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Separation of the ionospheric and thermospheric contributions in the data from the Triple Ionosophere Photo Meter onboard the Feng-Yun 3E satellite

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Science China Earth Sciences 2025年第1期68卷 172-184页

作者： Fang JIANG Tian MAO Jin-Song WANG Xiu-Qing HU Xiao-Xin ZHANG Liping FU Nan JIA Tianfang WANG National Space Science center Chinese Academy of Sciences Beijing Key Laboratory of Space Environment Exploration Key Laboratory of environmental Space Situation Awareness Technology National Satellite meteorological center China Meteorological Administration

The Triple Ionosphere Photo Meter （TRIPM） is a far ultraviolet nadir-view photometer that is onboard the secondgeneration,polar-orbiting Chinese meteorological satellite Feng-Yun 3E （FY-3E）,which was launched on July 5,*** has three channels,and each is used to measure different types of emissions:（1） 135.6 nm airglow produced by the recombination of the O+ions and electrons in the absence of sunlight （nighttime channel）;（2） 135.6 nm airglow from the OI when sunlight is present （daytime/dusk-dawn 135.6 nm channel）;and （3） Airglow in the N2LBH of the TRIPM （daytime/dusk-dawn N2LBH channel）.FY-3E is a satellite operating in the early morning ***,the data are mostly distributed on the dawndusk side or at times when the solar zenith angle is relatively *** this study,combined with simulation calculations,the data are *** further explore the application value of the data products,a model is used to separate the ionospheric radiative recombination contribution from the thermosphere photoelectron impact excitation contribution in the data from the daytime/dusk-dawn 135.6 nm *** approach not only improves the accuracy of O/N2derived from the 135.6 nm channel and N2LBH channel but also provides the ionospheric 135.6 nm radiance at the same time as the *** results show that the 135.6 nm radiance originating from the combination of O+and electrons extracted from the measurement data exhibits similar equatorial anomaly peak structure characteristics and seasonal variations as the corresponding GPS total electron content （TEC） *** the other hand,the separated 135.6 nm radiance generated from the thermosphere photoelectron collision excitation does not contain radiative recombination contributions;thus,the ionosphere influence is greatly avoided when the O/N2is obtained.

关键词： Far ultraviolet 135.6 nm emission intensity Photoelectron impact excitation Radiative recombination excitation

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Spatiotemporal characteristics and influencing factors of vegetation water use efficiency on the Tibetan Plateau in 2001–2020

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Journal of Geographical Sciences 2025年第1期35卷 39-64页

作者： HE Chenyang WANG Yanjiao YAN Feng LU Qi School of Ecological and environmental Science East China Normal University Institute of Ecological Conservation and Restoration Chinese Academy of Forestry National Climate center China Meteorological Administration

Water use efficiency （WUE）,as a pivotal indicator of the coupling degree within the carbon–water cycle of ecosystems,holds considerable importance in assessment of the carbon–water balance within terrestrial ***,in the context of global warming,WUE evolution and its primary drivers on the Tibetan Plateau remain *** study employed the ensemble empirical mode decomposition method and the random forest algorithm to decipher the nonlinear trends and drivers of WUE on the Tibetan Plateau in 2001–*** indicated an annual mean WUE of 0.8088 gC/mm·m2across the plateau,with a spatial gradient reflecting decrease from the southeast toward the *** manifesting monotonous trends of increase or decrease in WUE accounted for 23.64%and 9.69%of the total,***,66.67%of the region exhibited trend reversals,i.e.,39.94%of the area of the Tibetan Plateau showed transition from a trend of increase to a trend of decrease,and 26.73%of the area demonstrated a shift from a trend of decrease to a trend of *** factors accounted for 70.79%of the variability in *** leaf area index and temperature served as the major driving forces of WUE variation.

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Nano high-entropy oxide cathode with enhanced stability for direct borohydride fuel cells

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Journal of Energy Chemistry 2025年第1期100卷 309-316页

作者： Lei Zhang Lingfeng Kuang Lianke Zhang Wen Chu Haiying Qin Jing Zhang Junjing He Hualiang Ni Hongzhong Chi New Energy Materials Research center College of Materials and Environmental Engineering Hangzhou Dianzi University School of Materials Science and Engineering Zhejiang University Key Laboratory of MEMS of Ministry of Education School of Integrated Circuits Southeast University

High-entropy materials have become high-activity electrocatalysis owing to their high-entropy effect and multiple active ***,we synthesize a series of carbon-supported nano high-entropy oxides（HEOs/C）,specifically （PtFeCoNiCu）O/C,using a carbothermal shock （CTS） method for application as a cathode catalyst in direct borohydride fuel cells （DBFCs）.The microstructure of the prepared catalysts was characterized by X-ray photoelectron spectroscopy,X-ray absorption fine structure,and transmission electron *** prepared （PtFeCoNiCu）O/C,with particle sizes ranging from 2 to 4 nm,demonstrates 3.94 transferred electrons towards the oxygen reduction reaction in an alkaline environment,resulting in a minimal H2O2yield of 2.6%.Additionally,it exhibits a Tafel slope of 61 mV dec-1,surpassing that of commercial Pt/C (82 mV dec-1).Furthermore,after 40,000 cycles of cyclic voltammetry（CV） testing,the half-wave potential of （PtFeCoNiCu）O/C shows a positive shift of 3 mV,with no notable decline in the limiting current *** （PtFeCoNiCu）O/C is used as a cathode catalyst in DBFCs,the DBFC achieves a maximum power density of 441 mW cm-2at 60°C and sustains a cell voltage of approximately 0.73 V after 52 h at 30°*** findings confirm that HEO/C is a promising cathode catalyst for DBFCs.

关键词： Direct borohydride fuel cells (DBFC)

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Interannual variability of boreal summer intraseasonal oscillation over the northwestern Pacific influenced by the Pacific Meridional Mode

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Atmospheric and Oceanic Science Letters 2025年第1期18卷 6-11页

作者： Haoyu Zhou Pang-Chi Hsu Lin Chen Yitian Qian Key Laboratory of meteorological Disaster Ministry of Education/Joint International Research Laboratory of Climate and Environmental Change/Collaborative Innovation Center on Forecast and Evaluation of Meteorological DisastersNanjing University of Information Science and TechnologyNanjingChina

During the boreal summer,intraseasonal oscillations exhibit significant interannual variations in intensity over two key regions:the central-western equatorial Pacific(5°S-5°N,150°E-150°W)and the subtropical Northwestern Pacific(10°-20°N,130°E-175°W).The former is well-documented and considered to be influenced by the ENSO,while the latter has received comparatively less attention and is likely influenced by the Pacific Meridional Mode(PMM),as suggested by partial correlation analysis *** elucidate the physical processes responsible for the enhanced(weakened)intraseasonal convection over the subtropical northwestern Pacific during warm(cold)PMM years,the authors employed a moisture budget *** findings reveal that during warm PMM years,there is an increase in summer-mean moisture over the subtropical northwestern *** increase interacts with intensified vertical motion perturbations in the region,leading to greater vertical moisture advection in the lower troposphere and consequently resulting in convective *** a process is pivotal in amplifying intraseasonal convection *** observational findings were further verified by model experiments forced by PMM-like sea surface temperature patterns.

关键词： Boreal summer intraseasonal oscillation Interannual variability Pacific Meridional Mode Moisture budget analysis

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Sulfolane‑Based Flame‑Retardant Electrolyte for High‑Voltage Sodium‑Ion Batteries

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Nano-Micro Letters 2025年第2期17卷 498-516页

作者： Xuanlong He Jie Peng Qingyun Lin Meng Li Weibin Chen Pei Liu Tao Huang Zhencheng Huang Yuying Liu Jiaojiao Deng Shenghua Ye Xuming Yang Xiangzhong Ren Xiaoping Ouyang Jianhong Liu Biwei Xiao Jiangtao Hu Qianling Zhang Graphene Composite Research center College of Chemistry and Environmental EngineeringShenzhen UniversityShenzhen 518060People’s Republic of China center of Electron Microscopy State Key Laboratory of Silicon and Advanced Semiconductor MaterialsSchool of Materials Science and EngineeringZhejiang UniversityHangzhou 310027People’s Republic of China GRINM(Guangdong)Research Institute for Advanced Materials and Technology FoshanGuangdong 528051People’s Republic of China College of Energy Engineering Zhejiang UniversityHangzhouZhejiang 310027People’s Republic of China School of Materials Science and Engineering Xiangtan UniversityXiangtan 411105People’s Republic of China Shenzhen Eigen-Equation Graphene Technology Co.Ltd Shenzhen 518000People’s Republic of China

Sodium-ion batteries hold great promise as next-generation energy storage ***,the high instability of the electrode/electrolyte interphase during cycling has seriously hindered the development of *** particular,an unstable cathode–electrolyte interphase(CEI)leads to successive electrolyte side reactions,transition metal leaching and rapid capacity decay,which tends to be exacerbated under high-voltage ***,constructing dense and stable CEIs are crucial for high-performance *** work reports localized high-concentration electrolyte by incorporating a highly oxidation-resistant sulfolane solvent with non-solvent diluent 1H,1H,5H-octafluoropentyl-1,1,2,2-tetrafluoroethyl ether,which exhibited excellent oxidative stability and was able to form thin,dense and homogeneous *** excellent CEI enabled the O3-type layered oxide cathode NaNi_(1/3)Mn_(1/3)Fe_(1/3)O_(2)(NaNMF)to achieve stable cycling,with a capacity retention of 79.48%after 300 cycles at 1 C and 81.15%after 400 cycles at 2 C with a high charging voltage of 4.2 *** addition,its nonflammable nature enhances the safety of *** work provides a viable pathway for the application of sulfolane-based electrolytes on SIBs and the design of next-generation high-voltage electrolytes.

关键词： Sodium-ion batteries Sulfolane-based electrolyte High voltage Layered oxide cathode Flame retardant

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Effect of Urbanization on the Urban Meteorology and Air Pollution in hangzhou

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Journal of meteorological Research 2015年第6期29卷 950-965页

作者：刘红年马万里钱俊龙蔡菊珍叶贤满李佳慧王学远 School of Atmospheric Sciences Nanjing University hangzhou environmental meteorological center Zhejiang Climate center hangzhou environmental Monitoring Central Station

Urbanization has a substantial effect on urban *** can alter the atmospheric diffusion capability in urban areas and therefore affect pollutant *** study the effects of hangzhou’s urban development in most recent decade on its urban meteorological characteristics and pollutant diffusion,90 weather cases were simulated,covering 9 weather types,with the Nanjing University City Air Quality Prediction System and high-resolution surface-type data and urban construction data for 2000 and *** results show that the most recent decade of urban development in hangzhou substantially affected its urban ***,the average urban wind speed decreased by 1.1 m s-1;the average intensity of the heat island increased by 0.5℃;and the average urban relative humidity decreased by 9.7%.Based on one case for each of the nine weather types,the impact of urbanization on air pollution diffusion was investigated,revealing that the changes in the meteorological environment decreased the urban atmosphere’s diffusion capability,and therefore increased urban pollutant *** instance,the urban nitrogen oxides concentration increased by 2.1 μg m-3 on average;the fine particulate matter（diameter of 2.5 μm or less;PM2.5） pollution concentration increased by 2.3 μg m-3 on average;in highly urbanized areas,the PM2.5concentration increased by 30 μg m-3 and average visibility decreased by 0.2 km,with a maximum decrease of 1 km;the average number of daily hours of haze increased by 0.46 h;and the haze height lifted by 100-300 *** ＂self-cleaning time＂ of pollutants increased by an average of 1.5 h.

关键词： hangzhou urbanization atmospheric environment haze

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Impact of meteorological conditions on a nine-day particulate matter pollution event observed in December 2013,Shanghai,China

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Particuology 2015年第3期13卷 69-79页

作者： Jianming Xu Fengxia Yan Ying Xie Fengyun Wang Jianbin Wu Qingyan Fu Shanghai meteorological Bureau meteorological center of Traffic Management Bureau of East China Shanghai environmental Monitoring center

A severe particulate matter pollution event occurred in Shanghai from 1 to 9 December 2013. The mean hourly mass concentrations of PM2.5 and PM10 were 211.9 and 249.0 μg/m3, respectively. Reanalysis data, in situ, and remote-sensing measurements were used to examine the impacts of meteorological conditions on this event. It was found that the synoptic pattern of weak pressure, the reduced planetary boundary layer height, and the passage of two cold fronts were key factors causing the event. Four stages were identified during this event based on the evolution of its PM2.5 levels and weather conditions. The highest concentration of PM2.5 （602 μg/m3） was observed in stage 3. High PM2.5 concentrations were closely associated with a low local ventilation index, with an average of 505 m2/s, as well as with the influx of pollutants from upstream, transported by the cold fronts.

关键词： Particulate matterPM2.5Pollution eventPlanetary boundary layerCold frontUrban air pollution

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Seasonal variations and size distributions of water-soluble ions in atmospheric aerosols in Beijing, 2012

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Journal of environmental Sciences 2015年第8期27卷 197-205页

作者： Yongjie Yang Rui Zhou Jianjun Wu Yue Yu Zhiqiang Ma Lejian Zhang Yi'an Di National Research center for environmental Analysis and Measurement Jiangsu Institute of meteorological Sciences Beijing Urban meteorological Engineering Technology Research center meteorological Observation center China Meteorological Administration

The characteristics of water-soluble ions in airborne particulate matter in Beijing were investigated using ion chromatography. The results showed that the total concentrations of ions were 83.7 ± 48.9 μg/m3 in spring, 54.0 ± 17.0 μg/m3 in summer, 54.1 ± 42.9 μg/m3 in autumn, and 88.8 ± 47.7 μg/m3 in winter, respectively. Furthermore, out of all the ions, NO3-,SO42-and NH4＋accounted for 81.2% in spring, 78.5% in summer, 74.6% in autumn, and 76.3%in winter. Mg2＋and Ca2＋were mainly associated with coarse particles, with a peak that ranged from 5.8 to 9.0 μm. Na＋, NH4＋and Cl-had a multi-mode distribution with peaks that ranged from 0.43 to 1.1 μm and 4.7 to 9.0 μm. K＋, NO3-, and SO42-were mainly associated with fine particles, with a peak that ranged from 0.65 to 2.1 μm. The concentrations of Na＋, K＋,Mg2＋, Ca2＋, NH4＋, Cl-, NO3-and SO42-were 2.69, 2.32, 1.01, 4.84, 16.9, 11.8, 42.0, and 44.1 μg/m3 in particulate matter（PM） on foggy days, respectively, which were 1.4 to 7.3 times higher than those on clear days. The concentrations of these ions were 2.40, 1.66, 0.92, 4.95, 17.5,7.00, 32.6, and 34.7 μg/m3 in PM on hazy days, respectively, which were 1.2–5.7 times higher than those on clear days.

关键词： Water-soluble ions Size distribution Hazy day Foggy day Beijing

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The comparison of ensemble or deterministic dispersion modeling on global dispersion during Fukushima Dai-ichi nuclear accident

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Science China Earth Sciences 2015年第3期58卷 356-370页

作者： SHENG Li SONG ZhenXin HU JiangKai Lü Kai TONG Hua LI Bing QIAO QingDang National meteorological center China Meteorological Administration Nuclear and Radiation Safety center Ministry of Environmental Protection of the People's Republic of China

Ensemble forcasting,originally developed for weather prediction,is lately being extended to atmospheric dispersion applications,which is a new,effective methodology for improving the atmospheric dispersion numerical *** March 2011,due to the massive 9.0 earthquakes and ensuing tsunami that struck off the northern coast of the island of Honshu,the Fukushima Nuclear Plant I had the substantial leak of radioactive materials into surrounding environment and *** aim at the global dispersion modeling of atmospheric radionuclides from Fukushima Nuclear Accident,this paper presents two approaches of atmospheric dispersion forecasting:ensemble dispersion modeling(EDM) and deterministic dispersion modeling(DDM),conducts the globally dispersion modeling cases for Fukushima nuclear accident,and analyzes and evaluates the simulation results using observation *** this paper,EDM includes three different perturbation methods:meteorological perturbation method,turbulence perturbation method,and physical parameterization ensemble forecasting *** simulation results show that the trajectories from EDM have a better performance,which is in better agreement with the atmospheric circulation and observation data; the spread from DDM is slower and not as far as ***,the results from EDM display a better performance in the modeling of transport from Japan to China East Sea on April *** reasons for these results are:the techniques of MET and TUR are performed by adding perturbations on mean wind and turbulent velocity,respectively; the various different flow fields will result in far spreading in horizontal and the simulation results closer to observation; PHY is performed by using different diffusion physical parameterizations and produces the perturbations on vertical wind,which results the spreading in smaller range and discontinuous in ***,the comparative analysis between modeling results and observation data shows that all cases r

关键词： ensemble dispersion modeling deterministic dispersion modeling atmospheric dispersion Fukushima nuclear accident

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FY-4A/GIIRS Temperature Validation in Winter and Application to Cold Wave Monitoring

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Journal of meteorological Research 2022年第4期36卷 658-676页

作者： Suling REN Jianying JIANG Xiang FANG Hui LIU Zhiqiang CAO Key Laboratory of Radiometric Calibration and Validation for environmental Satellites Innovation Center for Fengyun Meteorological Satellite(FYSIC)National Satellite Meteorological CenterChina Meteorological AdministrationBeijing 100081 National meteorological center China Meteorological AdministrationBeijing 100081

In order to improve the operational application ability of the Fengyun-4A(FY-4A)new sounding dataset,in this paper,validation of the FY-4A Geosynchronous Interferometric Infrared Sounder(FY-4A/GIIRS)temperature was carried out using the balloon sounding temperature from meteorological sounding *** than 350,000 samples were obtained through time–space matching,and the results show that the FY-4A/GIIRS temperature mean bias(MB)is 0.07°C,the mean absolute error(MAE)is 1.80°C,the root-mean-square error(RMSE)is 2.546°C,and the correlation coefficient(RR)is *** FY-4A/GIIRS temperature error is relatively larger in the upper and lower troposphere,and relatively smaller in the middle troposphere;that is,the temperature at 500 hPa is better than that at 850 *** temporal variation is smaller in the upper and middle troposphere than in the lower *** reconstruction of missing data of FY-4A/GIIRS temperature in cloudy areas is also carried out and the results are *** spatial distribution of reconstructed FY-4A/GIIRS temperature and the fifth generation ECMWF reanalysis(ERA5)data is consistent and completely retains the minimum temperature center with high precision of FY-4A/*** are more detailed characteristics of intensity and position at the cold center than that of the reanalysis ***,an operational satellite retrieval temperature product with time–space continuity and high accuracy is *** reconstructed FY-4A/GIIRS temperature is used to monitor a strong cold wave event in November *** results show that the product effectively monitors the movement and intensity of cold air activities,and it also has good indication for the phase transition of rain and snow triggered by cold wave.

关键词： Fengyun-4A Geosynchronous Interferometric Infrared Sounder(FY-4A/GIIRS) temperature profile,cold wave Cressman interpolation algorithm

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