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Regulation of photophysical and electronic properties of I-III-VI quantum dots for light-emitting diodes

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Science China Materials 2024年第9期67卷 2737-2748页

作者： Xiaofei Dong Xianggao Li Shougen Yin Zheng Li Longwu Li Jingling Li School of Science Langfang Normal UniversityLangfang 065000China School of Chemical Engineering and Technology Tianjin UniversityTianjin 300350China institute of Material Physics Key Laboratory for Optoelectronic Materials and Devices of TianjinKey Laboratory of Display Materials and Photoelectric Devices of Ministry of EducationTianjin University of TechnologyTianjin 300384China College of Chemistry and Materials Science Langfang Normal UniversityLangfang 065000China School of Materials Science and Hydrogen Energy Foshan UniversityFoshan 528000China

Quantum dot light-emitting diodes(QLEDs)have become an important research direction in the pursuit of next-generation display technology owing to their favorable attributes,including high energy efficiency,wide color gamut,and low *** in the luminous efficiency and operating life of QLEDs have been achieved by enhancing the photoluminescence efficiency of the quantum dots(QDs)and optimizing the device ***,the current mainstream QDs contain heavy metal elements such as lead and cadmium,which restrict the development and application of QD *** new types of environmentally friendly QDs is crucial.I-III-VI semiconductor QDs have been developed as luminescent materials for constructing high color rendering index QLEDs,owing to the outstanding photophysical properties of these QDs,such as composition-dependent tunable bandgap,large Stokes shift,and highefficiency ***,the microstructures of heterojunctions,especially the surface states and interface states,affect the recombination and transport of carriers in electroluminescent(EL)devices with multilayer thin film structures,which in turn influence the luminous efficiency and stability of the *** review focuses on the synthesis strategies of I-III-VI multi-component QDs and provides an in-depth understanding of the luminescence mechanism and the regulation of photophysical and electronic ***,the application of I-III-VI QDs in multi-color and white EL QLEDs is discussed and the challenges and outlook are addressed.

关键词： Ⅰ-Ⅲ-Ⅵquantum dots synthesis method defect states luminescence mechanism light-emitting diodes

Revealing the key role of non-solvating diluents for fast-charging and low temperature Li-ion batteries

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Journal of Energy Chemistry 2024年第7期94卷 171-180页

作者： Yuping Zhang Siyin Li Junkai Shi Jiawei Lai Ziyue Zhuang Jingwen Liu Wenming Yang Liang Ma Yue-Peng Cai Jijian Xu Qifeng Zheng School of Chemistry Guangzhou Key Laboratory of Materials for Energy Conversion and StorageSouth China Normal UniversityGuangzhou 510006GuangdongChina Guangzhou foreign language School Guangzhou 511455GuangdongChina Department of Chemistry City University of Hong KongHong Kong 999077China

Fast-charging and low temperature operation are of vital importance for the further development of lithium-ion batteries(LIBs),which is hindered by the utilization of conventional carbonate-based electrolytes due to their slow kinetics,narrow operating temperature and voltage ***,an acetonitrile(AN)-based localized high-concentration electrolyte(LHCE)is proposed to retain liquid state and high ionic conductivity at ultra-low temperatures while possessing high oxidation *** originally reveal the excellent thermal shielding effect of non-solvating diluent to prevent the aggregation of Li^(+) solvates as temperature drops,maintaining the merits of fast Li transport and facile desolvation as at room temperature,which bestows the graphite electrode with remarkable low temperature performance(264 mA h g^(-1) at-20 C).Remarkably,an extremely high capacity retention of 97%is achieved for high-voltage high-energy graphite||NCM batteries after 250 cycles at-20 C,and a high capacity of 110 mA h g^(-1)(71%of its room-temperature capacity)is retained at-30°*** study unveils the key role of the non-solvating diluents and provides instructive guidance in designing electrolytes towards fast-charging and low temperature LIBs.

关键词： Li-ion battery Fast-charging Low temperature Non-solvating diluent Shielding effect

Deep Broad Learning for Emotion Classification in Textual Conversations

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Tsinghua Science and Technology 2024年第2期29卷 481-491页

作者： Sancheng Peng Rong Zeng Hongzhan Liu Lihong Cao Guojun Wang Jianguo Xie Center for Linguistics and Applied Linguistics and Laboratory of Language Engineering and ComputingGuangdong University of Foreign StudiesGuangzhou 510006China Guangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices South China Normal UniversityGuangzhou 510006China School of Computer Science and Cyber Engineering Guangzhou UniversityGuangzhou 510006China Modern Education Technology Center Guangdong University of Foreign StudiesGuangzhou 510006China

Emotion classification in textual conversations focuses on classifying the emotion of each utterance from textual *** is becoming one of the most important tasks for natural language processing in recent ***,it is a challenging task for machines to conduct emotion classification in textual conversations because emotions rely heavily on textual *** address the challenge,we propose a method to classify emotion in textual conversations,by integrating the advantages of deep learning and broad learning,namely *** aims to provide a more effective solution to capture local contextual information(i.e.,utterance-level)in an utterance,as well as global contextual information(i.e.,speaker-level)in a conversation,based on Convolutional Neural Network(CNN),Bidirectional Long Short-Term Memory(Bi-LSTM),and broad *** experiments have been conducted on three public textual conversation datasets,which show that the context in both utterance-level and speaker-level is consistently beneficial to the performance of emotion *** addition,the results show that our proposed method outperforms the baseline methods on most of the testing datasets in weighted-average F1.

关键词： emotion classification textual conversation Convolutional Neural Network(CNN) Bidirectional Long Short-Term Memory(Bi-LSTM) broad learning

Research on“Chinese+Law”Teaching Resources in Thailand

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Journal of Contemporary Educational Research 2024年第7期8卷 169-173页

作者： Wenbo Yang institute for the Development of International Chinese language Education Tianjin Normal UniversityTianjin 300380China

This article details the distinctive progress in Thailand’s“Chinese+Law”*** then examines the development of related teaching resources,culminating in three key conclusions:(1)The integration of“Chinese”and“Law”in Thai vocational education is insufficient;(2)Teaching resources for“Chinese+Law”in Thailand are scarce and of subpar ***,there are only print textbooks available,with no accompanying digital or multimedia resources developed;(3)The optimal approach for“Chinese+Law”teaching materials in Thailand should involve collaborative efforts between Chinese and Thai experts.

关键词： “Chinese+Law” Teaching resources Case analysis

PbrARF4 contributes to calyx shedding of fruitlets in ‘Dangshan Suli’ pear by partly regulating the expression of abscission genes

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Horticultural Plant Journal 2024年第2期10卷 341-354页

作者： Guoling Guo Pengfei Wei Tao Yu Haiyan Zhang Wei Heng Lun Liu Liwu Zhu Bing Jia School of Horticulture Anhui Agricultural UniversityHefeiAnhui 230036China Huayuan foreign language School Zhejiang Normal UniversityJinhuaZhejiang 322100China Agricultural Experimental Center of Guiyang Guiyang Agriculture and Rural BureauGuiyangGuizhou 550018China

Fruitlet calyx shedding in pear plants is apparently regulated via numerous pathways that involve both environmental triggers and phytohormones cues such as auxin. In this study, we found at 10 days after full bloom (DAFB) higher levels of indoleacetic acid (IAA) and tryptophan (Trp) in calyx persistence fruitlet (CPF) than calyx shedding fruitlet (CSF) ofDanshan Suli’ pear (Pyrus bretschneideri Rhed.). Consisting with this, the activity of indolealdehyde oxidase (IAAIdO), which promotes IAA synthesis, was remarkably increased, and that of peroxidase(POD), which degrades IAA, dropped markedly in CPF but not in CSF. Further, qRT-PCR results revealed that most of 31 PbrARFs (encoding auxin response factors) in Pyrus bretschneideri were highly expressed in CPF, whereas PbrARF4, PbrARF24 and PbrARF26 were significantly downregulated in CPF vis-a-vis CSF. Phylogenetic analysis revealed that 6 PbrARFs clustered in the group III, where PbrARF4 showed the closest affinity with AtARF1 that promotes organ abscission, indicating a putative role of PbrARF4 in mediating the process of calyx shedding in pear. In fact, the ectopic overexpression of PbrARF4 in Solanum lycopersicum resulted in an earlier-formed and deeper abscission layer (AL) in the transgenic plants, whose calyxes were more prone to wilt at the mature red stage (MR) compared with the control plants (wild-type). More importantly, expression levels of the abscission genes SILS and Sl Cel2 in transgenic plants overexpressing PbrARF4 were significantly upregulated in comparation with the WT, whereas those of Sl BI and Sl TAPG2 were considerably inhibited. Further, PbrJOINTLESS and PbrIDA,the two genes related to calyx shedding in pear, were up-regulated more in CSF than CPF. The findings contribute to a better understanding of PbrARFs involved in fruitlet calyx shedding of pear, which could prove beneficial to improving the quality of pear fruit.

关键词： Pear Pyrus bretschneideri Rehd Calyx shedding IAA PbrARF4 Abscission genes

Event-triggered adaptive output feedback control for hyperbolic PDEs: swapping-based design

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Science China(Information Sciences) 2024年第5期67卷 327-328页

作者： Chunting JI Zhengqiang ZHANG Xue-Jun XIE School of Engineering Qufu Normal University institute of Automation Qufu Normal University

Partial differential equations(PDEs) characterize transport phenomena and fluid flow, and common cases include heat exchangers and road traffic [1]. Recently, scholars have become enthusiastic about event-triggered control(ETC) of hyperbolic PDEs, primarily because it can help conserve computing and communication resources. For example,Ref. [2] presented an output feedback ETC scheme for 2 × 2hyperbolic PDEs.

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The biological functions and metabolic pathways of valine in swine

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Journal of Animal Science and Biotechnology 2024年第1期15卷 20-34页

作者： Chuni Wang Yao Peng Yiru Zhang Juan Xu Sheng Jiang Leli Wang Yulong Yin institute of Subtropical Agriculture Chinese Academy of SciencesChangshaChina Hunan Provincial Key Laboratory of Animal Intestinal Function and Regulation College of Life SciencesHunan Normal UniversityChangshaChina tianjin institute of Industrial Biotechnology Chinese Academy of SciencesTianjinChina

Valine is an essential amino acid and a type of branched-chain amino acid. Due to the involvement of branchedchain amino acids in various metabolic pathways, there has been a surge of interests in valine nutrition and its role in animal physiology. In pigs, the interactions between valine and other branched-chain amino acids or aromatic amino acids are complex. In this review, we delve into the interaction mechanism, metabolic pathways, and biological functions of valine. Appropriate valine supplementation not only enhances growth and reproductive performances, but also modulates gut microbiota and immune functions. Based on past observations and interpretations, we provide recommended feed levels of valine for weaned piglets, growing pigs, gilts, lactating sows, barrows and entire males. The summarized valine nutrient requirements for pigs at different stages offer valuable insights for future research and practical applications in animal husbandry.

关键词： Additional dosage Biological function Metabolic pathway Pig Valine

Design and synthesis of polyoxovanadate-based framework for efficient dye degradation

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Tungsten 2024年第2期6卷 447-453页

作者： Qing Lan Su-Juan Jin Zheng Wang Xu-Yang Li Yan Xiong Zhuo-Cheng Wang Shan-Shan Liu Zhi-Ming Zhang Qiang Zhao Engineering Technology Research Center of Henan Province for Solar Catalysis School of Chemical and Pharmaceutical EngineeringNanyang Normal UniversityNanyang 473061China institute of New Energy Materials&Low Carbon Technology Tianjin University of TechnologyTianjin 300384China

A new polyoxovanadate-based framework material[Cu(en)_(2)]_(4)V_(18)O_(42)(H_(2)O)·6H_(2)O(1)was designed and synthesized by hydrothermal reaction of NaVO_(3),Cu(NO_(3))_(2)·6H_(2)O and 1,2-diaminoethane(en)via carefully adjusting the pH value of the reaction *** structure of the title compound has been determined by single-crystal X-ray diff raction analysis,thermogravimetric analysis,infrared spectra and elemental *** structural analysis demonstrate the three-dimensional(3D)framework structure of compound 1,which was composed of the[V_(18)O_(42)(H_(2)O)]_(8)−({V_(18)O_(42)(H_(2)O)})anions linked by the Cu^(2+)*** 1 represents the fi rst 3D framework based on{V_(18)O_(42)(H_(2)O)}polyoxoanions and copper ***-driven degradation of residual organic pollutants in industrial wastewater is still a major problem for human *** experiments reveal that compound 1 possesses of excellent photocatalytic activity for the degradation of methylene blue and rhodamine B.

关键词： Polyoxovanadate Framework Polyoxovanadate-based framework Photocatalytic Organic pollutants

A single micro-LED manipulation system based on micro-gripper

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Nanotechnology and Precision Engineering 2024年第2期7卷 45-52页

作者： Jie Bai Pingjuan Niu Erdan Gu Jianming Li Clarence Augustine TH Tee School of Mechanical Engineering Tiangong University School of Electronic and Information Engineering Tiangong University institute of Photonics University of Strathclyde tianjin Key Laboratory of Micro Low Gravity Environment Simulation Technology Tianjin Aerospace Electromechanical Equipment Research Institute Department of Electrical and Information Engineering School of Physics and Electrical Information EngineeringZhejiang Normal University

Micro-LEDs(μLEDs) have advantages in terms of brightness, power consumption, and response speed. In addition, they can also be used as micro-sensors implanted in the body via flexible electronic skin. One of the key techniques involved in the fabrication of μLED-based devices is transfer printing. Although numerous methods have been proposed for transfer printing, improving the yield of μLED arrays is still a formidable task. In this paper, we propose a novel method for improving the yield of μLED arrays transferred by the stamping method, using an innovative design of piezoelectrically driven asymmetric micro-gripper. Traditional grippers are too large to manipulate μLEDs, and therefore two micro-sized cantilevers are added at the gripper tips. A μLED manipulation system is constructed based on the micro-gripper together with a three-dimensional positioning system. Experimental results using this system show that it can be used successfully to manipulate μLED arrays.

关键词： Micro-gripper Micro-LED Transfer printing Manipulation