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Radioisotope production using lasers:From basic science to applications

Matter and Radiation at Extremes 2024年第3期9卷 31-44页

作者： M.R.D.Rodrigues A.Bonasera M.Scisciò J.A.Pérez-Hernández M.Ehret F.Filippi P.L.Andreoli M.Huault H.Larreur D.Singappuli D.Molloy D.Raffestin M.Alonzo G.G.Rapisarda D.Lattuada G.L.Guardo C.Verona Fe.Consoli G.Petringa A.McNamee M.La Cognata S.Palmerini T.Carriere M.Cipriani G.di Giorgio G.Cristofari R.De Angelis G.A.P.Cirrone D.Margarone L.Giuffrida D.Batani P.Nicolai K.Batani R.Lera L.Volpe D.Giulietti S.Agarwal M.Krupka S.Singh Fa.Consoli Cyclotron Institute Texas A&M UniversityCollege StationTexas 77840USA Laboratori Nazionali del Sud Istituto Nazionale di Fisica Nucleare(LNS-INFN)CataniaItaly ENEA Fusion and Technologies for Nuclear Safety and Security Department-CFrascatiItaly Centro de Láseres Pulsados(clpu) VillamayorSpain Universidad de Salamanca SalamancaSpain Centre Lasers Intenses et Applications(CELIA) Universitéde BordeauxCNRSCEATalenceFrance HB11 Energy Holdings Pty FreshwaterNew South WalesAustralia School of Mathematics and Physics Queen’s University BelfastBelfastUnited Kingdom dipartimento di fisica e Astronomia“E.Majorana ”Università di CataniaCataniaItaly Facoltàdi Ingegneria e Architettura Universitàdegli Studi di Enna“Kore”EnnaItaly dipartimento di Ingegneria Industriale Universitàdi Roma“Tor Vergata”RomaItaly dipartimento di fisica e Geologia Universitàdegli Studi di PerugiaPerugiaItaly Istituto Nazionale di fisica Nucleare Sezione di PerugiaPerugiaItaly ELI Beamlines Facility the Extreme Light Infrastructure ERICDolni BrezanyCzech Republic ETSIA Universidad Politécnica de MadridMadridSpain dipartimento fisica “E.Fermi”Universitàdi Pisa and INFNPisaItaly FZU–Institute of Physics of Czech Academy of Sciences PragueCzech Republic Institute of Plasma Physics of Czech Academy of Sciences PragueCzech Republic

The discovery of chirped pulse amplification has led to great improvements in laser technology,enabling energetic laser beams to be compressed to pulse durations of tens of femtoseconds and focused to a few micrometers.Protons with energies of tens of MeV can be accelerated using,for instance,target normal sheath acceleration and focused on secondary targets.Under such conditions,nuclear reactions can occur,with the production of radioisotopes suitable for medical application.The use of high-repetition lasers to produce such isotopes is competitive with conventional methods mostly based on accelerators.In this paper,we study the production of^(67)Cu,^(63)Zn,^(18)F,and^(11)C,which are currently used in positron emission tomography and other applications.At the same time,we study the reactions^(10)B(p,α)^(7)Be and^(70)Zn(p,4n)^(67)Ga to put further constraints on the proton distributions at different angles,as well as the reaction^(11)B(p,α)^(8)Be relevant for energy production.The experiment was performed at the 1 PW laser facility at VegaⅢin Salamanca,Spain.Angular distributions of radioisotopes in the forward(with respect to the laser direction)and backward directions were measured using a high purity germanium detector.Our results are in reasonable agreement with numerical estimates obtained following the approach of Kimura and Bonasera[Nucl.Instrum.Methods Phys.Res.,Sect.A 637,164–170(2011)].

关键词： purity estimates backward

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One-neutron stripping process in the^(209)Bi(^(6)Li,^(5)Li)^(210)Bi*reaction reaction

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Nuclear Science and Techniques 2024年第6期35卷 120-129页

作者： Gao-Long Zhang Zhen-Wei Jiao Guang-Xin Zhang E.N.Cardozo B.Paes Shi-Peng Hu Jian-Qiang Qian Daniele Mengoni Wei-Wei Qu Cong-Bo Li Yun Zheng Huan-Qiao Zhang Hui-Bin Sun Nan Wang Chun-Lei Zhang J.J.Valiente-Dobón D.Testov M.Mazzocco A.Gozzelino C.Parascandolo D.Pierroutsakou M.La Commara A.Goasduff D.Bazzacco D.R.Napoli F.Galtarossa F.Recchia A.Illana S.Bakes I.Zanon S.Aydin Gde Angelis M.Siciliano R.Menegazzo S.M.Lenzi S.Akkoyun L.F.Canto J.Lubian School of Physics Beihang UniversityBeijing 100191China Sino-French Institute of Nuclear Engineering and Technology Sun Yat-Sen UniversityZhuhai 519082China Instituto de Física Universidade Federal Fluminense24210-340 NiteróiRio de JaneiroBrazil Laboratorio TANDAR Comisión Nacional de Energía AtómicaBKNA1650 San MartíınArgentina Institute for Advanced Study in Nuclear Energy and Safety Shenzhen UniversityShenzhen 518060China Shenzhen Key Laboratory of Research and Manufacture of High Purity Germanium Materials and Fetectors Shenzhen UniversityShenzhen 518060China infn Sezione di PadovaPaduaItaly dipartimento di fisica Astronomia dell’Universita di padova PaduaItaly State Key Laboratory of Radiation Medicine and Protection School of Radiation Medicine and ProtectionSoochow UniversitySuzhou 215123China China Institute of Atomic Energy Beijing 102413China The Key Laboratory of Beam Technology and Material Modification of Ministry of Education College of Nuclear Science and TechnologyBeijing Normal UniversityBeijing 100875China Laboratori Nazionali di Legnaro INFN35020 LegnaroItaly infn Sezione di Napoli80126 NaplesItaly dipartimento di Farmacia Universitàdi Napoli“Federico II”80131 NaplesItaly Department of Natural and Mathematical Sciences Faculty of EngineeringTarsus University33480 MersinTurkey Physics division Argonne National LaboratoryLemontILUSA Department of Physics Sivas Cumhuriyet UniversitySivasTurkey Instituto de Física Universidade Federal do Rio de JaneiroRio de Janeiro CP 6852821941-972Brazil

One-neutron stripping process between^(6)Li and^(209)Bi was studied at 28,30,and 34 MeV using the in-beam-ray spectroscopy method.The-coincident analysis clearly identified two-rays feeding the ground and long-lived isomeric states,which were employed to determine the cross section.The one-neutron stripping cross sections were similar to the cross sections of complete fusion in the^(6)Li+^(209)Bi system,but the one-neutron stripping cross sections decreased more gradually at the sub-barrier region.A coupled-reaction-channel calculation was performed to study the detailed reaction mechanism of the one-neutron stripping process in^(6)Li.The calculations indicated that the first excited state of 5 Li is critical in the actual one-neutron transfer mechanism,and the valence proton of 209Bi can be excited to the low-lying excited state in(^(6)Li,^(5)Li)reaction,unlike in the(d,p)reaction.

关键词： Transfer reaction Weakly bound nuclei Cross section

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A novel way to study the nuclear collective excitations

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Nuclear Science and Techniques 2023年第12期34卷 109-111页

作者： Gianluca Colò dipartimento di fisica“Aldo Pontremoli” Universitàdegli Studi di MilanoVia Celoria 1620133 MilanoItaly infn Sezione di MilanoVia Celoria 1620133 MilanoItaly

Typically, the unambiguous determination of the quantum numbers of nuclear states is a challenging task. Recently, it has been proposed to utilize to this aim vortex photons in the MeV energy region and, potentially, this could revolutionize nuclear spectroscopy because of the new and enhanced selectivity of this probe. Moreover, nuclei may become diagnostic tools for vortex photons. Still, some open questions have to be dealt with.Nuclei exhibit intricate excitation spectra. Indeed, not all states within these spectra are equally significant. Some are not sensitive to specific terms in the nuclear Hamiltonian or do not display novel features, so that investigating them is not helpful to enhance our overall understanding of nuclear structure. On the other hand, there are states that manifest themselves as prominent peaks, e.g., in the inelastic scattering spectra. Among the best examples are the so-called Giant Resonances that lie at energies of the order of tens of MeV [1].

关键词： spectra structure excitation

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Thermal management for the underwater frontend and readout electronics of JUNO 20‑inch PMTs

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Radiation Detection Technology and Methods 2023年第3期7卷 418-426页

作者： Yangfu Wang Xiaoshan Jiang Jun Hu Peiliang Wang Lei Fan Shaojing Hou Zhe Ning Yunhua Sun Xiongbo Yan Zheng Wang Ziyue Yan Peiran Ye Jie Zhang Alberto Garfagnini Antonio Bergnoli Riccardo Brugnera Beatrice Jelmini Filippo Marini Marco Grassi Mariia Redchuk Andrea Serafini Katharina von Sturm Institute of High Energy Physics BeijingChina University of China Academy of Sciences Beijing 100049China infn sezione di Padova PaduaItaly dipartimento di fisica e Astronomia Universita di PadovaPaduaItaly

Background The Jiangmen underground neutrino observatory(JUNO)is a new generation of long-term operation neutrino experimental platform under construction in Jiangmen,Guangdong province of southern China.The underwater frontend and readout electronics(F&R electronics)are placed nearby the 20-inch PMTs and readout current signals from three PMTs.The electronics are sealed in a stainless-steel underwater box to keep them dry,and temperature control of the electronics plays a significant role in their reliability.Methods A conductive cooling structure based on the passive cooling method is designed for the 20-inch PMT F&R electronics.Both numerical simulation and experimental tests were performed to evaluate the cooling structures'thermal performance.Results The results show that the case temperature of the respective chip for 20-inch PMT F&R electronics is less than 30℃in ambient still water.Conclusion The case temperature of the respective chip meets the strict temperature requirement for the F&R electronics.The JUNO collaboration has adopted this cooling structure for the 20-inch PMT readout electronics.

关键词： Thermal management JUNO PMT Electronics

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Nuclear liquid-gas phase transition within a Brueckner-Hartree-Fock approach

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Chinese Physics C 2022年第11期46卷 231-237页

作者：张晶刘宏铭李增花 G.F.Burgio H.-J.Schulze Institute of Modern Physics Key Laboratory of Nuclear Physics and Ion-beam Application(MOE)Fudan UniversityShanghai 200433China infn sezione di Catania Dipartimento di Fisica e AstronomiaUniversitàdi CataniaVia S.Sofia 64I-95123 CataniaItaly

The critical parameters of the liquid-gas phase transition of symmetric nuclear matter are computed using the Brueckner-Hartree-Fock method at finite temperature by employing different realistic nucleon-nucleon potentials.Temperature effects on single-particle potentials,defect functions,and three-body forces are discussed in detail.Results obtained from the full procedure and frozen-correlations approximation are compared.We find critical temperatures of approximately 14 to 19 MeV and critical densities in the range of 0.05 to 0.08fm^(-3),depending on the interactions employed.

关键词： nuclear liquid-gas phase transition Brueckner-Hartree-Fock approach symmetric nuclear matter

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Two-flavor hybrid stars with the Dyson-Schwinger quark model

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Chinese Physics C 2017年第11期41卷 110-116页

作者：魏金标陈欢 H.-J.Schulze School of Mathematics and Physics China University of Geosciences infn sezione di Catania Dipartimento di FisicaUniversitá di Catania

We study the properties of two-flavor quark matter in the Dyson-Schwinger model and investigate the possible consequences for hybrid neutron stars,with particular regard to the two-solar-mass limit.We find that with some extreme values of the model parameters,the mass fraction of two-flavor quark matter in heavy neutron stars can be as high as 30 percent and the possible energy release during the conversion from nucleonic neutron stars to hybrid stars can reach 1052 erg.

关键词： hybrid stars quark matter equation of state Dyson-Schwinger equations

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The HEPD particle detector of the CSES satellite mission for investigating seismo-associated perturbations of the Van Allen belts

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Science China(Technological Sciences) 2018年第5期61卷 643-652页

作者： AMBROSI Giovanni BARTOCCI Simona BASARA Laurent BATTISTON Roberto BURGER William J. CARFORA Luca CASTELLINI Guido CIPOLLONE Piero CONTI Livio CONTIN Andrea DE DONATO Cinzia DE SANTIS Cristian FOLLEGA Francesco M. GUANDALINI Cristina IONICA Maria IUPPA Roberto LAURENTI Giuliano LAZZIZZERA Ignazio LOLLI Mauro MANEA Christian MARCELLI Laura MASCIANTONIO Giuseppe MERGE Matteo OSTERIA Giuseppe PACINI Lorenzo PALMA Francesco PALMONARI Federico PANICO Beatrice PATRIZII Laura PERFETTO Francesco PICOZZA Piergiorgio POZZATO Michele PUEL Matteo RASHEVSKAYA Irina RICCI Ester RICCI Marco RICCIARINI Sergio Bruno SCOTTI Valentina SOTGIU Alessando SPARVOLI Roberta SPATARO Bruno VITALE Vincenzo Istituto Nazionale di fisica Nucleare (infn) Sezione di Perugia Perugia 06123 Italy Uninettuno University Rome 00186 Italy Istituto Nazionale di fisica Nucleare (infn) Sezione di Roma Tor Vergata Rome 00133 Italy Istituto Nazionale di fisica Nucleare (infn) TIFPA Povo (TN) 38123 Italy dipartimento di fisica Universita di Trento Povo (TN) 38123 Italy dipartimento di fisica Universita di Roma Tor Vergata Rome 00133 Italy IFAC-CNR Sesto Fiorentino (FI) 50019 Italy dipartimento di fisica e Astronomia Universita di Bologna Bologna 40127 Italy Istituto Nazionale di fisica Nucleare (infn) Sezione di Bologna Bologna 40127 Italy Istituto Nazionale di fisica Nucleare (infn) Sezione di Napoli Naples 80126 Italy Istituto Nazionale di fisica Nucleare (infn) LNE Frascati (RM) 00044 Italy Agenzia Spaziale Italiana (ASI) SSDC Rome 00133 Italy

CSES(China Seismo-Electromagnetic Satellite) is a mission developed by CNSA(Chinese National Space Administration) and ASI(Italian Space Agency), to investigate the near-Earth electromagnetic, plasma and particle environment, for studying the seismo-associated disturbances in the ionosphere-magnetosphere transition zone. The anthropogenic and electromagnetic noise,as well as the natural non-seismic electromagnetic emissions is mainly due to tropospheric activity. In particular, the mission aims to confirming the existence of possible temporal correlations between the occurrence of earthquakes for medium and strong magnitude and the observation in space of electromagnetic perturbations, plasma variations and precipitation of bursts with highenergy charged particles from the inner Van Allen belt. In this framework, the high energy particle detector(HEPD) of the CSES mission has been developed by the Italian LIMADOU Collaboration. HEPD is an advanced detector based on a tower of scintillators and a silicon tracker that provides good energy and angular resolution and a wide angular acceptance, for electrons of 3–100 Me V, protons of 30–200 Me V and light nuclei up to the oxygen. CSES satellite has been launched on February 2^(nd), 2018 from the Jiuquan Satellite Launch Center(China).

关键词：卫星发射中心粒子带子空间管理合作开发空间机构轻原子核意大利

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中子的内部结构:来自BESIII的研究

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Science Bulletin 2022年第6期67卷 557-560页

作者： Simone Pacetti Rinaldo Baldini Ferroli Andrea Bianconi Egle Tomasi-Gustafsson dipartimento di fisica e Geologia and INFN Sezione di Perugia1-06123 PerugiaItaly Laboratori Nazionali di Frascati dell'infn 1-00044 FrascatiItaly dipartimento di Ingegneria dell'Informazione Brescia1-25133 BresciaItaly INFN Sezione di Pavia1-27100 PaviaItaly DPhN IRFUCEAUniversitéParis-Saclay1-91191 Gif-sur-Yvette CedexFrance

The BESⅢCollaboration has recently published a new precise measurement of the time-like neutron form factor(FF)[1].In the light of the remarkable accuracy and of the wideness of the explored kinematical range,these data represent an unprecedented tool for highlighting and studying specific features of the neutron FF.Until a few years ago,the only available data were those obtained by the FENICE experiment at Frascati,in the’90s[2].

关键词： BESⅢ precise

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Competition between fusion-evaporation and multifragmentation in central collisions in ^(58)Ni+^(48)Ca at 25A MeV

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Nuclear Science and Techniques 2013年第5期24卷 82-88页

作者： FRANCALANZA L ABBONDANNO U AMORINI F BARLINI S BINI M BOUGAULT R BRUNO M CARDELLA G CASINI G AGOSTINO M D' De FILIPPO V De SANCTIS J GERACI E GIUSSANI A GRAMEGNA F GUIOT B KRAVCHUK V La GUIDARA E LANZALONE G Le NEINDRE N MAIOLINO C MARINI P MORELLI L OLMI A PAGANO A PAPA M PIANTELLI S PIRRONE S POLITI G POGGI G PORTO F RUSSOTTO P RIZZO F VANNINI G VANNUCCI L infn Laboratori Nazionali del Sud-LNS Catania 95123Italy dipartimento di fisica Universitàdi Catania I-95129Italy infn sezione di Trieste Trieste I-34127Italy dipartimento di fisica Universitàdi FirenzeINFN Sezione di Firenze 1-50139Italy LPC Caen IN2P3-CNRS/ENSICAEN and UniversitéF-14050 Caen cedex 5-140France dipartimento di fisica Universitàdi Bologna and INFN Sezione di Bologna 4-50121Italy infn sezione di Catania I-95129 Italy infn sezione di Firenze I-50139 Italy dipartimento di fisica Universitàdi Milano and INFN Sezione di Milano1-20126Italy infn Laboratori Nazionali di Legnaro 1-35020 Italy Centro Siciliano di fisica Nucleare e Struttura della Materia Catania 1-95129Italy UniversitàKore Enna 1-94100Italy

The experimental data concerning the58Ni+48Ca reaction at Elab(Ni)=25A MeV,collected by using the CHIMERA 4π device,have been analyzed in order to investigate the competition among different reaction mechanisms for central collisions in the Fermi energy domain.As a main criterion for centrality selection we have chosen the flow angle(flow) method,making an event-by-event analysis that considers the shape of events,as it is determined by the eigenvectors of the experimental kinetic-energy tensor.For the selected central events(flow >60°) some global variables,good to characterize the pattern of central collisions have been constructed.The main features of the reaction products were explored by using different constraints on some of the relevant observables,like mass and velocity distributions and their correlations.Much emphasis was devoted,for central collisions,to the competition between fusion-evaporation processes with subsequent identification of a heavy residue and a possible multifragmentation mechanism of a well defined(if any) transient nuclear system.Dynamical evolution of the system and pre-equilibrium emission were taken into account by simulating the reactions in the framework of transport theories.different approaches have been envisaged(dynamical stochastic BNV calculations + sequential SIMON code,QMD,CoMD,etc.).Preliminary comparison of the experimental data with BNV calculations shows reasonable agreement with the assumption of sequential multifragmentation emission in the mass region of IMFs close to the heavy residues.Possible deviations from sequential processes were found for those IMFs in the region of masses intermediate between the mass of heavy residues and the mass of light IMFs.Further simulations are in progress.The experimental analysis will be enriched also by information obtained inspecting the IMF-IMF correlation function,in order to elucidated the nature of space-time decay property of the emitting source associated with events having the largest IMF multiplicity.

关键词：多重碎裂中心碰撞蒸发过程 MeV 竞争熔合国际货币基金组织事件分析

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Orbital angular momentum based intra- and interparticle entangled states generated via a quantum dot source

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先进光子学(英文) 2023年第4期5卷 74-84页

作者： Alessia Suprano Danilo Zia Mathias Pont Taira Giordani Giovanni Rodari Mauro Valeri Bruno Piccirillo Gonzalo Carvacho Nicolo Spagnolo Pascale Senellart Lorenzo Marrucci Fabio Sciarrino Sapienza Universitàdi Roma Dipartimento di FisicaRomaItaly Universite Paris-Saclay UMR 9001Centre for Nanosciences and NanotechnologyCNRSPalaiseauFrance Universitàdi Napoli Federico II Complesso Universitario di Monte Sant’AngeloDipartimento di Fisica“Ettore Pancini”NapoliItaly infn-sezione di Napoli NapoliItaly

Engineering single-photon states endowed with orbital angular momentum (OAM) is a powerful toolfor quantum information photonic implementations. Indeed, due to its unbounded nature, OAM is suitable forencoding qudits, allowing a single carrier to transport a large amount of information. Most of the experimentalplatforms employ spontaneous parametric down-conversion processes to generate single photons, evenif this approach is intrinsically probabilistic, leading to scalability issues for an increasing number of qudits.Semiconductor quantum dots (QDs) have been used to get over these limitations by producing on-demand pure and indistinguishable single-photon states, although only recently they have been exploitedto create OAM modes. Our work employs a bright QD single-photon source to generate a complete set ofquantum states for information processing with OAM-endowed photons. We first study hybrid intraparticleentanglement between OAM and polarization degrees of freedom of a single photon whose preparationwas certified by means of Hong–Ou–Mandel visibility. Then, we investigate hybrid interparticle OAM-based entanglement by exploiting a probabilistic entangling gate. The performance of our approach isassessed by performing quantum state tomography and violating Bell inequalities. Our results pave theway for the use of deterministic sources for the on-demand generation of photonic high-dimensionalquantum states.

关键词： orbital angular momentum quantum dot intraparticle entanglement interparticle entanglement Bell violation

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