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Investigations of the mechanical response of dummy HTPB propellant grain under ultrahigh acceleration overload conditions using onboard flight-test measurements

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Defence Technology（防务技术） 2024年第2期32卷 473-484页

作者： Yiming Zhang Ningfei Wang Weihua Ma Ran Wang Long Bai Yi Wu School of Aerospace Engineering Beijing Institute of TechnologyBeijing 100081China Beijing System Design Institute of Electro-mechanic Engineering Beijing 100854China Xi'an Changfeng research Institute of Mechanism and electricity Xi'an 710065China

In this paper,to study the mechanical responses of a solid propellant subjected to ultrahigh acceleration overload during the gun-launch process,specifically designed projectile flight tests with an onboard measurement system were *** projectiles containing dummy HTPB propellant grains were successfully recovered after the flight tests with an ultrahigh acceleration overload value of 8100 *** onboard-measured time-resolved axial displacement,contact stress and overload values were successfully obtained and *** compression tests of the dummy HTPB propellant used in the gunlaunched tests were carried out at low and intermediate strain rates to characterize the propellant's dynamic properties.A linear viscoelastic constitutive model was employed and applied in finite-element simulations of the projectile-launching *** the launch process,the dummy propellant grain exhibited large deformation due to the high acceleration overload,possibly leading to friction between the motor case and propellant *** calculated contact stress showed good agreement with the experimental results,though discrepancies in the overall displacement of the dummy propellant grain were *** dynamic mechanical response process of the dummy propellant grain was analysed in *** results can be used to estimate the structural integrity of the analysed dummy propellant grain during the gun-launch process.

关键词： Gun-launched flight test Dummy HTPB propellant Onboard measurements Utrahigh overload Mechanical response

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Incorporation sodium ions into monodisperse lead-free double perovskite Cs_(2)AgBiCl_(6) nanocrystals to improve optical properties

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Chinese Chemical Letters 2024年第3期35卷 549-553页

作者： Song Wang Ying Xie Wenchao Jiang Binghang Liu Keying Shi Kai Pan Key laboratory of Functional Inorganic Material Chemistry Ministry of EducationHeilongjiang UniversityHarbin 150080China School of Materials Science and Engineering Jiangsu Engineering Laboratory of Light-Electricity-Heat Energy-Converting Materials and ApplicationsChangzhou UniversityChangzhou 213164China State Key laboratory of Catalysis Dalian National Laboratory for Clean EnergyDalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China

Lead-free double perovskite nanocrystals(NCs)have emerged as a promising candidate in the optical field,owing to their non-toxic,good moist heat and chemical ***,their poor optical properties limited their *** improve the optical properties of lead-free double perovskite NCs,metal ion doping or alloying had been suggested as a promising ***,we prepared monodisperse,uniformly sized,cubic morphology of Cs_(2)AgBiCl_(6)NCs with different Na^(+)incorporation amounts via a simple hot-injection *** Na^(+)incorporation broke the parity-forbidden transition by reducing the inversion symmetry of the electron wave function at the Ag site,which changed the parity of the self-trapped exciton wave function and thus allowed radiative *** a result,the photoluminescence quantum yield(PLQY)of Na^(+)-alloyed Cs_(2)AgBiCl_(6)NCs(12.1%)was higher than that of Cs_(2)AgBiCl_(6)NCs(2.4%),and the exciton lifetime of Na^(+)-alloyed Cs_(2)AgBiCl_(6)NCs increased to 36.98 ns from 17.58 ns for Cs_(2)AgBiCl_(6)*** adjusting the amount of Na^(+)incorporation,the band gap of Cs_(2)AgBiCl_(6)NCs can be significantly tuned from~2.90 eV to~3.50 ***,the temperature-dependent photoluminescence spectra indicated that the Na^(+)-alloyed Cs_(2)AgBiCl_(6)NCs possessed higher longitudinal optical phonon energy and exciton binding energy compared to Cs_(2)AgBiCl_(6)*** suggested that there were strong exciton-phonon interactions during exciton recombination,a reduced probability of non-radiative processes,and excellent thermal *** offers a promising strategy for improving the optical properties of lead-free double perovskite NCs,and have the potential to replace traditional lead halide perovskite NCs in future optoelectronic applications.

关键词： Nanocrystals Alloy Double perovskites Optical properties Exciton binding energy

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Trialkylsilyl-thiophene-conjugated acceptor for efficient organic solar cells compatible with spin-coating and blade-coating technologies

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Science China Chemistry 2024年

作者： Tengfei Li Qiang Wu Zefan Yao Hairui Bai Wenyan Su Rui Sun Lingxiao Tang Zhaozhao Bi Xiaojun Li Weiguo Zhu Jie Min Qunping Fan Wei Ma State Key laboratory for Mechanical Behavior of Materials Xi'an Jiaotong University College of Chemistry and Molecular Engineering Peking University School of Materials Science and Engineering Xi'an University of Science and Technology Jiangsu Engineering research Center of Light-electricity-Heat Energy-Converting Materials and Applications School of Materials Science and Engineering and Changzhou University The Institute for Advanced Studies Wuhan University Beijing National laboratory for Molecular Sciences CAS Key Laboratory of Organic Solids Institute of Chemistry Chinese Academy of Sciences

Sidechain engineering as an efficient and convenient strategy has been widely used to optimize molecular structure of photovoltaic materials for boosting power conversion efficiency(PCE) of organic solar cells(OSCs). Herein, a new Y-series acceptor named Y-ThSi with trialkylsilyl-substituted thiophene as conjugated sidechain is developed. Compared with its parental Y6 with multiple intermolecular interactions, Y-ThSi has a unitary molecular packing due to the additional steric hindrance from twodimensional(2D)-conjugated trialkylsilyl-thiophene. Therefore, Y-ThSi shows an obviously blue-shifted absorption with an onset of ～850 nm but significantly up-shifted lowest unoccupied molecular orbital energy level. For the PM6:Y-ThSi pair, the spin-coating OSCs achieve a decent PCE of 14.56% with an impressively high photovoltage(VOC) of 0.936 V. Inspired by its high VOCand narrow absorption, Y-ThSi is introduced into near-infrared absorbing binary PM6:BTP-eC9 host to construct ternary OSCs. Thanks to the complementary absorption, optimized morphology, and minimized energy loss properties, the PM6:BTP-eC9:Y-ThSi-based OSCs offer a higher PCE of 18.34%. Moreover, our developed strategy can overcome the commonly existed PCE drop when the blade-coating towards large-scale printing is used instead. Therefore, a comparable PCE of 18.34% is achieved, which is one of the best values for the blade-coating OSCs so far.

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Promising thermal photonic management materials for sustainable human habitat

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Nano research 2024年第1期17卷 112-131页

作者： Houze Yao Qihua Liao Huhu Cheng Liangti Qu Key laboratory of Organic Optoelectronics&Molecular Engineering Ministry of EducationDepartment of ChemistryLaboratory of Flexible Electronics TechnologyTsinghua UniversityBeijing 100084China State Key laboratory of Tribology in Advanced Equipment(SKLT) Department of Mechanical EngineeringTsinghua UniversityBeijing 100084China

The spectral characteristics of outdoor structures,such as automobiles,buildings,and clothing,determine their energy interaction with the environment,from broad-spectrum absorption of light energy to high-efficiency thermal *** developed spectrally selective absorption(SSA)materials permit the reduction of energy loss from human habitat eco-system in the sustainable way and further reduce the utilization of fossil energy to achieve carbon *** we review recent advances in SSA materials that enable rational and efficient management of thermal energy and provide new solutions for the resource base that supports human life like comfortable heat management,electricity production,and water *** basic principles of thermal photonic management,the regulation of SSA materials,and functional properties are *** outlook discussing challenges and opportunities in SSA material energy management for comfortable living environments is finally presented,which expects the enormous potential of this interdisciplinary research in solving growing resource-shortage of human society.

关键词： spectrally selective absorption passive cooling solar power eco-system

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Magnetoimpedance of Electroplated Wires with Large Core Diameters

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Journal of Materials Science & Technology 2009年第6期25卷 825-828页

作者： C. Sirisathitkul P. Jantaratana Magnet laboratory Molecular Technology Research Unit School of Science Walailak University electricity and magnetism properties research laboratory Department of Physics Faculty of Science Kasetsart University

Monolayered Co and trilayered Co/Cu/Co were electroplated on 485 μm-diameter Cu wires using the bath pH 2.5. These wires can be functioned as magnetic sensors owing to their magnetoimpedance （MI） effect. By measuring at four different frequencies （100, 250, 500, and 1000 kHz） and Co thicknesses （2.5, 5.0, 10.0, and 25.0μm）, the MI ratio of electroplated Co on Cu wires tended to increase with increasing Co thickness and frequency of the driving current. The Co/Cu/Co on Cu wires exhibited even higher MI ratio. The magnetic layer also regulated the magnetic inductions and anisotropy regardless of the size of nonmagnetic core. Nevertheless, the diameter of the Cu core had a significant effect on the MI ratio. By comparing with the 47.7 μm-diameter Ag cores electroplated by Co and Co/Cu/Co of the same thickness, the Cu cores with a larger diameter gave rise to a larger MI ratio because their lower electrical resistance enhanced the crossing effect. Substantial MI ratio was observed even in a low frequency regime because the skin effect occurred at a low frequency in the case of electroplated wires with large core diameters.

关键词： Magnetoimpedance Electroplated wire Copper Cobalt

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Rational design of natural leather-based water evaporator for electricity generation and functional applications

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Journal of Energy Chemistry 2024年第9期96卷 129-144页

作者： Bingyuan Zhang Xiaoyu Guan Qingxin Han Haoxiang Guo Sai Zheng Xuhui Sun Afnan H.El-Gowily Mohammed A.Abosheasha Yanxia Zhu Motoki Ueda Meng An Haojun Fan Yoshihiro Ito College of Bioresources Chemical and Materials Engineering Key Laboratory of Auxiliary Chemistry and Technology for Chemical IndustryMinistry of EducationShaanxi Collaborative Innovation Center of Industrial Auxiliary Chemistry and TechnologyShaanxi University of Science&TechnologyXi'an 710021ShaanxiChina Nano Medical Engineering laboratory RIKEN Cluster for Pioneering Research2-1 HirosawaWako 351-0198SaitamaJapan Key laboratory of Leather Chemistry and Engineering(Sichuan University) Ministry of EducationChengdu 610065SichuanChina College of Mechanical and Electrical Engineering Shaanxi University of Science&TechnologyXi'an 710021ShaanxiChina Biochemistry Division Chemistry DepartmentFaculty of ScienceTanta UniversityTanta 31527Egypt

In recent years,water evaporation-induced electricity has attracted a great deal of attention as an emerging green and renewable energy harvesting *** abundant materials have been developed to fabricate hydrovoltaic devices,the limitations of high costs,inconvenient storage and transport,low environmental benefits,and unadaptable shape have restricted their wide ***,an electricity generator driven by water evaporation has been engineered based on natural biomass leather with inherent properties of good moisture permeability,excellent wettability,physicochemical stability,flexibility,and *** numerous nano/microchannels together with rich oxygen-bearing functional groups,the natural leather-based water evaporator,Leather_(Emblic-NPs-SA/CB),could continuously produce electricity even staying outside,achieving a maximum output voltage of∼3 V with six-series ***,the leather-based water evaporator has enormous potential for use as a flexible self-powered electronic floor and seawater demineralizer due to its sensitive pressure sensing ability as well as its excellent photothermal conversion efficiency(96.3%)and thus fast water evaporation rate(2.65 kg m^(−2)h^(−1)).This work offers a new and functional material for the construction of hydrovoltaic devices to harvest the sustained green energy from water evaporation in arbitrary ambient environments,which shows great promise in their widespread applications.

关键词： Energy conversion Water evaporation-induced electricity Functional leather Flexible self-powered sensor Desalination

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Enhancement of GMI Effect in Silicon Steels by Furnace Annealing

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Journal of Materials Science & Technology 2009年第5期25卷 619-621页

作者： C.Sirisathitkul P.Jantaratana Magnet laboratory Molecular Technology Research UnitSchool of ScienceWalailak UniversityNakon Si Tham-marat 80161Thailand electricity and magnetism properties research laboratory Department of PhysicsFaculty of ScienceKasetsart UniversityBangkok 10900Thailand

The ratio and sensitivity of giant magnetoimpedance （GMI） in grain oriented silicon steels （Fe-4.5%Si） are improved after furnace annealing in air for 20 min. By annealing at 800℃, the GMI sensitivity rises from 1.29%/Oe to 1.91%/Oe and the ratio increases from 237% to 294% with decreasing characteristic frequency. The results are attributable to an increase in the transverse magnetic permeability during the heat treatment. From simulation by finite element method, the GMI effect can be interpreted as the modification of the current distribution by the applied magnetic field via the transverse permeability. In the case of annealed samples,the larger transverse permeability allows a higher GMI ratio and sensitivity.

关键词： Silicon steels Giant magnetoimpedance Furnace annealing Skin depth Transverse permeability

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Solvation Engineering via Fluorosurfactant Additive Toward Boosted Lithium-Ion Thermoelectrochemical Cells

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Nano-Micro Letters 2024年第4期16卷 253-268页

作者： Yinghong Xu Zhiwei Li Langyuan Wu Hui Dou Xiaogang Zhang Jiangsu Key laboratory of Electrochemical Energy Storage Technologies College of Material Science and TechnologyNanjing University of Aeronautics and AstronauticsNanjing 211106People’s Republic of China

Lithium-ion thermoelectrochemical cell(LTEC), featuring simultaneous energy conversion and storage, has emerged as promising candidate for low-grade heat harvesting. However, relatively poor thermosensitivity and heat-to-current behavior limit the application of LTECs using LiPF_6 electrolyte. Introducing additives into bulk electrolyte is a reasonable strategy to solve such problem by modifying the solvation structure of electrolyte ions. In this work, we develop a dual-salt electrolyte with fluorosurfactant(FS) additive to achieve high thermopower and durability of LTECs during the conversion of low-grade heat into electricity. The addition of FS induces a unique Li~+ solvation with the aggregated double anions through a crowded electrolyte environment,resulting in an enhanced mobility kinetics of Li~+ as well as boosted thermoelectrochemical performances. By coupling optimized electrolyte with graphite electrode, a high thermopower of 13.8 mV K^(-1) and a normalized output power density of 3.99 mW m^(–2) K^(–2) as well as an outstanding output energy density of 607.96 J m^(-2) can be *** results demonstrate that the optimization of electrolyte by regulating solvation structure will inject new vitality into the construction of thermoelectrochemical devices with attractive properties.

关键词： Solvation engineering Fluorosurfactant Ionic thermoelectric Lithium-ion thermoelectrochemical cell Low-grade heat

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Aggregating structure in coal water slurry studied by eDLVO theory and fractal dimension

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Frontiers in Energy 2023年第2期17卷 306-316页

作者： Qiang LI Qian WANG Jian HOU Jiansheng ZHANG Yang ZHANG Key laboratory for Thermal Science and Power Engineering of the Ministry of Education Department of Energy and Power EngineeringTsinghua UniversityBeijing 100084China Energy and electricity research Center Jinan UniversityZhuhai 519070China

Coal water slurry gasification is a main source of hydrogen in the developing hydrogen ***,biomass and waste can be added,making gasification process *** expand the application of coal water slurry and gasification process,it is necessary to understand the micro-structure in this large particle suspension *** this paper,the micro-structure in coal water slurry was studied by extended DLVO(eDLVO)theory and fractal dimension,which is used to explain the mechanism of stability in large particle suspension *** interaction between two coal particles was characterized from the interparticle potential and energy barrier based on the eDLVO *** rheology and stability between different types of coals are measured and explained by the aggregating structure and fractal dimension in coal water *** results indicated that there would be an aggregating structure in high rank coals,due to the interparticle potential caused by the surface properties,but probably not in low rank *** aggregating structure can be described and characterized by fractal *** aggregation of particles is the source of the stability for high rank coals,as the close-packed 3D network structure in large particle suspension can support coal particles from settling *** results have demonstrated that the combination of the eDLVO theory and rheological measurement is an effective way to investigate the stability of large particle suspension systems.

关键词： coal water slurry extended DLVO(eDLVO) fractal dimension stability

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Highly stretchable kirigami-patterned nanofiber-based nanogenerators for harvesting human motion energy to power wearable electronics

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Materials Futures 2024年第2期3卷 131-140页

作者： Chuan Ning Shengxin Xiang Xiupeng Sun Xinya Zhao Chuanhui Wei Lele Li Guoqiang Zheng Kai Dong College of Materials Science and Engineering Key Laboratory of Material Processing and Mold(Ministry of Education)Zhengzhou UniversityZhengzhou 450001People’s Republic of China Key laboratory of Materials Physics Ministry of EducationSchool of Physics and MicroelectronicsZhengzhou UniversityZhengzhou 450001People’s Republic of China CAS Center for Excellence in Nanoscience Beijing Key Laboratory of Micro-Nano Energy and SensorBeijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijing 101400People’s Republic of China School of Nanoscience and Technology University of Chinese Academy of SciencesBeijing 100049People’s Republic of China

Wearable electronics are advancing towards miniaturization and ***,traditional energy supply methods have largely hindered their *** effective solution to this problem is to convert human mechanical energy into electricity to power wearable electronic ***,it is greatly attractive to design flexible,foldable and even stretchable energy harvesting ***,we use the electrospinning and kirigami approach to develop a type of highly stretchable kirigami-patterned nanofiber-based triboelectric nanogenerator(K-TENG).Due to its innovative structural design,the K-TENG can achieve a tensile strain of 220%,independent of the tensile properties of the material *** a person swings their arms,the K-TENG fixed to the clothing can convert mechanical energy from human movement into electrical *** produced electricity can directly drive 50 LED lights and a digital watch,or be stored in a lithium battery to charge the smartwatch and smartphone,*** study employs a new method to fabricate a stretchable triboelectric nanogenerator and demonstrates its promising applications in wearable power technology.

关键词： stretchable triboelectric nanogenerators kirigami energy harvesting

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