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Deciphering the role of mtH2O2 in hepatic ischemia-reperfusion injury mechanisms with low-background super-resolution fluorogenic probe

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Science China Chemistry 2025年第01期 297-307页

作者： Bin Fang Limin Wang Haoqin Li Jiaxin Zhang Yang Ding Pan Pan Li Bo Peng Hua Bai Lin Li Frontiers Science Center for Flexible electronics Xi'an Institute of Flexible Electronics (IFE) and Xi'an Institute of Biomedical Materials &Engineering Northwestern Polytechnical University institute of Flexible electronics (IFE Future Technologies) Xiamen University

Hepatic ischemia-reperfusion injury（HIRI） is characterized by mitochondrial dysfunction and oxidative stress. Monitoring mitochondrial hydrogen peroxide（mtH2O2） levels in real-time through super-resolution imaging is crucial for elucidating its distribution in live cells and its mechanism of action during HIRI. However, low-background fluorogenic probes have been overlooked in the context of super-resolution imaging. In this study, we developed a low-background fluorogenic probe（MitoWG） with the potential for super-resolution morphology-correlated mitochondrial identification to track the fluctuates of mtH2O2in HIRI. Activation of the desirable fluorescence properties of the probe by mtH2O2was confirmed using structural illumination microscopy（SIM）, enabling high-quality mitochondrial imaging with exceptional specificity and *** in mtH2O2levels were successfully observed in both cellular and rat models of HIRI. Furthermore, we associated the decline in mitochondrial redox homeostasis with accelerated mtH2O2production during HIRI, which triggered mitophagy deficiency and led to cell death. In conclusion, Mito-WG possesses excellent photophysical and low-background properties for SIM imaging, making it a promising tool for mtH2O2tracking in HIRI research and clinical diagnosis.

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Wafer‑Scale Ag_(2)S‑Based Memristive Crossbar Arrays with Ultra‑Low Switching‑Energies Reaching Biological Synapses

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Nano-Micro Letters 2025年第3期17卷 328-339页

作者： Yuan Zhu Tomas Nyberg Leif Nyholm Daniel Primetzhofer Xun Shi Zhen Zhang Division of Solid‑State electronics Department of Electrical EngineeringUppsala University75121 UppsalaSweden Department of Chemistry Uppsala UniversityUppsalaSweden Department of Physics and Astronomy Uppsala UniversityUppsalaSweden State Key Laboratory of high Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050People’s Republic of China

Memristive crossbar arrays(MCAs)offer parallel data storage and processing for energy-efficient neuromorphic ***,most wafer-scale MCAs that are compatible with complementary metal-oxide-semiconductor(CMOS)technology still suffer from substantially larger energy consumption than biological synapses,due to the slow kinetics of forming conductive paths inside the memristive *** we report wafer-scale Ag_(2)S-based MCAs realized using CMOS-compatible processes at temperatures below 160℃.Ag_(2)S electrolytes supply highly mobile Ag+ions,and provide the Ag/Ag_(2)S interface with low silver nucleation barrier to form silver filaments at low energy *** further enhancing Ag+migration in Ag_(2)S electrolytes via microstructure modulation,the integrated memristors exhibit a record low threshold of approximately−0.1 V,and demonstrate ultra-low switching-energies reaching femtojoule values as observed in biological *** low-temperature process also enables MCA integration on polyimide substrates for applications in flexible ***,the intrinsic nonidealities of the memristive units for deep learning can be compensated by employing an advanced training *** impressive accuracy of 92.6%in image recognition simulations is demonstrated with the MCAs after the *** demonstrated MCAs provide a promising device option for neuromorphic computing with ultra-high energy-efficiency.

关键词： Wafer-scale Ag_(2)S films Reactive sputter Silver nucleation Ag^(+)migration Energy-efficient neuromorphic computing

Pulsed high-current discharge in water:adiabatic model of expanding plasma channel and acoustic wave

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Plasma Science and Technology 2022年第3期24卷 123-129页

作者： A KOZYREV A ZHERLITSYN N SEMENIUK institute of high-current electronics Russian Academy of SciencesTomsk 634055Russia

This paper presents the results of a theoretical and experimental study of the use of a pulsed discharge in water to obtain a strong acoustic wave in a liquid medium.A discharge with a current amplitude of 10 kA,a duration of 400 ns,and an amplitude pulsed power of 280 MW in water at atmospheric pressure created an expanding acoustic wave with an amplitude of more than 100 *** describe the formation of the discharge channel,an isothermal plasma model has been developed,which made it possible to calculate both the expansion dynamics of a high-current channel and the strong acoustic wave generated by *** calculations show that the number density of plasma in the channel reaches 10^(20) cm^(-3),while the degree of water vapor ionization is about 10%,and the channel wall extends with a velocity of 500 m s^(−1).The calculations for the acoustic wave are in good agreement with measurements.

关键词： plasma applications electrical discharge in water dense plasma channel

Constructing quasi-2D perovskite to collect hot carriers to reduce open-circuit voltage loss for efficient inverted perovskite solar cells

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Science China Chemistry 2025年

作者： Lei Gu Xing Li Chao Wu Yang Feng Chunming Yang Lin Song Frontiers Science Center for Flexible electronics Institute of Flexible Electronics Northwestern Polytechnical University Shanghai Synchrotron Radiation Facility Shanghai Advanced Research Institute Chinese Academy of Sciences

Inverted perovskite solar cells （PSCs） have received great attention owing to the high certificated power conversion efficiency（PCE） reaching 26.7%. However, interfacial charge recombination is far superior to perovskite bulk charge recombination due to the use of fullerenes and their derivatives in inverted perovskite solar cells, which induces devastating open circuit voltage（VOC） losses. For this reason the present work attempts to use 4-chloropiperidine hydrochloride for the upper surface modification of perovskite to construct a quasi-two-dimensional （2D） structure with suitable 2D layer widths （n=2, 3 dominant）,which has a smaller electron carrier transport barrier without sacrificing short-circuit current （JSC） in the device. This strategy effectively passivates the interfacial defect states while promoting energy level alignment to achieve carrier dissociation and equilibrium transport at the interface, which in turn resulted in improved fill factor （FF）. In addition, additional energy levels are provided by 2D perovskites to collect hot carriers, resulting in improved device open circuit voltage （VOC）. As a result, the device PCE increases from 22.37%to 24.11%after the 4CPD treatment. In addition, the 4CPD-treated PSCs maintain 90%of the initial PCE after storage in an N2atmosphere at 50°C for 1,080 h, whereas the control devices show a 15%PCE loss under the same aging conditions. This work provides new opportunities to suppress interfacial charge recombination in inverted devices.

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Force and impulse multi-sensor based on flexible gate dielectric field effect transistor

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 214-220页

作者： Chao Tan Junling Lü Chunchi Zhang Dong Liang Lei Yang Zegao Wang College of Materials Science and Engineering Sichuan UniversityChengdu 610065China The 54th Research institute of China electronics Technology Group Corporation Shijiazhuang 050081China

Nowadays,force sensors play an important role in industrial production,electronic information,medical health,and many other ***-dimensional material-based filed effect transistor(2D-FET)sensors are competitive with nano-level size,lower power consumption,and accurate ***,few of them has the capability of impulse detection which is a path function,expressing the cumulative effect of the force on the particle over a period of *** we fabricated the flexible polymethyl methacrylate(PMMA)gate dielectric MoS_(2)-FET for force and impulse sensor *** systematically investigated the responses of the sensor to constant force and varying forces,and achieved the conversion factors of the drain current signals(I_(ds))to the detected impulse(I).The applied force was detected and recorded by I_(ds)with a low power consumption of~30 *** sensitivity of the device can reach~8000%and the 4×1 sensor array is able to detect and locate the normal force applied on ***,there was almost no performance loss for the device as left in the air for two months.

关键词： flexible gate dielectric transistor force sensor impulse sensor force sensor array

Tempering Behavior of M50 Steel with Different Austenite Proportion Induced by high current Pulsed Electron Beam

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稀有金属材料与工程 2012年第S1期41卷 475-477页

作者： G.E.Ozure institute of high current electronics 4Academichesky Av.Tomsk 634055Russia

M50 steel was irradiated by high current pulsed electron beam(HCPEB)with different *** subsequent tempering was carried out between 500 and 625℃.Microstructure evolution was analyzed by scanning electron microscopy and X-ray *** is found that the HCPEB treatment could constrain martainsite transformation in the surface layer of the *** behavior of HCPEB remelted layer strongly depends on the proportion of retained *** saturated more carbon and metallic elements depict higher tempering *** tempered process,carbides precipitates among the grain and phase *** decreased solution of the elements promotes the retained austenite into martensite.

关键词： electron beam irradiation M50 steel tempering microstructure

Methods for recording the time profile of single ultrashort pulses of electron beams and discharge currents in real-time mode

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high Voltage 2016年第1期1卷 43-51页

作者： Victor F.Tarasenko Dmitry V.Rybka institute of high current electronics Siberian Branch Russian Academy of SciencesTomsk 634055Russia

The collectors for measuring the time profile of a current pulse of the runaway electron beam that are generatedunder atmospheric pressure are described. An analysis of changes in pulse shape depending on the bandwidth of theregistration path with a temporal resolution of up to 20 ps was performed. It is shown that the electron beam detectedbehind small-diameter diaphragms has a complex structure, which depends on the parameters of the gas diode. Thereis a design of the current shunts with a temporal resolution of up to 100 ps in this study. Measurement techniques ofvoltage pulses with subnanosecond and nanosecond duration are briefly described.

关键词： ultrashort pulse recording

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超高功率体放电的形成及其应用(英文)

光学精密工程 2011年第2期19卷 273-283页

作者： TARASENKO V F BAKSHT E KH BURACHENKO A G LOMAEV M I RYBKA D V SHULEPOV M A SOROKIN D A SHUT'KO V high current electronics institute

研究了氮气中的高压体（扩散）放电特性,实验中施加的极间隙脉冲电压达数百千伏,持续时间为数纳秒,上升时间为几个纳秒,给出了实验结果。研究了氦气压强为（0.42）×10^5Pa时,从扩散形式到火花放电的放电转换过程。确定了在氮气压强下... 详细信息

研究了氮气中的高压体（扩散）放电特性,实验中施加的极间隙脉冲电压达数百千伏,持续时间为数纳秒,上升时间为几个纳秒,给出了实验结果。研究了氦气压强为（0.42）×10^5Pa时,从扩散形式到火花放电的放电转换过程。确定了在氮气压强下电流幅度与逃逸电子束电流脉宽的关系。结果表明,导致隙间扩散放电的超短雪崩电子束（SAEB）对放电过程有重要的影响。在该压强下得出了SAEB瞬间产生相对放电电流的时延与压强的关系,根据该关系,时延随着压强增加而变化,并且在压强为2×10^5Pa时最小,同时扩散放电电流脉冲的峰值随压强增加而减小。在0.5×10^5Pa的压强下,使用刀片电极和6 cm长的N2∶SF6=10∶1的激活媒质,得到了输出能量为2 mJ、脉冲功率为0.55 MW的激光。最后,在大气压强下,对AlBe箔片进行了重复频率放电处理（REP）,其表层清除了碳而且氧原子以450 nm/300pulse渗入箔片。

关键词：体放电扩散放电非均匀电场逃逸电子紫外激光器修饰及清洁

Ru/NiMnB spherical cluster pillar for highly proficient green hydrogen electrocatalyst at high current density

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Journal of Energy Chemistry 2025年第1期100卷 397-408页

作者： Md Ahasan Habib Shusen Lin Mehedi Hasan Joni Sumiya Akter Dristy Rutuja Mandavkar Jae-Hun Jeong Jihoon Lee Department of Electronic Engineering College of Electronics and Information Kwangwoon University

Advanced OER/HER electrocatalytic alternatives are crucial for the wide adaptation of green hydrogen ***,Ru/NiMnB spherical cluster pillar （SCP）,denoted as Ru/NiMnB,is synthesized using a combination of electro-deposition and hydrothermal *** investigation of Ru doping in the NiMnB matrix revealed significant improvements in electrocatalytic *** Ru/NiMnB SCPs demonstrate superior OER/HER activity with low overpotentials of 150 and 103 mV at 50mA/cm2in 1 M KOH,making them highly competitive with state-of-the-art ***,the Ru/NiMnB SCPs exhibit a low 2-E cell voltage of 2.80 V at ultra-high current density of 2,000 m A/cm2in 1 M KOH,outperforming the standard benchmark electrodes of RuO2||Pt/C,thereby positioning Ru/NiMnB as one of the best bifunctional *** SCPs exhibit exceptional high-current characteristics,stability and corrosion resistance,as evidenced by continuous operation at 1,000 mA/cm2high-current density for over 150 h in 6 M KOH at elevated temperatures under harsh industrial *** a small amount of Ru incorporation significantly enhances the electrocatalytic performances of NiMnB,attributed to increased active sites and improved intrinsic properties such as conductivity,adsorption/desorption capability and reaction ***,Ru/NiMnB SCPs present a promising bi-functional electrode concept for efficient green H2production.

关键词： Potassium hydroxide