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Magnetism Measurements of Two-Dimensional van der Waals Antiferromagnet CrPS_(4)Using Dynamic Cantilever Magnetometry

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Chinese Physics letters 2024年第10期41卷 123-128页

作者： Qi Li Weili Zhen Ning Wang Meng Shi Yang Yu Senyang Pan Lin Deng Jiaqiang Cai Kang Wang Lvkuan Zou Zhongming Zeng Zhaosheng Wang Jinglei Zhang Anhui Province Key Laboratory of Condensed Matter Physics at Extreme Conditions High Magnetic Field LaboratoryHFIPSChinese Academy of SciencesHefei 230031China science Island Branch of Graduate School University of Science and Technology of ChinaHefei 230026China School of Advanced Manufacturing Engineering Hefei UniversityHefei 230601China Suzhou Institute of Nano-tech and Nano-bionics Chinese Academy of SciencesSuzhou 215123China

Recent experimental and theoretical work has focused on two-dimensional van der Waals(2D vdW)magnets due to their potential applications in sensing and spintronics *** measurements of these emerging materials,conventional magnetometry often encounters challenges in characterizing the magnetic properties of small-sized vdW materials,especially for antiferromagnets with nearly compensated magnetic ***,we investigate the magnetism of 2D antiferromagnet CrPS_(4)with a thickness of 8nm by using dynamic cantilever magnetometry(DCM).

关键词： (4) magnets Magnet

Optical secret sharing by multi-step liquid crystal planar doublet panning and coupling

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Chinese Optics letters 2024年第8期22卷 21-28页

作者： Zhichang Mo Yi Chen Xiangyu Zhu Zhouhao Zhang Dawei Li Jianda Shao Yuanan Zhao Jianguo Wang Laboratory of Thin Film Optics Shanghai Institute of Optics and Fine MechanicsChinese Academy of SciencesShanghai 201800China Center of Materials science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Key Laboratory of Materials for High Power Laser Chinese Academy of SciencesShanghai 201800China Henan Key Laboratory of Infrared Materials&Spectrum Measures and Applications School of PhysicsHenan Normal UniversityXinxiang 453007China Hangzhou Institute for Advanced Study University of Chinese Academy of SciencesHangzhou 310024China

The hologram, which is formed by phases coupled through cascade devices for secret information sharing, still carries a cracking risk. We propose a liquid crystal planar doublet as the information carrier, and new holograms generated by the new coupled phases when the relative displacements of the different liquid crystal layers change. The designed geometrical phases are generated by an optimized iterative restoration algorithm, and each holographic image formed by these phases is readable. This scheme achieves an increase in the capacity of the stored secret information and provides more misdirection, which is expected to have potential value in optical steganography and storage.

关键词： liquid crystal holography optical steganography displacement coupled geometrical phase

The remarkable effect of amino hydrogen on membrane permeability and organelle staining of 1,8-naphthalimide dyes

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Chinese Chemical letters 2024年第2期35卷 347-351页

作者： Zhifeng Li Qinglong Qiao Ning Xu Kai An Wenchao Jiang Yi Tao Pengjun Bao Yinchan Zhang Zhaochao Xu School of Chemistry Dalian University of TechnologyDalian 116024China CAS Key Laboratory of Separation science for Analytical Chemistry Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China University of Chinese academy of sciences Beijing 100049China

Membrane permeability and intracellular diffusion of fluorescent probes determine staining selectivity of intracellular ***,the relationship between the molecular structure of fluorescent probes and their membrane permeability and intracellular distribution is poorly *** this paper,we reported a series of 1,8-naphthalimide dyes and carried out cell imaging experiments,and found that the presence of amino hydrogen in these dyes played a crucial role in their cell membrane permeability and intracellular *** secondary amino group containing compounds 1-4 show excellent membrane permeability and strong fluorescence in living *** the tertiary amine containing dyes 5 and 6 can hardly permeate the cell membrane though they show extremely similar structure with compounds *** 1 can selectively image lipid droplets by selecting the wavelength of excitation *** the specificity for lysosomes,2 and 4 have been used in long-term time-lapses imaging of lysosomal dynamics and tracking the process of lysosome-lysosome interaction,fusion and *** effect of hydrogen-containing amino substituent on the cell membrane permeability of fluorescent molecules is promising for the development of better biocompatible probes.

关键词： Amino hydrogen 1,8-Naphthalimide Cell permeability Lipid droplet Lysosome

Gd_(3)Al_(3)Ga_(2)O_(12):Ce^(3+), Yb^(3+) fluorescent ceramic with highly increased trap density for optical information storage

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Chinese Optics letters 2024年第7期22卷 59-65页

作者： Jiaocheng Yin Renjie Jiang Junwei Zhang Qiao Hu Miao Zhao Xiaoxia Wang Anlian Pan Hao Ruan College of Materials science and Engineering Hunan UniversityChangsha 410082China Photonic Integrated Circuits Center Shanghai Institute of Optics and Fine MechanicsChinese Academy of SciencesShanghai 201800China

Electron-trapping materials,due to their exceptional ability of energy storage and controllable photon release under external stimulation,have attracted considerable attention in the field of optical information storage(OIS).In this work,Gd_(3)Al_(3)Ga_(2)O_(12):Ce^(3+), Yb^(3+)fluorescent ceramics,were developed using air and vacuum sintering *** co-doping Ce^(3+)and Yb^(3+),the trap density was significantly increased by 7.5 times compared to samples containing only Ce^(3+).Vacuum annealing further enhanced trap density by 1.6 times compared to samples sintered solely in air,while generating deep traps(1.44 eV),making Gd_(3)Al_(3)Ga_(2)O_(12):Ce^(3+), Yb^(3+) an excellent OIS *** work is expected to facilitate the development of OIS materials.

关键词： electron-trapping materials optical information storage Gd_(3)Al_(3)Ga_(2)O_(12):Ce^(3+),Yb^(3+) two-step sintering method.

A comparison of model choice strategies for logistic regression

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Journal of Data and Information science 2024年第1期9卷 37-52页

作者： Markku Karhunen Built Environment Solutions unit Finnish Environment Institute(Syke)Latokartanonkaari 1100790 HelsinkiFinland

Purpose:The purpose of this study is to develop and compare model choice strategies in context of logistic *** choice means the choice of the covariates to be included in the ***/methodology/approach:The study is based on Monte Carlo *** methods are compared in terms of three measures of accuracy:specificity and two kinds of sensitivity.A loss function combining sensitivity and specificity is introduced and used for a final ***:The choice of method depends on how much the users emphasize sensitivity against *** also depends on the sample *** a typical logistic regression setting with a moderate sample size and a small to moderate effect size,either BIC,BICc or Lasso seems to be *** limitations:Numerical simulations cannot cover the whole range of data-generating processes occurring with real-world ***,more simulations are *** implications:Researchers can refer to these results if they believe that their data-generating process is somewhat similar to some of the scenarios presented in this ***,they could run their own simulations and calculate the loss ***/value:This is a systematic comparison of model choice algorithms and heuristics in context of logistic *** distinction between two types of sensitivity and a comparison based on a loss function are methodological novelties.

关键词： Model choice Logistic regression Logit regression Monte Carlo simulations Sensitivity Specificity

Structurally Flexible 2D Spacer for Suppressing the Electron-Phonon Coupling Induced Non-Radiative Decay in Perovskite Solar Cells

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Nano-Micro letters 2024年第9期16卷 325-340页

作者： Ruikun Cao Kexuan Sun Chang Liu Yuhong Mao Wei Guo Ping Ouyang Yuanyuan Meng Ruijia Tian Lisha Xie Xujie Lü Ziyi Ge Zhejiang Provincial Engineering Research Center of Energy Optoelectronic Materials and Devices Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201People’s Republic of China School of Materials science and Chemical Engineering Ningbo UniversityNingbo 315211People’s Republic of China Center of Materials science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049People’s Republic of China Center for High Pressure science and Technology Advanced Research(HPSTAR) Shanghai 201203People’s Republic of China

This study presents experimental evidence of the dependence of non-radiative recombination processes on the electron-phonon coupling of perovskite in perovskite solar cells(PSCs).Via A-site cation engineering,a weaker electron-phonon coupling in perovskite has been achieved by introducing the structurally soft cyclohexane methylamine(CMA^(+))cation,which could serve as a damper to alleviate the mechanical stress caused by lattice oscillations,compared to the rigid phenethyl methylamine(PEA^(+))*** demonstrates a significantly lower non-radiative recombination rate,even though the two types of bulky cations have similar chemical passivation effects on perovskite,which might be explained by the suppressed carrier capture process and improved lattice geometry *** resulting PSCs achieve an exceptional power conversion efficiency(PCE)of 25.5%with a record-high opencircuit voltage(V_(OC))of 1.20 V for narrow bandgap perovskite(FAPbI_(3)).The established correlations between electron-phonon coupling and non-radiative decay provide design and screening criteria for more effective passivators for highly efficient PSCs approaching the Shockley-Queisser limit.

关键词： Electron-phonon coupling A-site cation engineering Non-radiative recombination

Hot Deformation Behavior and Workability of a New Ni–W–Cr Superalloy for Molten Salt Reactors

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Acta Metallurgica Sinica(English letters) 2024年第8期37卷 1453-1466页

作者： Long Liu Zijian Zhou Jie Yu Xinguang Wang Chuanyong Cui Rui Zhang Yizhou Zhou Xiaofeng Sun Shi‑Changxu Innovation Center for Advanced Materials Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China School of Materials science and Engineering University of Science and Technology of ChinaShenyang 110016China Fushun Special Steel Co. LtdFushun 113000China

The hot deformation behavior of a newly developed Ni–W–Cr superalloy for use in 800℃molten salt reactors(MSRs)was looked into by isothermal compression tests in the temperature range of 1050–1200℃with a strain rate of 0.001–1 s^(−1)under a true strain of *** Arrhenius-type model for the Ni–W–Cr superalloy was constructed by fitting the corrected flow stress *** this model,the effect of dispersion of solid solution elements during thermal deformation on microstructure evolution was considered,as well as the effects of friction and adiabatic heating on the temperature and strain rate-dependent variation of flow *** hot deformation activation energy of the Ni–W–Cr superalloy was 323 kJ/mol,which was less than that of the Hastelloy N alloy(currently used in MSRs).According to the rectified flow stress data,processing maps were *** conjunction with the corresponding deformation microstructures,the flow instability domains of the Ni–W–Cr superalloy were determined to be 1050–1160℃/0.03–1 s^(−1)and 1170–1200℃/0.001–0.09 s^(−1).In these deformation conditions,a locally inhomogeneous microstructure was caused by flow-i.e.,incomplete dynamic recrystallization and hot working parameters should avoid sliding into these *** ideal processing hot deformation domain for the Ni–W–Cr superalloy was determined to be 1170–1200℃/0.6–1 s^(−1).

关键词： Ni-W-Cr Superalloy Hot deformation behavior Constitutive equation Processing map Microstructure evolution

Influence of the Atlantic Multidecadal Oscillation and Interdecadal Pacific Oscillation on Antarctic surface air temperature during 1900 to 2015

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Acta Oceanologica Sinica 2024年第3期43卷 48-58页

作者： Cuijuan Sui Lejiang Yu Alexey YuKarpechko Licheng Feng Shan Liu Key Laboratory of Marine Hazards Forecasting National Marine Environmental Forecasting CenterMinistry of Natural ResourcesBeijing 100081China Key Laboratory for Polar science Polar Research Institute of ChinaMinistry of Natural ResourcesShanghai 200136China finnish Meteorological Institute HelsinkiFI-00101Finland

The importance of the Atlantic Multidecadal Oscillation(AMO)and Interdecadal Pacific Oscillation(IPO)in influencing zonally asymmetric changes in Antarctic surface air temperature(SAT)has been ***,previous studies have primarily concentrated on examining the combined impact of the contrasting phases of the AMO and IPO,which have been dominant since the advent of satellite observations in *** study utilizes long-term reanalysis data to investigate the impact of four combinations of+AMO+IPO,–AMO–IPO,+AMO–IPO,and–AMO+IPO on Antarctic SAT over the past 115 ***+AMO phase is characterized by a spatial mean temperature amplitude of up to 0.5℃over the North Atlantic Ocean,accompanied by positive sea surface temperature(SST)anomalies in the tropical eastern Pacific and negative SST anomalies in the extratropical-mid-latitude western Pacific,which are indicative of the+IPO *** Antarctic SAT exhibits contrasting spatial patterns during the+AMO+IPO and+AMO–IPO ***,during the–AMO+IPO period,apart from the Antarctic Peninsula and the vicinity of the Weddell Sea,the entire Antarctic region experiences a warming *** most pronounced signal in the SAT anomalies is observed during the austral autumn,whereas the combination of–AMO and–IPO exhibits the smallest magnitude across all the *** wavetrain excited by the SST anomalies associated with the AMO and IPO induces upper-level and surface atmospheric circulation anomalies,which alter the SAT ***,downward longwave radiation anomalies related to anomalous cloud cover play a crucial *** the future,if the phases of AMO and IPO were to reverse(AMO transitioning to a negative phase and IPO transitioning to a positive phase),Antarctica could potentially face more pronounced warming and accelerated melting compared to the current observations.

关键词： Atlantic Multidecadal Oscillation(AMO) Interdecadal Pacific Oscillation(IPO) surface air temperature Antarctic wavetrain Rossby wave source

Mn incorporated RuO_(2) nanocrystals as an efficient and stable bifunctional electrocatalyst for oxygen evolution reaction and hydrogen evolution reaction in acid and alkaline

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Chinese Chemical letters 2024年第10期35卷 194-200页

作者： Jing Cao Dezheng Zhang Bianqing Ren Ping Song Weilin Xu State Key Laboratory of Electroanalytical Chemistry Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China University of science and Technology of China Hefei 230026China

The development of efficient and stable bifunctional overall water-splitting is a crucial goal for clean and renewable energy,which is a challenging ***,we report an Mn-incorporated RuO_(2)(MnRuO_(2))catalyst for highly efficient electrocatalytic oxygen evolution reaction(OER)and hydrogen evolution reaction(HER)in acid and alkaline *** from a more electrochemical active area with the incorporation of Mn,the Mn-RuO_(2)required an overpotential of 200 mV to attain a current density of 10 mA/cm^(2)for OER in *** result indicates that the doping of Mn into RuO_(2)can enhance the OER *** acidic overall water-splitting electrolyzer with good stability constructed by bifunctional Mn-RuO_(2)only requires a cell voltage of 1.50 V to afford 10 m A/cm^(2)and can operate stably for 50 h at50 mA/cm^(2),which is better than the state-of-the-art Ru-based ***,the Mn-Ru O_(2)exhibits excellent HER and OER activity in alkaline media,and it shows superior activity and durability for overall water-splitting,only needing a cell voltage of 1.49 V to attain 10 m A/cm^(2).The present work provides an efficient approach to designing and constructing efficient Ru-based electrocatalysts for overall water-splitting.

关键词： RuO_(2)-based solid solution electrocatalysts Oxygenevolution reaction Hydrogen evolution reaction Overall watersplitting Acid andalkaline