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An Effective Approach for the Preparation of High Performance Thermal Conductive Polymer Composites Containing Liquid Metal

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Chinese Journal of Polymer science 2024年第7期42卷 992-1001,I0010页

作者： Xin Chen Xue-Zhong Zhang Yi-Fei Yuan Chuan-Liang Chen Lian-Hu Xiong Qiang Fu Hua Deng College of Polymer science and engineering State Key Laboratory of Polymer Materials EngineeringSichuan UniversityChengdu610065China Department of Materials science and engineering Sichuan University-Pittsburgh InstituteSichuan UniversityChengdu610065China

The preparation of high-performance thermal conductive composites containing liquid metals(LM)has attracted significant ***,the stable dispersion of LM within polymer solution and effective property contribution of liquid metals remains significant challenges that need to be *** by the properties of the dendritic structure of the tree root system in grasping the soil,“shear-induced precipitation-interfacial reset-reprotonation”processing strategy is proposed to prepare nanocomposites based on aramid micron fibers(AMFs)with hierarchical dendritic *** to the combination of van der Waals force provided by hierarchical dendritic structure,electrostatic interaction between AMFs and LM,coordinative bonding of―NH to LM,together with interfacial re-setting and multi-step protonation,several features can be achieved through such strategy:conducive to the local filler network construction,improvement of interfacial interaction,improvement of the stability of filler dispersion in the solvent,and enhancement of mechanical and thermal properties of the *** resulting AMFsp H=4/LM films demonstrate a thermal conductivity of 10.98 W·m^(-1)·K^(-1)at 70%filler content,improvement of 126.8%compared to ANFs/LM film;while maintaining a strength of~85.88 MPa,improvement of 77%compared to AMFs/LM *** also possess insulation properties,enable heat dissipation for high power *** work provides an effective strategy for the preparation of high performance polymer composites containing liquid metal.

关键词： Shear-induced Reprotonation AMFs LM Filler dispersion

The origins of catalytic selectivity for the electrochemical conversion of carbon dioxide to methanol

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Nano Research 2024年第1期17卷 5-17页

作者： Tian Wang Yating Wang Yuhang Li Chunzhong Li Key Laboratory for Ultrafine Materials of Ministry of Education Shanghai Engineering Research Center of Hierarchical NanomaterialsFrontiers Science Center for Materiobiology and Dynamic ChemistrySchool of Materials Science and EngineeringEast China University of Science&TechnologyShanghai 200237China School of Chemical engineering East China University of Science&TechnologyShanghai 200237China

The electrocatalytic conversion of carbon dioxide(CO_(2))into useful fuels and chemical feedstocks is an emerging route to alleviate global warming and reduce reliance on fossil ***(CH_(3)OH),as one of the most significant and widely used liquid fuels that can be generated by CO_(2)reduction,is essential in the chemical *** this minireview,we unravel the origins of the selective formation of CH_(3)OH via CO_(2)reduction,including catalyst composition designs,local structure modulations,and electrolyte/catalyst interface ***,the remaining challenges and perspectives for the CO_(2)-to-CH_(3)OH reduction are proposed.

关键词： methanol carbon dioxide(CO_(2))reduction reaction electrochemistry electrocatalyst catalyst-electrolyte interface

Nonlinear dynamics of a circular curved cantilevered pipe conveying pulsating fluid based on the geometrically exact model

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Applied Mathematics and Mechanics(English Edition) 2024年第2期45卷 261-276页

作者： Runqing CAO Zilong GUO Wei CHEN Huliang DAI Lin WANG Department of engineering Mechanics School of Aerospace EngineeringHuazhong University of Science and TechnologyWuhan 430074China Hubei Key Laboratory for engineering Structural Analysis and Safety Assessment Wuhan 430074China State Key Laboratory of Intelligent Manufacturing Equipment and Technology School of Mechanical Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China

Due to the novel applications of flexible pipes conveying fluid in the field of soft robotics and biomedicine,the investigations on the mechanical responses of the pipes have attracted considerable *** fluid-structure interaction(FSI)between the pipe with a curved shape and the time-varying internal fluid flow brings a great challenge to the revelation of the dynamical behaviors of flexible pipes,especially when the pipe is highly flexible and usually undergoes large *** this work,the geometrically exact model(GEM)for a curved cantilevered pipe conveying pulsating fluid is developed based on the extended Hamilton's *** stability of the curved pipe with three different subtended angles is examined with the consideration of steady fluid *** attention is concentrated on the large-deformation resonance of circular pipes conveying pulsating fluid,which is often encountered in practical *** constructing bifurcation diagrams,oscillating shapes,phase portraits,time traces,and Poincarémaps,the dynamic responses of the curved pipe under various system parameters are *** mean flow velocity of the pulsating fluid is chosen to be either subcritical or *** numerical results show that the curved pipe conveying pulsating fluid can exhibit rich dynamical behaviors,including periodic and quasi-periodic *** is also found that the preferred instability type of a cantilevered curved pipe conveying steady fluid is mainly in the flutter of the second *** a moderate value of the mass ratio,however,a third-mode flutter may occur,which is quite different from that of a straight pipe system.

关键词： curved pipe conveying fluid pulsating fluid geometrically exact model(GEM) nonlinear dynamics parametric vibration flutter

Unraveling electrolyte solvation architectures for high-performance lithium-ion batteries

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science China(Technological sciences) 2024年第3期67卷 958-964页

作者： YANG MengHao SHI Zhe HE ZhiYuan WANG Dan School of Materials science and engineering Tongji UniversityShanghai 201804China Department of Nuclear science and engineering Massachusetts Institute of Technology CambridgeMassachuseis 02139USA School of Materials science and engineering Beijing Institute of TechnologyBeijing 100081China

The design of advanced electrolytes hinges critically on a comprehensive comprehension of lithium-ion migration mechanisms within these electrochemical systems. Fluorination generally improves the stability and reduces the reactivity of organic compounds, making them potentially suitable for use in harsh conditions such as those found in a battery electrolyte. However,the specific properties, such as the solvation power, diffusivity, ion mobility, and so forth, would depend on the exact nature and extent of the fluorination. In this work, we introduce a theoretical framework designed to facilitate the autonomous creation of electrolyte molecular structures and craft methodologies to compute transport coefficients, providing a physical interpretation of fluoride systems. Taking fluorinated-1,2-diethoxyethanes as electrolyte solvents, we present and analyze the relationship between the electronic properties and atomic structures, and further correlate these properties to the transport coefficients, resulting in a good alignment with the experimental diffusion behaviors and Li-solvation structures. The insights derived from this research contribute to the methodological basis for high-throughput evaluation of prospective electrolyte systems, and consequently, propose strategic directions for the improvement of electrochemical cycle characteristics. This comprehensive exploration of the transport mechanisms enhances our understanding, offering avenues for further advancements in the field of lithium-ion battery technology.

关键词： Unraveling electrolyte solvation architectures for high-performance lithium-ion batteries

Recent Advances in Patterning Strategies for Full‑Color Perovskite Light‑Emitting Diodes

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Nano-Micro Letters 2024年第3期16卷 99-137页

作者： Gwang Heon Lee Kiwook Kim Yunho Kim Jiwoong Yang Moon Kee Choi Graduate School of Semiconductor Materials and Devices engineering Center for Future Semiconductor Technology(FUST)Ulsan National Institute of Science and Technology(UNIST)Ulsan 44919Republic of Korea Department of Energy science and engineering Daegu Gyeongbuk Institute of Science and Technology(DGIST)Daegu 42988Republic of Korea Energy science and engineering Research Center Daegu Gyeongbuk Institute of Science and Technology(DGIST)Daegu 42988Republic of Korea Department of Materials science and engineering Ulsan National Institute of Science and Technology(UNIST)Ulsan 44919Republic of Korea Center for Nanoparticle Research Institute for Basic Science(IBS)Seoul 08826Republic of Korea

Metal halide perovskites have emerged as promising light-emitting materials for next-generation displays owing to their remarkable material characteristics including broad color tunability,pure color emission with remarkably narrow bandwidths,high quantum yield,and solution *** recent advances have pushed the luminance efficiency of monochromic perovskite light-emitting diodes(PeLEDs)to their theoretical limits,their current fabrication using the spincoating process poses limitations for fabrication of full-color *** integrate PeLEDs into full-color display panels,it is crucial to pattern red–green–blue(RGB)perovskite pixels,while mitigating issues such as cross-contamination and reductions in luminous ***,we present state-of-the-art patterning technologies for the development of full-color ***,we highlight recent advances in the development of efficient ***,we discuss various patterning techniques of MPHs(i.e.,photolithography,inkjet printing,electron beam lithography and laserassisted lithography,electrohydrodynamic jet printing,thermal evaporation,and transfer printing)for fabrication of RGB pixelated *** patterning techniques can be classified into two distinct approaches:in situ crystallization patterning using perovskite precursors and patterning of colloidal perovskite *** review highlights advancements and limitations in patterning techniques for PeLEDs,paving the way for integrating PeLEDs into full-color panels.

关键词： Perovskite Light-emitting diode Full-color display High-resolution patterning Electroluminescence

A Wideband High-Gain Sawtooth Slot Array Antenna with Frequency-Scanning at Lower Frequency and Fixed-Beam at Higher Frequency

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Chinese Journal of Electronics 2024年第2期33卷 463-471页

作者： Qiang SUN Yongling BAN Jun HU School of Electronic science and engineering University of Electronic Science and Technology of China

Exploring the multifunctional array antenna suitable for complex communication environment has very important research value. In this paper, a millimeter wave(mm-wave) double longitudinal sawtooth slot array antenna(DLSA) based on substrate integrated waveguide(SIW) technology is proposed, which has wideband, highgain and novel beam characteristics. Two irregular longitudinal slots are etched on the SIW conductor surface as the radiation structure. To improve the bandwidth of the DLSA, the metallized vias are added at the transition point of the slots to construct multiple resonant frequency points. By adjusting the size of the slots and the position of the metallized vias, the phase constant can be regulated, and the unusual beam characteristics can be obtained. That is to say, in the lower frequency band, the beam pointing angle increases with frequency. In the higher frequency band,the beam pointing angle is maintained at a fixed angle. Finally, to improve the antenna gain, a 16 × 8 DLSA is fabricated, measured and discussed. The proposed antenna has an impedance matching bandwidth close to 9.7 *** 27 to 33 GHz, the beam pointing angle changes from 8° to 29°. From 33 to 37 GHz, the beam pointing angle is fixed at 29°, and the pointing angle error range is ±1°. In addition, the measured maximum gain is 22.9 d Bi at32 GHz.

关键词： Antenna measurements Slot antennas Surface waves Resonant frequency Gain measurement Conductors Frequency measurement

TiO_(2)-Fe_(2)TiO_(5)heterostructure hollow spheres enable high-performance lithium-sulfur batteries via interfacial engineering

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Rare Metals 2024年第8期43卷 4006-4012页

作者： Kai-Tao Liu Hong-Qiang Wang Zhuo Chen Shi-Lin Zhang Ying-Ying Song Fang Liu Qiao-Ling Li Jiao Li School of Materials science and engineering Shandong University of TechnologyZibo 255049China College of Chemistry&Environmental science Hebei UniversityBaoding 071002China School of Chemical engineering Faculty of SciencesEngineering and TechnologyUniversity of AdelaideAdelaide 5005Australia School of Materials science and engineering Hebei University of TechnologyTianjin 300130China

The shuttle effect of lithium polysulfides between sulfur cathode and lithium anode is a notorious problem in the commercial application of lithium-sulfur ***,heterostructured TiO_(2)-Fe_(2)TiO_(5)hollow spheres were ... 详细信息

关键词： lithium sulfide (5)

Sawtooth-enhanced bend sensor for gesture recognition

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science China(Technological sciences) 2024年第6期67卷 1727-1736页

作者： BAI YanRu ZHANG ZiHang WANG HaoYu GUO Rui LI XiSheng School of Automation and Electrical engineering University of Science and Technology BeijingBeijing100083China School of Advanced engineering University of Science and Technology BeijingBeijing100083China School of Precision Instrument and Opto-Electronics engineering Tianjin UniversityTianjin300072China School of Computer and Communication engineering University of Science and Technology BeijingBeijing100083China

Gesture recognition has diverse application prospects in the field of human-computer ***,gesture recognition devices based on strain sensors have achieved remarkable results,among which liquid metal materials have considerable advantages due to their high tensile strength and *** improve the detection sensitivity of liquid metal strain sensors,a sawtooth-enhanced bending sensor is proposed in this *** with the results from previous studies,the bending sensor shows enhanced resistance *** addition,combined with machine learning algorithms,a gesture recognition glove based on the sawtooth-enhanced bending sensor is also fabricated in this study,and various gestures are accurately *** the fields of human-computer interaction,wearable sensing,and medical health,the sawtooth-enhanced bending sensor shows great potential and can have wide application prospects.

关键词： liquid metal bending sensor gesture recognition machine learning

An online value iteration method for linear-quadratic mean field social control with unknown dynamics

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science China(Information sciences) 2024年第4期67卷 38-39页

作者： Bing-Chang WANG Shumei LI Ying CAO School of Control science and engineering Shandong University

Mean field(MF) models have been widely applied to economics, control theory, and other fields. Its prominent feature is that the individual influence on the overall population is negligible and the impact of the entire system to the single agent is significant and cannot be ignored. As a classical problem in control theory, linear quadratic(LQ) control for MF models has been widely investigated(e.g., [1, 2]).

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