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Non-thermal plasma enhanced catalytic conversion of methane into value added chemicals and fuels

Journal of Energy Chemistry 2024年第10期97卷 265-301页

作者： Shanza Baig Baharak Sajjadi Mewbourne School of petroleum and geological engineering University of Oklahoma

Plasma catalysis has recently gained increased attention for its application in gas conversion,notably in processes like the dry reforming of methane aimed at transforming them into valuable chemicals and *** this field is still in its early developmental stages,there is a crucial necessity to explore the synergistic mechanism between plasma and *** optimization of catalysts is imperative to improve their selectivity and conversion rates for desired products in a plasma ***,delving into microscale investigations of plasma characteristics,such as electron temperature and the density of energetic species,is essential to enhance the stability and activity of *** review examines recent advancements in various methane conversion techniques,encompassing Dry Reforming of Methane,Steam Methane Reforming,Pa rtial Oxidation of Metha ne,and Methane Decomposition utilizing non-thermal dielectric barrier discharge（DBD） *** aim is to gain a deeper understanding of plasma-catalyst interactions and to refine catalyst selection strategies for maximizing the production of desired products such as syngas,oxygenates,or higher *** review delves into the catalytic mechanisms that delineate the synergistic effects between DBD plasma and catalyst in each technology,shedding light on the role of diverse catalytic properties in activating methane molecules-a pivotal step in hybrid plasma-catalytic *** approaches employed by researchers in exploring suitable catalysts and optimal reaction conditions to bolster CH4conversion rates and selectivity using DBD plasma are ***,the review identifies gaps in the realm of plasma catalysis,underscoring the necessity for further research to fully understand the underlying principles of plasma and catalyst which are not trivial to uncover.

关键词： Catalyst DBD Methane Non-thermal plasma

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Optimizing sampling frequency of surface and downhole measurements for efficient stick-slip vibration detection

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petroleum 2024年第1期10卷 30-38页

作者： Saket Srivastava Aditya Sharma Catalin Teodoriu Mewbourne School of petroleum and geological engineering The University of Oklahoma

Drilling vibrations significantly impact drilling operations with high costs due to early downhole equipment failure and loss of productive time. Stick-slip vibrations, a severe form of torsional vibrations,is known to be present up to 50% of total drilling time, making it a topic of immense concern and research. An ongoing discussion in the industry is regarding the reliability of surface measurements for early detection of severe downhole bit sticking. Moreover, most surface measurements are sampled at lower frequency rates closer to 1 Hz. Recently, the implementation of advanced data acquisition modules in downhole subs has greatly improved our understanding of drilling vibrations through high resolution data, sampled up to 10 kHz. However, with a wide range of sampling frequency to choose from different available tools, a critical question remains unanswered. What is an optimal and adequate sampling frequency for early detection of downhole vibrations using both surface and downhole measurements?The paper addresses the question with a focus on stick-slip vibrations through an experimental investigation. Stick slip tests are repeated for different sampling frequencies of surface and downhole measurements and the stick slip index for each case is calculated. The stick-slip index varies for different sampling frequency even though the vibration tests remain completely identical. It was inferred that sampling frequency of measurements greatly impact the detection of downhole vibrations. Even though stick-slip vibrations are characteristically low frequency vibrations(≤2Hz), a minimum of 10Hz sampling frequency is recommended for detection of stick-slip vibrations. Moreover, all characteristics of stick-slip vibrations including bit sticking, bit RPM peaks and negative bit RPMs are clearly observed at a minimum of 100Hz sampling rate.

关键词： Stick-slip

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Distribution and geochemical significance of alkylbenzenes for crude oil with different depositional environments and thermal maturities

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petroleum Science 2024年第2期21卷 777-790页

作者： Bing-Kun Meng Dao-Fu Song Yuan Chen Sheng-Bao Shi School of petroleum engineering and Environmental engineering Yan'an UniversityYan'an716000ShaanxiChina State Key Laboratory of petroleum Resources and Prospecting College of GeosciencesChina University of PetroleumBeijing102249China

A total of 45 alkylbenzenes were detected and identified in crude oils with different depositional environments and thermal maturities from the Tarim Basin,Beibuwan Basin,and Songliao Basin using comprehensive two-dimensional gas chromatography time-of-flight mass spectrometry(GC×GCTOFMS).By analyzing the distribution characteristics of C0-C5alkylbenzenes,it is found that the content of some alkylbenzenes varies greatly in crude *** on the distribution characteristics of 1,2,4,5-tetramethylbenzene(Te MB)and 1,2,3,4-Te MB,the ratio of 1,2,4,5-Te MB to 1,2,3,4-Te MB is proposed to indicate the organic matter origin and depositional environment of ancient *** samples originated mainly from lower hydrobiont,algae,bacteria and source rocks deposited under reducing/anoxic conditions have low 1,2,4,5-/1,2,3,4-Te MB values(less than 0.6),while oil samples originated mainly from terrestrial higher plants and source rocks deposited under oxic/sub-oxic conditions have higher 1,2,4,5-/1,2,3,4-Te MB values(greater than 1.0).The significant difference of 1,2,4,5-/1,2,3,4-Te MB values is controlled by 1,2,4,5-Te MB content.1,2,4,5-Te MB content in oils derived from source rocks deposited in oxidized sedimentary environment(greater than 1.0 mg/g whole oil)is higher than that in oils from source rocks deposited in reduced sedimentary environment(less than 1.0 mg/g whole oil).1,2,4,5-/1,2,3,4-Te MB ratio might not or slightly be affected by evaporative fractionation,biodegradation and thermal maturity.1,2,4,5-/1,2,3,4-Te MB ratio and 1,2,4,5-Te MB content can be used as supplementary parameter for the identification of sedimentary environment and organic matter *** should be noted that compared to the identification of organic matter sources,the 1,2,4,5-/1,2,3,4-Te MB parameter is more effective in identifying sedimentary environments.

关键词： 1 2 4 5-Tetramethylbenzene GC×GC-TOFMS Organic matter origin Depositional environment

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Application of machine learning and deep learning in geothermal resource development: Trends and perspectives

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Deep Underground Science and engineering 2024年第3期3卷 286-301页

作者： Abdulrahman Al‐Fakih Abdulazeez Abdulraheem Sanlinn Kaka College of petroleum engineering and geosciences King Fahd University of Petroleum MineralsDhahranSaudi Arabia

This study delves into the latest advancements in machine learning and deep learning applications in geothermal resource development,extending the analysis up to *** focuses on artificial intelligence's transformative role in the geothermal industry,analyzing recent literature from Scopus and Google Scholar to identify emerging trends,challenges,and future *** results reveal a marked increase in artificial intelligence(AI)applications,particularly in reservoir engineering,with significant advancements observed post‐*** study highlights AI's potential in enhancing drilling and exploration,emphasizing the integration of detailed case studies and practical *** also underscores the importance of ongoing research and tailored AI applications,in light of the rapid technological advancements and future trends in the field.

关键词： artificial intelligence deep learning geothermal energy development machine learning

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Prediction of Ground Vibration Induced by Rock Blasting Based on Optimized Support Vector Regression Models

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Computer Modeling in engineering & Sciences 2024年第6期139卷 3147-3165页

作者： Yifan Huang Zikang Zhou Mingyu Li Xuedong Luo Faculty of engineering China University of GeosciencesWuhan430074China Institute of geological Survey China University of GeosciencesWuhan430074China

Accurately estimating blasting vibration during rock blasting is the foundation of blasting vibration *** this study,Tuna Swarm Optimization(TSO),Whale Optimization Algorithm(WOA),and Cuckoo Search(CS)were used to optimize two hyperparameters in support vector regression(SVR).Based on these methods,three hybrid models to predict peak particle velocity(PPV)for bench blasting were ***-eight samples were collected to establish the PPV database,eight initial blasting parameters were chosen as input parameters for the predictionmodel,and the PPV was the output *** predictive performance evaluation indicators,the coefficient of determination(R2),rootmean square error(RMSE),mean absolute error(MAE),and a10-index were *** normalizedmutual information value is then used to evaluate the impact of various input parameters on the PPV prediction *** to the research findings,TSO,WOA,and CS can all enhance the predictive performance of the SVR *** TSO-SVR model provides the most accurate *** performances of the optimized hybrid SVR models are superior to the unoptimized traditional prediction *** maximum charge per delay impacts the PPV prediction value the most.

关键词： Blasting vibration metaheuristic algorithms support vector regression peak particle velocity normalized mutual information

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Quaternary Activity Characteristics and Regional Tectonic Significance of the Jiulong Fault in Jiujiang,Jiangxi Province,China

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Journal of Earth Science 2024年第4期35卷 1107-1117页

作者： Xin Qi Yuyong Jiao Qinghua Li Bin Li Faculty of engineering China University of GeosciencesWuhan430074China Wuhan Center China Geological SurveyWuhan430205China Institute of geological Survey China University of GeosciencesWuhan430074China

Obtaining geological and landform dislocation features,as well as the measured stratigraphic activity age,provides direct evidence to evaluate fault activity,which is more difficult to do in areas with low tectonic activity,such as eastern and central China.A detailed investigation of the fault activity,trenching,drilling joint geological profile,geological survey,and chronological analysis were used to obtain the spatial geometry,fault kinematics,and activity chronology of the Jiulong *** conclusions are as follows:(1)The Jiulong fault was a fracture zone composed of four branch faults,with a width of around 30–40 m and good extendibility,while the maximum surface rupture length was 373 m.(2)The Jiulong fault has many strata dislocations,and the dislocation distance decreased from bottom to top,demonstrating synsedimentary structure characteristics,with a maximum stratigraphic dislocation distance of 18.2 m.(3)Preliminary analysis suggested the Jiulong fault as a secondary fracture of the Xiangfan-Guangji fault zone and provided evidence of the southeastward extension of the Xiangfan-Guangji fault.A preliminary hypothesis purported the Xiangfan-Guangji fault as the seismogenic fault of the Ms 5.0 magnitude earthquake in 1911.(4)According to OSL and ESR dating analyses,the upper breakpoint of the Jiulong fault cuts into the Late Pleistocene Xingang Formation(Qp3x)strata,and the latest active age of the Jiulong fault was 57.6 *** chronology analysis confirmed an active fault from the Late Pleistocene and identified a weak tectonic in Jiujiang Province,which represents the largest active fault outcrop uncovered in the area so *** study provides evidence and research materials for the evaluation of fault activity and seismic stability in this region.

关键词： active fault regional tectonic earthquakes seismic intensity tectonics

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Influences of shale microstructure on mechanical properties and bedding fractures distribution

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petroleum Science 2024年第3期21卷 1944-1954页

作者： Ming-Zhe Gu Mao Sheng Shi-Zhong Cheng Fan-Hao Gong Gen-Sheng Li State Key Laboratory of petroleum Resources and engineering China University of Petroleum-BeijingBeijing2249China College of petroleum engineering China University of Petroleum-BeijingBeijing102249China Shenyang Center of China geological Survey ShenyangLiaoning110034China

The difference in microstructure leads to the diversity of shale mechanical properties and bedding fractures distribution *** this paper,the microstructure and mechanical properties of Longmaxi marine shale and Qingshankou continental shale were studied by X-ray diffractometer(XRD),field emission scanning electron microscope(FE-SEM)with mineral analysis system,and ***,the typical bedding layers area was properly stratified using Focused Ion Beam(FIB),and the effects of microstructure and mechanical properties on the distribution patterns of bedding fractures were *** results show that the Longmaxi marine shale sample contains more clay mineral grains,while the Qingshankou continental shale sample contains more hard brittle mineral grains such as *** Longmaxi marine shale sample,hard brittle minerals with grain sizes larger than 20μm is18.24%and those with grain sizes smaller than 20μm is 16.22%.For Qingshankou continental shale sample,hard brittle minerals with grain sizes larger than 20μm is 40.7%and those with grain sizes smaller than 20μm is 11.82%.In comparison to the Qingshankou continental shale sample,the Longmaxi marine shale sample has a lower modulus,hardness,and *** shales are formed by alternating coarse-grained and fine-grained layers during *** average single-layer thickness of Longmaxi marine shale sample is greater than Qingshankou continental shale *** two types of shale have similar bedding fractures distribution patterns and fractures tend to occur in the transition zone from coarse-grained to fine-grained *** orientation of the fracture is usually parallel to the bedding plane and detour occurs in the presence of hard brittle *** fracture distribution density of the Longmaxi marine shale sample is lower than that of the Qingshankou continental shale sample due to the strong heterogeneity of the Qingshankou continental *** current resea

关键词： Shale Nanoindentation Microstructure Mechanical property Fracture

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The effects of various factors on spontaneous imbibition in tight oil reservoirs

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petroleum Science 2024年第1期21卷 315-326页

作者： Cheng Liu Tian-Ru Wang Qing You Yue-Chun Du Guang Zhao Cai-Li Dai School of Energy Resources China University of GeosciencesBeijing100083PR China School of petroleum engineering China University of PetroleumQingdao266580ShandongPR China

Slickwater fracturing fluids have gained widespread application in the development of tight oil reservoirs. After the fracturing process, the active components present in slickwater can directly induce spontaneous imbibition within the reservoir. Several variables influence the eventual recovery rate within this procedure, including slickwater composition, formation temperature, degree of reservoir fracture development, and the reservoir characteristics. Nonetheless, the underlying mechanisms governing these influences remain relatively understudied. In this investigation, using the Chang-7 block of the Changqing Oilfield as the study site, we employ EM-30 slickwater fracturing fluid to explore the effects of the drag-reducing agent concentration, imbibition temperature, core permeability, and core fracture development on spontaneous imbibition. An elevated drag-reducing agent concentration is observed to diminish the degree of medium and small pore utilization. Furthermore, higher temperatures and an augmented permeability enhance the fluid flow properties, thereby contributing to an increased utilization rate across all pore sizes. Reduced fracture development results in a lower fluid utilization across diverse pore types. This study deepens our understanding of the pivotal factors affecting spontaneous imbibition in tight reservoirs following fracturing. The findings act as theoretical, technical, and scientific foundations for optimizing fracturing strategies in tight oil reservoir transformations.

关键词： Tight oil reservoir Spontaneous imbibition Nuclear magnetic resonance Slickwater fracturing fluid Fluid utilization degree

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Sand control mechanism of radial well filled with phase change material in hydrate reservoir

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petroleum Science 2024年第4期21卷 2571-2582页

作者： Xiao-Qiang Liu Zhong-Xi Han Zhi-Lin Luo Hai-Long Lu Ying Sun Qing You Tian-Kui Guo Zhan-Qing Qu School of Energy Resources China University of Geosciences (Beijing) Beijing Key Laboratory of Unconventional Natural Gas geological Evaluation and Development engineering China University of Geosciences (Beijing) China Research Institute of petroleum Exploration and Development engineering Technology Research Institute of Southwest Oil & Gas Field Company PetroChina Beijing International Center for Gas Hydrate School of Earth and Space Sciences Peking University School of Advanced Material Peking University Shenzhen Graduate School School of petroleum engineering China University of Petroleum (East China)

Radial well filled with phase change material has been proposed as a novel sand control method for hydrate exploitation. In order to reveal the sand control mechanism, CFD-DEM coupling method is applied to simulate the migration, settlement, and blockage processes of sand particles in the radial *** obtained results indicate that three scenarios have been recognized for sand particles passing through sand control medium, based on the diameter ratio of sand control medium to sand particle（Dd）:fully passing（Dd= 8.75-22.5）, partially passing and partially blocked（Dd= 3.18-5.63）, and completely blocked（Dd= 2.18-3.21）. After being captured by the sand control medium, sand particles can block pores, which increases fluid flow resistance and causes a certain pressure difference in the radial *** pressure in the radial well should be lower than the hydrate phase equilibrium pressure during sand control design, for the purpose of promoting hydrate decomposition, and sand capture. The length of the radial well should be optimized based on the reservoir pore pressure, production pressure difference,bottom hole pressure, and the pressure gradient in the radial well. It should be noticed that the sand control medium leads to a decrease in permeability after sand particles captured. Even the permeability is reduced to several hundred millidarcy, it is still sufficient to ensure the effective flow of gas and water after hydrate decomposition. Increasing fluid velocity reduces the blocking capacity of the sand control medium, mainly because of deterioration in bridging between sand particles.

关键词： Hydrate reservoir Sand control Radial well CFD-DEM

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Influence of tectonic preservation conditions on the nanopore structure of shale reservoir: A case study of Wufeng-Longmaxi Formation shale in western Hubei area, south China

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petroleum Science 2024年第4期21卷 2203-2217页

作者： Meng Xiang Shang Xu Ya-Ru Wen Qi-Yang Gou Bing-Chang Liu National Key Laboratory of Deep Oil and Gas China University of Petroleum (East China) Hubei Key Laboratory of Resources and Eco-environment Geology Hubei Geological Survey Key Laboratory of Tectonics and petroleum Resources Ministry of Education China University of Geosciences

Tectonism is one of the dominant factors affecting the shale pore structure. However, the control of shale pore structure by tectonic movements is still controversial, which limits the research progress of shale gas accumulation mechanism in the complex tectonic region of southern China. In this study, 34 samples were collected from two exploratory wells located in different tectonic locations. Diverse experiments,e.g., organic geochemistry, XRD analysis, FE-SEM, low-pressure gas adsorption, and high-pressure mercury intrusion, were conducted to fully characterize the shale reservoir. The TOC, Ro, and mineral composition of the shale samples between the two wells are similar, which reflects that the shale samples of the two wells have proximate pores-generating capacity and pores-supporting ***, the pore characteristics of shale samples from two wells are significantly different. Compared with the stabilized zone shale, the porosity, pore volume, and specific surface area of the deformed zone shale were reduced by 60.61%, 64.85%, and 27.81%, respectively. Moreover, the macroscopic and fine pores were reduced by 54.01% and 84.95%, respectively. Fault activity and uplift denudation are not conducive to pore preservation, and the rigid basement of Huangling uplift can promote pore preservation. These three factors are important reasons for controlling the difference in pore structure between two wells shales. We established a conceptual model of shale pores evolution under different tectonic preservation conditions. This study is significant to clarify the scale of shale gas formation and enrichment in complex tectonic regions, and helps in the selection of shale sweet spots.

关键词： Shale gas Pore structure Tectonic preservation conditions Shale gas enrichment mechanism

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