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Study on crustal thickness and the prediction of prolific depressions:the Bohai Basin as an example

Acta Oceanologica Sinica 2024年第4期43卷 92-104页

作者： Mengke Cai Gongcheng Zhang Wanyin Wang Dingding Wang College of Geological Engineering and Geomatics Chang’an UniversityXi’an 710054China China National Offshore Oil Corporation(cnooc)Research Institute Co. Ltd.Beijing 100028China Key Laboratory of Marine Geology and Environment Chinese Academy of SciencesQingdao 266071China National Engineering Research Center of Offshore Oil and Gas Exploration Beijing 100028China Department of Earth Environment and Resources SciencesUniversity of Naples FedericoⅡNaples 80138Italy

The deep crustal structure is closely related to oil and gas *** the oil and gas enrichment of depressions based on the Moho depth and crustal thickness is a promising research topic with significant implications for guiding exploration in petroliferous *** this study,seismic data were used as a constraint on the use of satellite gravity anomaly inversion to obtain the distribution of Moho depth and crustal thickness in the Bohai *** factors were calculated to analyze the differential distribution of deep crustal structural *** indicators,including the minimum Moho depth,minimum crustal thickness,sum of Moho stretching factors,and sum of crustal stretching factors,were *** component analysis was applied to reduce the dimensionality of the multi-indicator system and obtain an oil and gas enrichment score for quantitative prediction of favorable prolific *** deviation between the inverted Moho depth and seismic constraints was small;thus,the data effectively reflect the variations in the characteristics of each *** analysis revealed significant statistical features related to the minimum Moho depth/crustal thickness and the sum of Moho/crustal stretching factors associated with prolific *** on the oil and gas enrichment score,the depressions were classified into four categories related to their different deep crustal structural *** active ClassⅠ,ClassⅡ,and ClassⅢdepressions are predicted to be favorable prolific *** study expands the research on quantitatively predicting favorable prolific depressions in the Bohai Basin using the deep crustal structure and can contribute to reducing production costs and improving exploration efficiency in future explorations.

关键词： Bohai Basin satellite gravity anomaly deep crustal structure Moho depth crustal thickness favorable prolific depression

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Genesis and Accumulation of Paleo-Oil Reservoir in Dabei Area,Kuqa Depression,Northwest China:Implications for Tight-Gas Accumulation

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Journal of Earth Science 2024年第2期35卷 655-665页

作者： Fujie Jiang Xiao Chen Pengwei Wang Xinghe Shao Haijun Yang State Energy Center for Shale Oil Research and Development Beijing102206China National Key Laboratory of Oil and Gas Resources and Engineering Beijing102249China College of Geosciences China University of PetroleumBeijing102249China cnooc International ltd. Beijing100027China Research Institute of Petroleum Exploration&Production SINOPECBeijing100083China Research Institute of Petroleum Exploration and Development Tarim OilfieldPetroChinaKorla841000China

Paleo-oil reservoir is of great importance to understand hydrocarbon enrichment mechanism and hydrocarbon exploration potential,but is yet poorly investigated in Kuqa *** occurrence of the paleo-oil reservoir in Dabei area was proved by quantitative grain fluorescence(QGF)and fluid inclusion *** history of the paleo-oil reservoir was reconstructed through:(1)oil-source correlation;(2)time coupling of source rock maturation,porosity evolution and migration *** impact of paleo-oil reservoir on tight-gas accumulation was consequently *** suggest that considerable oil was accumulated in the K_(1)bs reservoir with paleo oil-water contact in Dabei 2 Well and Dabei 201 Well at 5800 and 6040 m,*** oil was primarily sourced from Triassic source rocks with Jurassic source rocks of secondary importance,which was at oil generation window(0.7%–1.1%Ro)during 9–6 and 7.5–5 Ma,*** occurrence of K_(1)bs tight reservoir(porosity<12%)was about 25 Ma,while faults and associated fractures at Kelasue structural belt were developed approximately from 8 to 3.5 ***,the tight oil accumulation was formed during 8–5 *** paleo-oil reservoir in Dabei 1 gas field was destroyed by the evaporation fractionation in later stage.

关键词： Paleo-oil reservoir Dabei area Kuqa Depression Northwest China petroleum geology

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Unraveling the coordination behavior and transformation mechanism of Cr^(3+) in Fe–Cr redox flow battery electrolytes

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Materials Reports(Energy) 2024年第2期4卷 54-63页

作者： Xiaojun Zhao Xinwei Niu Xinyuan Liu Chongchong Wu Xinyu Duan Zhiqi Ma Yan Xu Hao Li Weijie Yang Department of Electrical Engineering North China Electric Power UniversityBaoding071003PR China Department of Energy Power and Mechanical Engineering North China Electric Power UniversityBaoding071003PR China cnooc Institute of Chemicals&Advanced Materials Beijing102200PR China Shanghai LongVault Energy Technology Co. Ltd.Shanghai201615PR China Advanced Institute for Materials Research(WPI-AIMR) Tohoku UniversitySendai980-8577Japan

Currently,the iron chromium redox flow battery(ICRFB)has become a research hotspot in the energy storage field owing to its low cost and ***,the activity of electrolyte is still ambiguous due to its complicated solution ***,we performed a pioneering investigation on the coordination behavior and transformation mechanism of Cr^(3+)in electrolyte and prediction of impurity ions impact through quantum chemistry *** on the structure and symmetry of electrostatic potential distribution,the activity of different Cr^(3+)complex ions is confirmed as[Cr(H2O)5Cl]^(2+)>[Cr(H2O)4Cl2]+>[Cr(H2O)6]^(3+).The transformation mechanism between[Cr(H2O)6]^(3+)and[Cr(H2O)5Cl]^(2+)is *** find the metal impurity ions(especially Mg^(2+))can exacerbate the electrolyte deactivation by reducing the transformation energy barrier from[Cr(H2O)5Cl]^(2+)(24.38 kcal mol^(−1))to[Cr(H2O)6]^(3+)(16.23 kcal mol^(−1)).The solvent radial distribution and mean square displacement in different solvent environments are discussed and we conclude that the coordination configuration limits the diffusivity of Cr^(3+).This work provides new insights into the activity of electrolyte,laying a fundamental sense for the electrolyte in ICRFB.

关键词： Fe-Cr redox flow battery Coordination Electrolyte Quantum chemistry computation

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Dissolution mechanism of a deep-buried sandstone reservoir in a deep water area:A case study from Baiyun Sag,Zhujiang River(Pearl River)Mouth Basin

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Acta Oceanologica Sinica 2023年第3期42卷 151-166页

作者： Jihua Liao Keqiang Wu Lianqiao Xiong Jingzhou Zhao Xin Li Chunyu Zhang China National Offshore Oil Corporation(cnooc)Research Institute Co. Ltd.Beijing 100028China hainan branch of China National Offshore Oil Corporation(cnooc)Co. Ltd.Haikou 570311China School of Earth Sciences and Engineering Xi’an Shiyou University Xi’an Petroleum UniversityXi’an 710065China

Dissolution mechanism and favorable reservoir distribution prediction are the key problems restricting oil and gas exploration in deep-buried *** this paper,the Enping Formation and Zhuhai Formation in Baiyun Sag of South China Sea was taken as a *** on the thin section,scanning electron microscopy,X-ray diffraction,porosity/permeability measurement,and mercury injection,influencing factors of dissolution were examined,and a dissolution model was ***,high-quality reservoirs were predicted temporally and *** results show that dissolved pores constituted the main space of the Paleogene sandstone *** primarily occurred in the coarse-and medium-grained sandstones in the subaerial and subaqueous distributary channels,while dissolution was limited in fine-grained sandstones and inequigranular *** main dissolved minerals were feldspar,tuffaceous matrix,and diagenetic *** of feldspar and illitization of kaolinite are the main dissolution pathways,but they occur at various depths and temperatures with different geothermal *** is controlled by four factors,in terms of depositional facies,source rock evolution,overpressure,and fault activities,which co-acted at the period of 23.8–13.8 Ma,and resulted into strong ***,based on these factors,high-quality reservoirs of the Enping and Zhuhai formations are predicted in the northern slope,southwestern step zone,and Liuhua uplift in the Baiyun Sag.

关键词： dissolution mechanism deep-buried reservoir diagenesis evolution reservoir prediction deep water region Baiyun Sag

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Multifractal estimation of NMR T_(2) cut-off value in low-permeability rocks considering spectrum kurtosis: SMOTE-based oversampling integrated with machine learning

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Petroleum Science 2023年第6期20卷 3411-3427页

作者： Xiao-Jun Chen Rui-Xue Zhang Xiao-Bo Zhao Jun-Wei Yang Zhang-Jian Lan Cheng-Fei Luo Jian-Chao Cai MOE Key Laboratory of Tectonics and Petroleum Resources Wuhan430074HubeiChina Department of Chemical Engineering and Analytical Science The University of ManchesterManchesterM139PLUK Jianghan Oilfied SINOPECQianjiang430063HubeiChina hainan branch of cnooc ltd Haikou570311HainanChina cnooc EnerTech-Drilling&Production Co.cnooc Central Laboratory(Zhanjiang) Zhanjiang524057GuangdongChina National Key Laboratory of Petroleum Resources and Engineering China University of PetroleumBeijing102249China

The transverse relaxation time (T_(2)) cut-off value plays a crucial role in nuclear magnetic resonance for identifying movable and immovable boundaries, evaluating permeability, and determining fluid saturation in petrophysical characterization of petroleum reservoirs. This study focuses on the systematic analysis of T_(2) spectra and T_(2) cut-off values in low-permeability reservoir rocks. Analysis of 36 low-permeability cores revealed a wide distribution of T_(2) cut-off values, ranging from 7 to 50 ms. Additionally, the T_(2) spectra exhibited multimodal characteristics, predominantly displaying unimodal and bimodal morphologies, with a few trimodal morphologies, which are inherently influenced by different pore types. Fractal characteristics of pore structure in fully water-saturated cores were captured through the T_(2) spectra, which were calculated using generalized fractal and multifractal theories. To augment the limited dataset of 36 cores, the synthetic minority oversampling technique was employed. Models for evaluating the T_(2) cut-off value were separately developed based on the classified T_(2) spectra, considering the number of peaks, and utilizing generalized fractal dimensions at the weight 0. The primary objective of this work is to gain insights into the relationship between the kurtosis of the T_(2) spectrum and pore types, as well as to predict the T_(2) cut-off value of low-permeability rocks using machine learning and data augmentation techniques.

关键词： Nuclear magnetic resonance Low-permeability porous media T_(2)cut-off value Fractal and multifractal Data augmentation Machine learning

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Controlling factors on the charging process of oil and gas in the eastern main sub-sag of the Baiyun Sag,Zhujiang River(Pearl River)Mouth Basin

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Acta Oceanologica Sinica 2023年第3期42卷 189-200页

作者： Cong Chen Xiangtao Zhang Guangrong Peng Zulie Long Baojun Liu Xudong Wang Puqiang Zhai Bo Zhang Shenzhen branch of China National Offshore Oil Corporation(cnooc)Co. Ltd.Shenzhen 518054China cnooc Deepwater Development Shenzhen 518054China

The eastern main sub-sag(E-MSS)of the Baiyun Sag was the main zone for gas exploration in the deep-water area of the Zhujiang River(Pearl River)Mouth Basin at its early exploration stage,but the main goal of searching gas in this area was broken through by the successful exploration of the W3-2 and H34B volatile oil reservoirs,which provides a new insight for exploration of the Paleogene oil reservoirs in the ***,it is not clear on the distribution of“gas accumulated in the upper layer,oil accumulated in the lower layer”(Gas_(upper)-Oil_(lower))under the high heat flow,different source-rock beds,multi-stages of oil and gas charge,and multi-fluid phases,and not yet a definite understanding of the genetic relationship and formation mechanism among volatile oil,light oil and condensate gas reservoirs,and the migration and sequential charge model of oil and *** puzzles directly lead to the lack of a clear direction for oil exploration and drilling zone in this *** this work,the PVT fluid phase,the origin of crude oil and condensate,the secondary alteration of oil and gas reservoirs,the evolution sequence of oil and gas formation,the phase state of oil and gas migration,and the configuration of fault activity were analyzed,which established the migration and accumulation model of Gas_(upper)-Oil_(lower)cocontrolled by source and heat,and fractionation controlled by facies in the ***,the fractionation evolution model among common black reservoirs,volatile reservoirs,condensate reservoirs and gas reservoirs is discussed,which proposed that the distribution pattern of Gas_(upper)-Oil_(lower)in the E-MSS is controlled by the generation attribute of oil and gas from source rocks,the difference of thermal evolution,and the fractionation controlled by phases after mixing the oil and ***,we suggest that residual oil reservoirs should be found in the lower strata of the discovered gas reservoirs in the oil-source fault and diapir-devel

关键词： volatile oil oil-oil correlation phase-controlled fractionation sequential charge model Baiyun Sag

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无模板插层-剥离勃姆石合成具有优异稳定性的多孔硅掺杂氧化铝二维纳米片

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Science China Materials 2024年第1期67卷 261-271页

作者：赵振祥杨军王春霖薛岩涛吴浩谢威龙吴萍萍王纯正邢伟汪毅庞春霞庞泉德王晓化南军白鹏阎子峰 State Key Laboratory of Heavy Oil Processing CNPC Key Laboratory of CatalysisCollege of Chemistry and Chemical EngineeringChina University of Petroleum(East China)Qingdao 266580China PetroChina Lanzhou Petrochemical Research Center Lanzhou 730060China Shandong Xinbo Chemical Technology Co. LtdWeifang 262404China Petrochemical Research Institute PetroChina Company LimitedBeijing 100195China cnooc Tianjin Chemical Research and Design Institute Co. LtdTianjin 300131China

高比表面积和大孔容的多孔氧化铝已被广泛应用在各种领域,但不使用有机模板合成多孔氧化铝仍面临巨大挑战.在此,我们报道了基于插层-剥离策略的多孔氧化铝合成方法,利用硅物种削弱勃姆石(氧化铝前体)的层间作用力,从而在不使用有机模板... 详细信息

高比表面积和大孔容的多孔氧化铝已被广泛应用在各种领域,但不使用有机模板合成多孔氧化铝仍面临巨大挑战.在此,我们报道了基于插层-剥离策略的多孔氧化铝合成方法,利用硅物种削弱勃姆石(氧化铝前体)的层间作用力,从而在不使用有机模板的情况下将勃姆石剥离成二维纳米片.该合成过程可放大到3 L,并获得厚度为2 nm的二维纳米片.此外,这些二维纳米片可组装成比表面为542 m^(2)g^(-1)和孔容为2.43 cm^(3)g^(-1)的勃姆石.在不同温度下对二维纳米片进行热/水热处理得到的多孔氧化铝其孔结构优于多数有机模板法合成的氧化铝,并表现出优异的吸附性能.本研究为合成二维勃姆石纳米片和多孔氧化铝材料提供了一种新策略.

关键词：多孔氧化铝纳米片模板合成勃姆石水热处理层间作用插层硅掺杂

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Origin of hydrocarbon fluids and discussion of abnormal carbon isotopic compositions in the Lishui-Jiaojiang Sag,East China Sea Shelf Basin

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Acta Oceanologica Sinica 2023年第3期42卷 76-88页

作者： Jingqi Xu Shanghai branch of China National Offshore Oil Corporation(cnooc)Co. Ltd.Shanghai 200335China

The hydrocarbon gases in the L1 gas field of the Lishui-Jiaojiang Sag have been commonly interpreted to be an accumulation of pure sapropelic-type thermogenic *** this study,chemical components,stable isotopic compositions,and light hydrocarbons were utilized to shed light on the origins of the hydrocarbon fluids in the L1gas *** hydrocarbon fluids in the L1 gas pool are proposed to be a mixture of three unique components:mid-maturity oil from the middle Paleocene coastal marine Lingfeng source rock,oil-associated(late oil window)gas generated from the lower Paleocene lacustrine Yueguifeng source rock,and primary microbial gas from the paralic deposits of the upper Paleocene Mingyuefeng source ***,for the first time,the hydrocarbon gases in the L1 gas pool are diagnosed as mixed oil-associated sapropelic-type gas and microbial gas via four pieces of principal evidence:(1)The abnormal carbon isotopic distributions of all methane homologues from C_(1)(CH_(4)or methane)to C_(5)(C_(5)H_(12)or pentane)shown in the Chung plot;(2)the diagnostic~(13)C-depleted C_(1)compared with the thermogenic sapropelic-type gas model,whileδ^(13)C_(2)(C_(2)H_(6)or ethane)andδ^(13)C_(3)(C_(3)H_(8)or propane)both fit perfectly;(3)the excellent agreement of the calculated carbon isotopic compositions of the pure thermogenic gas with the results of the thermal simulated gas from the type-II1 kerogen-rich Yueguifeng source rock;and(4)the oil-associated gas inferred from various binary genetic diagrams with an abnormally elevated gas oil ***,the natural gases of the L1 gas pool were quantified in this study to comprise approximately 13%microbial gas,nearly 48%oil-associated sapropelic-type gas,and 39%of nonhydrocarbon *** microbial gas is interpreted to have been codeposited and entrained in the humic-kerogen-rich Mingyuefeng Formation under favorable lowtemperature conditions during the late Paleocene-middle *** microbial gas subsequently leaked into the stru

关键词： origin of hydrocarbons carbon isotope hydrogen isotope light hydrocarbon East China Sea Shelf Basin Lishui-Jiaojiang Sag

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Influence of lithospheric thickness distribution on oil and gas basins,China seas and adjacent areas

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Acta Oceanologica Sinica 2024年第4期43卷 1-14页

作者： Jing Ma Wanyin Wang Hermann Zeyen Yimi Zhang Zhongsheng Li Tao He Dingding Wang School of Geology Engineering and Geomatics Key Laboratory of Western China’s Mineral Resources and Geological Engineering of Ministry of EducationChang’an UniversityXi’an 710054China UMR8148 GEOPS CNRS/UniversitéParis-SaclayDépartement des Sciences de la TerreBât.50491405France cnooc Research Institute Co. Ltd.Beijing 100027China Qingdao Institute of marine geology Qingdao 266071China Department of Earth Sciences Memorial University of NewfoundlandSt.John’sNewfoundland AlB3X5Canada University of Naples Federico Ⅱ Department of Earth SciencesNaples80138Italy

The distribution of oil and gas resources is intricately connected to the underlying structure of the ***,investigating the characteristics of lithospheric thickness and its correlation with oil and gas basins is highly *** research utilizes recently enhanced geological–geophysical data,including topographic,geoid,rock layer thickness,variable rock layer density,and interface depth *** the principles of lithospheric isostasy and heat conduction,we compute the laterally varying lithospheric thickness in the China seas and adjacent *** these results,two pivotal parameters for different types of oil and gas basins were statistically analyzed:the minimum lithospheric thickness and the relative fluctuation in lithospheric thickness.A semiquantitative analysis was used to explore the connection between these parameters and the hydrocarbon abundance within the oil and gas *** study unveils distinct variations in lithospheric thickness among basins,with oil and gas rich basins exhibiting a thicker lithosphere in the superimposed basins of central China and a thinner lithosphere in the rift basins of eastern ***,the relative fluctuations in lithospheric thickness in basins demonstrate significant disparities:basins rich in oil and gas often exhibit greater thickness ***,in the offshore basins of China,a conspicuous negative linear correlation is observed between the minimum lithospheric thickness and the relative fluctuation in lithospheric *** study posits that deep-seated thermal upwelling results in lithospheric undulations and extensional thinning in oil and gas ***,sustained deep-seated heat influences sedimentary materials in basins,creating favorable conditions for oil and gas *** insights derived from this study contribute to a quantitative understanding of the intricate relationships between deep lithospheric structures and oil and gas basins.

关键词： China seas and adjacent areas lithospheric thickness oil and gas basins

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Application of seismic sedimentology in characterization of fluvial-deltaic reservoirs in Xihu sag, East China Sea shelf basin

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Petroleum Exploration and Development 2023年第1期50卷 138-151页

作者： LOU Min CAI Hua HE Xianke LIU Yinghui HUANG Xin ZHANG Xianguo LIU Huafeng Shanghai branch of cnooc Shanghai 200335China cnooc Research Institute Co. Ltd.Beijing 100028China China University of Petroleum(East China) Qingdao 266580China

The fluvial-deltaic reservoirs of the Oligocene Huagang Formation in the Xihu sag of the East China Sea shelf basin reflect rapid lateral change in sedimentary facies and poor morphology of conventional slice attributes,which bring difficulties to the reservoir prediction for subsequent exploration and development of lithologic *** traditional seismic sedimentology technology is optimized by applying the characteristic technologies such as frequency-boosting interpretation,inversion-conventional–90°phase shift joint construction of seismic lithologic bodies,nonlinear slices,paleogeomorphology restoration,and multi-attribute fusion,to obtain typical slice attributes,which are conducive to geological form description and sedimentary *** Huagang Formation developed three types of sedimentary bodies:braided river,meandering river and shallow water delta,and the vertical sedimentary evolution was controlled by the mid-term base-level cycle and *** the early–middle stage of the mid-term base-level ascending cycle,braided channel deposits were dominant,and vertical superimposed sand bodies were *** the late stage of the ascending half-cycle and the early stage of the descending half-cycle,meandering river deposits were dominant,and isolated sand bodies were *** the middle–late stage of the descending half-cycle,shallow-water delta deposits were dominant,and migratory medium–thick sand bodies were *** paleogeomorphology controlled the sand body distribution,while non-restricted paleogeomorphology had little effect on the sand body *** on reservoir characterization,the fault sealing type and reservoir updip pinch-out type structural lithological traps are proposed as the main directions for future exploration and development in the Xihu sag.

关键词： East China Sea shelf basin Xihu sag Oligocene Huagang Formation fluvial-deltaic facies reservoir characterization seismic sedimentology

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