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Microwave-Assisted Confining Growth and Liquid Exfoliation of sp^(3)-Hybrid Carbon Nitride Nano/Micro-Crystals

Energy & Environmental materials 2024年第6期7卷 399-408页

作者： Chenglong Shen Qing Lou Kaikai Liu Guangsong Zheng Runwei Song Jinhao Zang Xigui Yang Xing Li Lin Dong Chongxin Shan Henan Key Laboratory of Diamond Optoelectronic materials and devices Key Laboratory of Material PhysicsMinistry of EducationSchool of Physics and Laboratory of Zhongyuan LightZhengzhou UniversityZhengzhou 450052China

As one promising carbon-based material,sp^(3)-hybrid carbon nitride has been predicted with various novel physicochemical ***,the synthesis of sp^(3)-hybrid carbon nitride is still limited by the nanaoscale,low crystallinity,complex source,and expensive ***,we have presented a facile approach to the sp^(3)-hybrid carbon nitride nano/micro-crystals with microwave-assisted confining growth and liquid ***,the carbon nitride nano/micro-crystals can spontaneously emerge and grow in the microwave-assisted polymerization of citric acid and urea,and the liquid exfoliation can break the bulk disorder polymer to retrieve the highly crystalline carbon nitride nano/*** obtained carbon nitride nano/micro-crystals present superior blue light absorption strength and surprising photoluminescence quantum yields of 57.96%in ethanol and 18.05%in solid *** experimental characterizations and density functional theory calculations reveal that the interface-trapped localized exciton may contribute to the excellent intrinsic light emission capability of carbon nitride nano/micro-crystals and the interparticle staggered stacking will prevent the aggregation-caused-quenching ***,the carbon nitride nano/micro-crystals are demonstrated to be potentially useful as the phosphor medium in light-emitting-diode for interrupting blue light-induced eye *** work paves new light on the synthesis strategy of sp^(3)-hybrid carbon nitride materials and thus may push forward the development of multiple carbon nitride research.

关键词： confining growth density functional theory liquid exfoliation luminescence sp^(3)-hybrid carbon nitride

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New Strategy for Boosting Cathodic Performance of Protonic Ceramic Fuel Cells Through Incorporating a Superior Hydronation Second Phase

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Energy & Environmental materials 2024年第4期7卷 83-92页

作者： Chuan Zhou Xixi Wang Dongliang Liu Meijuan Fei Jie Dai Daqin Guan Zhiwei Hu Linjuan Zhang Yu Wang Wei Wang Ryan O'Hayre San Ping Jiang Wei Zhou Meilin Liu Zongping Shao State Key Laboratory of materials-Oriented Chemical Engineering College of Chemical Engineering Nanjing Tech University Max Planck Institute for Chemical physics of Solids Key Laboratory of Interfacial physics and Technology Shanghai Institute of Applied Physics Chinese Academy of Sciences Department of Metallurgical and materials Engineering Colorado School of Mines WA School of Mines: Minerals Energy and Chemical Engineering (WASM-MECE) Curtin University Suzhou Laboratory School of materials Science and Engineering Georgia Institute of Technology

For protonic ceramic fuel cells,it is key to develop material with high intrinsic activity for oxygen activation and bulk proton conductivity enabling water formation at entire electrode ***,a higher water content which benefitting for the increasing proton conductivity will not only dilute the oxygen in the gas,but also suppress the O2adsorption on the electrode surface.

关键词： cathode high-hydrating capability proton conductivity protonic ceramic fuel cells

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A nitric oxide-triggered hydrolysis reaction to construct controlled self-assemblies with complex topologies

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Science China Chemistry 2024年第4期67卷 1289-1299页

作者： Wenzhuo Chen Yuping Tang Shuai Chen Zipei Chen Jia He Hongbin Huo Juan Zhang Jiajia Li Fei Yan Wei Tian Laboratory of Shaanxi Administration of Traditional Chinese Medicine for TCM Compatibility Shaanxi Key Laboratory of Chinese Medicine Fundamentals and New Drugs ResearchCollege of PharmacyShaanxi University of Chinese MedicineXianyang 712046China Shaanxi Key Laboratory of Macromolecular Science and Technology Xi’an Key Laboratory of Hybrid Luminescent Materials and Photonic DeviceMOE Key Laboratory of Material Physics and Chemistry under Extraordinary ConditionsSchool of Chemistry and Chemical EngineeringNorthwestern Polytechnical UniversityXi’an 710072China Department of Polymeric materials School of Materials Science and EngineeringTongji UniversityShanghai 201804China

Hydrolysis reactions are capable of directing the non-equilibrium assembly of biomolecular scaffolds to realize sophisticated structures and functions in natural ***,utilizing the proper hydrolysis reactions to construct controlled assemblies with complex topologies is still an arduous challenge in artificial systems and needs to be ***,we report a nitric oxide(NO)-triggered slow hydrolysis strategy for the controlled construction of biomimetic supramolecular toroids(STs),thus realizing their visualization of intermediate structures and regulation of geometry *** presented protocol harnesses hydrolysis reactions to control of non-equilibrium self-assembly processes for the construction of self-assemblies with complex topologies successfully,which sheds light on how the hydrolysis reaction rate can modulate the kinetic pathway of assembly,thus realizing the artificial establishment of bio-inspired hierarchical structures.

关键词： supramolecular toroids controlled self-assembly nitic oxide-triggered hydrolysis pathway regulation

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Pressure-induced emission(PIE)in halide perovskites toward promising applications in scintillators and solid-state lighting

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Aggregate 2024年第1期5卷 9-15页

作者： Wenya Zhao Guanjun Xiao Bo Zou State Key Laboratory of Superhard materials College of PhysicsJilin UniversityChangchunChina

High-pressure chemistry has provided a huge boost to the development of scientific ***-induced emission(PIE)in halide perovskites is gradually showing its unique charm in both pressure sensing and optoelectronic device ***,the PIE retention of halide perovskites under ambient conditions is of great commercial ***,we mainly focus on the potential applications of PIE and PIE retention in metal halide perovskites for scintillators and solid-state *** on the performance requirements of scintillator and single-component white light-emitting diodes(WLEDs),the significance of PIE and PIE retention is critically clarified,aiming to design and synthesize materials used for high-performance optoelectronic *** perspective not only demonstrates promising applications of PIE in the fields of scintillators and WLEDs,but also provides potential applications in display imaging and anti-counterfeiting of PIE ***,solving the scientific disputes that exist under ambient conditions is also simply discussed as an outlook by introducing high-pressure dimension to produce PIE.

关键词： halide perovskites high pressure light-emitting diode pressure-induced emission scintillators solidstate lighting

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Modulating low-frequency tribocatalytic performance through defects in uni-doped and bi-doped SrTiO_(3)

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Journal of Advanced Ceramics 2024年第8期13卷 1153-1163页

作者： Yjing Xu Yingzhi Meng Xu Xiang Qing Tang Hongfang Zhang Lajun Liu Ju Gao Bo Xu Renhong Liang Longlong Shu Yanmin Jia Wanping Chen School of Physical Science and Technology Suzhou University of Science and TechnologySuzhou 215009China College of materials Science and Engineering Guilin University of TechnologyGuilin 541004China Key Laboratory of Advanced Electrode materials for Novel Solar Cells for Petroleum and Chemical Industry of China Suzhou University of Science and TechnologySuzhou 215009China School of Science and Key Laboratory of Biomedical Functional materials China Pharmaceutical UniversityNanjing 211198China School of physics and materials Science Guangzhou UniversityGuangzhou 510006China School of physics and materials Science Nanchang UniversityNanchang 330031China School of physics and Information Technology Shaanxi Normal UniversityXi'an 710062China School of physics and Technology Wuhan UniversityWuhan 430072China

Triboelectrification,a process that transforms mechanical energy into electrical energy through friction,holds promise for eco-friendly wastewater *** study delves into the enhancement of tribocatalytic dye degradation using SrTiO_(3),a material notable for its non-piezoelectric and centrosymmetric *** synthesis of uni-and bi-doped SrTiOs particles,achieved through a solid-state reaction at 100℃,results in a high-purity cubic perovskite *** with rhodium(Rh)and carbon(C)causes crystal lattice contraction,internal stress,and significant oxygen *** changes notably improve tribocatalytic efficiency under solar irradiation,with Rh-doped SrTiO_(3) demonstrating an impressive degradation rate of approximately 88% for Rhodamine B(RhB),along with reaction rate constants near 0.9 h^(-1) at 554 nm and a noticeable *** study highlights that defects introduced by doping are integral to this process,boosting catalytic activity through energy state modification and enhancing surface redox radical ***,these defects are instrumental in generating a flexoelectric field,which markedly influences the separation of electron-hole pairs under solar *** findings illuminate the complex interplay between material composition,defect states,and environmental conditions,paving the way for advanced strategies in environmental remediation through optimized tribocatalytic activity.

关键词： tribocatalysis SrTiO_(3)(STO) doping-induced defects blueshift flexoelectric field

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Vacancy healing for stable perovskite solar cells via bifunctional potassium tartrate

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Journal of Energy Chemistry 2024年第1期88卷 64-70,I0002页

作者： Jing Dou Yue Ma Xiuxiu Niu Wentao Zhou Xueyuan Wei Jie Dou Zhenhua Cui Qizhen Song Tinglu Song Huanping Zhou Cheng Zhu Yang Bai Qi Chen Experimental Centre for Advanced materials School of Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China Beijing Key Laboratory for Theory and Technology of Advanced Battery materials Key Laboratory of Polymer Chemistry and Physics of Ministry of EducationBIC-ESATSchool of Materials Science and EngineeringPeking UniversityBeijing 100871China

Perovskite solar cell has gained widespread attention as a promising technology for renewable ***, their commercial viability has been hampered by their long-term stability and potential Pb leakage. Herein, we demonstrate a bifunctional passivator of the potassium tartrate(PT) to address both challenges. PT minimizes the Pb leakage in perovskites and also heals cationic vacancy defects, resulting in improved device performance and stability. Benefiting from PT modification, the power conversion efficiency(PCE) is improved to 23.26% and the Pb leakage in unencapsulated films is significantly reduced to 9.79 ppm. Furthermore, the corresponding device exhibits no significant decay in PCE after tracking at the maximum power point(MPP) for 2000 h under illumination(LED source, 100 mW cm^(-2)).

关键词： Perovskite Potassium tartrate Lead leakage Long-term stability

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One-step hydrothermal synthesis of few-layered metallic phase MoS2 for high-performance supercapacitors

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Progress in Natural Science:materials International 2024年第2期34卷 429-436页

作者： Jing Xu Xulong Yuan Yujie Zhao Shaoqi Rui Qingling Jia Han Li Shun Lu Bing Li Yongxing Zhang Xuebin Zhu Anhui Province Key Laboratory of Pollutant Sensitive materials and Environmental Remediation Anhui Province Key Laboratory of Intelligent Computing and Applications Anhui Province Industrial Generic Technology Research Center for Alumics Materials Huaibei Normal University Chongqing Institute of Green and Intelligent Technology Chinese Academy of Sciences Key Laboratory of materials physics Institute of Solid State Physics HFIPS Chinese Academy of Sciences

In recent years,molybdenum disulfide（MoS2） has gained significant attention in the scientific *** MoS2demonstrates unique properties and potential ***,the synthesis of few-layered and high-purity 1T-MoS2is still a *** this study,we successfully employed a hydrothermal method to synthesize few-layered and high-purity *** purity of the material is controlled by a combination of sodium borohydride and ***,the few-layered 1T-MoS2exhibits exceptional performance as a supercapacitor,including the high specific capacitance(250.3 F g-1at a current density of 1 A g-1) and excellent long-trem cycling stability（90.7 % after 5000 cycles）.Meanwhile,the asymmetric device assembled by 6-FL-1TMoS2and active carbon on carbon cloths exhibits excellent flexibility and high energy and power density(23.1μWh cm-2at 600 μW cm-2,55 μWh cm-2at 12000 μW cm-2).This work provides valuable insights into the synthesis of few-layered and high-purity 1T-MoS2,opening up new avenues for further research and applications.

关键词： 1T-MoS2 Few-layered High-purity One-pot hydrothermal method Supercapacitor

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Emerging materials and transistors for integrated circuits

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National Science Review 2024年第3期11卷 7-8页

作者： Ming Liu Lian-Mao Peng Lab of Nanofabrication and Novel device Integration Institute of Microelectronics Chinese Academy of Sciences Key Laboratory for the physics and Chemistry of Nanodevices and Center for Carbon-based Electronics School of Electronics Peking University

The device technology for integrated circuits(ICs) has received a great deal of attention in the past decade since the mainstream silicon-based complementary metal-oxide-semiconductor(CMOS) field-effect transistor(FET) for modern ICs had been encountering development bottlenecks due to the combination of power constraints, physics, cost and fabrication processes.

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Synthesis,structure,and thermal expansion in CaZrF_(6) with two polymorphs

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Nano Research 2024年第9期17卷 8618-8626页

作者： Peixian Zhang Yongqiang Qiao Kaiyue Zhao Qingjie Wang Huan Zhao Juan Guo Erjun Liang Tao Sun Jiangwei Zhang Qilong Gao Key Laboratory of materials physics of Ministry of Education School of Physics and MicroelectronicsZhengzhou UniversityZhengzhou 450052China College of Energy materials and Chemistry Inner Mongolia UniversityHohhot 010021China First Affiliated Hospital of Dalian Medical University 222 Zhongshan RoadDalian 116011China Ordos Laboratory Ordos 017000China

Due to the high structural flexibility and controllable thermal expansion,cubic double ReO_(3)-type negative thermal expansion(NTE)fluorides provide a solution for solving the prominent phenomenon of thermal expansion mismatch between ***,the expensive raw materials and complex synthesis steps limit its practical *** this work,we have designed a more advantageous method for the synthesis of NTE material CaZrF_(6),and it is expected to be generalized to the synthesis of other double ReO_(3)-***,a new orthorhombic phase CaZrF_(6) has been synthesized via this method in a lower *** the strong isotropic NTE of the cubic phase CaZrF_(6),the orthorhombic phase shows the strong anisotropic positive thermal expansion(PTE).The combined analysis of temperature-dependent X-ray diffraction(XRD),Raman spectra,and first-principles calculations shows that the low frequency phonon vibration mode with negative Grüneisen parameter in cubic CaZrF_(6) are strongly correlated with the transverse thermal vibration of F atoms and dominates the NTE of the material.

关键词： negative thermal expansion fluorides polymorph lattice dynamics first principles calculations

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High-power all-polarization-maintaining fiber femtosecond pulse laser at 780 nm and its engineering integration

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中国激光 2024年

作者：罗韬温俊鹏王文龙李梓晗朱喆杨家豪吴垠修昊范怡衡刘亚龙韦小明杨中民 Guangzhou Yangming Laser Technology Co. Ltd 3. Research Institute of Future Technology South China Normal University School of physics and Optoelectronics State Key Laboratory of Luminescent Materials and Devices Guangdong Engineering Technology Research and Development Center of Special Optical Fiber Materials and Device Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques South China University of Technology

We present a high-power, high-stability all-polarization-maintaining (all-PM)fiber femtosecond pulse laser source at 780 nm with full engineering integration that comprises an all-PM fiber amplified chirped pulse laser at 1560 nm, a grating pair compressorandasecond-harmonicgeneration(SHG)***-PMfiber amplified chirped pulse laser at 1560 nm operates with a repetition rate of 111.5 MHz and an average power of 5.37 W, which is compressed with a pulse width of～204 *** 780-nm pulses are subsequently generated by SHG in a frequency-doubling *** achieve an average power of 2.22 W at 780 nm with a pulse width of 288 fs, an SHG efficiency of 52%, and a root-mean-square power fluctuation of 0.23%, which is *** integrated for practical application with reliable laser operation. We anticipate that this780-nmall-PMfiberfemtosecondpulselaserwithfullengineeringintegrationis promising for frontier applications, like two-photon imaging, nanofabrication, terahertz generation, etc.

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