LiaoningChina University of Chinese Academy of Sciences Beijing 100049China Qingdao Industrial energy Storage Research Institute Qingdao Institute of Bioenergy and Bioprocess TechnologyChinese Academy of SciencesQingdao 266101ShandongChina

Solid polymer electrolytes(SPEs)have become increasingly important in advanced lithium-ion batteries(LIBs)due to their improved safety and mechanical properties compared to organic liquid ***-linked polymers have the potential to further improve the mechanical property without trading off Li-ion *** this study,focusing on a recently developed cross-linked SPE,i.e.,the one based on poly(vinylene carbonate)-poly(ethylene oxide)cross-linked network(PVCN),we used solid-state nuclear magnetic resonance(NMR)techniques to investigate the fundamental interaction between the chain segments and Li ions,as well as the lithium-ion *** utilizing homonuclear/heteronuclear correlation,CP(cross-polarization)kinetics,and spin-lattice relaxation experiments,etc.,we revealed the structural characteristics and their relations to lithium-ion *** is found that the network formation prevents poly(ethylene oxide)chains from crystallization,which could create sufficient space for segmental tumbling and Li-ion co nductio *** such,the mechanical property is greatly improved with even higher Li-ion mobilities compared to the poly(vinylene carbonate)or poly(ethylene oxide)based SPE analogues.

关键词： ssNMR Lithium-ion mobility Cross-link Solid polymer electrolyte

A process insight into production of ethyl levulinate via a stepwise fractionation

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Journal of Bioresources and Bioproducts 2024年第2期9卷 233-242页

作者： Yan Ma Hongxiao Wang Ziyang Wu Weihong Tan Guodong Feng Jianchun Jiang Institute of Chemical Industry of Forest Products Chinese Academy of ForestryNanjing 210042China Jiangsu Province Key Lab.of Biomass energy and Material Nanjing 210042China National Engineering Lab.for Biomass Chemical utilization Nanjing 210042China Co-innovation Center of Efficient Processing and utilization of Forest Resources Nanjing Forestry UniversityNanjing 210037China

Ethyl levulinate(EL)is a key biomass-derived compounds due to its socio-economic benefits for the synthesis of commodity ***,we proposed an efficient one-step bamboo conversion to EL in ethanol,and a novel stepwise fractionation to purify EL and lignocellulose degradation products.A proton acid,due to its high catalytic efficiency,yielded 26.65%EL in 120 min at 200℃.The productions of ethyl glucoside and 5-ethoxymethylfurfural were analyzed in terms of by-products *** the best of our knowledge,there is no single report on catalyst for one step synthesis of EL directly from bamboo,as well as a stepwise fractionation to purify *** to similar physiochemical properties in each fraction,the platform molecules could broaden a new paradigm of bamboo biomass utilization for renewable energy and value-added *** addition,glucose,ethyl glucoside,corn starch,and microcrystalline cellulose were also investigated as substrates,so that the reaction intermediates of this one-pot procedure were identified and a possible reaction mechanism was proposed.

关键词： Ethyl levulinate Liquefaction Biomass Ethanol By-products

Climate bonds toward achieving net zero emissions and carbon neutrality:Evidence from machine learning technique

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Journal of Management Science and Engineering 2024年第1期9卷 1-15页

作者： Hermas Abudu Presley K.Wesseh Jr. Boqiang Lin College of Overseas Education Chengdu UniversityChengdu610106SichuanChina School of Management China Institute for Studies in Energy PolicyCollaborative Innovation Center for Energy Economics and Energy PolicyXiamen UniversityFujian361005China Center for African Development Strategy(CFADS) MonroviaLiberia

The Conference of the Parties(COP26 and 27)placed significant emphasis on climate financing policies with the objective of achieving net zero emissions and carbon ***,studies on the implementation of this policy proposition are *** address this gap in the literature,this study employs machine learning techniques,specifically natural language processing(NLP),to examine 77 climate bond(CB)policies from 32 countries within the context of climate *** findings indicate that“sustainability”and“carbon emissions control”are the most outlined policy objectives in these CB ***,the study highlights that most CB funds are invested toward energy projects(i.e.,renewable,clean,and efficient initiatives).However,there has been a notable shift in the allocation of CB funds from climate-friendly energy projects to the construction sector between 2015 and *** shift raises concerns about the potential redirection of funds from climate-focused investments to the real estate industry,potentially leading to the greenwashing of climate ***,policy sentiment analysis revealed that a minority of policies hold skeptical views on climate change,which may negatively influence climate ***,the findings highlight that the effective implementation of CB policies depends on policy goals,objectives,and ***,this study contributes to the literature by employing NLP techniques to understand policy sentiments in climate financing.

关键词： Climate bonds funds utilization Climate bonds policy text mining Machine learning technique Net zero emissions Policy sentiment analysis

Hybrid Network Model Based on Data Enhancement for Short-term Power Prediction of New PV Plants

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Journal of Modern Power Systems and Clean energy 2024年第1期12卷 77-88页

作者： Shangpeng Zhong Xiaoming Wang Bin Xu Hongbin Wu Ming Ding the Anhui Province Key Laboratory of Renewable energy utilization and energy Saving Hefei University of TechnologyHefei 230009China the State Grid Anhui Electric Power Research Institute Hefei 230061China

This study proposes a hybrid network model based on data enhancement to address the problem of low accuracy in photovoltaic(PV)power prediction that arises due to insuffi cient data samples for new PV ***,a time-series gener ative adversarial network(TimeGAN)is used to learn the distri bution law of the original PV data samples and the temporal correlations between their features,and these are then used to generate new samples to enhance the training ***,a hybrid network model that fuses bi-directional long-short term memory(BiLSTM)network with attention mechanism(AM)in the framework of deep&cross network(DCN)is con structed to effectively extract deep information from the origi nal features while enhancing the impact of important informa tion on the prediction ***,the hyperparameters in the hybrid network model are optimized using the whale optimi zation algorithm(WOA),which prevents the network model from falling into a local optimum and gives the best prediction *** simulation results show that after data enhance ment by TimeGAN,the hybrid prediction model proposed in this paper can effectively improve the accuracy of short-term PV power prediction and has wide applicability.

关键词： New photovoltaic(PV)plant short-term predic tion time-series generative adversarial network(TimeGAN) hy brid network hyperparameter

Supported Atomically Dispersed Pd Catalyzed Direct Alkoxylation and Allylic Alkylation

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Chinese Journal of Chemistry 2024年第7期42卷 719-724页

作者： Ruixuan Qin Ziwen Chen Qingyuan Wu Nanfeng Zheng Pengxin Liu New Cornerstone Science Laboratory State Key Laboratory for Physical Chemistry of Solid SurfacesCollaborative Innovation Center of Chemistry for Energy Materialsand National&Local Joint Engineering Research Center of Preparation Technology of NanomaterialsCollege of Chemistry and Chemical EngineeringXiamen UniversityXiamenFujian 361005China innovation Laboratry for Scences and Technoogies of energy Materials of Fujan Province(IKKM) Xiamen Fujian 361102China School of Physical Science and Technology Shanghai Tech UniversityShanghai 201210China Fujian Key Laboratory of Rare-earth Functional Materials Fujian Shanhai Collaborative Innovation Center of Rare-earth Functional MaterialsLongyanFujian 366300China

A new approach to allylic alkylation is realized using an atomically dispersed palladium catalyst(Pd1/TiO2-EG).Unlike conventional methods that require derivation of substrates and utilization of additives,this method allows for direct allylic alkylation from allylic alcohols,producing H2O as the sole *** catalyst's high efficiency is attributed to the local hydrogen bonding at the or-ganic-inorganic interface(Pd-EG interface),facilitating hydroxyl group activation forη3π-allyl complex *** system demonstrates successful direct C—O and C—C coupling reactions with high selectivity,requiring no *** study highlights the potential of supported atomically dispersed catalysts for greener and more efficient catalysis,meanwhile,offers unique insights into the distinct behavior of atomically dispersed catalysts in comparison to homogeneous or nanoparticle-based catalysts.

关键词： Atomically dispersed catalyst Alkylation C—C coupling Organic-inorganic Interface Hydrogen bond Tsuji-Trost reaction Green catalysis

Armoring lithium metal anode with soft±rigid gradient interphase toward high-capacity and long-life all-solid-state battery

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Green energy & Environment 2024年第8期9卷 1279-1289页

作者： Rui Zhang Biao Chen Yuhan Ma Yue Li Junwei Sha Liying Ma Chunsheng Shi Naiqin Zhao School of Materials Science and Engineering and Tianjin Key Laboratory of Composite and Functional Materials Tianjin University Joint School of National University of Singapore and Tianjin University International Campus of Tianjin University Department of Chemical and Biomolecular Engineering National University of Singapore collaborative innovation centre of Chemical Science and Engineering

Solid polymer electrolytes （SPEs） are highly promising for realizing high-capacity,low-cost,and safe Li metal ***,the Li dendritic growth and side reactions between Li and SPEs also plague these ***,a fluorinated lithium salt coating （FC） with organicinorganic gradient and soft-rigid feature is introduced on Li surface as an artificial protective layer by the in-situ reaction between Li metal and fluorinated carboxylic *** FC layer can improve the interface stability and wettability between Li and SPEs,assist the transport of Li ions,and guide Li nucleation,contributing to a dendrite-free Li deposition and long-lifespan Li metal *** symmetric cell with FC-Li anodes exhibits a high areal capacity of 1 mAh cm-2at 0.5 mA cm-2,and an ultra-long lifespan of 2000 h at a current density of 0.1 m A ***,the full cell paired with the LiFePO4cathode exhibits improved cycling stability,remaining 83.7%capacity after 500 cycles at 1 *** matching with the S cathode,the FC layer can prevent the shuttle effect,contributing to stable and high-capacity Li-S *** work provided a promising way for the construction of stable all-solid-state lithium metal batteries with prolonged lifespan.

关键词： All-solid-state battery Solid polymer electrolyte Li metal anode Li nucleation Interface stability