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Rational design of continuous and short-range lithium ion pathways based on polydopamine-anchored metal-organic frameworks for all-solid-state electrolytes

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Journal of Energy Chemistry 2024年第12期99卷 712-724页

作者： Kun Shi Changsong Yu Dawei Zheng Zeheng Yang Weixin Zhang School of Chemistry and Chemical engineering Anhui Province Engineering Research Center of Flexible and Intligent MaterialsHefei University of TechnologyHefei 230009AnhuiChina

The immerging three dimensional(3D) metal-organic framework(MOF)-reinforced composite solid-state electrolytes have attracted great interest because of the enhanced ionic conductivity and mechanical properties. However, the defective spatial arrangement of MOFs restricted by fabrication methodology leads to insufficient lithium ion transport in electrolytes. Herein, a 3D interconnected MOF framework tailored for all-solid-state electrolytes is rationally designed by a universal polydopamine(PDA)-engineered "double-sided tape" strategy. The PDA serves as a double-sided tape, firmly adhering on the special single-layer Nylon grid as well as offering uniform nucleation sites to anchor the metal nodes to ensure continuous growth of well-ordered MOFs. Benefiting from the Lewis acid feature of MOFs and its cage effect toward TFSI^(-), a fast and homogeneous lithium ion transport can be achieved through the internal channels within neighboring MOFs and the continuous MOFs/polymer interfaces both along the short-range circumferential boundary of Nylon fiber. The resultant composite electrolytes exhibit high lithium ion conductivity and prominent mechanical properties, rendering excellent cyclic stability whether used in coin or pouch cells. This work demonstrates a widely applicable "double-sided tape"strategy for controllable spatial arrangement of MOF nanoparticles on optional substrates, which provides a scalable approach to rationally construct desired lithium ion pathways within composite electrolytes.

关键词： All-solid-state electrolytes “Double-sided tape”strategy Continuous lithium ion pathways Short-range pathways Mechanical properties

Hysteresis loss reduction in self-bias FeSi/SrFe_(12)O_(19)soft magnetic composites

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Chinese Physics B 2022年第2期31卷 576-580页

作者： Shuangjiu Feng Jiangli Ni Feng Hu Xucai Kan Qingrong Lv Xiansong Liu engineering technology research center of Magnetic Materials of anhui province School of Physics and Materials ScienceAnhui UniversityHefei 230601China engineering technology research center of Preparation and Application of Industrial Ceramics of anhui province School of Chemistry and Material EngineeringChaohu UniversityHefei 238000China

The magnetic field provided by magnetized SrFe_(12)O_(19)particles in FeSi/SrFe_(12)O_(19)composites is used to replace the applied transverse magnetic field,which successfully reduces the magnetic loss of the composites with minor reduction of *** magnetic loss reduction mainly comes from the decrease in hysteresis loss,while the eddy current loss is basically *** hysteresis loss reduction in magnetized composites is believed to be due to the decrease in domain wall displacement caused by the increase in the average magnetic domain size in a DC magnetic *** is an effective method for reducing the magnetic loss of soft magnetic composites with wide application potential,and there is no problem of increasing the cost and the volume of the magnetic cores.

关键词： soft magnetic composites FeSi SrFe_(12)O_(19) magnetic loss

Transforming waste particles into valuable adsorbents via amyloid-mediated molecular engineering

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Science China Chemistry 2025年第01期 317-328页

作者： Qingmin Yang Jian Zhao Yujia Zhang Xingyu Zhou Hao Ren Bowen Hu Zhongli Lei Lixin Chen Peng Yang School of Material and Chemical engineering Bengbu University anhui Provincial engineering Laboratory of Silicon-Based Materials School of Chemistry and Chemical engineering Northwestern Polytechnical University Key Laboratory of Applied Surface and Colloid Chemistry Ministry of Education School of Chemistry and Chemical EngineeringShaanxi Normal University Xi'an Key Laboratory of Polymeric Soft Matter School of Chemistry and Chemical Engineering Shaanxi Normal University International Joint research center on Functional Fiber and Soft Smart Textile School of Chemistry and Chemical EngineeringShaanxi Normal University

The high-value utilization of industrial solid waste using a facile and eco-friendly process is of great interest and significance in reducing environmental pollution and developing a green circular economy. Herein, we propose an amyloid-mediated molecular engineering strategy to transform particulate waste into valuable adsorbents for metal ions. Our method has the advantage of aqueous solution fabrication under mild conditions without the use of high-temperature hydrothermal methods and toxic chemical reagents. Amyloid-mediated molecular engineering manipulates the phase transition of bovine serum albumin(BSA)on particulate waste surfaces, resulting in a remarkable ～3.1 times improvement in the adsorption capacity of fly ash, a typical industrial solid waste for gold ions after modification with the phase-transitioned BSA(PTB). The resultant adsorption ability was 69–1,980 times higher than those of conventional and emerging adsorbent materials such as ion exchange resins, activated carbon(AC), covalent organic frameworks(COFs), and metal-organic frameworks(MOFs). We further demonstrated the application of our PTB-modified materials in the recovery of precious metals from low-grade gold ore and electronic waste leachates. Consequently, this strategy could increase the value of waste materials nearly 27 times. In addition, this method is generally extendable to other conventional industrial adsorbents such as resin, clay, and Al2O3, and enhances their adsorption capabilities at least twofold. Overall, this work provides a simple and green approach for improving the adsorption performance of solid particles, and is expected to develop into a universal strategy for transforming waste particles into high-value-added products.

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Hysteresis loss free soft magnetic ferrites based on Larmor precession

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Chinese Physics B 2023年第8期32卷 433-438页

作者：冯双久赵幸丽朱守金吕庆荣阚绪材刘先松 engineering technology research center of Magnetic Materials of anhui province School of Materials Science and EngineeringAnhui UniversityHefei 230601China School of Physics and Optoelectronic engineering Anhui UniversityHefei 230601China

A big enough transverse magnetic field applied to soft magnetic ferrite toroid can magnetize the ferrite to a saturation level in transverse direction and almost completely suppresses magnetic domain structures in the ferrite,the response to the longitudinal alternating electromagnetic field changes from the original domain wall displacements and spin rotations to the precession of magnetization around the transverse field,and the hysteresis loss disappears in the *** theoretical and experimental results indicate that the permeability and magnetic loss in the ferrite can be controlled by adjusting the transverse magnetic field.A higher Q value with relatively low permeability can be achieved by increasing the transverse field,which ensures that the ferrite can be operated at high frequencies,with magnetic loss being very low.

关键词： ferrites Larmor precession magnetic losses hysteresis loss free

Effect of carbon solution-loss reaction on properties of coke in blast furnace

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Journal of Iron and Steel research International 2020年第5期27卷 489-499页

作者： Qi-hang Liu Shuang-ping Yang Chen Wang Yi-long Ji School of Metallurgical engineering Xi’an University of Architecture and TechnologyXi’an 710055ShaanxiChina Metallurgical engineering technology research center of Shaanxi province Xi’an 710055ShaanxiChina anhui province Key Laboratory of Metallurgical engineering and Resources Recycling Anhui University of TechnologyMa’anshan 243002AnhuiChina

The pore structure of coke under CO2 atmosphere was investigated by the carbon solution-loss reaction *** results show that the pore size distribution of coke gradually changes from dispersion to relative concentration with the increase in carbon loss rate,but it tends to be dispersed again in the late stage of the reaction,and the pore volume and specific surface area also increase first and then decrease with the increase in carbon loss *** electron microscopy results show that the evolution of coke pores is from the formation of micropores to the expansion of micropores,and finally the micropore and mesopores collapse to form a large number of string *** chemical bonds and functional groups of different reacted cokes were analyzed by Fourier-transform infrared ***,the microstructure of reacted cokes was analyzed by optical microscopy,and then the ordering of the affinity of different microstructures with CO2 was *** volume hypothesis which was the theory about energy size of comminution was adopted to analyze the degradation behavior of reacted *** breakage energy of reacted cokes was calculated by volume hypothesis,and the power consumption coefficient CK of different reacted cokes was determined by drum experiment,and then the degradation behavior of reacted cokes under different power consumptions was predicted.

关键词： Coke property Carbon solution-loss reaction Coke degradation Coke pore Volume hypothesis Breakage energy

Quantum Discord in any Mixture of Two Bi-Qubit Arbitrary Product States

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Communications in Theoretical Physics 2013年第12期60卷 667-672页

作者：王胜房刘益民李国锋刘先松张战军 engineering technology research center of Magnetic Materials Anhui Province School of Physics & Materials ScienceAnhui University Department of Physics Shaoguan University

Quantum discord in any mixture of two bi-qubit arbitrary product states is studied with two different approaches. In the first approach the maximM classicM correlations are obtained via numerical computations, while in the second approach they are analytically derived. Quantum correlations captured with both approaches completely coincide, as is in accord with the conclusion of Cen et al. [Phys. Rev. A 83 （2011） 054101]. The symmetry reduction of the concerned states concerning quantum correlations is accomplished. The captured discords are amply analyzed so that some inherent distinct properties are revealed.

关键词： quantum discord numerical computation approach analytic expression any mixture two bi-qubit arbitrary product states

Removal of rubidium from brine by an integrated film of sulfonated polysulfone/graphene/potassium copper ferricyanide

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Chinese Journal of Chemical engineering 2024年第5期69卷 112-121页

作者： Huanxi Xu Peihua Lin Pei-Jun Liu Hai-Gang Liu Hui-Bin Guo Chao-Xiang Wu Ming Fang Xu Zhang Guan-Ping Jin anhui province engineering research center of Flexible and Intelligent Materials School of Chemistry and Chemical EngineeringHefei University of TechnologyHefei 230009China Chemical Design and research Institute Co. LTD of Qinghai ProvinceQinghai Engineering and Technology Research Center of Fine ChemicalXining 810008China

A novel integrated film of sulfonated polysulfone/graphene/potassium copper ferricyanide(KCuFC/SPSG)was used for selectively extracting rubidium ion(Rb^(+))from *** form KCuFC/SPSG,the precursor film of sulfonated polysulfone/graphene(SPSG)was synthesized by phase conversion process,which was alternately immersed in 0.1 mol·L^(-1)CuSO_(4)/K_(4)[Fe(CN)_(6)]by in-situ adsorption coupled co-precipitation *** data such as nuclear magnetic resonance spectrometer,Fourier transform infrared spectroscope,X-ray photoelectron spectroscope,X-ray diffraction,scanning electron microscope,and energy dispersive spectroscopy all verified that abundant KCuFC were uniformly located on the *** resulting KCuFC/SPSG was used in film separation *** the solution was fed into the system,the Rb^(+)could be selectively adsorption by KCuFC/*** the saturation adsorption,0.5 mol·L^(-1)NH_(4)Cl/HCl was fed into the film cell,Rb^(+)could be quickly desorbed by ion-exchange between Rb^(+)and NH_(4)^(+)in the lattice of *** purpose of separating and recovering Rb^(+)from the brine can be achieved after the repeated *** effects of pH,adsorption time,and interferential ions on the adsorption capacity of Rb^(+)were investigated by batch *** adsorption behavior fits the pseudo-second order kinetic process,while KCuFC has a higher adsorption capacity(Langmuir maximum sorption 165.4 mg·g^(-1)).In addition,KCuFC/SPSG shows excellent selectivity for Rb^(+)even in complex brine ***/SPSG could maintain 93.5%extraction efficiency after five adsorption/desorption cycles.

关键词： Rubidium extraction Potassium copper ferricyanide Sulfonated polysulfone Graphene oxide Adsorption

Quantum Correlations in Werner Derivatives

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Communications in Theoretical Physics 2013年第10期60卷 405-409页

作者：王胜芳刘益民李国锋刘先松张战军 engineering technology research center of Magnetic Materials Anhui ProvinceSchool of Physics & Materials ScienceAnhui University Department of Physics Shaoguan University

Quantum correlations in Werner derivatives are studied with two different approaches, i.e., measurement- induced disturbance （MID） [Phys. Rev. A 77 （2008） 022301] and ameliorated MID （AMID） [J, Phys. A 44 （2011） 352002]. They are derived via strict deductions with MID while numerically calculated via the measurement optimization with AMID. Interestingly, quantum correlations captured with both approaches are completely coincident. Moreover, some distinct features of the quantum correlations and their underlying physics are exposed via analyses and discussions.

关键词： quantum correlation Werner derivatives measurement-induced disturbance (MID) amelioratedMID (AMID)

Upregulation of CDGSH iron sulfur domain 2 attenuates cerebral ischemia/reperfusion injury

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Neural Regeneration research 2023年第7期18卷 1512-1520页

作者： Miao Hu Jie Huang Lei Chen Xiao-Rong Sun Zi-Meng Yao Xu-Hui Tong Wen-Jing Jin Yu-Xin Zhang Shu-Ying Dong Department of Pharmacology School of PharmacyBengbu Medical CollegeBengbuAnhui ProvinceChina Key Laboratory of Cardiovascular and Cerebrovascular Diseases Bengbu Medical CollegeBengbuAnhui ProvinceChina anhui engineering technology research center of Biochemical Pharmaceutical BengbuAnhui ProvinceChina

CDGSH iron sulfur domain 2 can inhibit ferroptosis,which has been associated with cerebral ischemia/reperfusion,in individuals with head and neck ***,CDGSH iron sulfur domain 2 may be implicated in cerebral ischemia/reperfusion *** validate this hypothesis in the present study,we established mouse models of occlusion of the middle cerebral artery and HT22 cell models of oxygen-glucose deprivation and reoxygenation to mimic cerebral ischemia/reperfusion injury in vivo and in vitro,*** found remarkably decreased CDGSH iron sulfur domain 2 expression in the mouse brain tissue and HT22 *** we used adeno-associated virus and plasmid to up-regulate CDGSH iron sulfur domain 2 expression in the brain tissue and HT22 cell models separately,mouse neurological dysfunction was greatly improved;the cerebral infarct volume was reduced;the survival rate of HT22 cells was increased;HT22 cell injury was alleviated;the expression of ferroptosis-related glutathione peroxidase 4,cystine-glutamate antiporter,and glutathione was increased;the levels of malondialdehyde,iron ions,and the expression of transferrin receptor 1 were decreased;and the expression of nuclear-factor E2-related factor 2/heme oxygenase 1 was *** of CDGSH iron sulfur domain 2 upregulation via the nuclear-factor E2-related factor 2 inhibitor ML385 in oxygen-glucose deprived and reoxygenated HT22 cells blocked the neuroprotective effects of CDGSH iron sulfur domain 2 up-regulation and the activation of the nuclear-factor E2-related factor 2/heme oxygenase 1 *** data indicate that the up-regulation of CDGSH iron sulfur domain 2 can attenuate cerebral ischemia/reperfusion injury,thus providing theoretical support from the perspectives of cytology and experimental zoology for the use of this protein as a therapeutic target in patients with cerebral ischemia/reperfusion injury.

关键词： cerebral ischemia/reperfusion injury CDGSH iron sulfur domain 2 ferroptosis glutathione peroxidase 4 heme oxygenase 1 HT22 nuclear-factor E2-related factor 2 oxygen-glucose deprivation/reoxygenation injury stroke transferrin receptor 1