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Landscape of human organoids:Ideal model in clinics and research

The Innovation 2024年第3期5卷 146-164页

作者： Xinxin Han Chunhui Cai Wei Deng Yanghua Shi Lanyang Li Chen Wang Jian Zhang Mingjie Rong Jiping Liu Bangjiang Fang Hua He Xiling Liu Chuxia Deng Xiao He Xin Cao Organ Regeneration X Lab Lisheng East China Institute of BiotechnologyPeking UniversityJiangsu 226200China Shanghai Lisheng Biotech Shanghai 200092China LongHua Hospital Shanghai University of Traditional Chinese Medicine725 Wanping South RoadXuhui DistrictShanghai 200032China Department of Oncology Shanghai Ninth People’s HospitalShanghai Jiao Tong University School of MedicineShanghai 200125China Department of Neurosurgery Third Affiliated HospitalNaval Medical UniversityShanghai 200438China Shanghai Key laboratory of Forensic Medicine Shanghai Forensic Service PlatformAcademy of Forensic ScienceMinistry of JusticeShanghai 200063China Cancer Center Faculty of Health SciencesUniversity of MacaoTaipaMacao SARChina Ministry of Education Frontiers Science Center for Precision Oncology University of MacaoTaipaMacao SAR 999078China CAS Key Lab for Biomedical Effects of nanomaterials and Nanosafety Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China Zhongshan Hospital Institute of Clinical Science Fudan University Shanghai Medical CollegeShanghai 200032China

In the last decade,organoid research has entered a golden era,signifying a pivotal shift in the biomedical *** year 2023 marked a milestone with the publication of thousands of papers in this arena,reflecting exponential ***,amid this burgeoning expansion,a comprehensive and accurate overview of the field has been conspicuously *** review is intended to bridge this gap,providing a panoramic view of the rapidly evolving organoid *** meticulously analyze the organoid field from eight distinctive vantage points,harnessing our rich experience in academic research,industrial application,and clinical *** present a deep exploration of the advances in organoid technology,underpinned by our long-standing involvement in this *** narrative traverses the historical genesis of organoids and their transformative impact across various biomedical sectors,including oncology,toxicology,and drug *** delve into the synergy between organoids and avant-garde technologies such as synthetic biology and single-cell omics and discuss their pivotal role in tailoring personalized medicine,enhancing high-throughput drug screening,and constructing physiologically pertinent disease *** comprehensive analysis and reflective discourse provide a deep dive into the existing landscape and emerging trends in organoid *** spotlight technological innovations,methodological evolution,and the broadening spectrum of applications,emphasizing the revolutionary influence of organoids in personalized medicine,oncology,drug discovery,and other *** ahead,we cautiously anticipate future developments in the field of organoid research,especially its potential implications for personalized patient care,new avenues of drug discovery,and clinical *** trust that our comprehensive review will be an asset for researchers,clinicians,and patients with keen interest in personalized medical *** offer a broad view of the

关键词： landscape intended advances

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Interfacial engineering of metallic rhodium by thiol modification approach for ambient electrosynthesis of ammonia

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Nano Research 2022年第10期15卷 8826-8835页

作者： Meng Jin Xinyuan Zhang Xian Zhang Hongjian Zhou Miaomiao Han Yunxia Zhang Guozhong Wang Haimin Zhang laboratory of Materials Physics Centre for Environmental and Energy NanomaterialsAnhui Key Laboratory of Nanomaterials and NanotechnologyCAS Center for Excellence in NanoscienceInstitute of Solid State PhysicsHFIPSChinese Academy of SciencesHefei 230031China University of Science and Technology of China Hefei 230026China School of Science Huzhou UniversityHuzhou 313000China

Here we report a vapor-phase reaction approach to fabricate rhodium(I)-dodecanethiol complex coated on carbon fiber cloth(Rh(I)-SC_(12)H_(25)/CFC),followed by low-temperature pyrolysis to achieve dodecanethiol modified Rh(Rh@SC_(12)H_(2)5/CFC)for electrocatalytic nitrogen reduction reaction(NRR).The results demonstrate that after pyrolysis for 0.5 h at 150℃,the obtained Rh@SC_(12)H_(2)5/CFC-0.5 exhibits excellent NRR activity with an NH3 yield rate of 121.2±6.6μg∙h^(−1)∙cm^(−2)(or 137.7±7.5μg∙h^(−1)∙mgRh^(−1))and a faradaic efficiency(FE)of 51.6%±3.8%at−0.2 V(***)in 0.1 M Na_(2)SO_(4).The theoretical calculations unveil that the adsorption of dodecanethiol on the hollow sites of Rh(111)plane is thermodynamically favorable,effectively regulating the electronic structure and surface wettability of metallic ***,the dodecanethiol modification on Rh(111)obviously decreases the surface H*coverage,thus inhibiting the competitive hydrogen evolution reaction and concurrently reducing the electrocatalytic NRR energy barrier.

关键词： dodecanethiol modification electrocatalysis low temperature pyrolysis nitrogen reduction reaction surface H*coverage

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Integration of advanced biotechnology for green carbon

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Green Carbon 2024年第2期2卷 164-175页

作者： Miao Wang Yixiang Wang Jingyuan Liu Hua Yu Peng Liu Yujing Yang Dan Sun Heng Kang Yanting Wang Jingfeng Tang Chunxiang Fu Liangcai Peng Key laboratory of Fermentation Engineering(Ministry of Education) National"111"Center for Cellular Regulation&Molecular PharmaceuticsCooperative Innovation Center of Industrial Fermentation(Ministry of Education&Hubei Province)Hubei Key Laboratory of Industrial MicrobiologyBiomass&Bioenergy Research CenterHubei University of TechnologyWuhan 430068China College of Plant Science&Technology Huazhong Agricultural UniversityWuhan 430070China Shandong Provincial Key laboratory of energy Genetics CAS Key Laboratory of BiofuelsQingdao Institute of Bioenergy&Bioprocess TechnologyChinese Academy of SciencesQingdao 266101China Shandong energy Institute Qingdao 266101China

Carbon neutralization has been introduced as a long-term policy to control global warming and climate *** plant photosynthesis produces the most abundant lignocellulosic biomass on Earth,its conversion to biofuels and bioproducts is considered a promising solution for reducing the net carbon ***,natural lignocellulose recalcitrance crucially results in a costly biomass process along with secondary waste *** updating recent advances in plant biotechnology,biomass engineering,and carbon nanotechnology,this study proposes a novel strategy that integrates the genetic engineering of bioenergy crops with green-like biomass processing for cost-effective biofuel conversion and high-value *** selecting key genes and appropriate genetic manipulation approaches for precise lignocellulose modification,this study highlights the desirable genetic site mutants and transgenic lines that are raised in amorphous regions and inner broken chains account for high-density/length-reduced cellulose nanofiber assembly in *** the amorphous regions and inner-broken chains of lignocellulose substrates are defined as the initial breakpoints for enhancing biochemical,chemical,and thermochemical conversions,desirable cellulose nanofibers can be employed to achieve nearcomplete biomass enzymatic saccharification for maximizing biofuels or high-quality biomaterials,even under cost-effective and green-like biomass processes in *** study emphasizes the optimal thermal conversion for generating high-performance nanocarbons by combining appropriate nanomaterials generated from diverse lignocellulose ***,this study provides a perspective on the potential of green carbon productivity as a part of the fourth industrial revolution.

关键词： Lignocellulose Biofuels nanomaterials Nanocarbon Genetic engineering

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Hierarchical and self-supporting honeycomb LaNi_5 alloy on nickel foam for overall water splitting in alkaline media

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Green energy & Environment 2022年第4期7卷 799-806页

作者： Yanze Wu Yalan Liu Kui Liu Lin Wang Lei Zhang Degao Wang Zhifang Chai Weiqun Shi Engineering laboratory of Advanced energy Materials Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo315201ZhejiangChina laboratory of Nuclear energy Chemistry and Key laboratory for Biomedical Effects of nanomaterials and Nanosafety Institute of High Energy PhysicsChinese Academy of SciencesBeijing100049China University of Chinese Academy of Sciences Beijing100049China

Ni-based metallic foams possessing large specific surfaces and open cell structures are of specific interest as catalysts or catalyst carriers for electrolysis of *** fabrication of Nickel foam limits the element modification choices to several inert transition metals only on polymer foam precursor and subsequent preparation of foam-based catalysts in aqueous solution or organic *** expand the modification horizon,molten salt with wide electrochemical window and fast ion diffusion can achieve the reduction of highly active ***,we reported is a general and facile method to deposit directly of highly reactive element La and prepare hierarchical honeycomb LaNi_(5) alloy on Ni foam(ho-LaNi_(5)/NF).This self-supporting electrode presents excellent electrical coupling and conductivity between the Ni foam and LaNi_(5),which provides a 3D self-supported heterostructure with outstanding electrocatalytic activity and excellent durability for the hydrogen evolution reaction(HER)and oxygen evolution reaction(OER).It exhibits excellent overpotential(1.86 V)comparable to commercial coupled IrO_(2)//Pt/C(1.85 V)at a high current density of 100 m A cm^(-2).This work may pave the way for fabricating novel 3D self-supported honeycomb alloy that can be applied as electrode for usage of clean energy.

关键词： Honeycomb alloy Hierarchical structures Molten salt Hydrogen evolution reaction Oxygen evolution reaction

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Advanced 2D molybdenum disulfide for green hydrogen production: Recent progress and future perspectives

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Frontiers in energy 2024年第3期18卷 308-329页

作者： Meng FANG Yuqin PENG Puwei WU Huan WANG Lixin XING Ning WANG Chunmei TANG Ling MENG Yuekuan ZHOU Lei DU Siyu YE Huangpu Hydrogen energy Innovation Centre School of Chemistry and Chemical EngineeringGuangzhou UniversityGuangzhou 510006China Sustainable energy and Environment Thrust Function HubThe Hong Kong University of Science and Technology(Guangzhou)Guangzhou 511400China Department of Mechanical and Aerospace Engineering The Hong Kong University of Science and TechnologyHong KongChina SinoHykey Technology Company Ltd. Guangzhou 510760China

The development of renewable and affordable energy is crucial for building a sustainable society. In this context, establishing a sustainable infrastructure for renewable energy requires the integration of energy storage, specifically use of renewable hydrogen. The hydrogen evolution reaction (HER) of electrochemical water splitting is a promising method for producing green hydrogen. Recently, two-dimensional nanomaterials have shown great promise in promoting the HER in terms of both fundamental research and practical applications due to their high specific surface areas and tunable electronic properties. Among them, molybdenum disulfide (MoS2), a non-noble metal catalyst, has emerged as a promising alternative to replace expensive platinum-based catalysts for the HER because MoS_(2)has a high inherent activity, low cost, and abundant reserves. At present, greatly improved activity and stability are urgently needed for MoS_(2)to enable wide deployment of water electrolysis devices. In this regard, efficient strategies for precisely modifying MoS_(2)are of interest. Herein, the progress made with MoS_(2)as an HER catalyst is reviewed, with a focus on modification strategies, including phase engineering, morphology design, defect engineering, heteroatom doping, and heterostructure construction. It is believed that these strategies will be helpful in designing and developing high-performance and low-cost MoS2-based catalysts by lowering the charge transfer barrier, increasing the active site density, and optimizing the surface hydrophilicity. In addition, the challenges of MoS_(2)electrocatalysts and perspectives for future research and development of these catalysts are discussed.

关键词： molybdenum disulfide(MoS_(2)) hydrogen evolution reaction(HER) active site electrocatalyst modification strategie

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Luminescence properties of rare earth complexes bonded to novel mesoporous spherical hybrid materials

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Journal of Rare Earths 2023年第1期41卷 60-66页

作者： Lin Huang Juan Wang Haipeng Zhang Guannan Zu Zhentao Wang Yonghong Fu Shaanxi Key laboratory of nanomaterials and Nanotechnology Xi'an University of Architecture and TechnologyXi'an 710055China

YVO_(4):Eu^(3+) phosphors have been widely used in optoelectronic integration fields of its chemical and thermal ***,the excitation spectrum band of VO_(4)^(3-) is too narrow for high-efficiency luminescence,restricting its further ***,flower-like and linear-like YVO_(4):Eu^(3+) hollow mesoporous spheres were synthesized and connected with Eu organic ligand,to obtain a new hybrid luminescent *** characterization shows that the pores of microspheres are in size of about 2-50 nm,sticked with regular morphology,well crystallized,and in uniform *** emission intensity of hybrid luminescent material is higher than that of single YVO_(4):Eu^(3+) and single Eu co mplexes realizing the purpose of mutually reinforcing luminesce *** paper provides a new idea to connect rare earth complexes for a new non-silicon-based mesoporous spherical matrix.

关键词： YVO_(4):Eu^(3+) Mesoporous spheres Hybrid material Luminescence Rare earths

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Polyoxometalates for continuous power generation by atmospheric humidity

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Nano Research 2024年第3期17卷 1875-1885页

作者： Tuo Ji Weilin Chen Zhenhui Kang Liming Zhang Key laboratory of Polyoxometalate and Reticular Material Chemistry of Ministry of Education Northeast Normal UniversityChangchun 130024China Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&Devices DepartmentSoochow UniversitySuzhou 215123China Macao Institute of Materials Science and Engineering Macao University of Science and TechnologyTaipaMacao 999078China Institute of Functional State Key laboratory of Luminescence and Applications Changchun Institute of OpticsFine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China

Atmospheric humidity is a sustainable low-value energy widely existing in natural environment,which is a promising candidate to solve the noncontinuous and low efficiency of low-value energy power *** the mono-substituted Dawson-type polyoxometalates are constructed to be highly dispersed organic ammonium-polyoxoanion clusters and are assembled into thin films power generators with micropores,working in atmospheric *** optimal polyoxometalates generator with the thickness of 7.2μm and the area of 0.36 cm^(2) produces a voltage of 0.68 V and a current density of 19.5μA·cm^(-2) under simulated natural environment,and works continuously and stably under almost all-natural environments(humidity 10%–90%).The highly dispersed polyoxometalate nanoclusters can form microporous in polyoxometalate films to effectively absorb atmospheric humidity and spontaneously form distribution gradient of water,which is the structural basis of power *** continuous power generation may be maintained by the effective adsorption and utilization of H_(2)O,the huge electrostatic field of organic ammonium-polyoxoanion clusters,and the reasonably designed polyoxometalates containing inorganic small ions with high *** is the first humidity generator designed with polyoxometalates,which may provide a new research direction for polyoxometalates in sustainable utilization of low-value energy.

关键词： atmospheric humidity continuous power generations nanomaterials polyoxoanions polyoxometalates

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Fullerenes and derivatives as electrocatalysts: Promises and challenges

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Green energy & Environment 2024年第1期9卷 7-27页

作者： Kun Guo Ning Li Lipiao Bao Xing Lu State Key laboratory of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan430074China

Carbon-based metal-free nanomaterials are promising alternatives to precious metals as electrocatalysts of key energy storage and conversion *** paramount signiﬁcance are the establishment of design principles by understanding the catalytic mechanisms and identifying the active *** from sp2-conjugated graphene and carbon nanotube,fullerene possesses unique characteristics that are growingly being discovered and exploited by the electrocatalysis *** instance,the well-deﬁned atomic and molecular structures,the good electron afﬁnity to tune the electronic structures of other substances,the intermolecular self-assembly into superlattices,and the on-demand chemical modiﬁcation have endowed fullerene with incomparable advantages as electrocatalysts that are otherwise not applicable to other carbon *** increasing studies are being reported on this intriguing topic,it is necessary to provide a state-of-the-art overview of the recent *** review takes such an initiative by summarizing the promises and challenges in the electrocatalytic applications of fullerene and its *** content is structured according to the composition and structure of fullerene,including intact fullerene(e.g.,fullerene composite and superlattices)and fullerene derivatives(e.g.,doped,endohedral,and disintegrated fullerene).The synthesis,characterization,catalytic mechanisms,and deﬁciencies of these fullerene-based materials are explicitly *** conclude it by sharing our perspectives on the key aspects that future efforts shall consider.

关键词： Fullerene Fullerene derivative Metal-free catalyst Structural defect Electrocatalyst

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Atomically dispersed metal sites in COF-based nanomaterials for electrochemical energy conversion

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Green energy & Environment 2023年第2期8卷 360-382页

作者： Yaqi Cao Wenchao Peng Yang Li Fengbao Zhang Yuanzhi Zhu Xiaobin Fan State Key laboratory of Chemical Engineering School of Chemical Engineering and TechnologyTianjin UniversityTianjin300350China Yunnan Provincial Key laboratory of energy Saving in Phosphorus Chemical Engineering and New Phosphorus Materials Faculty of Chemical EngineeringKunming University of Science and TechnologyKunming650500China

Atomically dispersed metal sites(ADMSs)play key roles in electrochemical energy *** covalent organic frameworks(COFs)enable the precise control of the chemical compositions and structures at the molecular level,making them ideal substrates for supporting *** this review,we systematically summarize the recent progress on the design and synthesis of ADMSs in COFs,including embedding molecular catalysts into COFs,immobilizing ADMSs on heteroatom-containing COFs,and preparing COF-derived carbon materials through *** electrocatalytic performance of the resulting catalysts is presented for various electrochemical reactions,involving oxygen reduction reaction(ORR),carbon dioxide reduction reaction(CO_(2)RR),oxygen evolution reaction(OER),hydrogen evolution reaction(HER),and nitrogen reduction reaction(NRR).The modulation strategies of AMDSs in COFs for enhanced activity,selectivity,and stability are highlighted,together with a perspective of the current challenges and the future opportunities in this field.

关键词： Covalent organic frameworks Metal sites Single-atom catalysts Electrochemical energy conversion

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Photoelectrocatalytic principles for meaningfully studying photocatalyst properties and photocatalysis processes:From fundamental theory to environmental applications

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Journal of energy Chemistry 2023年第11期86卷 84-117,I0003页

作者： Jiafang Liu Shengbo Zhang Weikang Wang Haimin Zhang Key laboratory of Materials Physics Centre for Environmental and Energy NanomaterialsAnhui Key Laboratory of Nanomaterials and NanotechnologyCAS Center for Excellence in NanoscienceInstitute of Solid State PhysicsChinese Academy of SciencesHefei 230031AnhuiChina University of Science and Technology of China Hefei 230026AnhuiChina School of Materials Science and Engineering Jiangsu UniversityZhenjiang 212013JiangsuChina

Photocatalysis is critically important for environmental remediation and renewable energy *** ability to objectively characterize photocatalyst properties and photocatalysis processes is paramount for meaningful performance evaluation and fundamental studies to guide the design and development of high-performance photocatalysts and photocatalysis *** is essentially an electron transfer process,and photoelectrocatalysis(PEC)principles can be used to directly quantify transferred electrons to determine the intrinsic properties of photocatalysts and photocatalysis processes in isolation,without interference from counter reactions due to physically separated oxidation and reduction *** this review,we discuss emphatically the PEC-based principles for characterizing intrinsic properties of photocatalysts and important processes of photocatalysis,with a particular focus on their environmental applications in the degradation of pollutants,disinfection,and detection of chemical oxygen demand(COD).An outlook towards the potential applications of PEC technique is given.

关键词： Photoelectrocatalysis Photocatalytic intrinsic properties Photocatalytic characterization Environmental remediation Photoelectrocatalysis-based application

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