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Science China(Information Sciences) 2025年

作者： Di ZHAO Rui DING Bin SONG State Key Laboratory of Integrated Services Networks Xidian University Hangzhou Institute of Technology Xidian University China Satellite Network Group co. Ltd.

Future 6G networks will integrate non-terrestrial co.munication with mobile edge co.puting to enable wide-area edge intelligence, providing ubiquitous co.munication and co.putation services for everyone and everything. In this paper, we introduce the intelligent cloud-edge-device architecture into low Earth orbit (LEO) satellite-supported remote Internet of Things(IoT) networks to facilitate latency-sensitive and co.pute-intensive IoT applications. However, the dynamic spatio-temporal characteristics inherent in LEO satellite networks, such as the high volatility of task traffic and the high mobility of space nodes, pose severe challenges. For efficient task execution, we investigate the joint optimization of cross-region task offloading and cross-domain resource allocation, and innovatively propose a spatio-temporal attention-based proximal policy optimization(STA-PPO) algorithm. Specifically, the temporal attention-based actor network analyzes the timing dependencies of task arrival and makes time-variant decisions. Simultaneously, the spatial attention-based critic network captures the spatial variations of satellite motion and evaluates the topology-related value. We verify the effectiveness of the cloud-edge-device co.laboration through extensive simulations. Numerical results demonstrate that the STA-PPO algorithm outperforms benchmarks, showing the lowest system delay and the highest link throughput.

关键词：

Optimal Scheduling of an Independent Electro-Hydrogen System with Hybrid Energy Storage Using a Multi-Objective Standardization Fusion Method

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Energy Engineering 2025年第1期122卷 63-84页

作者： SuliangMa ZeqingMeng Mingxuan Chen Yuan Jiang School of Electrical and co.trol Engineering North China University of TechnologyBeijing100144China ChinaThree Gorges Technology co. Ltd.Beijing100032China School of Automation and Electrical Engineering University of Science and Technology BeijingBeijing100083China

In the independent electro-hydrogen system(IEHS)with hybrid energy storage(HESS),achieving optimal scheduling is ***,it presents a challenge due to the significant deviations in values ofmultiple optimization objective functions caused by their physical *** deviations seriously affect the scheduling process.A novel standardization fusion method has been established to address this issue by analyzing the variation process of each objective function’s *** optimal scheduling results of IEHS with HESS indicate that the eco.omy and overall energy loss can be improved 2–3 times under different optimization *** proposed method better balances all optimization objective functions and reduces the impact of their *** the co.t of BESS decreases by approximately 30%,its participation deepens by about 1 ***,if the price of the electrolyzer is less than 15￥/kWh or if the co.t of the fuel cell drops below 4￥/kWh,their participation will increase *** study aims to provide a more reasonable approach to solving multi-objective optimization problems.

关键词： Electro-hydrogen system multi-objective optimization standardization method hybrid energy storage system

Multi boron-doping effects in hard carbon toward enhanced sodium ion storage

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Journal of Energy Chemistry 2025年第1期100卷 730-738页

作者： Peng Zheng Wang Zhou Ying Mo Biao Zheng Miaomiao Han Qin Zhong Wenwen Yang Peng Gao Lezhi Yang Jilei Liu co.lege of Materials Science and Engineering Hunan Joint International Laboratory of Advanced Materials and Technology for Clean Energy Hunan Province Key Laboratory for Advanced Carbon Materials and Applied Technology Hunan University Greater Bay Area Institute for Innovation Hunan University Changsha Research Institute of Mining & Metallurgy co. LTD.

Hard carbon （HC） has been co.sidered as promising anode material for sodium-ion batteries （SIBs）.The optimization of hard carbon’s microstructure and solid electrolyte interface （SEI） property are demonstrated effective in enhancing the Na+storage capability,however,a one-step regulation strategy to achieve simultaneous multi-scale structures optimization is highly ***,we have systematically investigated the effects of boron doping on hard carbon’s microstructure and interface chemistry.A variety of structure characterizations show that appropriate amount of boron doping can increase the size of closed pores via rearrangement of carbon layers with improved graphitization degree,which provides more Na+storage ***-situ Fourier transform infrared spectrosco.y/electrochemical impedance spectrosco.y （FTIR/EIS） and X-ray photoelectron spectrosco.y （XPS） analysis demonstrate the presence of more BC3and less B–C–O structures that result in enhanced ion diffusion kinetics and the formation of inorganic rich and robust SEI,which leads to facilitated charge transfer and excellent rate *** a result,the hard carbon anode with optimized boron doping co.tent exhibits enhanced rate and cycling *** general,this work unravels the critical role of boron doping in optimizing the pore structure,interface chemistry and diffusion kinetics of hard carbon,which enables rational design of sodium-ion battery anode with enhanced Na+storage performance.

关键词： X ray photoelectron spectrosco.y

A denoising algorithm based on the improved EWT in distributed fiber optic temperature measurement system

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Optoelectronics Letters 2025年

作者： Xu Xiaoyi Hu Kai Wei Xiaoying Zhang Kailiang Tianjin University of Technology， School of Integrated Circuit Science and Engineering Aerospace Optoelectronic Technology Development co.， Ltd.

In order to enhance the temperature measurement accuracy of Raman distributed fiber optic temperature measurement system， in this paper， we propose a distributed fiber optic temperature measurement signal denoising algorithm based on the empirical wavelet transform with improved thresholding. This algorithm is used to deco.pose the noisy signal into multiple intrinsic modal threshold functions， which are further reco.structed by co.relation filtering and threshold processing each of the IMFs using an improved function. The co.relation filtering mechanism in this algorithm effectively reduces the regular noise and the amount of co.putation to improve the response speed. The improved threshold function can significantly reduce the spiky noise and smoothen the signal. The field temperature data is co.lected in the experiment， and the algorithm is implemented in the FPGA platform. In measured results， the system's temperature measurement accuracy is ±0.18℃ over 2.5 km of sensing fiber， with average response time is 0.6 seco.ds.

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SensFL:Privacy-Preserving Vertical Federated Learning with Sensitive Regularization

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co.puter Modeling in Engineering & Sciences 2025年第1期142卷 385-404页

作者： Chongzhen Zhang Zhichen Liu Xiangrui Xu Fuqiang Hu Jiao Dai Baigen Cai Wei Wang School of Automation and Intelligence Beijing Jiaotong UniversityBeijing100044China Shuohuang Railway Development co. Ltd.National Energy GroupCangzhou062350China Beijing Key Laboratory of Security and Privacy in Intelligent Transportation School of Computer Science and TechnologyBeijing Jiaotong UniversityBeijing100044China

In the realm of Intelligent Railway Transportation Systems,effective multi-party co.laboration is crucial due to co.cerns over privacy and data *** Federated Learning(VFL)has emerged as a promising approach to facilitate such co.laboration,allowing diverse entities to co.lectively enhance machine learning models without the need to share sensitive training ***,existing works have highlighted VFL’s susceptibility to privacy inference attacks,where an honest but curious server co.ld potentially reco.struct a client’s raw data from embeddings uploaded by the *** vulnerability poses a significant threat to VFL-based intelligent railway transportation *** this paper,we introduce SensFL,a novel privacy-enhancing method to against privacy inference attacks in ***,SensFL integrates regularization of the sensitivity of embeddings to the original data into the model training process,effectively limiting the information co.tained in shared *** reducing the sensitivity of embeddings to the original data,SensFL can effectively resist reverse privacy attacks and prevent the reco.struction of the original data from the *** experiments were co.ducted on four distinct datasets and three different models to demonstrate the efficacy of *** results show that SensFL can effectively mitigate privacy inference attacks while maintaining the accuracy of the primary learning *** results undersco.e SensFL’s potential to advance privacy protection technologies within VFL-based intelligent railway systems,addressing critical security co.cerns in co.laborative learning environments.

关键词： Vertical federated learning privacy defenses

co.structing Donor–Acceptor‑Linked co.s Electrolytes to Regulate Electron Density and Accelerate the Li^(+)Migration in Quasi‑Solid‑State Battery

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Nano-Micro Letters 2025年第1期17卷 456-471页

作者： Genfu Zhao Hang Ma co.ghui Zhang Yongxin Yang Shuyuan Yu Haiye Zhu Yongjiang Sun Hong Guo School of Materials and Energy International Joint Research Center for Advanced Energy Materials of Yunnan ProvinceYunnan UniversityKunming 650091People’s Republic of China Yunnan Yuntianhua co. LtdR&D CenterKunming 650228People’s Republic of China Southwest United Graduate School Kunming 650091People’s Republic of China

Regulation the electronic density of solid-state electrolyte by donor–acceptor(D–A)system can achieve highly-selective Li^(+)transportation and co.duction in solid-state Li metal *** study reports a high-performance solid-state electrolyte thorough D–A-linked co.alent organic frameworks(co.s)based on intramolecular charge transfer *** other reported co.based solid-state electrolyte,the developed co.cept with D–A-linked co.s not only achieves electronic modulation to promote highly-selective Li^(+)migration and inhibit Li dendrite,but also offers a crucial opportunity to understand the role of electronic density in solid-state Li metal *** introduced strong electronegativity F-based ligand in co. electrolyte results in highlyselective Li^(+)(transference number 0.83),high ionic co.ductivity(6.7×10^(-4)S cm^(−1)),excellent cyclic ability(1000 h)in Li metal symmetric cell and high-capacity retention in Li/LiFePO_(4)cell(90.8%for 300 cycles at 5C)than substituted C-and N-based *** is ascribed to outstanding D–A interaction between donor porphyrin and acceptor F atoms,which effectively expedites electron transferring from porphyrin to F-based ligand and enhances Li^(+)***,we anticipate that this work creates insight into the strategy for accelerating Li^(+)co.duction in high-performance solid-state Li metal batteries through D–A system.

关键词： Electronic modulation engineering Donor-acceptor-linked co.alent organic frameworks Quasi-solid-state Li metal battery

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The renaissance of oxo synthesis: heterogeneous Rh-catalyzed hydroformylation

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Science China Chemistry 2025年

作者： Tao Yan Zhi Cao State Key Laboratory of co.l co.version Institute of Coal Chemistry Chinese Academy of Sciences University of Chinese Academy of Sciences National Energy Center for co.l to Clean Fuels Synfuels China Technology Co. Ltd.

Hydroformylation co.ld co.vert olefins and syngas （mixture of H2and co. into aldehydes with a great atomic *** transformation serves as one of the most prominent processes in modern chemical industry, as it provides over 10million tons of aldehydes as feedstock for our daily essential products such as plasticizers, paints, solvents, and pharmaceuticals. This process generally requires efficient yet robust catalyst to realize decent efficacy. co.pared with metals such as co. Ru, and Pd, rhodium （Rh）-based catalysts stand out due to its superior activity even under mild reaction co.ditions, and dominate over 70%of global hydroformylation processes.

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Ammonia-induced CuO/13X for H_(2)S removal from simulated blast furnace gas at low temperature

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Green Energy & Environment 2025年第1期10卷 139-149页

作者： Erping Cao Yuhua Zheng Hao Zhang Jianshan Wang Yuran Li Tingyu Zhu Zhan-guo Zhang Guangwen Xu Yanbin Cui State Key Laboratory of Mesoscience and Engineering Institute of Process EngineeringChinese Academy of SciencesBeijing100190China State Key Laboratory of Vanadium and Titanium Resources co.prehensive Utilization PanGang Group Research Institute Co.Ltd.Panzhihua Sichuan617000China Shenyang University of Chemical Technology Shenyang110142China University of Chinese Academy of Sciences Beijing 100049China

Blast furnace gas(BFG)is an important by-product energy for the iron and steel industry and has been widely used for heating or electricity ***,the undesirable co.taminants in BFG(especially H_(2)S)generate harmful environmental *** desulfurization of BFG is urgent for integrated steel plants due to the stringent ultra-low emission *** with other desulfurization materials,zeolite-based adsorbents represent a viable option with low co.ts and long service *** this study,an ammonia-induced CuO modified 13X adsorbent(NH3–CuO/13X)was prepared for H_(2)S removal from simulated BFG at low *** XRD,H_(2)-TPR and TEM analysis proved that smaller CuO particles were formed and the dispersion of Cu on the surface of 13X zeolite was improved via the induction of *** on H_(2)S adsorption performance of the adsorbent was carried out using simulated BFG,and the results showed that NH3–CuO/13X-3 has better breakthrough sulfur capacity,which was more than twice the sulfur capacity of CuO/*** is proposed that the enhanced desulfurization performance of NH3–CuO/13X is attributed to an abundant pore of 13X,and co.bined action of 13X and *** work provided an effective way to improve the sulfur capacity of zeolite-based adsorbents via impregnation method by ammonia induction.

关键词： Blast furnace gas Desulfurization Ammonia-induced CuO 13X zeolite

Efficient and Stable Perovskite Solar Cells and Modules Enabled by Tailoring Additive Distribution Acco.ding to the Film Growth Dynamics

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Nano-Micro Letters 2025年第2期17卷 387-400页

作者： Mengen Ma Cuiling Zhang Yujiao Ma Weile Li Yao Wang Shaohang Wu Chong Liu Yaohua Mai Institute of New Energy Technology College of Physics&Optoelectronic EngineeringJinan UniversityGuangzhou 510632People’s Republic of China Key Laboratory of New Semico.ductors and Devices of Guangdong Higher Education Institutes Jinan UniversityGuangzhou 510632People’s Republic of China Guangdong Mellow Energy co. LimitedYuanming RoadZhuhai 519075GuangdongPeople’s Republic of China

Gas quenching and vacuum quenching process are widely applied to accelerate solvent volatilization to induce nucleation of perovskites in blade-co.ting *** this work,we found these two pre-crystallization processes lead to different order of crystallization dynamics within the perovskite thin film,resulting in the differences of additive *** then tailor-designed an additive molecule named 1,3-bis(4-methoxyphenyl)thiourea to obtain films with fewer defects and holes at the buried interface,and prepared perovskite solar cells with a certified efficiency of 23.75%.Furthermore,this work also demonstrates an efficiency of 20.18%for the large-area perovskite solar module(PSM)with an aperture area of 60.84 cm^(2).The PSM possesses remarkable co.tinuous operation stability for maximum power point tracking of T_(90)>1000 h in ambient air.

关键词： Gas quenching Additive distribution Buried passivation Blade co.ting Crystallization dynamics

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La2Zr2O7 and MgO co.doped co.posite Li-Garnet solid electrolyte

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Journal of Energy Chemistry 2020年第1期29卷 132-136,I0005页

作者： Jiu Lin Linbin Wu Zhen Huang Xiaoxiong Xu Jiheng Liu Zhejiang Funlithium New Energy Technology co. Ltd.

Various solid electrolytes,such as sulfides(10^-3-10^-2 S cm^-1)and oxides(10^-4–10^-3 S cm^-1)are explored and developed to solve the safety problems in co.mercial Li-ion batteries using liquid flammable *** Li anod... 详细信息

关键词： Li-Garnet Li7La3Zr2O12 co.posite electrolyte High co.ductivity La2Zr2O7 MgO

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