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On-demand engineerable visible spectrum by fine control of electrochemical reactions

National science Review 2024年第3期11卷 239-249页

作者： Qirong Liu Lei Liu Yongping Zheng Min Li Baofu Ding Xungang Diao Hui-Ming Cheng Yongbing Tang advanced Energy Storage technology Research Center Shenzhen Institute of Advanced TechnologyChinese Academy of Sciences institute of technology for Carbon Neutrality Shenzhen Institute of Advanced Technology Chinese Academy of Sciences School of Energy and Power Engineering North University of China School of Resource Environment and Safety EngineeringHunan University of Science and Technology School of Energy and Power Engineering Beihang University Shenzhen Key Laboratory of Energy Materials for Carbon Neutrality Shenzhen Institute of Advanced Technology Chinese Academy of Sciences Shenyang National Laboratory for Materials science Institute of Metal Research Chinese Academy of Sciences

Tunability of optical performance is one of the key technologies for adaptive optoelectronic applications,such as camouflage clothing, displays, and infrared shielding. High-precision spectral tunability is of great importance for some special applications with on-demand adaptability but remains challenging. Here we demonstrate a galvanostatic control strategy to achieve this goal, relying on the finding of the quantitative correlation between optical properties and electrochemical reactions within materials. An electrochromic electro-optical efficiency index is established to optically fingerprint and precisely identify electrochemical redox reactions in the electrochromic device. Consequently, the charge-transfer process during galvanostatic electrochemical reaction can be quantitatively regulated, permitting precise control over the final optical performance and on-demand adaptability of electrochromic devices as evidenced by an ultralow deviation of <3.0%. These findings not only provide opportunities for future adaptive optoelectronic applications with strict demand on precise spectral tunability but also will promote in situ quantitative research in a wide range of spectroelectrochemistry, electrochemical energy storage, electrocatalysis, and material chemistry.

关键词： electrochromics fine control spectral tunability high precision galvanostatic control

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Parameter selection for the hydroconversion of waste polyethylene plastic under mild conditions: A comprehensive evaluation

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science China(Technological sciences) 2024年第8期67卷 2413-2426页

作者： CHENG LeiLei CHEN RuiZhe ZHU WeiQiang TIAN ShaoNan GU Jing YUAN HaoRan CHEN Yong guangzhou institute of Energy Conversion Chinese Academy of SciencesGuangzhou 510640China School of Energy science and Engineering University of Science and Technology of ChinaHefei 230026China institute of Process Engineering Chinese Academy of SciencesBeijing 100190China

The hydrogenolysis/hydrocracking of waste polyethylene(PE) has recently been intensively studied, with the general pursuit of low-temperature reaction conditions, increased oil-phase yield, and narrower carbon chain distribution. Before this, we utilized a ball-milled ZSM-22 catalyst loaded with Ru nanoparticles(NPs), which exhibited excellent hydroconversion performance. It deconstructed PE into >80 wt.% oil products under low temperatures and short reaction times. Herein, we investigated the influence of varying temperature/pressure parameters on the degree of specific hydrocracking/internal hydrogenolysis/terminal hydrogenolysis reactions. From the comprehensive energy efficiency perspective, including stirring, reaction, and product separation, as well as taking into account the degree of product isomerization and catalyst lifespan, we analyzed the optimization of parameters. This research abandons the notion that lower temperatures are better and proposes a more comprehensive evaluation framework for low-consumption hydroconversion of PE to produce high-value products.

关键词： plastic upcycling polyethylene hydrocracking hydrogenolysis comprehensive energy efficiency

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The Emergence of Functional Ultrasound for Noninvasive Brain-Computer Interface

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Research 2024年第2期6卷 301-317页

作者： Hairong Zheng Lili Niu Weibao Qiu Dong Liang Xiaojing Long Guanglin Li Zhiyuan Liu Long Meng institute of Biomedical and Health Engineering Shenzhen Institutes of Advanced TechnologyChinese Academy of SciencesShenzhen518055China Shenzhen institute of advanced Integration technology Chinese Academy of Sciences and The Chinese University of Hong KongShenzhen518055China

A noninvasive brain-computer interface is a central task in the comprehensive analysis and understanding of the brain and is an important challenge in international brain-science *** implanted brain-computer interfaces are cranial and invasive,which considerably limits their *** development of new noninvasive reading and writing technologies will advance substantial innovations and breakthroughs in the field of brain-computer ***,we review the theory and development of the ultrasound brain functional imaging and its ***,we introduce latest advancements in ultrasound brain modulation and its applications in rodents,primates,and human;its mechanism and closed-loop ultrasound neuromodulation based on electroencephalograph are also ***,high-frequency acoustic noninvasive brain-computer interface is prospected based on ultrasound super-resolution imaging and acoustic tweezers.

关键词： breakthrough computer Computer

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How to build a habitable planet:an interview with Charles H. Langmuir

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National science Review 2024年第6期11卷 76-80页

作者： Yi-Gang Xu the guangzhou institute of Geochemistry Chinese Academy of Sciences

Earth is the only known habitable planet in the solar system. Understanding how Earth developed its unique habitability has been the frontier of Earth sciences and has become one of the main themes of current deep-space explorations. What are the decisive factors that led to a habitable planet? What is the role of solid Earth processes in the origin of life and in modulating the surface environment? Are Earth’s habitability studies relevant to current challenges that human beings face? These questions have attracted the interest of both scientists and the public alike.

关键词： Earth (planet)

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The influence of silica on reaction rates and molecular hydrogen(H_(2))generation during olivine hydrothermal alteration

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science China Earth sciences 2024年第1期67卷 222-233页

作者： Ruifang HUANG Weidong SUN Xing DING Yusheng ZHAO Yibing LI Xiuqi SHANG CAS Key Laboratory of Ocean and Marginal Sea Geology South China Sea Institute of OceanologyChinese Academy of SciencesGuangzhou 510301China SUSTech academy for advanced Interdisciplinary Studies Southern University of Science and TechnologyShenzhen 518055China Center of Deep Sea Research Institute of OceanologyChinese Academy of SciencesQingdao 266071China State Key Laboratory of Isotope Geochemistry Guangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou 510640China Institue of Geology Chinese Academy of Geological SciencesBeijing 100037China

Hydrothermal alteration of olivine greatly influences geodynamics and the recycling of volatiles(such as water and carbon)in subduction *** is an important component of geological fluids,and its influence on the hydrothermal alteration of olivine remains poorly *** this study,we performed experiments at 300–515℃ and 3.0 kbar(1 bar=10^(5)Pa)by reacting well homogenized mixtures of olivine and silica powders with saline solutions(0.5 mol L^(−1)NaCl).Silica greatly influences the reaction pathways,reaction rates,and molecular hydrogen(H_(2))formation during olivine hydrothermal *** experiments at 300℃ and 3.0 kbar with mixtures of olivine and 10 wt%silica,olivine was replaced by serpentine and *** proportions of serpentine and talc were determined according to standard curves based on infrared spectroscopy *** 6.5%serpentine and 12%talc were produced after an experimental duration of 7 days,which had no change after a longer period(14 days).Compared to the kinetics in silica-free systems,the rates of olivine hydrothermal alteration in experiments with 10 wt%silica are much *** overall reaction is:4.5Forsterite+5.5SiO_(2),aq+4H_(2)O=Serpentine+*** the addition of more silica(20 wt%and 40 wt%),olivine was transformed into *** rates of reaction were much faster,e.g.,for experiments with olivine and 20 wt%silica,43%of talc was produced after 14 days,which increased to 77%for experiments with 40 wt%silica over the same *** overall reaction is:3Forsterite+5SiO_(2),aq+2H_(2)O=*** experiments at 400–505℃ and 3.0 kbar,the promoting effect of silica on olivine hydrothermal alteration was also observed,which is closely associated with a decrease in Gibbs free energies of olivine hydrothermal *** 300℃ and 3.0 kbar,silica decreased H_(2)formed during olivine hydrothermal alteration by around an order of magnitude,resulting in an increase in oxygen *** on measured H_(2),we calibrated ox

关键词： Olivine hydrothermal alteration Silica Serpentinization Hydrogen Serpentine

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Single-wall carbon nanotube fiber non-woven fabrics with a high electrothermal heating response

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Nano Research 2024年第6期17卷 5621-5628页

作者： Xinyu Jiao Lele Xu Xinyang Sun Chao Shi Peng-Xiang Hou Chang Liu Hui-Ming Cheng Shenyang National Laboratory for Materials science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China School of Materials science and Engineering University of Science and Technology of ChinaHefei 230026China Faculty of Materials science and Engineering/institute of technology for Carbon Neutrality Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China

Carbon nanotube(CNT)fibers have great promise for constructing multifunctional fabrics with high electrical conductivity,good electro-heating ability,excellent flexibility,and a low ***,the inter-fiber contacts in the fabric greatly reduce these advantages and limit their ***,a simple pressure-fusing method to fabricate single-wall CNT(SWCNT)fiber non-woven fabrics(NWFs)that are composed of interconnected SWCNT fibers with fused joints is reported,which have good flexibility,a low density of 0.46 g/cm^(3),a high electrical conductivity of 3.7×10^(5)S/m,and a record high specific electrical conductivity of 803(S·m^(2))/*** also showed excellent electrical heating ability,so that a temperature of~160℃was rapidly reached at a low voltage of 2 *** with their low density,the SWCNT fiber NWFs are promising for use as a heating unit for low temperature battery protection and de-icing applications.

关键词： carbon nanotube fiber nonwoven fabrics fusing electrothermal heating

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Li-promoted C3N4 catalyst for efficient isomerization of glucose into fructose at 50℃ in water

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Green Energy & Environment 2024年第9期9卷 1419-1426页

作者： Wang Liu Yanfei Zhang Mengya Sun Xinpeng Zhao Shenggang Li Xinqing Chen Liangshu Zhong Lingzhao Kong CAS Key Laboratory of Low-Carbon Conversion science and Engineering Shanghai Advanced Research Institute Chinese Academy of Sciences University of chinese academy of sciences School of Physical science and technology Shanghai Tech University School of Environmental science and Engineering Suzhou University of Science and Technology

Efficient and selective glucose-to-fructose isomerization is a crucial step for production of oxygenated chemicals derived from sugars,which is usually catalyzed by base or Lewis acid heterogeneous ***,high yield and selectivity of fructose cannot be simultaneously obtained under mild conditions which hamper the scale of application compared with enzymatic ***,a Li-promoted C3N4catalyst was exploited which afforded an excellent fructose yield （40.3 wt%） and selectivity （99.5%） from glucose in water at 50~oC,attributed to the formation of stable Li–N bond to strengthen the basic sites of ***,the so-formed N6–Li–H2O active site on Li–C3N4catalyst in aqueous phase changes the local electronic structure and strengthens the deprotonation process during glucose isomerization into *** superior catalytic performance which is comparable to biological pathway suggests promising applications of lithium containing heterogeneous catalyst in biomass refinery.

关键词： Glucose Fructose Isomerization Li–C 3 N 4 Density functional theory calculations

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Model-driven CT reconstruction algorithm for nano-resolution x-ray phase contrast imaging

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chinese Physics B 2024年第7期33卷 646-650页

作者：谭雨航蔡学宝杨杰成苏婷郑海荣梁栋朱佩平葛永帅 Research Center for Medical Artificial Intelligence Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China institute of Electronic Paper Displays South China Academy of Advanced OptoelectronicsSouth China Normal UniversityGuangzhou 510006China Paul C Lauterbur Research Center for Biomedical Imaging Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China institute of High Energy Physics Chinese Academy of SciencesBeijing 100049China

The low-density imaging performance of a zone plate-based nano-resolution hard x-ray computed tomography(CT)system can be significantly improved by incorporating a grating-based Lau interferometer. Due to the diffraction, however,the acquired nano-resolution phase signal may suffer splitting problem, which impedes the direct reconstruction of phase contrast CT(nPCT) images. To overcome, a new model-driven nPCT image reconstruction algorithm is developed in this study. In it, the diffraction procedure is mathematically modeled into a matrix B, from which the projections without signal splitting can be generated invertedly. Furthermore, a penalized weighted least-square model with total variation(PWLSTV) is employed to denoise these projections, from which nPCT images with high accuracy are directly *** experiments demonstrate that this new algorithm is able to work with phase projections having any splitting distances. Moreover, results also reveal that nPCT images of higher signal-to-noise-ratio(SNR) could be reconstructed from projections having larger splitting distances. In summary, a novel model-driven nPCT image reconstruction algorithm with high accuracy and robustness is verified for the Lau interferometer-based hard x-ray nano-resolution phase contrast imaging.

关键词： splitting phase image reconstruction algorithm grating interferometer

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Identifying malicious traffic under concept drift based on intraclass consistency enhanced variational autoencoder

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science China(Information sciences) 2024年第8期67卷 238-252页

作者： Xiang LUO Chang LIU Gaopeng GOU Gang XIONG Zhen LI Binxing FANG institute of Information Engineering Chinese Academy of Sciences School of Cyber Security University of Chinese Academy of Sciences School of Computer science and technology Harbin Institute of Technology (Shenzhen)

Accurate identification of malicious traffic is crucial for implementing effective defense countermeasures and has led to extensive research efforts. However, the continuously evolving techniques employed by adversaries have introduced the issues of concept drift, which significantly affects the performance of existing methods. To tackle this challenge, some researchers have focused on improving the separability of malicious traffic representation and designing drift detectors to reduce the number of false ***, these methods often overlook the importance of enhancing the generalization and intraclass consistency in the representation. Additionally, the detectors are not sufficiently sensitive to the variations among different malicious traffic classes, which results in poor performance and limited robustness. In this paper, we propose intraclass consistency enhanced variational autoencoder with Class-Perception detector(ICE-CP) to identify malicious traffic under concept drift. It comprises two key modules during training:intraclass consistency enhanced(ICE) representation learning and Class-Perception(CP) detector construction. In the first module, we employ a variational autoencoder(VAE) in conjunction with Kullback-Leibler(KL)-divergence and cross-entropy loss to model the distribution of each input malicious traffic flow. This approach simultaneously enhances the generalization, interclass consistency, and intraclass differences in the learned representation. Consequently, we obtain a compact representation and a trained classifier for nondrifting malicious traffic. In the second module, we design the CP detector, which generates a centroid and threshold for each malicious traffic class separately based on the learned representation, depicting the boundaries between drifting and non-drifting malicious traffic. During testing, we utilize the trained classifier to predict malicious traffic classes for the testing samples. Then, we use the CP det

关键词： concept drift malicious traffic identification variational autoencoder intrusion detection cyberspace security

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Solar energetic particles intensity variations associated with a tilted-dipole 3D corotating interaction region

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Earth and Planetary Physics 2024年第5期8卷 797-810页

作者： YuJi Zhu Fang Shen Xi Luo Yang Wang BoFeng Tang State Key Laboratory of Space Weather National Space Science Center Chinese Academy of Sciences Shandong institute of advanced technology (SDIAT) College of Earth and Planetary sciences University of Chinese Academy of Sciences School of science Harbin Institute of Technology

The effect of a tilted-dipole three-dimensional corotating interaction region(CIR) on the transport and acceleration of solar energetic particles(SEPs) is *** this work,we discussed how the particle intensity longitudinal and radial dependence might be influenced by the background ***,we investigate how the spectral index distribution is modulated by the CIR structure We use the focused transport equation(FTE) to describe the propagation and acceleration of SEPs in a tilt-dipole 3D CIR,generated by the high-resolution 3D magnetohydrodynamic(MHD) *** forward stochastic differential method is used to solve the *** protons with theE～(-4.4)spectrum from 0.5 to 15 MeV are injected uniformly at the heliographic equator of 0.15 *** quantities are extracted along each interplanetary magnetic field(IMF) line to show the *** the tilted-dipole CIR background,if injected from the solar equator at the inner boundary,particles in the slow flow are transported to higher latitudes due to the extension of the IMF lines to higher *** longitudinal patterns of the particles are dominated by the density of IMF *** focusing effect modulates the longitudinal variation of the particle intensity and gives rise to new longitudinal intensity *** adiabatic effect largely increases the intensity fluctuation along the *** structure of the solar wind can also lead to the difference of the index α in the empirical functionI＿(max)=kR～(-α),describing the radial variation of peak intensity according to our *** the influence of the CIR structure,the index α varies from 1.9 to 3.4 at 0.3-1.0 *** variation of the solar wind speed should be considered when estimating the radial dependence of the SEP peak *** spectra indices rise near the CIR boundaries and drop near the stream interface(SI).The adiabatic effect makes the spatial variability of the spectral index *** spectral index could be sim

关键词： solar energetic particle (SEP) corotating interaction regions (CIR) magnetohydrodynamic (MHD)

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