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Inhibiting shuttle effect of lithium polysulfides by double metal selenides for high-performance lithium-sulfur batteries

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Rare Metals 2024年第6期43卷 2546-2559页

作者： Lei Li Xue-Jing Yang Yi-Yang Li Bo Jin Hui Liu Meng-Yang Cui Dong-Bo Guan Xing-You Lang Qing Jiang Key Laboratory of automobile Materials Ministry of Educationand College of Materials Science and EngineeringJilin UniversityChangchun 130022China

Lithium-sulfur batteries(LSBs)have attracted the attention of more and more researchers due to the advantages of high energy density,environmental friendliness,and low production ***,the low electronic conductivity of active material and shuttling effect of lithium polysulfides(LiPSs)limit the commercial development of *** solve these problems,we design a core-shell composite with nitrogen-doped carbon(NC)and two types of selenides(FeSe_(2)-NC@ZnSe-NC).The FeSe_(2)-NC@ZnSe-NC has a strong adsorption capacity,and can effectively adsorb *** the same time,it also effectively alleviates the shuttling effect of LiPSs,and improves the utilization of the active substance during the charge/discharge reaction *** mechanism involved in FeSe_(2)-NC@ZnSe-NC is demonstrated by both experiments and density-functional theory(DFT)*** electrochemical test results indicate that LSB with S/FeSe_(2)-NC@ZnSe-NC delivers an initial discharge capacity of 1260 mAh·g^(-1)at *** after 500 cycles at 1C,the capacity decay rate per cycle is 0.031%,and the capacity retention rate is 85%.The FeSe_(2)-NC@ZnSe-NC core-shell structure verifies a rational strategy to construct an electrode material for high-performance LSBs.

关键词： Lithium-sulfur batteries Shuttling effect Metal selenide Nitrogen-doped carbon Lithium polysulfides

High-efficiency sodium storage of Co_(0.85)Se/WSe_(2) encapsulated in N-doped carbon polyhedron via vacancy and heterojunction engineering

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Carbon Energy 2024年第1期6卷 94-107页

作者： Ya Ru Pei Hong Yu Zhou Ming Zhao Jian Chen Li Xin Ge Wei Zhang Chun Cheng Yang Qing Jiang Key Laboratory of automobile Materials(Jilin University) Ministry of EducationSchool of Materials Science and EngineeringJilin UniversityChangchunChina Jilin Provincial International Cooperation Key Laboratory of High-Efficiency Clean Energy Materials Electron Microscopy CenterJilin UniversityChangchunChina

With the advantage of fast charge transfer,heterojunction engineering is identified as a viable method to reinforce the anodes'sodium storage ***,vacancies can effectively strengthen the Na+adsorption ability and provide extra active sites for Na+***,their synchronous engineering is rarely ***,a hybrid of Co_(0.85)Se/WSe_(2) heterostructure with Se vacancies and N-doped carbon polyhedron(CoWSe/NCP)has been fabricated for the first time via a hydrothermal and subsequent selenization *** aberration-corrected transmission electron microscopy confirms the phase interface of the Co_(0.85)Se/WSe_(2) heterostructure and the existence of Se *** functional theory simulations reveal the accelerated charge transfer and enhanced Na+adsorption ability,which are contributed by the Co_(0.85)Se/WSe_(2) heterostructure and Se vacancies,*** expected,the CoWSe/NCP anode in sodium-ion battery achieves outstanding rate capability(339.6 mAh g^(−1) at 20 A g^(−1)),outperforming almost all Co/W-based selenides.

关键词： Co_(0.85)Se/WSe_(2)heterostructure density functional theory simulations N-doped carbon polyhedron Se vacancies sodium-ion batteries

Computation of the exact time delay margin for vehicle platoon under generic communication topologies

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Journal of Traffic and Transportation engineering(English Edition) 2024年第4期11卷 761-775页

作者： Xu Zhu Maode Yan Panpan Yang Yongtao Liu School of Electronic and Control engineering Chang'an UniversityXi'an 710064China School of automobile Chang'an UniversityXi'an 710064China

Due to the limited bandwidth and transmission congestion of the vehicle platoon's communication,it is inevitable to induce time delay,which significantly degrades the control performance of the vehicle platoon,even resulting in *** paper focuses on analyzing the internal stability under generic communication topologies and presents a method of computing the exact time delay margin(ETDM).The proposed method can offer a necessary and sufficient internal stability condition with no ***,to reduce the analytical complexity and computational burden elegantly,we decompose the closed-loop platoon dynamics into a set of individual subsystems via similarity transformation and matrix *** decomposition approach is applicable for any general communication ***,an explicit formula is deduced to compute the ETDM by surveying the characteristic roots'distribution of all these individual *** is further demonstrated that only the positive purely imaginary roots need to be considered to compute the ***,simulations are conducted to demonstrate the effectiveness of the theoretical claims.

关键词： Vehicle platoon Exact time delay margin Generic communication topologies System decomposition Characteristic roots'distribution

Beyond fossil:the synthetic fuel surge for a green-energy resurgence

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Clean Energy 2024年第5期8卷 1-18页

作者： Sreejaun Thothaathiri Janaki Dinesh Kumar Madheswaran G.Naresh Thangavelu Praveenkumar Electric Vehicle Technology Laboratory Department of Automobile EngineeringSRM Institute of Science and TechnologyKattankulathur CampusTamilnadu 603203India

This review offers a comprehensive overview of synthetic fuels as promising alternatives to conventional fossil *** carbon-neutral potential of synthetic fuels when produced using renewable energy and captured CO_(2),offering significant opportunities to mitigate CO_(2) emissions,is ***,the efficiency of synthetic fuels is presented,as they do not require dedicated agricultural land or substantial water resources,addressing concerns related to the land-use change and water scarcity associated with traditional *** economic viability of synthetic fuels is explored,highlighting the advancements in technology and decreased renewable-energy costs,coupled with their independence from food crops,mitigating concerns about potential impacts on food *** investments by industry leaders such as Porsche,Highly Innovative Fuels Global,and ExxonMobil,totalling$1 billion,aimed at achieving an annual production of 550 million litres by 2026,are covered in *** study is further extended by emphasizing the scalability of synthetic fuel production through modular processes,enabling tailored facilities to meet regional demands and contribute to a decentralized and resilient energy ***,the‘drop-in’nature of synthetic fuels that are seamlessly compatible with existing fuel storage,pipelines,and pumps,facilitating a smooth transition without requiring extensive infrastructure changes,is *** such as the current high cost of synthetic fuel production are acknow-ledged,necessitating supportive government policies and incentives for widespread ***,synthetic fuels have emerged as promising contenders in the pursuit of sustainable and adaptable energy solutions,with tangible benefits for the environment,economy,and existing energy infrastructure.

关键词： synthetic fuels biofuels carbon neutrality sustainable energy e-fuel ‘drop-in’nature

Identification of the Hammerstein nonlinear system with noisy output measurements

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Control Theory and Technology 2024年第2期22卷 203-212页

作者： Qiming Zha Feng Li Ranran Liu School of Electrical and Information engineering Jiangsu University of TechnologyChangzhou213001JiangsuChina School of automobile and Traffic engineering Jiangsu University of TechnologyChangzhou213001JiangsuChina

In this research, we present a methodology to identify the Hammerstein nonlinear system with noisy output measurements. The Hammerstein system presented is comprised of neural fuzzy model (NFM) as its static nonlinear block and auto-regressive with extra input (ARX) model as its dynamic linear block, and a two-step procedure is accomplished using signal combination. In the first step, in the case of input–output of Gaussian signals, the correlation function-based least squares (CF-LS) technique is utilized to identify the linear block, solving the problem that the intermediate variable connecting nonlinear and linear blocks cannot be measured. In the second step, to improve the identification accuracy of the nonlinear block parameters, an improved particle swarm optimization technique is developed under input–output of random signals. The validity and accuracy of the presented scheme are verified by a numerical simulation and a practical nonlinear process, and the results illustrate that the proposed methodology can identify well the Hammerstein nonlinear system with noisy output measurements.

关键词： Hammerstein nonlinear system Signal combination Auto-regressive with extra input Improved particle swarm optimization

Reliability evaluation of IGBT power module on electric vehicle using big data

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Journal of Semiconductors 2024年第5期45卷 50-60页

作者： Li Liu Lei Tang Huaping Jiang Fanyi Wei Zonghua Li Changhong Du Qianlei Peng Guocheng Lu The School of Electrical engineering Chongqing UniversityChongqing 400044China The Deepal automobile Technology Co. Ltd.Chongqing 400023China

There are challenges to the reliability evaluation for insulated gate bipolar transistors(IGBT)on electric vehicles,such as junction temperature measurement,computational and storage *** this paper,a junction temperature estimation approach based on neural network without additional cost is proposed and the lifetime calculation for IGBT using electric vehicle big data is *** direct current(DC)voltage,operation current,switching frequency,negative thermal coefficient thermistor(NTC)temperature and IGBT lifetime are *** the junction temperature(T_(j))is *** the rain flow counting method,the classified irregular temperatures are brought into the life model for the failure *** fatigue accumulation method is then used to calculate the IGBT *** solve the limited computational and storage resources of electric vehicle controllers,the operation of IGBT lifetime calculation is running on a big data *** lifetime is then transmitted wirelessly to electric vehicles as input for neural *** the junction temperature of IGBT under long-term operating conditions can be accurately estimated.A test platform of the motor controller combined with the vehicle big data server is built for the IGBT accelerated aging ***,the IGBT lifetime predictions are derived from the junction temperature estimation by the neural network method and the thermal network *** experiment shows that the lifetime prediction based on a neural network with big data demonstrates a higher accuracy than that of the thermal network,which improves the reliability evaluation of system.

关键词： IGBT junction temperature neural network electric vehicles big data

High-stability double-layer polymer-inorganic composite electrolyte fabricated through ultraviolet curing process for solid-state lithium metal batteries

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Frontiers of Materials Science 2024年第2期18卷 117-128页

作者： Xinghua Liang Pengcheng Shen Lingxiao Lan Yunmei Qin Ge Yan Meihong Huang Xuanan Lu Qiankun Hun Yujiang Wang Jixuan Wang Guangxi Key Laboratory of automobile Components and Vehicle Technology Guangxi University of Science&TechnologyLiuzhou 545006China Guangxi automobile Group Co. Ltd.Liuzhou 545006China School of Automotive engineering Guangdong Polytechnic of Industry and CommerceGuangzhou 510510China

Electrolyte interface resistance and low ionic conductivity are essential issues for commercializing solid-state lithium metal batteries(SSLMBs).This work details the fabrication of a double-layer solid composite electrolyte(DLSCE)for *** composite comprises poly(vinylidene fluoride-co-hexafluoropropylene)(PVDF-HFP)and poly(methyl methacrylate)(PMMA)combined with 10 wt.%of Li_(6.4)La_(3)Zr_(1.4)Ta_(0.6)O_(12)(LLZTO),synthesized through an ultraviolet curing *** ionic conductivity of the DLSCE(2.6×10^(-4) S·cm^(-1))at room temperature is the high lithium-ion transference number(0.57),and the tensile strength is 17.8 *** this DLSCE was assembled,the resulted LFP/DLSCE/Li battery exhibited excellent rate performance,with the discharge specific capacities of 162.4,146.9,93.6,and 64.0 mA·h·g^(-1) at 0.1,0.2,0.5,and 1 C,***,the DLScE demonstrates remarkable stability with lithium metal batteries,facilitating the stable operation of a Li/Li symmetric battery for over 200 h at both 0.1 and 0.2 mA-cm^(-2).Notably,the formation of lithium dendrites is also effectively inhibited during *** work provides a novel design strategy and preparation method for solid composite electrolytes.

关键词： electrochemicalreliability lithium metal battery lithium-ion transference number double-layer solid composite electrolyte

Thin-walled and large-sized magnesium alloy die castings for passenger car cockpit:Application,materials,and manufacture

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China Foundry 2024年第5期21卷 525-545页

作者： Lei Zhan Yu-meng Sun Yang Song Chun-hua Kong Kai Ma Bai-xin Dong Hong-yu Yang Shi-li Shu Feng Qiu School of Automotive engineering Jilin Communication PolytechnicChangchun 130012China Key Laboratory of automobile Materials of Ministry of Education School of Materials Science and EngineeringNanling CampusJilin UniversityChangchun 130025China

In order to effectively reduce energy consumption and increase range mile,new energy vehicles represented by Tesla have greatly aroused the application of integrated magnesium(Mg)alloy die casting technology in ***,the application of Mg alloys in automobiles,especially in automotive cockpit components,is quite extensive,while it has almost disappeared for a period of time due to its relatively high cost,causing a certain degree of information loss in the application technology of Mg alloy parts in *** rapid development of automotive technology has led to a higher requirement for the automotive components compared with those traditional ***,whatever the components themselves,or the Mg alloy materials and die casting process have to face an increasing challenge,needing to be *** addition,owing to its high integration characteristics,the application of Mg alloy die casting technology in large-sized and thin-walled automotive parts has inherent advantages and needs to be expanded ***,it necessitates exploring advance Mg alloys and new product structures and optimizing die casting *** article summarizes and analyzes the development status of thin-walled and large-sized die casting Mg alloy parts in passenger car cockpit and corresponding material selection methods,die casting processes as well as mold design ***,this work will aid researchers in establishing a comprehensive understanding of the manufacture of thin-walled and large-sized die casting Mg alloy parts in automobile *** will also assist them in developing new Mg alloys with improved comprehensive performance and new processes to meet the high requirements for die casting automotive components.

关键词： Mg alloys thin wall large size automotive part die casting

Moiré superlattices arising from growth induced by screw dislocations in layered materials

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Chinese Physics B 2024年第7期33卷 72-77页

作者：田伏钰 Muhammad Faizan 贺欣孙远慧张立军 State Key Laboratory of Integrated Optoelectronics Key Laboratory of automobile Materials of MOE and College of Materials Science and engineering Jilin UniversityChangchun 130012China Suzhou Laboratory Suzhou 215123China

Moiré superlattices(MSLs) are modulated structures produced from homogeneous or heterogeneous two-dimensional layers stacked with a twist angle and/or lattice mismatch. Enriching the methods for fabricating MSL and realizing the unique emergent properties are key challenges in its investigation. Here we recommend that the spiral dislocation driven growth is another optional method for the preparation of high quality MSL samples. The spiral structure stabilizes the constant out-of-plane lattice distance, causing the variations in electronic and optical properties. Taking SnS_(2) MSL as an example, we find prominent properties including large band gap reduction(~ 0.4 e V) and enhanced optical activity. Firstprinciples calculations reveal that these unusual properties can be ascribed to the locally enhanced interlayer interaction associated with the Moiré potential modulation. We believe that the spiral dislocation driven growth would be a powerful method to expand the MSL family and broaden their scope of application.

关键词： Moirésuperlattices interlayer interaction spiral dislocation layered materials