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Evidence for active generation and seepage of sub-salt natural gas/condensate blend in the east offshore Nile Delta, Egypt: Integrated geochemical, petrophysical and seismic attribute approaches

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Petroleum science 2025年第1期22卷 130-150页

作者： Mahmoud Leila Ahmed A.Radwan Amir Ismail Emad A.Eysa Geology Department Faculty of Science Mansoura University School of Mining and Geosciences Nazarbayev University Department of Geology Faculty of Science Al-Azhar UniversityAssiut Branch Department of Geology Faculty of Science Helwan University Department of Physical and Environmental sciences Texas A&M University—Corpus Christi Geology Department Faculty of Science Zagazig University

Offshore Nile Delta in Egypt represents an enormous hydrocarbon province with recent projected gas and condensate discoveries of more than 50 trillion cubic feet “TCF”. Most of these occur in the post-salt hydrocarbon plays where biogenic gases are dominant. This study integrates organic geochemistry,seismic geomorphology and petrophysics in order to decipher the origin, and accumulation conditions of the wet gas/condensate blend in the Upper Miocene sub-salt Wakar Formation sandstones in Port Fouad Marine “PFM” Field, offshore Nile Delta. Hydrocarbon pay zones are scattered thin（ 1 w.t.%, hydrogen index“HI” > 200 mg HC/g TOC） and mature(Tmax> 430°C, vitrinite reflectance “VR” > 0.6 %R_o), source rocks are restricted to Upper Miocene Wakar and Oligo-Miocene Tineh formations. The latter contains more mature organofacies（up to 1.2 %R_o） and type II/III kerogen, thereby demonstrating a good capability to generate wet gases. The studied gas is wet and has thermogenic origin with signs of secondary microbial alteration, whereas the condensate contains a mixture of marine and terrestrial input. Molecular biomarkers of the condensate, isotopic and molecular composition of the gas reveals a generation of condensate prior to gas expulsion from the source. The Wakar sandstones have a heterogeneous pore system where three reservoir rock types（RRTI, RRTII and RRTIII）. RRTI rocks present the bulk composition of the Wakar pay zones. Spatial distribution of RRTI facies likely control the accumulation of the sub-salt hydrocarbons. Our results provide a new evidence on an active petroleum system in the sub-salt Paleogene successions in the offshore Nile Delta where concomitant generation of ga

关键词： Petrophysical evaluation Source rock Hydrocarbon geochemistry Biomarkers Gas chimneys Rock-typing

Partial multi-label learning via label-specific feature corrections

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science China(Information sciences) 2025年第03期68卷 95-109页

作者： Jun-Yi HANG Min-Ling ZHANG School of Computer science and Engineering Southeast University Key Laboratory of Computer network and Information Integration(Southeast University) Ministry of Education

Partial multi-label learning（PML） allows learning from rich-semantic objects with inaccurate annotations, where a set of candidate labels are assigned to each training example but only some of them are valid. Existing approaches rely on disambiguation to tackle the PML problem, which aims to correct noisy candidate labels by recovering the ground-truth labeling information ahead of prediction model induction. However, this dominant strategy might be suboptimal as it usually needs extra assumptions that cannot be fully satisfied in real-world scenarios. Instead of label correction, we investigate another strategy to tackle the PML problem, where the potential ambiguity in PML data is eliminated by correcting instance features in a label-specific manner. Accordingly, a simple yet effective approach named PASE, i.e., partial multi-label learning via label-specific feature corrections, is proposed. Under a meta-learning framework, PASElearns to exert label-specific feature corrections so that potential ambiguity specific to each class label can be eliminated and the desired prediction model can be induced on these corrected instance features with the provided candidate labels. Comprehensive experiments on a wide range of synthetic and real-world data sets validate the effectiveness of the proposed approach.

关键词： machine learning multi-label learning partial multi-label learning label-specific features feature correction

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Effect of divalent cations(Co^(2+) and Ni^(2+)) on microstructure,physical properties and application of NdFeO_(3)

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Journal of Rare Earths 2025年第1期43卷 89-97,I0004页

作者： M.M.Arman Materials science Lab(1) Physics DepartmentFaculty of ScienceCairo UniversityGiza12613Egypt

The nanocrystalline samples Nd_(1-x)M_(x)FeO_(3)(x=0.0 and 0.1;M:Co^(2+)and Ni^(2+))were prepared using the citrate combustion *** X-ray diffraction(XRD)pattern confirmed that the nanoparticles were synthesized in an orthorhombic *** particle size of Nd_(1-x)M_(x)FeO_(3) is in the range of 29-59 *** selected area electron diffraction(SAED)indicates the samples were prepared in a polycrystalline *** samples Nd_(1-x)M_(x)FeO_(3)(x=0.0 and 0.1;M:Co^(2+)and Ni^(2+))have anti ferromagnetic *** Fe^(3+)spins are aligned antiparallel,forming the antiferromagnetic(AFM)properties,which are affected by many factors such as the bond angle between the Fe^(3+)(Fe^(3+)-O_(2)--Fe^(3+))and the Dzyaloshinskii-Moriya(D-M)*** doping of Co^(2+)and Ni^(2+)ions in NdFeO_(3) enhances the magnetic properties of the NdFeO_(3).The saturation magnetization(Ms)of Nd_(0.90)Co_(0.10)FeO_(3) increases 1.8times more than that of NdFeO_(3).The exchange bias field(HEX)of the Co-doped sample is two times greater than that of NdFeO_(3).The magnetic anisotropy constant(K)of the 10%Co-doped sample increases by 11 factors compared to that of NdFeO_(3).The Tauc plot illustrates that the samples have a direct optical *** divalent cation substitution(Co^(2+)and Ni^(2+))decreases the optical band gap of NdFeO_(3),leading to the recommendation of using the samples Nd_(0.90)Co_(0.10)FeO_(3) and Nd_(0.90)Ni_(0.10)FeO_(3) in photocatalysis of dye degradation from *** removal efficiencies of Cr6+at pH=6 are 88.06%,85.54%,and 85.52%for the samples NdFeO_(3),Nd_(0.90)Co_(0.10)FeO_(3),and Nd_(0.90)Ni_(0.10)FeO_(3),*** Freundlich isotherm mode is the best-fit model for NdFeO_(3) to adsorb Cr6+ions from aqueous solutions.

关键词： Optical properties Nanoparticles Magnetic properties Perovskites Removal efficiency Rareearths

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Privacy-preserving explainable AI: a survey

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science China(Information sciences) 2025年第1期68卷 23-56页

作者： Thanh Tam NGUYEN Thanh Trung HUYNH Zhao REN Thanh Toan NGUYEN Phi Le NGUYEN Hongzhi YIN Quoc Viet Hung NGUYEN School of Information and Communication Technology Griffith University School of Computer and Communication sciences Ecole Polytechnique Federale de Lausanne faculty of Mathematics and Computer science University of Bremen faculty of Information Technology HUTECH University Department of Computer science Hanoi University of Science and Technology School of Electrical Engineering and Computer science The University of Queensland

As the adoption of explainable AI(XAI) continues to expand, the urgency to address its privacy implications intensifies. Despite a growing corpus of research in AI privacy and explainability, there is little attention on privacy-preserving model explanations. This article presents the first thorough survey about privacy attacks on model explanations and their countermeasures. Our contribution to this field comprises a thorough analysis of research papers with a connected taxonomy that facilitates the categorization of privacy attacks and countermeasures based on the targeted explanations. This work also includes an initial investigation into the causes of privacy leaks. Finally, we discuss unresolved issues and prospective research directions uncovered in our analysis. This survey aims to be a valuable resource for the research community and offers clear insights for those new to this domain. To support ongoing research, we have established an online resource repository, which will be continuously updated with new and relevant findings.

关键词： privacy-preserving explainable AI privacy attacks privacy defences PrivEx PPXAI

Cu/TiO_(2)adsorbents modified by air plasma for adsorption-oxidation of H_(2)S

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Journal of Environmental sciences 2025年第2期148卷 476-488页

作者： Yongqi Yan Xinyu Yang Ping Ning Chi Wang Xin Sun Fei Wang Peng Gao Kai Li faculty of Environmental science and Engineering Kunming University of Science and TechnologyKunming 650500China National-Regional Engineering Center for Recovery of Waste Gases from Metallurgical and Chemical Industries Kunming University of Science and TechnologyKunming 650500China faculty of Chemical Engineering Kunming University of Science and TechnologyKunming 650500China City College Kunming University of Science and TechnologyKunming 650500China

In this study,non-thermal plasma(NTP)was employed to modify the Cu/TiO_(2)adsorbent to efficiently purify H_(2)S in low-temperature and micro-oxygen *** effects of Cu loading amounts and atmospheres of NTP treatment on the adsorption-oxidation performance of the adsorbents were *** NTP modification successfully boosted the H_(2)S removal capacity to varying degrees,and the optimized adsorbent treated by air plasma(Cu/TiO_(2)-Air)attained the best H_(2)S breakthrough capacity of 113.29 mg H_(2)S/gadsorbent,which was almost 5 times higher than that of the adsorbent without NTP *** studies demonstrated that the superior performance of Cu/TiO_(2)-Air was attributed to increased mesoporous volume,more exposure of active sites(CuO)and functional groups(amino groups and hydroxyl groups),enhanced Ti-O-Cu interaction,and the favorable ratio of active oxygen ***,the X-ray diffraction(XRD)and X-ray photoelectron spectroscopy(XPS)results indicated the main reason for the deactivationwas the consumption of the active components(CuO)and the agglomeration of reaction products(CuS and SO_(4)^(2−))occupying the active sites on the surface and the inner pores of the adsorbents.

关键词： Non-thermal plasma(NTP) Surface modification Simultaneous adsorption-oxidation Cu/TiO_(2)(TiO_(2)loaded with copper) H_(2)S

Hourglass-GCN for 3D Human Pose Estimation Using Skeleton Structure and View Correlation

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Computers, Materials & Continua 2025年第1期82卷 173-191页

作者： Ange Chen Chengdong Wu Chuanjiang Leng faculty of Robot science and Engineering Northeastern UniversityShenyang110169China

Previous multi-view 3D human pose estimation methods neither correlate different human joints in each view nor model learnable correlations between the same joints in different views explicitly,meaning that skeleton structure information is not utilized and multi-view pose information is not completely ***,existing graph convolutional operations do not consider the specificity of different joints and different views of pose information when processing skeleton graphs,making the correlation weights between nodes in the graph and their neighborhood nodes *** Graph Convolutional networks(GCNs)cannot extract global and deeplevel skeleton structure information and view correlations *** solve these problems,pre-estimated multiview 2D poses are designed as a multi-view skeleton graph to fuse skeleton priors and view correlations explicitly to process occlusion problem,with the skeleton-edge and symmetry-edge representing the structure correlations between adjacent joints in each viewof skeleton graph and the view-edge representing the view correlations between the same joints in different *** make graph convolution operation mine elaborate and sufficient skeleton structure information and view correlations,different correlation weights are assigned to different categories of neighborhood nodes and further assigned to each node in the *** on the graph convolution operation proposed above,a Residual Graph Convolution(RGC)module is designed as the basic module to be combined with the simplified Hourglass architecture to construct the Hourglass-GCN as our 3D pose estimation ***-GCNwith a symmetrical and concise architecture processes three scales ofmulti-viewskeleton graphs to extract local-to-global scale and shallow-to-deep level skeleton features *** results on common large 3D pose dataset Human3.6M and MPI-INF-3DHP show that Hourglass-GCN outperforms some excellent methods in 3D pose estimati

关键词： 3D human pose estimation multi-view skeleton graph elaborate graph convolution operation Hourglass-GCN

Dissolved carbon in biochar:Exploring its chemistry,iron complexing capability,toxicity in natural redox environment

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Journal of Environmental sciences 2025年第1期147卷 217-229页

作者： Chaochao Lai Juhong Zhan Qiuyun Chai Changlu Wang Xiaoxia Yang Huan He Bin Huang Xuejun Pan faculty of Environmental science and Engineering Kunming University of Science and TechnologyKunming 650500China Research Institute for Environmental Innovation(Suzhou)Tsinghua Suzhou 215163China

Dissolved black carbon(DBC)plays a crucial role in the migration and bioavailability of iron in ***,the properties of DBC releasing under diverse pyrolysis conditions and dissolving processes have not been systematically ***,the compositions of DBC released from biochar through redox processes dominated by bacteria and light were thoroughly *** was found that the DBC released from straw biochar possess more oxygen-containing functional groups and aromatic *** content of phenolic and carboxylic groups in DBC was increased under influence of microorganisms and light,*** concentration of phenolic hydroxyl groups increased from 10.0~57.5 mmol/gC to 6.6~65.2 mmol/gC,and the concentration of carboxyl groups increased from49.7~97.5 mmol/gC to 62.1~113.3 mmol/*** the impacts of DBC on pyrite dissolution andmicroalgae growth were also *** complexing Fe^(3+)was proved to play a predominant role in the dissolution of ferrous mineral in DBC *** to complexing between iron ion and DBC,the amount of dissolved Fe in aquatic water may rise as a result of elevated number of aromatic components with oxygen containing groups and low molecular weight generated under light ***-DBC complexations in solution significantly promoted microalga growth,which might be attributed to the stimulating effect of dissolved Fe on the chlorophyll *** results of study will deepen our understanding of the behavior and ultimate destiny of DBC released into an iron-rich environment under redox conditions.

关键词： Dissolved black carbon Bacteria Light Iron complexes Toxicity

A Fully‑Printed Wearable Bandage‑Based Electrochemical Sensor with pH Correction for Wound Infection Monitoring

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Nano-Micro Letters 2025年第3期17卷 355-375页

作者： Kanyawee Kaewpradub Kornautchaya Veenuttranon Husanai Jantapaso Pimonsri Mittraparp‑arthorn Itthipon Jeerapan Center of Excellence for Trace Analysis and Biosensor Prince of Songkla UniversityHat Yai 90110SongkhlaThailand Division of Physical science Faculty of SciencePrince of Songkla UniversityHat Yai 90110SongkhlaThailand Center of Excellence for Innovation in Chemistry Faculty of SciencePrince of Songkla UniversityHat Yai 90110SongkhlaThailand The ijE Electrochemistry for All Laboratory Prince of Songkla UniversityHat Yai 90110SongkhlaThailand Division of Biological science Faculty of SciencePrince of Songkla UniversityHat Yai 90110SongkhlaThailand

Wearable sensing systems have been designed to monitor health conditions in real-time by detecting analytes in human *** diagnosis remains challenging,necessitating suitable materials for high-performance wearable sensors to offer prompt *** devices have limitations in measuring pH and the concentration of pH-dependent electroactive species simultaneously,which is crucial for obtaining a comprehensive understanding of wound status and optimizing ***,improving materials and analysis system accuracy is *** article introduces the first example of a flexible array capable of detecting pyocyanin,a bacterial virulence factor,while correcting dynamic pH *** demonstrate that this combined sensor enhances accuracy by mitigating the impact of pH variability on pyocyanin sensor *** screen-printable inks were developed to enhance analytical *** analytical performances of two sensitive sensor systems(i.e.,fully-printed porous graphene/multiwalled carbon nanotube(CNT)and polyaniline/CNT composites for pyocyanin and pH sensors)are *** least square regression is employed to analyze nonzero-order data arrays from square wave voltammetric and potentiometric measurements of pyocyanin and pH sensors to establish a predictive model for pyocyanin concentration in complex *** sensitive and effective strategy shows potential for personalized applications due to its affordability,ease of use,and ability to adjust for dynamic pH changes.

关键词： Pyocyanin Bandages Wound monitoring Biosensor Wearable device

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Effect of Cu/HZSM-5 sorbents with different Si/Al ratios on the adsorption and oxidation performance of H_(2)S

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Journal of Environmental sciences 2025年第5期151卷 161-173页

作者： Kaini Ma Kai Li Ping Ning Jiayu Feng Jiacheng Bao Lei Shi Xiangyu Wang Xin Sun faculty of Environmental science and Engineering Kunming University of Science and TechnologyKunming 650500China National-Regional Engineering Center for Recovery of Waste Gases from Metallurgical and Chemical Industries Kunming University of Science and TechnologyKunming 650500China

This study employed a wet impregnation method to synthesize five types of Cu/HZSM-5 adsorbents with Si/Al ratios of 25,50,85,200,and 300,used for the removal of H_(2)S in lowtemperature,low-oxygen *** impact of different Si/Al ratios on the adsorption oxidative performance of Cu_(30)/HZSM-5–85 adsorbents was *** to the performance test results,Cu_(30)/HZSM-5–85 exhibited the highest breakthrough capacity,reaching 231.75 mg H_(2)S/g_(sorbent).Cu/HZSM-5 sorbent maintains a strong ability to remove H_(2)S even under humid conditions and shows excellent water ***,BET,and XPS results revealed that CuO is the primary active species,with Cu_(30)/HZSM-5–85 having the largest surface area and highest CuO content,providing more active sites for H_(2)S adsorption.H_(2)-TPR and O_(2)-TPD results confirmed that Cu_(30)/HZSM-5–85 sorbent exhibits outstanding redox properties and oxygen storage capacity,contributing to excellent oxygen transferability in the molecular sieve adsorption-oxidation *** notable characteristics such as a large surface area,high desulfurization efficiency,and water resistance,Cu_(30)/HZSM-5–85 sorbents hold significant importance for industrial applications.

关键词： H_(2)S Si/Al ratio Adoration-oxidation Cu/HZSM-5-85(HZSM-5 with Si/Al ratio of 85 loaded Cu)