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Catalytic oxidation of toluene by manganese oxides:Effect of K^(+)doping on oxygen vacancy

Journal of Environmental Sciences 2024年第8期142卷 43-56页

作者： Zhenzhen Huang Haiyang Li Xuejun Zhang Yanli Mao Yinghan Wu Wei Liu Hongrun Gao Mengru Zhang Zhongxian Song Faculty of Environmental and Municipal Engineering Henan Key Laboratory of Water Pollution Control and Rehabilitation TechnologyHenan University of Urban ConstructionPingdingshan 467036China College of Environmental and Safety Engineering Shenyang University of Chemical TechnologyShenyang 110142China

Alkali metal potassium was beneficial to the electronic regulation and structural stability of transition metal ***,K ions were introduced into manganese oxides by different methods to improve the degradation efficiency of *** results of activity experiments indicated that KMnO_(4)-HT(HT:Hydrothermal method)exhibited outstanding low-temperature catalytic activity,and 90%conversion of toluene can be achieved at 243℃,which was 41℃and 43℃lower than that of KNO_(3)-HT and Mn-HT,*** largest specific surface area was observed on KMnO_(4)-HT,facilitating the adsorption of *** formation of cryptomelane structure over KMnO_(4)-HT could contribute to higher content of Mn^(3+)and lattice oxygen(Olatt),excellent low-temperature reducibility,and high oxygen mobility,which could increase the catalytic ***,two distinct degradation pathways were ***Ⅰ(KMnO_(4)-HT):toluene→benzyl→benzoic acid→carbonate→CO_(2)and H2O;PathwayⅡ(Mn-HT):toluene→benzyl alcohol→benzoic acid→phenol→maleic anhydride→CO_(2)and *** intermediates were detected on KMnO_(4)-HT,indicating its stronger oxidation capacity of toluene,which was originated from the doping of K^(+)and the interaction between *** intermediates were observed on Mn-HT,which can be attributed to the weaker oxidation ability of pure *** results indicated that the doping of K^(+)can improve the catalytic oxidation capacity of toluene,resulting in promoted degradation of intermediates during the oxidation of toluene.

关键词： Catalytic oxidation Preparation method Cryptomelane Mn^(3+)and lattice oxygen

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On the calibration of a shear stress criterion for rock joints to represent the full stress-strain profile

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第2期16卷 379-392页

作者： Akram Deiminiat Jonathan D.Aubertin Yannic Ethier department of construction Engineering École de Technologie Supérieure(ÉTS)MontréalCanada

Conventional numerical solutions developed to describe the geomechanical behavior of rock interfaces subjected to differential load emphasize peak and residual shear *** detailed analysis of preand post-peak shear stress-displacement behavior is central to various time-dependent and dynamic rock mechanic problems such as rockbursts and structural instabilities in highly stressed *** complete stress-displacement surface(CSDS)model was developed to describe analytically the pre-and post-peak behavior of rock interfaces under differential *** formulations of the CSDS model required extensive curve-fitting iterations which limited its practical applicability and transparent integration into engineering *** present work proposes modifications to the CSDS model aimed at developing a comprehensive and modern calibration protocol to describe the complete shear stressdisplacement behavior of rock interfaces under differential *** proposed update to the CSDS model incorporates the concept of mobilized shear strength to enhance the post-peak ***’s concepts of joint roughness coefficient(JRC)and joint compressive strength(JCS)are incorporated to facilitate empirical estimations for peak shear stress and normal closure ***/uniaxial compression test and direct shear test results are used to validate the updated model and exemplify the proposed calibration *** results illustrate that the revised model successfully predicts the post-peak and complete axial stressestrain and shear stressedisplacement curves for rock joints.

关键词： Full shear profile Post-peak shear behavior Rock joint Joint roughness coefficient(JRC) Axial stress-strain curve

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Topographic seismic effects and avalanche hazard:A case study of Mount Siella(L’Aquila,Central Italy)

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Journal of Mountain Science 2024年第2期21卷 662-675页

作者： Ferdinando TOTANI department of Civil construction-Architecture and Environmental Engineering University of L’AquilaL'Aquila 67100Italy

In mountainous areas,snow avalanches could be triggered by the shaking produced by *** forces induced by the earthquake can cause an irregular increase of shear strength load down the slope,for the presence of complex surface and buried *** irregularities generate maximum effects of waves amplification linked to wavelengths comparable to the horizontal dimension of the topographic *** this reason,the selected time-histories represent an appropriate input for the two-dimensional numerical response analyses when a dynamic phenomenon produce the resonant motion of a whole *** represents an important earthquake-induced hazard in snow-covered mountain areas with high probability of seismic *** valleys are located in regions with scare ground motion data and investments on infrastructures are not always accompanied by adequate protection against earthquake-induced *** paper points out a simple deterministic approach for selecting a set of real accelerograms applied to a real case of Siella Mountain(Central Italy)where a large avalanche destroying a tourist facility of Rigopiano resort on 18 January *** selected time histories were used as input for the two-dimensional numerical model of the subsoil to evaluate the topographic seismic amplification in ridge and compare it with the results of other *** methods suggest that morphology-related inertial effects should be considered as an overload action on snow layers when controlling multi-hazard studies and spatial planning.

关键词： Real accelerograms selection Deterministic approach Topographic amplification Avalanche induced by earthquake 2D seismic response.

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Finite Element Simulations of the Localized Failure and Fracture Propagation in Cohesive Materials with Friction

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Computer Modeling in Engineering & Sciences 2024年第7期140卷 997-1015页

作者： Chengbao Hu Shilin Gong Bin Chen Zhongling Zong Xingwang Bao Xiaojian Ru department of Civil Engineering Hangzhou City UniversityHangzhou310015China Zhejiang Engineering Research Center of Intelligent urban Infrastructure Hangzhou310015China Key Laboratory of Safe construction and Intelligent Maintenance for urban Shield Tunnels of Zhejiang Province Hangzhou310015China School of Civil and Ocean Engineering Jiangsu Ocean UniversityLianyungang222005China Institute of Municipal Engineering Hangzhou Shangcheng District Municipal Engineering Group Co.Ltd.Hangzhou310016China

Strain localization frequently occurs in cohesive materials with friction(e.g.,composites,soils,rocks)and is widely recognized as a fundamental cause of progressive structural ***,achieving high-fidelity simulation for this issue,particularly concerning strong discontinuities and tension-compression-shear behaviors within localized zones,remains significantly *** response,this study introduces an integrated algorithmwithin the finite element framework,merging a coupled cohesive zone model(CZM)with the nonlinear augmented finite elementmethod(N-AFEM).The coupledCZMcomprehensively describes tension-compression and compressionshear failure behaviors in cohesive,frictional materials,while the N-AFEM allows nonlinear coupled intraelement discontinuities without necessitating extra nodes or nodal *** CZM validation using existing experimental data,this integrated algorithm was utilized to analyze soil slope failure mechanisms involving a specific tensile strength and to assess the impact of mechanical parameters(e.g.,tensile strength,weighting factor,modulus)in soils.

关键词： FEM analysis strong discontinuity nonlinear soil rupture cohesive zone model tension-compression-shear coupling

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Tuning SMSI to stabilize metallic Pd species:A case study on Pd/TiO_(2) for HCHO oxidation

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Chinese Chemical Letters 2024年第3期35卷 162-166页

作者： Chunying Wang Xiaofeng Liu Jingyi Wang Yaobin Li Shaohua Xie Fudong Liu Changbin Zhang Yuming Zheng Wenpo Shan Hong He Center for Excellence in Regional Atmospheric Environment Key Laboratory of Urban Pollutant ConversionInstitute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China Zhejiang Key Laboratory of urban Environmental Processes and Pollution Control Ningbo Urban Environment Observation and Research StationChinese Academy of SciencesNingbo 315800China department of Civil Environmentaland Construction Engineering(CECE)Catalysis Cluster for Renewable Energy and Chemical Transformations(REACT)Nano Science Technology Center(NSTC)University of Central FloridaOrlandoFL 32816USA State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-environmental SciencesChinese Academy of SciencesBeijing 100085China

Pretreatment of the carrier for supported catalysts can effectively improve the strong metal-support interaction(SMSI)and increase the dispersion of precious metals,which are critical to many important catalytic *** this work,we tuned SMSI on Pd/TiO_(2)catalysts through inducing surface defects of TiO_(2)by pretreated with different atmospheres(H_(2)/N_(2),N_(2),O_(2)/N_(2))at the high temperature(800℃).Multiple characterization results illustrated that surface defects anchored Pd species and thus enhanced their *** reduction,Ti^(3+)species formed and transferred onto the metallic Pd species and then induced SMSI,which effectively stabilize Pd species in the metallic *** stronger MSI,the more stability of Pd *** a case,Pd/TiO_(2)–800H_(2),with strongest MSI,displayed the best HCHO oxidation performance at low temperature(10℃).

关键词： Pd/TiO_(2) Surface defects SMSI Formaldehyde Stability of Pd species

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Simplified seismic scenario analysis of existing masonry buildings accounting for local site effects

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Frontiers of Structural and Civil Engineering 2024年第2期18卷 309-318页

作者： Ayşe E.ÖZSOYÖZBAY Işıl SANRI KARAPINAR Zehra N.KUTLU İsmail E.KILIÇ department of Civil Engineering Maltepe UniversityIstanbul 34857Turkey School of Engineering and construction Oryx Universal CollegeDoha 12253Qatar

This study discusses the effects of local sites and hazard amplification on the seismic vulnerability assessment of existing masonry *** this context,a rapid seismic evaluation procedure was implemented on an old masonry building stock in the historical center Galata,located inİstanbul,to determine the seismic risk priority of the built *** scenarios were generated for all soil classes,different moment magnitudes,and source-to-site distances to obtain more accurate results for the seismic vulnerability assessment of the studied building ***,damage distributions estimated under nine different scenarios with/without site effects were compared and illustrated in maps to discuss changes in vulnerability owing to amplification *** this study,by re-examining the rapid seismic evaluation procedure by including geo-hazard-based assessment,the importance of site effects on the vulnerability and risk assessment of built heritage was *** proposed framework integrating field data and local site effects is believed to advance the current applications for vulnerability assessment of masonry buildings and provide an improvement in the application of rapid seismic assessment procedures with more reliable results.

关键词： masonry buildings seismic vulnerability assessment cultural heritage local site effect

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Ghost Module Based Residual Mixture of Self-Attention and Convolution for Online Signature Verification

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Computers, Materials & Continua 2024年第4期79卷 695-712页

作者： Fangjun Luan Xuewen Mu Shuai Yuan department of Computer Technology School of Computer Science and EngineeringShenyang Jianzhu UniversityShenyang110168China Liaoning Province Big Data Management and Analysis Laboratory of urban construction Shenyang Jianzhu UniversityShenyang110168China Shenyang Branch of National Special Computer Engineering Technology Research Center Shenyang Jianzhu UniversityShenyang110168China

Online Signature Verification (OSV), as a personal identification technology, is widely used in various ***, it faces challenges, such as incomplete feature extraction, low accuracy, and computational heaviness. Toaddress these issues, we propose a novel approach for online signature verification, using a one-dimensionalGhost-ACmix Residual Network (1D-ACGRNet), which is a Ghost-ACmix Residual Network that combines convolutionwith a self-attention mechanism and performs improvement by using Ghost method. The Ghost-ACmix Residualstructure is introduced to leverage both self-attention and convolution mechanisms for capturing global featureinformation and extracting local information, effectively complementing whole and local signature features andmitigating the problem of insufficient feature extraction. Then, the Ghost-based Convolution and Self-Attention(ACG) block is proposed to simplify the common parts between convolution and self-attention using the Ghostmodule and employ feature transformation to obtain intermediate features, thus reducing computational ***, feature selection is performed using the random forestmethod, and the data is dimensionally reducedusing Principal Component Analysis (PCA). Finally, tests are implemented on the MCYT-100 datasets and theSVC-2004 Task2 datasets, and the equal error rates (EERs) for small-sample training using five genuine andforged signatures are 3.07% and 4.17%, respectively. The EERs for training with ten genuine and forged signaturesare 0.91% and 2.12% on the respective datasets. The experimental results illustrate that the proposed approacheffectively enhances the accuracy of online signature verification.

关键词： Online signature verification feature selection ACG block ghost-ACmix residual structure

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Digital twin-enabled smart facility management: A bibliometric review

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Frontiers of Engineering Management 2024年第1期11卷 32-49页

作者： Obaidullah HAKIMI Hexu LIU Osama ABUDAYYEH department of Civil and construction Engineering Western Michigan UniversityKalamazooMI 49008-5316USA

In recent years,the architecture,engineering,construction,and facility management(FM)industries have been applying various emerging digital technologies to facilitate the design,construction,and management of infrastructure *** twin(DT)has emerged as a solution for enabling real-time data acquisition,transfer,analysis,and utilization for improved decision-making toward smart *** research on DT for FM has been undertaken in the past *** paper presents a bibliometric analysis of the literature on DT for FM.A total of 248 research articles are obtained from the Scopus and Web of Science *** is then utilized to conduct bibliometric analysis and visualize keyword co-occurrence,citation,and co-authorship networks;furthermore,the research topics,authors,sources,and countries contributing to the use of DT for FM are *** findings show that the current research of DT in FM focuses on building information modeling-based FM,artificial intelligence(AI)-based predictive maintenance,real-time cyber–physical system data integration,and facility lifecycle asset *** areas,such as AI-based real-time asset prognostics and health management,virtual-based intelligent infrastructure monitoring,deep learning-aided continuous improvement of the FM systems,semantically rich data interoperability throughout the facility lifecycle,and autonomous control feedback,need to be further *** review contributes to the body of knowledge on digital transformation and smart FM by identifying the landscape,state-of-the-art research trends,and future needs with regard to DT in FM.

关键词： digital twin building information modeling facility management semantic interoperability artificial intelligence intelligent monitoring autonomous control feedback

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Current Situation and Countermeasures of Household Waste Classification in Feixi County, Hefei City

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Meteorological and Environmental Research 2024年第3期15卷 77-81页

作者： Yaqi XU Yalong JIANG Enqing GAO Shimao FENG Yuchen QIANG School of urban construction College Anhui Xinhua UniversityHefei 230088China

Feixi County has made significant progress in promoting waste classification,such as establishing a comprehensive classification system,and effectively reducing environmental pollution and waste ***,with the increase in waste generation,the county faces multiple challenges especially in the disposal of kitchen waste and improvement of residents environmental *** address these issues,Feixi County has implemented various measures,such as strengthening the construction of infrastructure for waste classification,improving regulations and clearly defining responsibilities,enhancing residents environmental awareness to encourage their participation in waste classification through education and promotion,and increasing supervision to ensure effective implementation of the *** emphasizes community governance,encourage all parties to participate in it,and strengthen publicity,education and training to enhance residents *** County has achieved positive results,but efforts are needed to further improve facilities,raise awareness,enhance supervision,and ensure the continuous effectiveness of waste classification work to promote urban green sustainable development.

关键词： Household waste classification Current situation Countermeasures Feixi County

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Green building research in South Africa:A scoping review and future roadmaps

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Energy and Built Environment 2024年第2期5卷 316-335页

作者： Favour D.Agbajor Modupe Cecilia Mewomo department of construction Management and Quantity Surveying Durban University of TechnologySteve Biko CampusDurban4001South Africa

The construction industry is recognised to pose serious environmental threats due to its anthropogenic *** confront this challenge,green building has been famed as an auspicious strategy to alleviate energy-related carbon emissions alongside climate change ***,it has birthed diverse empirical studies and holistic reviews by the research ***,these previous studies have been carried out from a global and continental viewpoint regardless of the green building development specifically in emerging *** present study seeks to fill the sparse research upshots on the synthesis of green building research at the country level with core focus on South *** this light,the current study provides a scoping overview of the intellectual exploration on green building research in the South African *** study’s findings highlight the varying growth regarding the subject matter,the drivers,drawbacks,and socio-economic issues confronting in developing green building projects in the *** optimize the advancement of green building in the region,this study recommends the implementation of financing schemes,utilization of advanced digital technologies,and promotion of green and sustainable building curricula across the institutions as well as post-occupancy-related studies within the green building spectrum towards a safe and salutogenic built-environment in the country.

关键词： Green building Sustainable construction Energy efficiency Review South Africa

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