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Chinese Chemical Letters 2024年第3期35卷 443-448页

作者： Linhe Xu Xueshan Hu Shuang Zhou Ze Zhang Junxian Zhang Chao Li Daxian Zuo Hao Liu Gang Chen Jiayu Wan Jinsong Tao State Key lab of Pulp and Paper Engineering South China University of TechnologyGuangzhou 510640China future Battery Research Center Global Institute of Future TechnologyShanghai Jiao Tong UniversityShanghai 200240China

Accurate detection of uric acid(UA)is crucial for diagnosing gout,yet traditional sweat-based UA sensors continue to face challenges posed by complex and costly electrode fabrication methods,as well as weakly hydrophilic ***,we designed and developed simple,low-cost,and hydrophilic sweat UA detection sensors constructed by carbon electrodes and cellulose paper *** carbon electrodes were made by carbonized polyimide films through a simple,one-step laser engraving *** electrodes are porous,possess a large specific surface area,and are flexible and *** substrates were composed of highly hydrophilic cellulose paper that can effectively collect,store,and transport *** constructed electrodes demonstrate high sensitivity of 0.4μA Lμmol^(-1)cm^(-2),wide linear range of 2–100μmol/*** addition,our electrodes demonstrate high selectivity,excellent reproducibility,high flexibility,and outstanding stability against mechanical bending,temperature variations,and extended storage ***,our sensors have been proven to provide reliable results when detecting UA levels in real sweat and on real human *** envision that these sensors hold enormous potential for use in the prognosis,diagnosis,and treatment of gout.

关键词： Laser-engraved carbon Polyimide Cellulose paper Hydrophilicity Sweat uric acid

Highly responsive broadband Si-based MoS2 phototransistor on high-k dielectric

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Science China(Information Sciences) 2024年第6期67卷 180-189页

作者： Ali IMRAN Xin HE Jiwei LIU Qinghai ZHU Muhammad SULAMAN Fei XUE Mingsheng XU Deren YANG College of Integrated Circuits State Key Laboratory of Silicon and Advanced Semiconductor MaterialsZhejiang University ZJU-Hangzhou global Scientific and Technological Innovation Centre School of Materials Science and Engineering State Key Laboratory of Silicon and Advanced Semiconductor MaterialsZhejiang University Beijing Key lab of Nanophotonics and Ultrafine Optoelectronic Systems School of PhysicsBeijing Institute of Technology

The demand for photodetectors and image sensors has grown exponentially in the past decade in biomedical, security surveillance, robotics, automotive, quality control, image recognition, and military applications, due to their superior quality, broadband detection, lower noise, and economic viability. Here,we report a MoS2channel-based phototransistor over an HfO2/n-Si substrate isolated by an h BN layer. The high photoresponse is achieved through the integration of the photoconduction, photogating, and mobility enhancement process by utilizing excellent features of MoS2, HfO2/Si, and h BN. The capacitive coupling of the photogenerated carriers by high-k dielectric HfO2leads to modulation of MoS2Fermi level due to electrostatic doping. Furthermore, the MoS2also contributes to the photogeneration of carriers due to its semiconducting nature, leading to additional photocurrent. Ultimately, the combination of photogating,photoconduction, and swift carrier extraction with remarkable mobility of 11.65 cm2· V-1· s-1results in high responsivity, external quantum efficiency, and detectivity of 4.5 × 10～8A · W-1, 0.72 × 10～6, and 6.20× 1016Jones at 266 nm illumination, respectively. The device also demonstrates broadband photoresponse from 266–1000 nm wavelengths. The high responsivity distinguishes the potential of our device for the future of optoelectronics and broadband image sensing applications.

关键词： photogating photoconduction two-dimensional materials high $~k$ dielectric carrier scattering phototransistor

Healthy and low-carbon communities: Design, optimization, and new technologies

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建筑模拟(英文) 2023年第9期16卷 1583-1585页

作者： Jianlin Liu Xing Zheng Yixing Chen College of Environmental Science and Engineering Donghua UniversityChina future cities lab global Singapore-ETH CentreSingapore College of Civil Engineering Hunan UniversityChina

As the world grapples with the challenges of global warming,the urban heat island(UHI)effect,urban air pollution,and the imperative to transition towards low-carbon economies,the role of communities in fostering sustainability and innovation becomes more critical than *** example,the frequent occurrences of air pollution and extreme weather conditions have seriously threatened residents’health and property *** global warming and urban heat island effect bring challenges to the climate resilience of *** has accelerated the growth of building stock and urban energy consumption.

关键词： pollution island warming

Nonlinear relationship between urban form and transport CO2 emissions:Evidence from Chinese cities based on machine learning

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Journal of Geographical Sciences 2024年第08期34卷 1558-1588页

作者： LI Linna DENG Zilin HUANG Xiaoyan Faculty of Geographical Science Beijing Normal University Northwest Land and Resources Research Center Global Regional and Urban Research InstituteShaanxi Normal University

Reducing carbon emissions from the transport sector is essential for realizing the carbon neutrality goal in *** substantial studies on the influence of urban form on transport CO2emissions,most of them have treated the effects as a linear process,and few have studied their nonlinear *** research focused on 274 Chinese cities in2019 and applied the gradient-boosting decision tree （GBDT） model to investigate the nonlinear effects of four aspects of urban form,including compactness,complexity,scale,and fragmentation,on urban transport *** was found that urban form contributed20.48%to per capita transport CO2emissions （PTCEs）,which is less than the contribution of socioeconomic development but more than that of transport *** contribution of urban form to total transport CO2emissions （TCEs） was the lowest,at 14.3%.In particular,the effect of compactness on TCEs was negative within a threshold,while its effect on PTCEs showed an inverted U-shaped *** effect of complexity on PTCEs was positive,and its effect on TCEs was *** effect of scale on TCEs and PTCEs was positive within a threshold and negative beyond that *** effect of fragmentation on TCEs was also nonlinear,while its effect on PTCEs was positively *** results show the complex effects of the urban form on transport ***,strategies for optimizing urban form and reducing urban transport carbon emissions are recommended for the future.

关键词： urban form transport CO,emissions nonlinear effect sustainable transport gradient-boosting decision treemodel

Highly responsive broadband Si-based MoSphototransistor on high-k dielectric

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Science China(Information Sciences) 2024年

作者： Ali IMRAN Xin HE Jiwei LIU Qinghai ZHU Muhammad SULAMAN Fei XUE Mingsheng XU Deren YANG Beijing Key lab of Nanophotonics and Ultrafine Optoelectronic Systems School of PhysicsBeijing Institute of Technology ZJU-Hangzhou global Scientific and Technological Innovation Centre College of Integrated Circuits State Key Laboratory of Silicon and Advanced Semiconductor MaterialsZhejiang University School of Materials Science and Engineering State Key Laboratory of Silicon and Advanced Semiconductor MaterialsZhejiang University

The demand for photodetectors and image sensors has grown exponentially in the past decade in biomedical, security surveillance, robotics, automotive, quality control, image recognition, and military applications, due to their superior quality, broadband detection, lower noise, and economic viability. Here,we report a MoS2channel-based phototransistor over an HfO2/n-Si substrate isolated by an h BN layer. The high photoresponse is achieved through the integration of the photoconduction, photogating, and mobility enhancement process by utilizing excellent features of MoS2, HfO2/Si, and h BN. The capacitive coupling of the photogenerated carriers by high-k dielectric HfO2leads to modulation of MoS2Fermi level due to electrostatic doping. Furthermore, the MoS2also contributes to the photogeneration of carriers due to its semiconducting nature, leading to additional photocurrent. Ultimately, the combination of photogating,photoconduction, and swift carrier extraction with remarkable mobility of 11.65 cm2·V-1·s-1results in high responsivity, external quantum efficiency, and detectivity of 4.5×108A·W-1, 0.72×106, and 6.20×1016Jones at 266 nm illumination, respectively. The device also demonstrates broadband photoresponse from 266–1000 nm wavelengths. The high responsivity distinguishes the potential of our device for the future of optoelectronics and broadband image sensing applications.

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Advancements,strategies,and prospects of solid oxide electrolysis cells(SOECs):Towards enhanced performance and large-scale sustainable hydrogen production

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Journal of Energy Chemistry 2024年第7期94卷 688-715页

作者： Amina Lahrichi Youness El Issmaeli Shankara S.Kalanur Bruno G.Pollet Green Hydrogen lab(GH2lab) Hydrogen Research Institute(HRI)Universitédu QuébecàTrois-Rivières(UQTR)3351 boulevard des ForgesTrois-RivièresQuébec G9A 5H7Canada

Solid oxide electrolysis cells(SOECs)represent a crucial stride toward sustainable hydrogen generation,and this review explores their current scientific challenges,significant advancements,and potential for large-scale hydrogen *** SOEC technology,the application of innovative fabrication tech-niques,doping strategies,and advanced materials has enhanced the performance and durability of these systems,although degradation challenges persist,implicating the prime focus for future *** we provide in-depth analysis of the recent developments in SOEC technology,including Oxygen-SOECs,Proton-SOECs,and ***,Hybrid-SOECs,with their mixed ionic conducting electrolytes,demonstrate superior efficiency and the concurrent production of hydrogen and *** with the capacity to harness waste heat,these advancements in SOEC technology present signif-icant promise for pilot-scale applications in *** review also highlights remarkable achieve-ments and potential reductions in capital expenditure for future SOEC systems,while elaborating on the micro and macro aspects of sOECs with an emphasis on ongoing research for optimization and *** concludes with the potential of SOEC technology to meet various industrial energy needs and its significant contribution considering the key research priorities to tackle the global energy demands,ful-fillment,and decarbonization efforts.

关键词： Solid oxide electrolysis cells Proton-SOECs Oxygen-SoECs Hybrid-SOECs Intermediate-high temperature electrolysers Hydrogenproduction

Full-Scale Isogeometric Topology Optimization of Cellular Structures Based on Kirchhoff-Love Shells

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Computer Modeling in Engineering & Sciences 2024年第6期139卷 2479-2505页

作者： Mingzhe Huang Mi Xiao Liang Gao Mian Zhou Wei Sha Jinhao Zhang State Key lab of Intelligent Manufacturing Equipment and Technology Huazhong University of Science and TechnologyWuhan430074China

Cellular thin-shell structures are widely applied in ultralightweight designs due to their high bearing capacity and strength-to-weight *** this paper,a full-scale isogeometric topology optimization(ITO)method based on Kirchhoff-Love shells for designing cellular tshin-shell structures with excellent damage tolerance ability is *** method utilizes high-order continuous nonuniform rational B-splines(NURBS)as basis functions for Kirchhoff-Love shell *** geometric and analysis models of thin shells are unified by isogeometric analysis(IGA)to avoid geometric approximation error and improve computational *** topological configurations of thin-shell structures are described by constructing the effective density field on the *** volume constraints are imposed in the proximity of each control point to obtain bone-like cellular *** facilitate numerical implementation,the p-norm function is used to aggregate local volume constraints into an equivalent global *** numerical examples are provided to demonstrate the effectiveness of the proposed *** simulation and comparative analysis,the results indicate that the cellular thin-shell structures optimized by the proposed method exhibit great load-carrying behavior and high damage robustness.

关键词： Cellular thin-shell structures isogeometric analysis full-scale topology optimization Kirchhoff–Love shells

Physio-chemical modeling of the NO_(x)-O_(3) photochemical cycle and the air pollutants’ reactive dispersion around an isolated building

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建筑模拟(英文) 2023年第9期16卷 1735-1758页

作者： Yunfei Fu Xisheng Lin Xing Zheng Liangzhu Wang Chun-Ho Liu Xuelin Zhang Cruz Y.Li K.T.Tse Department of Civil and Environmental Engineering The Hong Kong University of Science and TechnologyClear Water BayKowloonHong KongChina future cities lab global Singapore-ETH CentreSingapore 138602 Department of Building Civil and Environmental Engineering at Concordia UniversityMontrealQuebecCanada Department of Mechanical Engineering The University of Hong KongPok-fu-lam RoadHong KongChina Department of Civil Engineering Chongqing UniversityChongqingChina School of Atmospheric Sciences Sun Yat-sen UniversityZhuhaiChina

A numerical physio-chemical model of the NO_(x)-O_(3) photochemical cycle in the near-wake region of an isolated residential/office building has been presented in this *** investigation delves into the dispersion of reactive air pollutants through the lens of fluid phenomenology and its impact on chemical reactivity,formation,transport,deposition,and *** fluid dynamics(CFD)simulations were conducted for the ground-point-source(GES)and roof-pointsource(RES)*** show that the Damköhler number(Da),which quantifies pollutants’physio-chemical timescales,displays a strong inverse proportionality with the magnitude and spread of NO–increasing Da reduces human exposure to the toxic NO and NO_(2) *** different wind directions were considered,the dispersion range of NO exhibited varying shrinking directions as Da ***,as Da increases,the concentration ratio KNO_(2)/KNO_(x),which quantifies the production of NO_(2) resulting from NO depletion,forms sharp high-low gradients near emission *** GES,the dispersion pattern is governed by the fluid’s phenomenological *** RES,the intoxicated area emanates from the building’s leading-edge,with the lack of shielding inhibiting pollutant interactions in the near-wake,resulting in scant physio-chemical *** NO_(2)/NO_(x) distribution follows a self-similar,stratified pattern,exhibiting consistent layering gradients and attributing to the natural deposition of the already-reacted pollutants rather than in-situ *** the end,building design guidelines have been proposed to reduce pedestrian and resident exposure to NO_(x)-O_(3).

关键词： reactive pollutant dispersion NO_(x)-O_(3)cycle air pollution isolated building physio-chemical modelling

A survey on blockchain-enabled federated learning and its prospects with digital twin

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Digital Communications and Networks 2024年第2期10卷 248-264页

作者： Kangde Liu Zheng Yan Xueqin Liang Raimo Kantola Chuangyue Hu State Key lab on Integrated Services Network School of Cyber EngineeringXidian UniversityXi'anChina Department of Communications and Networking Aalto UniversityEspooFinland Yangtze Delta Region Blockchain Technology Research Institute JiaxingChina

Digital Twin(DT)supports real time analysis and provides a reliable simulation platform in the Internet of Things(IoT).The creation and application of DT hinges on amounts of data,which poses pressure on the application of Artificial Intelligence(AI)for DT descriptions and intelligent *** Learning(FL)is a cutting-edge technology that enables geographically dispersed devices to collaboratively train a shared global model locally rather than relying on a data center to perform model ***,DT can benefit by combining with FL,successfully solving the"data island"problem in traditional ***,FL still faces serious challenges,such as enduring single-point failures,suffering from poison attacks,lacking effective incentive *** the successful deployment of DT,we should tackle the issues caused by *** from industry and academia have recognized the potential of introducing Blockchain Technology(BT)into FL to overcome the challenges faced by FL,where BT acting as a distributed and immutable ledger,can store data in a secure,traceable,and trusted ***,to the best of our knowledge,a comprehensive literature review on this topic is still *** this paper,we review existing works about blockchain-enabled FL and visualize their prospects with *** this end,we first propose evaluation requirements with respect to security,faulttolerance,fairness,efficiency,cost-saving,profitability,and support for ***,we classify existing literature according to the functionalities of BT in FL and analyze their advantages and disadvantages based on the proposed evaluation ***,we discuss open problems in the existing literature and the future of DT supported by blockchain-enabled FL,based on which we further propose some directions for future research.

关键词： Digital twin Artificial intelligence Federated learning Blockchain

Cloud-Assisted Distributed Edge Brains for Multi-Cell Joint Beamforming Optimization for 6G

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China Communications 2022年第3期19卷 36-49页

作者： Juan Deng Kaicong Tian Qingbi Zheng Jielin Bai Kuo Cui Yitong Liu Guangyi Liu Beijing University of Posts and Telecommunications Beijing 100876China future Research lab China Mobile Research InstituteBeijing 100032China

In 5G networks,optimization of antenna beam weights of base stations has become the key application of AI for network *** 6G,higher frequency bands and much denser cells are expected,and the importance of automatic and accurate beamforming assisted by AI will become more *** existing network,servers are“patched”to network equipment to act as a centralized brain for model training and inference leading to high transmission overhead,large inference latency and potential risks of data *** architectures have been proposed to achieve flexible parameter configuration and fast local response,but it is inefficient in collecting and sharing global information among base *** this paper,we propose a novel solution based on a collaborative cloud edge architecture for multi-cell joint beamforming *** analyze the performance and costs of the proposed solution with two other architectural solutions by *** with the centralized solution,our solution improves prediction accuracy by 24.66%,and reduces storage cost by 83.82%.Compared with the decentralized solution,our solution improves prediction accuracy by 68.26%,and improves coverage performance by 0.4 *** last,the future research work is prospected.

关键词： artificial intelligence collaborative cloud edge centralized cloud brain decentralized edge brain 6G mobile communication