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Atomistic mechanism of high ionic co.ductivity in lithium ytterbium-based halide solid electrolytes:A first-principles study

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Journal of Rare Earths 2024年第1期42卷 155-162,I0006页

作者： Limin Wang Wei Xiao Lu Sun Rong Yang Jinqiu Yu Ligen Wang State Key Laboratory of Nonferrous Metals and Processes China GRINM Group Co.Ltd.Beijing100088China GRIMAT Engineering Institute co. Ltd.Beijing101407China General Research Institute for Nonferrous Metals Beijing100088China China Automotive Battery Research Institute co. Ltd.Beijing101407China Rare Earth Functional Materials(Xiong'an)Innovation Center co. Ltd.Xiong'an071700China

As the next generation of co.mercial automotive power batteries begins replacing liquid lithium batteries,many look towards all-solid-state batteries to pioneer the ***-so lid-state batteries have attracted the attention of co.ntless researchers around the world because of their high safety and high energy *** recent times,halide solid-state electrolytes have beco.e a research hotspot within solid-state electrolytes because of their potentially superior *** this paper,in the framework of DFT,we investigated the atomic mechanisms of improving the ionic co.ductivity and stability of Li_(3)YbCl_(6).Our calculations show that both trigonal and orthorhombic Li_(3)YbCl_(6) exhibit wide electrochemical windows and metastable properties(100 meV/atom>Ehull>0 meV/atom).However,the orthorhombic Li_(3)YbCl_(6) can be stabilized at high temperatures by taking the vibrational entropy into acco.nt,which is supported by the experimental ***,it is expected that because of the Yb/Li synergistic interactions that,due to their strong mutual co.lomb repulsion,influence the Li^(+)transport behavior,the orthorhombic Li_(3)YbCl_(6) might have superior ionic co.ductivities with appropriate Li+migration paths determined by the Yb^(3+) ***,higher ionic co.ductivities can be obtained by regulating the random distribution of Li^(+) *** Li^(+)-deficiency can also largely increase the ionic co.ductivity by invoking *** study helps gain a deeper understanding of the laws that govern ionic co.ductivities and stabilities and provides a certain theoretical reference for the experimental development and design of halide solid-state electrolytes.

关键词： Halide solid-state electrolytes Phase stability Ionic co.ductivity First-principles calculations Rare earths

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Mechanism of a dual-phase Ti-Nb alloy exhibiting near-linear elastic deformation

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Rare Metals 2024年第5期43卷 2282-2289页

作者： Yan Guo Wang Ding Wen Ma Shun Guo Hao-Dong Meng Nian-Yao Xu School of Automotive Engineering Changzhou Institute of TechnologyChangzhou 213032China School of Materials Science and Engineering Jiangsu UniversityZhenjiang 212013China Youke Publishing co. LtdChina Grinm Group Co.LtdBeijing 100088China

In this work,the underlying mechanism responsible for the near-linear elastic deformation behavior of a dual-phase Ti-Nb alloy co.sisting of β and α'' phase with large reco.erable strain was systematically *** on in situ synchrotron X-ray diffraction(SXRD)analyses,it was found that besides intrinsic elastic deformation,a slight reversible β-α'' stress-induced martensitic(SIM)transformation,which proceeded in a co.secutive mode under the retarding effect of micro-defects,took place during the near-linear elastic *** unloading,a small amount of residual macrosco.ic strain remained in the specimen due to the inco.plete reverse α''→β transformation on *** high near-linear elastic deformability of the co.d drawing(CD)Ti-Nb alloy has been revealed to be attributed to the co.pling actions of intrinsic elasticity as well as the co.secutive and reversible β-α'' SIM *** research may co.tribute to a new avenue for the design and development of novel dual-phase Ti-based alloys with desirable elastic deformability.

关键词： Titanium alloys Dual-phase Near-linear elastic deformation Martensitictransformation

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Observer-based robust high-order fully actuated attitude autopilot design for spinning glide-guided projectiles

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Defence Technology（防务技术） 2024年第4期34卷 282-294页

作者： Wei Wang Yuchen Wang Shiwei Chen Yongcang Guo Zhongjiao Shi School of Aerospace Engineering Beijing Institute of TechnologyBeijing 10081China Northwest Industries group co. Ltd.Xi'an 710043China

This paper investigates the design of an attitude autopilot for a dual-channel co.trolled spinning glideguided projectile(SGGP),addressing model uncertainties and external *** on fixed-time stable theory,a disturbance observer with integral sliding mode and adaptive techniques is proposed to mitigate total disturbance effects,irrespective of initial *** introducing an error integral signal,the dynamics of the SGGP are transformed into two separate seco.d-order fully actuated ***,employing the high-order fully actuated approach and a parametric approach,the nonlinear dynamics of the SGGP are recast into a co.stant linear closed-loop system,ensuring that the projectile's attitude asymptotically tracks the given goal with the desired *** the proposed co.posite co.trol framework,the ultimately uniformly bounded stability of the closed-loop system is rigorously demonstrated via the Lyapunov *** of the effectiveness of the proposed attitude autopilot design is provided through extensive numerical simulations.

关键词： Spinning glide-guided projectile Attitude co.trol Sliding mode disturbance observer Fixed-time stable theory High-order fully actuated approach

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Electronic structure and spin state regulation of vanadium nitride via a sulfur doping strategy toward flexible zinc-air batteries

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Journal of Energy Chemistry 2024年第2期89卷 239-249,I0007页

作者： Daijie Deng Honghui Zhang Jianchun Wu Xing Tang Min Ling Sihua Dong Li Xu henan Li Huaming Li Institute for Energy Research Institute of Quantum and Sustainable TechnologySchool of Chemistry and Chemical EngineeringSchool of Materials Science and EngineeringJiangsu Province and Education Ministry Co-Sponsored Synergistic Innovation Center of Modern Agricultural EquipmentJiangsu UniversityZhenjiang 212013JiangsuChina Key Laboratory of Radio Frequency and Micro-Nano Electronics of Jiangsu Province Nanjing 210023JiangsuChina Zhenjiang Kangyuan Electrical Appliance co. Ltd.Zhenjiang 212013JiangsuChina co.lege of Chemical and Biological Engineering Zhejiang UniversityHangzhou 310027ZhejiangChina YTO group co.poration Dongfanghong(henan)Agricultural Service Technology co. Ltd.Luoyang 471033HenanChina

Owing to the distinctive structural characteristics,vanadium nitride(VN)is highly regarded as a catalyst for oxygen reduction reaction(ORR)in zinc-air batteries(ZABs).However,VN exhibits limited intrinsic ORR activity due to the weak adsorption ability to O-co.taining ***,the S-doped VN anchored on N,S-doped multi-dimensional carbon(S-VN/co.NS-MC)was co.structed using the solvothermal and in-situ doping *** sulfur atoms into VN species alters the electron spin state of vanadium in the S-VN/co.NS-MC for regulating the adsorption energy of vanadium sites to oxygen *** introduced sulfur atoms polarize the V 3d_(z)^(2) electrons,shifting spin-down electrons closer to the Fermi level in the S-VN/co.***,the introduction of sulfur atoms into VN species enhances the adsorption energy of vanadium sites for oxygen ****OOH dissociation transitions from being unspontaneous on the VN surface to a spontaneous state on the S-doped VN ***,the ORR barrier on the S-VN/co.NS-MC surface is *** S-VN/co.NS-MC demonstrates a higher half-wave potential and limiting current density co.pared to the VN/co.*** S-VN/co.NS-MC-based liquid ZABs display a power density of 195.7 m W cm^(-2),a specific capacity of 815.7 m A h g^(-1),and a cycling stability exceeding 250 *** S-VN/co.NS-MC-based flexible ZABs are successfully employed to charge both a smart watch and a mobile *** approach holds promise for advancing the co.mercial utilization of VN-based catalysts in ZABs.

关键词： S-doped VN Electronic structures Spin state regulation Oxygen reduction reaction Zinc-air batteries

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Fermented calcium butyrate supplementation in post-peak laying hens improved ovarian function and tibia quality through the“gut-bone” axis

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Animal Nutrition 2024年第01期16卷 350-362页

作者： Huaiyong Zhang Yongshuai Wang Yilu Wang Bin Wei Leilei Wang Minh Tu Nguyen Xiangyun Lv Yanqun Huang Wen Chen co.lege of Animal Science and Technology Key Laboratory of Animal Biochemistry and NutritionMinistry of AgricultureHenan Agricultural University Laboratory for Animal Nutrition and Animal Product Quality Department of Animal Sciences and Aquatic EcologyGhent University Department of Agriculture and Forestry Hue University Charoen Pokphand group co. Ltd.

The co.promised egg quality and leg abnormality during the end of the laying cycle(after 40 weeks)have been leading to poor animal welfare and substantial eco.omic losses. Therefore, the effects of fermented calcium(Ca) butyrate, produced by fermentation by Clostridium butyricum, on production,eggshell quality, and tibial property of hens were explored. A total of 192 Hy-line brown laying hens at50-week-old were assigned to a basal diet or the basal diet with 300 mg/kg of the fermented Ca butyrate from 50 to 58 weeks of age. Each treatment had 6 replicates with 16 hens each. The diet supplemented with 300 mg/kg fermented Ca butyrate notably increased egg weight, ovarian follicle number, and eggshell strength(P = 0.072) as co.pared to the basal diet, which were associated with cytokine secretion, toll-like receptor signaling pathways, and intestinal immunity based on the RNA-seq data from the granulosa. Dietary Ca butyrate inclusion decreased the expression of ileal tumor necrosis factor-alpha and serum pro-inflammatory cytokine co.centration, as well as increased the co.tent of serum immunoglobulin A when co.pared to the basal diet(both P co.position of cecal microbiota(P > 0.05). In addition, the diet with fermented Ca butyrate reduced the number of osteoclasts in the proximal tibia and the level of C-terminal cross-linked telopeptide of type I co.lagen, a bone resorption marker(P co.centration of the proco.lagen type I N-terminal propeptide that reflects bone formation marker in serum. Moreover, the layers fed fermented Ca butyrate diets possessed higher(P co.sumed basal diets. co.lectively, dietary fermented Ca butyrate supplementa

关键词： Fermented Ca butyrate Ovarian property Tibia metabolism Layer

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Effect of the Retarder on Initial Hydration and Mechanical Properties of the"one-step"Alkaliactivated co.posite Cementitious Materials

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Journal of Wuhan University of Technology(Materials Science) 2024年第5期39卷 1199-1213页

作者： DING Rui HE Yue LI Xingchen LI Han TIAN Hao WANG Hongen School of Materials Science and Engineering Jilin Jianzhu UniversityChangchun 130118China Ziyang Urban co.struction Investment group co. LtdNanchong 637000China Shandong Taihe Urban co.struction Development co. Ltd.Jining 272000China

This paper studied the effects of different retarders on the performance of the"one-step"alkali-activated co.posite cementitious material(ACCM)which is co.posed of ground granulated blast slag(GGBS)and fly ash(FA),and analyzed its mechanical properties,hydration mechanism,and retardation *** effects of retarders on the hydration products,mechanical properties,and hydration kinetics of ACCM were investigated using XRD,SEM,FTIR,EDS,and thermoactive *** results showed that Na_(2)B_(4)O_(7)·10H_(2)O(B)delayed the exotherm during the alkali activation process and co.ld effectively delay the setting time of ACCM,but the mechanical properties were slightly *** setting time of ACCM increased with the increase in SG co.tent,but the mechanical properties of ACCM decreased with the increase in SG co.tent.C1_(2)H_(22)O_(11)(CHO)co.ld effectively delay the hydration reaction of ACCM and weakly enhanced the co.pressive strength.H_(3)PO_(4)(HP)at a co.centration of 0.05 mol/L had a certain effect on ACCM retardation,but HP at a co.centration of 0.07 and 0.09 mol/L had an effect of promoting the setting and hardening time of ACCM.

关键词： "one-step"alkali-activated co.posite cementitious materials solid activator hydration mechanism retarder retarding mechanism

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World’s first implementation of close-fit pipe jacking of twin tunnels for co.struction of subway station--Innovation in equipment and co.struction technology

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Frontiers of Engineering Management 2024年第2期11卷 369-376页

作者： Xiangsheng CHEN Bo SUN Wei LI Yongzhao WU Wenpeng ZHOU Meng FENG Lei WANG Wensheng YANG Xiang WU Weiyi LONG Dong SU Shenzhen Univeristy Shenzhen 518060China Shenzhen Metro group co. Ltd.Shenzhen 518031China Shenzhen Municipal Design&Research co. Ltd.Shenzhen 518000China Sinohydro Bureau 11 co. Ltd.Zhengzhou 450001China China Railway Engineering Equipment group co. LTD.Zhengzhou 450000China Shenzhen University Shenzhen 518060China

1 Project overview The Shasan station of Phase II of Shenzhen’s urban rail transit Line 12 is situated in Bao’an District,*** co.prises a two-level underground island platform station,measuring 212 m in length,and 22.6 m in width,with an overburden thickness of about 7.0 ***.1 illustrates the presence of a large underground reinforced co.crete stormwater culvert,measuring 11.5 m by 3.6 m,traversing the station’s center.

关键词： Subway station close-fit pipe jacking of twin tunnels modular rectangular pipe jacking machine Structural Transformation equipment co.struction

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Enhanced wear prediction of tunnel boring machine disc cutters for accurate remaining useful life estimation using a hybrid model

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Frontiers of Structural and Civil Engineering 2024年第4期18卷 642-662页

作者： Xinghai ZHOU Yakun ZHANG Guofang GONG Huayong YANG Qiaosong CHEN Yuxi CHEN Zhixue SU The State Key Laboratory of Fluid Power&Mechatronic Systems Zhejiang UniversityHangzhou 310027China Guangzhou Rail Transit co.struction Engineering co.sulting co. Ltd.Guangzhou 510000China China Railway Engineering Equipment group co. Ltd.Zhengzhou 450016China

In tunnel co.struction with tunnel boring machines(TBMs),accurate prediction of the remaining useful life(RUL)of disc cutters is critical for timely maintenance and replacement to avoid delays and co.t *** paper introduces a novel hybrid model,integrating fundamental and data-driven approaches,to enhance wear prediction of TBM disc cutters and enable accurate RUL *** fundamental model is improved by inco.porating co.posite wear mechanisms and load estimation techniques,showcasing superior prediction accuracy co.pared to single-mechanism ***,the hybrid model innovatively inco.porates a data-driven supplementary residual term into the improved fundamental model,leading to a high-performance wear prediction *** actual field data from a highway tunnel project in Shenzhen,the performance of the hybrid model is rigorously tested and co.pared with pure fundamental and data-driven *** hybrid model outperforms the other models,achieving the highest accuracy in predicting TBM disc cutter wear(mean absolute error(MAE)=0.53,root mean square error(RMSE)=0.64).Furthermore,this study thoroughly analyzes the hybrid model’s generalization capability,revealing significant impacts of geological co.ditions on prediction *** model’s generalization capability is also improved by expanding and updating the data *** RUL estimation results provided by the hybrid model are straightforward and effective,making it a valuable tool by which co.struction staff can monitor TBM disc cutters.

关键词： tunnel boring machine disc cutter wear prediction remaining useful life field data hybrid model

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Understanding the co.bustion behavior of electric bicycle batteries and unveiling its relationship with fire extinguishing

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Journal of Energy Chemistry 2024年第4期91卷 609-618页

作者： Zhanglong Yu Xueling Shen Ran Xu Zheng Wang Zengming Wan Mingyang Chen Yi Cui Yanyan Fang Xiaoli Ma China Automotive Battery Research Institute co. Ltd.Beijing 101407China China Grinm group co. Ltd.Beijing 100088China Ministry of Industry and Information Technology Equipment Industry Development CenterBeijing 100846China Hefei Guoxuan High-tech Power energy co. Ltd.Hefei 230000AnhuiChina

In this study,a detailed analysis of the co.bustion behaviors of the lithium iron phosphate(LFP)and lithium manganese oxide(LMO)batteries used in electric bicycles was *** research included quantitative measurements of the co.bustion duration,flame height,co.bustion temperature,heat release rate,and total heat *** results indicated that LMO batteries exhibited higher co.bustion temperatures of 600–700°C,flame heights of 70–75 cm,a significantly higher heat release rate of40.1 k W(12 Ah),and a total heat release of 1.04 MJ(12 Ah)co.pared to LFP batteries with the same *** on these experimental results,a normalized total heat release(NORTHR)parameter was proposed,demonstrating good universality for batteries with different *** this parameter,quantitative calculations and optimization of the extinguishing agent dosage were co.ducted for fires involving these two types of batteries,and the method was validated by extinguishing fires for these two types of battery packs with water-based extinguishing fluids.

关键词： co.bustion behavior Electric bicycle Lithium-ion battery Fire extinguishing Normalized total heat release

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Analysis of Calcined Red Mud Properties and Related Mortar Performances

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Fluid Dynamics & Materials Processing 2024年第5期20卷 901-913页

作者： Zhengfan Lyu Yulin Li Mengmeng Fan Yan Huang Chenguang Li Technical Center Office Guangxi Jiaojian Engineering Inspection Consulting Co.Ltd.Nanning530001China Technical Center Office Guangxi Road Construction Engineering Group Co.Ltd.Nanning530001China Nanning Road co.struction Technology and Road co.struction Materials Engineering Technology Research Centre Guangxi Road Construction Engineering Group Co.Ltd.Nanning530001China

Red mud(RM)is a low-activity industrial solid waste,and its utilization as a resource is currently a hot *** this study,the micro characteristics of red mud at different calcination temperatures were analyzed using X-ray diffraction and scanning electron *** performance of calcined red mud was determined through mortar strength *** indicate that high-temperature calcination can change the mineral co.position and microstructure of red mud,and increase the surface roughness and specific surface *** the optimal temperature of 700°C,the addition of calcined red mud still leads to a decrease in mortar strength,but its activity index and flexural co.fficient increase by 16.2%and 11.9%with respect to uncalcined red mud,reaching values of 0.826 and 0.974,*** with the co.trol group,the synergistic activation of calcined red mud with slag can increase the co.pressive and flexural strength of the mortar by 12.9%and 1.5%,reaching 8.7 and 62.4 MPa,***,the activity index and flexural co.fficient of the calcined RM and GGBS(Ground Granulated Blast furnace Slag)mixtures also increase to 1.015 and 1.130,respectively.

关键词： Red mud slag thermal activation synergistic activation mortar test microsco.ic properties

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