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Effects of surface chlorine atoms on charge distribution and reaction barriers for photocatalytic CO_(2)reduction

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Nano Materials Science 2024年第2期6卷 235-243页

作者： Wendong Zhang Wenjun Ma Yuerui Ma Peng Chen Qingqing Ye Yi Wang Zhongwei Jiang Yingqing Ou Fan Dong Chongqing Key Laboratory of green Synthesis and Application&Chongqing Key Laboratory of Inorganic Functional Materials College of ChemistryChongqing Normal UniversityChongqing401331China Suzhou Industrial Technology Research institute of Zhejiang University Jiangsu215000China Department of Chemistry Faculty of ScienceNational University of SingaporeSingapore117543Singapore Yangtze Delta Region institute(Huzhou)&institute of Fundamental and Frontier Sciences University of Electronic Science and Technology of ChinaHuzhou313001China

Photocatalytic CO_(2)reduction to produce high value-added carbon-based fuel has been proposed as a promising approach to mitigate global warming ***,the conversion efficiency and product selectivity are still low due to the sluggish dynamics of transfer processes involved in proton-assisted multi-electron *** the formation energy barriers of intermediate products is an effective method to enhance the selectivity and productivity of final *** this study,we aim to regulate the surface electronic structure of Bi_(2)WO_(6)by doping surface chlorine atoms to achieve effective photocatalytic CO_(2)*** Cl atoms can enhance the absorption ability of light,affect its energy band structure and promote charge *** with DFT calculations,it is revealed that surface Cl atoms can not only change the surface charge distribution which affects the competitive adsorption of H_(2)O and CO_(2),but also lower the formation energy barrier of intermediate products to generate more intermediate*COOH,thus facilitating CO ***,this study demonstrates a promising surface halogenation strategy to enhance the photocatalytic CO_(2)reduction activity of a layered structure Bi-based catalyst.

关键词： Surface chlorine atoms Charge distribution Reaction barriers Photocatalytic CO_(2)reduction Bi_(2)WO_(6)

Diversity and ecological assembly process of aerobic anoxygenic phototrophic bacteria in a low irradiation area,Three Gorges Reservoir

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Journal of Environmental Sciences 2024年第9期143卷 116-125页

作者： Lixin Huo Anran Ma Hong Liu Xingzu Wang Cheng Song Chongqing institute of green and Intelligent Technology Chinese Academy of SciencesChongqing 400714China Chongqing School University of Chinese Academy of SciencesCollege of Resources and EnvironmentChongqing 400714China Key Laboratory of Reservoir Aquatic Environment Chinese Academy of SciencesChongqing 400714China University of Chinese Academy of Sciences Beijing 100049China

Aerobic anoxygenic phototrophic bacteria(AAPB)are significant bacterial groups in aquatic ecosystems,known for their rapid growth and photoheterotrophic ***,the distribution and ecological assembly process of AAPB in low irradiation freshwater basins remain unclear,warranting further *** this study,we present the diversity,abundance,spatial variations,ecological process,and community interaction of AAPB in sediment of Three Gorges Reservoir(TGR)under low *** findings demonstrate the dominant genera of AAPB community that exist in the TGR area also are appeared in different waters,with some regional ***,the concentration of pufM gene,an indicator for AAPB,maintains a consistently high numerical level ranging from(2.21±0.44)×10^(4)to(9.98±0.30)×10^(7)gene copies/*** solar irradiation is suggested as the major factor affecting AAPB,it remains unclear whether and how AAPB differ between regions due to varying solar irradiation *** results show spatial differences between total bacteria and AAPB communities,with significant differences observed only in *** and environmental factor contributed less than 10%to the spatial difference of community,with sediment type and environmental factors being the key factors influencing microbial community *** stochastic process plays a dominant role in the aggregation and replacement of AAPB communities,among which the most contribution is dispersal *** AAPB network,Yoonia and Gemmobacter are the hubs for *** results valuable insights into the AAPB communities in TGR with low irradiation.

关键词： Three Gorges Reservoir(TGR) Aerobic anoxygenic phototrophic bacteria(AAPB) Bacterial community Null model Community assembly

Fabrication of dense SiBCN monolith at a lower temperature and its high-temperature performance

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Journal of Advanced Ceramics 2024年第8期13卷 1198-1211页

作者： Zi-Bo Niu Daxin Li Dechang Jia Zhihua Yang Kunpeng Lin Yan Wang Paolo Colombo Ralf Riedel Yu Zhou institute for Advanced Ceramics School of Materials Science and EngineeringHarbin Institute of TechnologyHarbin 150080China Key Laboratory of Advanced Structural-Function Integrated Materials and green Manufacturing Technology Ministry of Industry and Information TechnologyHarbin 150080China State Key Laboratory of Advanced Welding and Joining Harbin Institute of TechnologyHarbin 150080China Department of Industrial Engineering University of PadovaPadova 3513iItaly Department of Materials Science and Engineering The Pennsylvania State UniversityUniversity Park 16802USA institute of Materials Science Darmstadt University of TechnologyDarmstadt 64287Germany School of Materials Science and Engineering Harbin Institute of Technology(Shenzhen)Shenzhen 518055China

In this study,a crack-free pyrolysis process of partially cured precursor powder compacts was developed to prepare dense silicon boron carbonitride(SiBCN)monoliths at much lower temperatures(1300℃),thereby circumventing the challenges of sintering densification(>1800℃).Unlike the elastic fracture in over-cured precursors or the viscoelastic deformation in under-cured precursors,the partially cured precursor,exhibiting elastic-plastic deformation behavior,facilitates limited nanoscale pore formation in a dense structure,achieving a balance between crack-free pyrolysis and *** to SiBCN derived from the over-cured precursor(σ=~159 MPa,K_(IC)=1.9 MPa:m^(1/2),Vickers hardness(HV)=7.8 GPa,and E=122 GPa),the resulting SiBCN monolith exhibited significantly improved mechanical properties(σ=~304 MPa,K_(IC)=3.7 MPa-m12,HV=10.6 GPa,and E=161 GPa)and oxidation *** addition,this study investigated the high-temperature performance of SiBCN monoliths,including crystallization and oxidation,and determined the oxidation kinetics induced by pore structure healing and the different oxidation mechanisms of Si-C-N and B-C-N clusters in the amorphous *** to its unique composition and structure,the SiBCN ceramic oxide layer exhibits exceptional self-healing effects on repairing the nanoporous system in the initial stage and shows outstanding high-temperature stability during prolonged oxidation,mitigating adverse effects from bubble formation and *** to the nanoporous structure,the oxidation rate is initially controlled by gas diffusion following a linear law before transitioning to oxide layer diffusion characterized by a parabolic ***,due to different valence bond configurations,Si-C-N transforms into an amorphous SiCNO structure after phase separation,unlike the nucleation and growth of residual B-N-C.

关键词： silicon boron carbonitride(SiBCN)ceramics crack-free pyrolysis amorphous structure oxidation mechanisms kinetic law

Saline-alkali soil reclamation and utilization in China:progress and prospects

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Frontiers of Agricultural Science and Engineering 2024年第2期11卷 216-228页

作者： Guangzhou WANG Gang NI Gu FENG Haley MBURRILL Jianfang LI Junling ZHANG Fusuo ZHANG State Key Laboratory of Nutrient Use and Management(SKLNUM) College of Resources and Environmental SciencesNational Academy of Agriculture Green DevelopmentChina Agricultural UniversityBeijing 100193China The institute of Ecology and Evolution University of OregonEugeneOR97403USA

Soil salinity is a global threat to the productivity of arable land. With the impact of population growth and development of social economy in China, the area of arable land has been shrinking in recent decades and is approaching a critical threshold of 120 Mha, the minimum area for maintaining the national food security. Saline-alkaline land, as important backup reserve, has been receiving increased attention as an opportunity to expand land resources. This review first summarizes the general principles and technologies of saline soil reclamation to support plant growth, including leaching salts or blocking the rise of salts, and soil fertility enhancement to improve the buffering *** the progress in this area in China is described including the customization of technologies and practices used in different saline-alkali regions. Following the soil management strategies, the concept of selecting crops for saline soil is proposed. This encompasses halophyte planting, salt-tolerant crop breeding and the application of saline-adapted functional microorganisms to improve the adaptation of crops. Finally, the current problems and challenges are evaluate, and future research directions and prospects proposed for managing this major soil constraint.

关键词： Food security land reserve reclamation saline-alkali soil utilization

Optimizing nitrogen management in the food system for sustainable development: a case study of Quzhou County

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Frontiers of Agricultural Science and Engineering 2024年第1期11卷 113-121页

作者： Fanlei MENG Menru WANG Yong HOU Lin MA Wenqi MA Xuejun LIU Fusuo ZHANG Wen XU College of Resources and Environmental Sciences National Academy of Agriculture Green DevelopmentState Key Laboratory of Nutrient Use and ManagementNational Observation and Research Station of Agriculture Green Development(QuzhouHebei)China Agricultural UniversityBeijing 100193China Water Systems and global Change Group Wageningen University&Research6700 AA Wageningenthe Netherlands Environmental Systems Analysis Group Wageningen University&Research6708 PB Wageningenthe Netherlands Key Laboratory of Agricultural Water Resources Hebei Key Laboratory of Soil EcologyCenter for Agricultural Resources ResearchInstitute of Genetic and Developmental BiologyChinese Academy of SciencesShijiazhuang 050021China College of Resources and Environment Science Hebei Agricultural UniversityBaoding 071001China

Nitrogen(N) is an essential nutrient for food production. The rapid increase in population requires high inputs of N to meet the growing food demand. If not managed well, the substantial loss of N from the food system has multiple impacts on grain yield, air and water pollution, and the economic benefits of agricultural. Multi-objective(food security, environmental sustainability and economic sustainability) synergistic consideration of N management in the food system is still lacking. This study employed strategies for optimizing N management in the food system, using Quzhou County as a typical example on the North China Plain. Firstly, a food chain approach was adopted to understand drivers and reasons behind N losses from the food ***, a top-down approach was used to define multi-objective N management, taking into consideration food security, environmental sustainability and economic sustainability. Multi-objective N management aims to reduce N losses to the environment and increase N use efficiencies,while simultaneously increasing yields and economic benefits. Thirdly, 3R(reduce-retain-recycle) N management strategies were identified for specific crops and animals through a bottom-up approach and then analyzed the potential of these strategies to achieve the multi-objectives. Finally, there is a discussion of how to engage different stakeholders to promote the technologies implementation. This study provides new insights into the synergistic achievement of multi-objective N management in the food system and the development of environmentally-friendly agriculture.

关键词： Agriculture green development food system multi-objective nitrogen management

Basic research and industrial development status of suancai in Northeast China: History， microflora diversity， processing technology， nutrition and safety

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Food Science and Human Wellness 2024年

作者： Qianqian Wang Jingbo Yang Yuqi Wang Meiru Xie Xiaoxi Qi Ramnarain Ramakrishna Libo Liu Wenkui Guo Guofang Zhang Chun Li Key Laboratory of Dairy Science， Ministry of Education， College of Food Science， Northeast Agricultural University Department of Plant Sciences， North Dakota State University Heilongjiang institute of green Food Science

Suancai has a lengthy history and a wide range of categories， which has some influence on the pickled diet culture around the world. Suancai production is transitioning to a large-scale， standardized production due to the growth of the market. It has a unique flavor and is rich in nutrients， and its abundance of free amino acids， vitamins and phenolics has many positive effects on the human body. This review gives the types and history of suancai， as well as its impact on the world's pickled culture. The changes in nutritional composition and flavor of suancai during fermentation are summarized. It presented the production technology and influencing factors of the northeast suancai， examined the quality and safety issues in suancai， and put forth some ideas and opinions on the standardization development of the suancai industry. It also summarized the geographic distribution and flora diversity of pickles around the world. In order to provide some knowledge and guidance for the promotion of modern industrial production in the suancai industry.

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Mutual feedback between algal blooming and global warming

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Journal of Oceanology and Limnology 2024年第3期42卷 787-801页

作者： Jianrong MA Guijun YANG Xianfu ZHAO Boqiang QIN Kun SHAN Botian ZHOU Yan ZENG Jingfu WANG Jingan CHEN Chongqing institute of green and Intelligent Technology Chinese Academy of SciencesChongqing 400714China State Key Laboratory of Environmental Geochemistry Institute of GeochemistryChinese Academy of SciencesGuiyang 550002China School of Environment and Ecology Jiangnan UniversityWuxi 214122China Key Laboratory of Ministry of Water Resources for Ecological Impacts of Hydraulic-projects and Restoration of Aquatic Ecosystem Institute of HydroecologyMinistry of Water Resources&Chinese Academy of SciencesWuhan 430079China State Key Laboratory of Lake Science and Environment Nanjing Institute of Geography and LimnologyChinese Academy of SciencesNanjing 210008China

global warming and algal blooms have been two of the most pressing problems faced by the world *** recent decades,numerous studies indicated that global warming promoted the expansion of algal ***,research on how algal blooms respond to global warming is *** warming coupled with eutrophication promoted the rapid growth of phytoplankton,which resulted in an expansion of algal *** blooms are affected by the combined effects of global warming,including increases in temperatures,CO_(2)concentration,and nutrient input to aquatic systems by extreme weather *** the growth of phytoplankton requires CO_(2),they appear to act as a carbon ***,algal blooms will release CH4,CO_(2),and inorganic nitrogen when they die and *** substrate nitrogen increases from decompose algal biomass,more N2O will be released by nitrification and *** comparison to CO_(2),CH4has 28-fold and N2O has 265-fold greenhouse ***,algal blooms in the polar regions may contribute to melting glaciers and sea ice(will release greenhouse gas,which contribute to global warming)by reducing surface albedo,which consequently would accelerate global ***,algal blooms and global warming could form feedback loops which prevent human survival and *** researches shall examine the mechanism,trend,strength,and control strategies involved in this mutual ***,it will promote global projects of environmental protection combining governance greenhouse gas emissions and algal blooms,to form a geoengineering for regulating the cycles of carbon,nitrogen,and phosphorus.

关键词： climate change carbon neutrality eutrophication greenhouse gas glaciers melting geoengineering

SiRAP2-12,a Positive Regulatory Factor,Effectively Improves the Waterlogging Tolerance of Foxtail Millet(Setaria italica)

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Phyton-International Journal of Experimental Botany 2024年第3期93卷 445-465页

作者： Xueyan Xia Xiaohong Fu Yu Zhao Jihan Cui Nuoya Xiao Jingxin Wang Yiwei Lu Meihong Huang Cheng Chu Jia Zhang Mengxin Yang Shunguo Li Jianfeng Liu institute of Millet Crops Hebei Academy of Agriculture and Forestry Sciences/Key Laboratory of Genetic Improvement and Utilization for Featured Coarse Cereals(Co-Construction byMinistry and Province)Ministry of Agriculture and Rural Affairs/The Key Research Laboratory of Minor Cereal Crops of Hebei ProvinceShijiazhuang050035China School of Life Sciences Institute of Life Science and Green DevelopmentHebei UniversityBaoding071002China

Foxtail millet(Setaria italica)growth was inhibited because of waterlogging stress,which has caused yield *** family plays an important role to plant adversity *** our study,we obtained 19,819 differential expressed genes(DEGs)between the two treatments based on the RNA-seq sequencing of foxtail millet of water-logging ***,a total of 28 ERF family members were obtained,which have a complete open read-ing *** studied the evolution and function of SiERF family and how they affected the waterlogging *** was found that SiERF1A/B/C(GenBank ID:OR775217,OR775219,OR775218)and SiRAP2-12(GenBank ID:OR775216)have similar functions to the known waterlogging tolerance genes of other *** them,the SiRAP2-12 expression was obviously signiﬁcantly up-regulated in foxtail millet after 5d water-logging *** SiRAP2-12 was silenced,the activity of defense enzymes in millet decreased signiﬁ*** details,superoxide dismutase(SOD),catalase(CAT)and peroxidase(POD),the osmotic regulator proline(Pro),and the activity of the anaerobic respiratory enzyme alcohol dehydrogenase(ADH)content were decreased by 78.61%,29.52%,79.95%,19.41%and 54.77%,*** contrast,the relative electrical conductivity contents(REC),malondialdehyde(MDA),and hydrogen peroxide(H_(2)O_(2))of the foxtail millet subjected to virus-induced gene silencing clearly increased by 1.03-fold,36.09%,and 15.21%,*** content of sodium(Na^(+))in the SiRAP2-12-silenced foxtail millet also increased,but that of potassium(K^(+))***,we found that ethylene content was signiﬁcantly ***,the SiAOC1 expression,an essential gene for ethylene synthesis,was inhibited in SiRAP2-12-silenced foxtail millet after waterlogging *** together,we hypothesized that SiRAP2-12 might be a positive regulator of millet tolerance to waterlogging stress.

关键词： Foxtail millet waterlogging SiRAP2-12 VIGS ethylene

Towards sustainable solar cells:unveiling the latest developments in bio-nano materials for enhanced DSSC efficiency

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Clean Energy 2024年第3期8卷 238-257页

作者： Sethu Narayanan Tamilselvan S.Shanmugan Research Centre for Solar Energy Department of Engineering PhysicsCollege of EngineeringKoneru Lakshmaiah Education FoundationGreen FieldsGuntur DistrictVaddeswaramAndhra Pradesh 522502India

Fossil fuels-instrumental in powering the nineteenth-century Industrial Revolution-are now under heightened scrutiny due to environmental concerns and carbon ***,there is a global impetus towards achieving carbon-neutral energy production,with solar energy emerging as a cornerstone in this *** the past three decades,dye-sensitized solar cells(DSSCs)have gained increasing prominence due to their unique *** review elucidates several crucial elements essential to DSSC construction,notably bio-nano materials,prized for their structural flexibility,cost-effectiveness and high molar absorption *** delves into the intricate relationship between molecular structure and DSSC performance,showcasing significant advancements with light-to-power conversion efficiencies reaching 11%.A comprehensive analysis of the photovoltaic performance of DSSCs utilizing bio-nano-based dyes offers invaluable insights into the state of this rapidly evolving *** components under scrutiny include transparent conductive oxide(TCO)layers,physical techniques for metal oxide deposition onto TCO thin films,diverse dye variants and foundational knowledge of components ripe for growth and ***,the review outlines the latest breakthroughs in the field,providing glimpses into the current status of prototype DSSCs.

关键词： DSSC performance TCO thin films environmental solution