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A general synthetic strategy for N, P co-doped graphene supported metal-rich noble metal phosphides for hydrogen generation

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Green Energy & Environment 2024年第1期9卷 152-162页

作者： Jingwen Ma Xiang Li Guangyu Lei Jun Wang Juan Wang Jian Liu Ming Ke Yang Li Chunwen Sun School of Chemical and environmental Engineering China University of Mining and Technology(Beijing)Beijing100083China State Key laboratory of Heavy Oil Processing China University of PetroleumBeijing102249China lab of Advanced Nano-structures&Transfer Processes Department of Chemical EngineeringTianjin UniversityTianjin300354China PetroChina planning and Engineering Institute Beijing100083China

The exploitation of electrocatalysts with high activity and durability for HER is desirable for future energy systems,but it is still a *** have attracted increasing attentions,but the preparation process often needs toxic regents or dangerous reaction ***,we develop a general green method to fabricate metal-rich NMPs anchored on NPG through pyrolyzing DNA cross-linked *** obtained Ru_(2) P-NPG exhibits an ultrasmall overpotential of 7 mV at 10 mA cm^(2) and ultralow Tafel slope of 33 mV dec^(-1) in 1.0 mol L?1 KOH,even better than that of commercial Pt/*** addition,Ru 2 P-NPG also shows low overpotentials of 29 and 78 mV in 0.5 mol L^(-1) H_(2)SO_(4) and 1.0 mol L^(-1) PBS,*** superior activity can be attributed to the ultrafine dispersion of Ru 2 P nanoparticles for more accessible sites,more defects formed for abundant active sites,the two-dimensional plane structure for accelerated electron transfer and mass transport,as well as the regulation of electron distribution of the ***,the synthetic method can also be applied to prepare other metal-rich noble metal phosphides(Pd_(3)P-NPG and Rh_(2)P-NPG),which also exhibits high activity for *** work provides an effective strategy for designing NMP-based electrocatalysts.

关键词： Noble metal phosphides Electrocatalyst Deoxyribonucleic acid Hydrogen evolution pH universal

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Retrieval of high spatial resolution mountainous land surface temperature considering topographic and adjacency effects

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Science China Earth Sciences 2024年第11期67卷 3610-3625页

作者： Zhiwei HE Bohui TANG Zhaoliang LI Faculty of Land Resources Engineering Kunming University of Science and Technology Key laboratory of Plateau Remote Sensing Department of Education of Yunnan Province State Key lab of Resources and environmental Information System Institute of Geographic Sciences and Natural Resources ResearchChinese Academy of Sciences Key laboratory of Agricultural Remote Sensing Ministry of Agriculture and Rural Affairs Institute of Agricultural Resources and Regional Planning Chinese Academy of Agricultural Sciences

Land surface temperature(LST) is a key parameter reflecting the interaction between land and atmosphere. Currently,thermal infrared(TIR) quantitative remote sensing technology is the only means to obtain large-scale, high spatial resolution LST. Accurately retrieving high spatial resolution mountainous LST(MLST) plays an important role in the study of mountain climate change. The complex terrain and strong spatial heterogeneity in mountainous areas change the geometric relationship between the surface and satellite sensors, affecting the radiation received by the sensors, and rendering the assumption of planar parallelism invalid. In this study, considering the influence of complex terrain in mountainous areas on atmospheric downward radiation and the thermal radiation contribution of adjacent pixels, a mountainous TIR radiative transfer model based on the sky view factor was developed. Combining with the atmospheric radiative transfer model MODTRAN 5.2, a nonlinear generalized split-window algorithm suitable for high spatial resolution MLST retrieval was constructed and applied to Landsat-9 TIRS-2satellite TIR remote sensing data. The analysis results indicate that neglecting the topographic and adjacency effects would lead to significant discrepancies in LST retrieval, with simulated data showing LST differences of up to 2.5 K. Furthermore, due to the lack of measured MLST in the field, the MLST accuracy obtained by this retrieval method was indirectly validated using the currently recognized highest-accuracy forward 3D radiative transfer model DART. The MLST and emissivity were input into the DART model to simulate the brightness temperature at the top of the atmosphere(TOA) of Landsat-9 band 10, and compared with the brightness temperature at TOA of Landsat-9 band 10. The RMSE(Root Mean Square Error) for the two subregions was0.50 and 0.61 K, respectively, indicating that the method proposed can retrieve high-precision MLST.

关键词： Mountainous land surface temperature Topographic and adjacency effects Nonlinear generalized split-window algorithm Landsat-9 data DART model

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Measuring urban thermal environment from accessibility-based perspective:A case study in a populous city

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Geography and Sustainability 2024年第3期5卷 329-342页

作者： Xinyu Dong Xiaoya Li Yanmei Ye Dan Su Runjia Yang Angela Lausch Department of Land Management Zhejiang UniversityHangzhou 310058China Department of Computational Landscape Ecology Helmholtz Centre for Environmental Research-UFZLeipzig 04318Germany Landscape Ecology lab Geography DepartmentHumboldt-Universität zu BerlinBerlin 10099Germany Department of Physical Geography and Geoecology Martin Luther University Halle-WittenbergHalle 06120Germany Department of Architecture Facility Management and GeoinformationAnhalt University of Applied SciencesDessau 06846Germany

Understanding the spatial interaction among residents,cooling service,and heat risk area in complex urban areas is conducive to developing targeted ***,traditional urban thermal environment assessments typically relied on simple linear integration of associated indicators,often neglecting the spatial interaction *** explore the spatial interaction among the three elements,this study proposes an accessibility-based urban thermal environment assessment *** Zhengzhou,a rapidly urbanizing city,as an example,remotely sensed images from three periods(2010,2015 and 2020)were applied to extract urban green space(UGS)and hot island area(HIA).An improved two-step floating catchment area(2SFCA)method and bivariate local Moran’s I were employed to explore whether residents’clustering locations are more likely to access cooling service or to be exposed to heat *** results demonstrate that the UGS in the city has been expanding,whereas the HIA shrank within the inner city in 2015 and then increased in *** though the urban thermal environment may have improved in the last decade,the spatial interaction among the residents,cooling service and heat risk area could be *** autocorrelation shows an increase in locations that are disadvantageous for resident *** when sufficient cooling services were provided,residents in these areas could still be exposed to high heat *** developed urban thermal environment framework provides a novel insight into the residents’heat risk exposure and cooling service accessibility,and the findings could assist urban planners in targeting the improvement of extra heat exposure risk locations.

关键词： Urban heat island Urban green space Accessibility Remote sensing Spatial autocorrelation analysis

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Modeling urban redevelopment:A novel approach using time-series remote sensing data and machine learning

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Geography and Sustainability 2024年第2期5卷 211-219页

作者： Li Lin Liping Di Chen Zhang Liying Guo Haoteng Zhao Didarul Islam Hui Li Ziao Liu Gavin Middleton Center for Spatial Information Science and Systems George Mason UniversityFairfaxVA22030USA Department of Geography and geoinformation Science George Mason UniversityFairfaxVA22030USA

Accurate mapping and timely monitoring of urban redevelopment are pivotal for urban studies and decisionmakers to foster sustainable urban *** mapping methods heavily depend on field surveys and subjective questionnaires,yielding less objective,reliable,and timely *** advancements in Geographic Information Systems(GIS)and remote-sensing technologies have improved the identification and mapping of urban redevelopment through quantitative analysis using satellite-based ***,challenges persist,particularly concerning accuracy and significant temporal *** study introduces a novel approach to modeling urban redevelopment,leveraging machine learning algorithms and remote-sensing *** methodology can facilitate the accurate and timely identification of urban redevelopment *** study’s machine learning model can analyze time-series remote-sensing data to identify spatio-temporal and spectral patterns related to urban *** model is thoroughly evaluated,and the results indicate that it can accurately capture the time-series patterns of urban *** research’s findings are useful for evaluating urban demographic and economic changes,informing policymaking and urban planning,and contributing to sustainable urban *** model can also serve as a foundation for future research on early-stage urban redevelopment detection and evaluation of the causes and impacts of urban redevelopment.

关键词： Urban redevelopment Urban sustainability Remote sensing Time-series analysis Machine learning

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A local rainfall-triggered giant landslide occurred in a region along a high-speed railway on the Qinghai‒Tibetan Plateau

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Journal of Mountain Science 2024年第9期21卷 2939-2955页

作者： LI Qingpeng LIU Wenhui HE Renjie YING Chunye LIU Hairui DOU Zengning LIU Yabing YANG Sha SONG Xianteng School of Geological Engineering Qinghai UniversityXining 810016China Key lab of Cenozoic Resource and Environment in North Margin of the Tibetan Plateau Qinghai UniversityXining 810016China College of Eco-environmental Engineering Qinghai UniversityXining 810016China Qinghai Transportation planning and Design Institute Co Ltd Xining 810000China Xining Center for Integrated Natural Resources Survey China Geological SurveyXining 810000QinghaiChina

An increasing number of geological hazards along high-speed railways on the Qinghai‒Tibetan Plateau have occurred and have resulted in a profound influence on old infrastructure,which has attracted increasing *** landslide event that occurred on September 15,2022,in Jiujiawan village,Xining city,Qinghai Province,is a typical *** on field investigations and remote sensing interpretations,a comprehensive analysis was conducted on the ***,the potential secondary failure of the current Jiujiawan landslide was assessed using Fast Lagrangian Analysis of Continua in Three Dimensions(FLAC3D).Based on the application of the small baseline subset-interferometric synthetic aperture radar(SBAS-InSAR)technique to SAR images from February 24,2017 to September 14,2022,a significant westward horizontal deformation was found to have been formed prior to the occurrence of the *** maximum annual average deformation rate in the line of sight(LOS)direction reached-45 mm/yr,with a maximum cumulative deformation of-178 *** value was consistent with the continual increase in annual precipitation(2.51 mm/yr)prior to the occurrence of the *** accumulated precipitation before the landslide was 279.8 mm,accounting for 54.2%of the total annual precipitation,with a particularly notable surge in monthly precipitation observed during August(250.3 mm).Additionally,the occurrence of a seismic event with a magnitude of Ms 6.9 in Menyuan County,80 km away from Xining,could be a potential triggering factor to the landslide,as evidenced by an abrupt subsidence alteration observed prior to and following the *** maximum subsidence in the line of sight(LOS)direction exceeded 11 mm,exhibiting a highly consistent spatial distribution with the occurrence range of *** results suggest that the Jiujiawan landslide was likely induced by earthquake events in the early stage and heavy rainfall in the later *** FLAC3D numerical

关键词： Landslide Development characteristic Driver Mudstone Xining Basin

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Spatiotemporal evolution and future simulation of land use/land cover in the Turpan-Hami Basin,China

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Journal of Arid Land 2024年第10期16卷 1303-1326页

作者： CHEN Yiyang ZHANG Li YAN Min WU Yin DONG Yuqi SHAO Wei ZHANG Qinglan Key laboratory of Digital Earth Science Aerospace Information Research InstituteChinese Academy of SciencesBeijing100094China International Research Center of Big Data for Sustainable Development Goals Beijing 100094China University of Chinese Academy of Sciences Beijing 100094China Xinjiang Uygur Autonomous Region Natural Resources planning and Research Institute Urumqi 830011China School of Geomatics and Marine Information Jiangsu Ocean UniversityLianyungang 222001China College of Geomatics and geoinformation Guilin University of TechnologyGuilin 541004China

The Turpan-Hami(Tuha)Basin in Xinjiang Uygur Autonomous Region of China,holds significant strategic importance as a key economic artery of the ancient Silk Road and the Belt and Road Initiative,necessitating a holistic understanding of the spatiotemporal evolution of land use/land cover(LULC)to foster sustainable planning that is tailored to the region's unique resource ***,existing LULC classification methods demonstrate inadequate accuracy,hindering effective regional *** this study,we established a two-level LULC classification system(8 primary types and 22 secondary types)for the Tuha *** employing Landsat 5/7/8 imagery at 5-a intervals,we developed the LULC dataset of the Tuha Basin from 1990 to 2020,conducted the accuracy assessment and spatiotemporal evolution analysis,and simulated the future LULC under various scenarios via the Markov-Future Land Use Simulation(Markov-FLUS)*** results revealed that the average overall accuracy values of our LULC dataset were 0.917 and 0.864 for the primary types and secondary types,*** with the seven mainstream LULC products(GlobeLand30,Global 30-meter Land Cover with Fine Classification System(GLC_FCS30),Finer Resolution Observation and Monitoring of Global Land Cover PLUS(FROM_GLC PLUS),ESA Global Land Cover(ESA_LC),Esri Land Cover(ESRI_LC),China Multi-Period Land Use Land Cover Change Remote Sensing Monitoring Dataset(CNLUCC),and China Annual Land Cover Dataset(CLCD))in 2020,our LULC data exhibited dramatically elevated overall accuracy and provided more precise delineations for land features,thereby yielding high-quality data backups for land resource analyses within the *** 2020,unused land(78.0%of the study area)and grassland(18.6%)were the dominant LULC types of the basin;although cropland and construction land constituted less than 1.0%of the total area,they played a vital role in arid land development and primarily situated within oases that form the urban co

关键词： land use/land cover(LULC) future simulation manual interpretation Markov-Future Land Use Simulation(Markov-FLUS)model Turpan-Hami(Tuha)Basin Xinjiang

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Climate change induced heat stress impact on workplace productivity in a net zero-carbon timber building towards the end of the century

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Building Simulation 2024年第6期17卷 893-906页

作者： Deepak Amaripadath Mattheos Santamouris Shady Attia School of Geographical Sciences and Urban planning Arizona State UniversityTempeAZUSA Urban Climate Research Center Arizona State UniversityTempeAZUSA School of Built Environment University of New South Wales2052SydneyAustralia Sustainable Building Design lab Department of UEEFaculty of Applied SciencesUniversity of Liege4000LiegeBelgium

Changing climate intensifies heat stress,resulting in a greater risk of workplace productivity decline in timber office buildings with low internal thermal *** impact of climate change induced heat exposure on indoor workplace productivity in timber office buildings has not been extensively ***,further investigation to reduce the work capacity decline towards the end of the century is ***,heat exposure in a net zero-carbon timber building near Brussels,Belgium,was evaluated using a reproducible comparative approach with different internal thermal mass *** analysis indicated that strategies with increased thermal mass were more effective in limiting the effects of heat exposure on workplace *** medium and high thermal mass strategies reduced workplace productivity loss to 0.1%in the current,0.3%and 0.2%in the midfuture,and 4.9%and 3.9%for future *** comparison,baseline with low thermal mass yielded a decline of 2.3%,3.3%,and 8.2%.The variation in maximum and minimum wet-bulb globe temperatures were also lower for medium and high thermal mass strategies than for low thermal mass *** study findings lead to the formulation of design guidelines,identification of research gaps,and recommendations for future work.

关键词： heat exposure office buildings work capacity thermal mass climate change

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Groundwater chromate removal by autotrophic sulfur disproportionation

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environmental Science and Ecotechnology 2024年第5期21卷 187-196页

作者： Yan-Ying Qiu Juntao Xia Jiahua Guo Xianzhe Gong Liang Zhang Feng Jiang Guangdong Provincial Key lab of environmental Pollution Control and Remediation Technology School of Environmental Science and EngineeringSun Yat-sen UniversityGuangzhou510275China Guangdong Provincial International Joint Research Center on Urban Water Management and Treatment Sun Yat-sen UniversityGuangzhouChina Institute of Marine Science and Technology Shandong UniversityQingdaoShandong266237China

Chromate[Cr(VI)]contamination in groundwater is a global environmental *** elemental sulfur-based biotechnologies for Cr(VI)removal depend heavily on the synthesis of dissolved organic carbon to fuel heterotrophic Cr(VI)reduction,a bottleneck in the remediation *** we show an alternative approach by leveraging sulfur-disproportionating bacteria(SDB)inherent to groundwater ecosystems,offering a novel and efficient Cr(VI)removal *** implemented SDB within a sulfur-packed bed reactor for treating Cr(VI)-contaminated groundwater,achieving a notable removal rate of 6.19 mg L^(-1) h^(-1) under oligotrophic *** identified the chemical reduction of Cr(VI)via sulfide,produced through sulfur disproportionation,as a key mechanism,alongside microbial Cr(VI)reduction within the sulfur-based ***-centric metagenomic analysis revealed a symbiotic relationship among SDB,sulfur-oxidizing,and chromate-reducing bacteria within the reactor,suggesting that Cr(VI)detoxification by these microbial communities enhances the sulfurdisproportionation *** research highlights the significance of sulfur disproportionation in the cryptic sulfur cycle in Cr(VI)-contaminated groundwater and proposes its practical application in groundwater remediation efforts.

关键词： Groundwater remediation Sulfide generation Sulfur-disproportionating bacteria Cr(VI)reduction Symbiotic interactions

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Fe nanoclusters anchored in biomass waste-derived porous carbon nanosheets for high-performance supercapacitor

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Chinese Chemical Letters 2024年第8期35卷 362-366页

作者： Yuchen Wang Yaoyu Liu Xiongfei Huang Guanjie He Kai Yan Guangdong Provincial Key laboratory of environmental Pollution Control and Remediation Technology School of Environmental Science and EngineeringSun Yat-sen UniversityGuangzhou 510275China Key laboratory of Advanced Energy Materials Chemistry(Ministry of Education) Nankai UniversityTianjin 300071China Electrochemical Innovation lab Department of Chemical EngineeringUniversity College LondonLondonWC1E 7JEUnited Kingdom

Metal-nanocluster materials have gradually become a promising electrode candidate for supercapaci-tor *** high-efficient and rational architecture of these metal-nanocluster electrode mate-rials with satisfied supercapacitive performance are full of ***,Fe-nanocluster anchored porous carbon(FAPC)nanosheets were constructed through a facile and low-cost impregnation-activation *** characterization methods documented that FAPC nanosheets possessed a mesopore-dominated structure with large surface area and abundant Fe-N4 active sites,which are crucial for su-percapacitive energy *** optimal FAPC electrode exhibited a high specific capacitance of 378 F/g at a specific current of 1 A/g and an excellent rate capability(271 F/g at 10 A/g),which are comparable or even superior to that of most reported carbon ***,the FAPC-based device achieved a desired specific energy of 14.8 Wh/kg at a specific power of 700 W/*** work opens a new avenue to design metal-nanocluster materials for high-performance biomass waste-based supercapacitors.

关键词： Fe nanoclusters Biomass waste Porous carbon nanosheets Supercapacitor Charge transfer

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Investigation on occupant presence and appliance operation schedules for university campus in south China sub-tropical area

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Building Simulation 2024年第2期17卷 301-318页

作者： Siwei Lou Zhongyuan Lin Yukai Zou Dawei Xia Yu Huang Zhuohong Li Zhaowen Gu School of Civil Engineering Guangzhou UniversityGuangzhou Higher Edu.Mega CenterGuangzhouChina School of Architecture and Urban planning Guangzhou UniversityGuangzhou Higher Edu.Mega CenterGuangzhouChina

Building occupant presence during varying periods is crucial to the performance studies of buildings and city ***,the understanding of the building occupancies on the university campus remains *** address this gap,our study employs field measurements,payment records,course arrangements,and building access systems to depict the occupancy patterns of the canteen,dormitory,library,and teaching and lab buildings during weekdays and *** found that the occupancy rates across different buildings are somehow interrelated,given that the total number of occupants on campus is generally ***,dormitory occupancy rates tend to be low during the morning and afternoon course hours,which inversely correlates with the high occupancy rates in the teaching and lab buildings during these ***,canteens experience surges in occupancy during meal times,which coincide with a decrease in library ***,we established appliance operation schedules for dormitories through surveys and on-site *** dispensers and electronic devices were identified as the primary energy consumers for both male and female occupants,with desk-top fans and hairdryers being significant energy users for male and female occupants,*** findings are essential for energy studies within a campus setting,underlining the importance of considering occupant behaviors on a regional scale.

关键词： building occupant behavior university campus occupancy schedule appliance operation schedule

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