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Energy & Environmental Materials 2024年第4期7卷 344-354页

作者： Jamil Ur Rahman Woo Hyun Nam Yong-Jae Jung Jong Ho Won Jong-Min Oh Nguyen Van Du Gul Rahman Víctor M.García-Suárez Ran He Kornelius Nielsch Jung Young Cho Won-Seon Seo Jong Wook Roh Sang-il Kim Soonil Lee Kyu Hyoung Lee Hyun Sik Kim Weon Ho Shin Leibniz Institute for Solid State and Materials Research Advanced Materials Convergence R&D Division Korea Institute of Ceramic Engineering & Technology department of Electronic Materials engineering Kwangwoon University department of Energy engineering Dankook University Faculty of Fundamental science Phenikaa University department of Physics Quaid-i-Azam University Departamento de Física Universidad de Oviedo Nanomaterials and Nanotechnology Research Center-CINN department of Materials science and engineering Yonsei University School of Nano & Materials science and engineering Kyungpook National University department of Materials science and engineering University of Seoul School of Materials science and engineering Changwon National University

Bi2Te3-based materials have drawn much attention from the thermoelectric community due to their excellent thermoelectric performance near room ***,the stability of existing n-type Bi2（Te,Se）3materials is still low due to the evaporation energy of Se (37.70 kJ mol-1) being much lower than that of Te (52.55 kJ mol-1).The evaporated Se from the material causes problems in interconnects of the module while degrading the efficiency.

关键词： Bi2Te3 energy harvesting FeTe2 nanoinclusion n-type materials thermoelectric

ReChoreoNet: Repertoire-based Dance Re-choreography with Music-conditioned Temporal and Style Clues

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Machine Intelligence Research 2024年第4期21卷 771-781页

作者： Ho Yin Au Jie Chen Junkun Jiang Yike Guo department of Computer science Hong Kong Baptist UniversityHong Kong 999077China department of Computer science and engineering The Hong Kong University of Science and EngineeringHong Kong 999077China

To generate dance that temporally and aesthetically matches the music is a challenging problem in three ***,the generated motion should be beats-aligned to the local musical ***,the global aesthetic style should be matched between motion and *** third,the generated motion should be diverse and *** address these challenges,we propose ReChoreoNet,which re-choreographs high-quality dance motion for a given piece of music.A data-driven learning strategy is proposed to efficiently correlate the temporal connections between music and motion in a progressively learned cross-modality embedding *** beats-aligned content motion will be subsequently used as autoregressive context and control signal to control a normalizing-flow model,which transfers the style of a prototype motion to the final generated *** addition,we present an aesthetically labelled music-dance repertoire(MDR)for both efficient learning of the cross-modality embedding,and understanding of the aesthetic connections between music and *** demonstrate that our repertoire-based framework is robustly extensible in both content and *** quantitative and qualitative experiments have been carried out to validate the efficiency of our proposed model.

关键词： Generative model cross-modality learning normalizing flow tempo synchronization style transfer.

Crystallographically vacancy‐induced MOF nanosheet as rational single‐atom support for accelerating CO_(2)electroreduction to CO

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Carbon Energy 2024年第8期6卷 49-62页

作者： Jin Hyuk Cho Joonhee Ma Chaehyeon Lee Jin Wook Lim Youngho Kim Ho Yeon Jang Jaehyun Kim Myung‐gi Seo Youngheon Choi Youn Jeong Jang Sang Hyun Ahn Ho Won Jang Seoin Back Jong‐Lam Lee Soo Young Kim department of Materials science and engineering Korea UniversitySeoulRepublic of Korea department of Chemical and Biomolecular engineering Sogang UniversitySeoulRepublic of Korea department of Materials science and engineering Pohang University of Science and Technology(POSTECH)PohangRepublic of Korea department of Materials science and engineering Research Institute of Advanced MaterialsSeoul National UniversitySeoulRepublic of Korea Lotte Chemical R&D Center DaejeonRepublic of Korea department of Chemical engineering Hanyang UniversitySeoulRepublic of Korea School of Chemical engineering and Material science Chung‐Ang UniversitySeoulRepublic of Korea

To attain a circular carbon economy and resolve CO_(2)electroreduction technology obstacles,single‐atom catalysts(SACs)have emerged as a logical option for electrocatalysis because of their extraordinary catalytic *** SACs,metal–organic frameworks(MOFs)have been recognized as promising support materials because of their exceptional ability to prevent metal *** study shows that atomically dispersed Ni single atoms on a precisely engineered MOF nanosheet display a high Faradaic efficiency of approximately 100%for CO formation in H‐cell and three‐compartment microfluidic flow‐cell reactors and an excellent turnover frequency of 23,699 h−1,validating their intrinsic catalytic *** results suggest that crystallographic variations affect the abundant vacancy sites on the MOF nanosheets,which are linked to the evaporation of Zn‐containing organic linkers during ***,using X‐ray absorption spectroscopy and density functional theory calculations,a comprehensive investigation of the unsaturated atomic coordination environments and the underlying mechanism involving CO^(*)preadsorbed sites as initial states was possible and provided valuable insights.

关键词： 2‐dimensional material carbon dioxide reduction metal-organic frameworks single‐atom catalysts vacancy sites

Refinement modeling and verification of secure operating systems for communication in digital twins

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Digital Communications and Networks 2024年第2期10卷 304-314页

作者： Zhenjiang Qian Gaofei Sun Xiaoshuang Xing Gaurav Dhiman School of Computer science and engineering Changshu Institute of TechnologySuzhou215500China University Centre for Research and Development Department of Computer Science and EngineeringChandigarh UniversityMohali140413India department of Computer science and engineering Graphic Era Deemed to be UniversityDehradun248002India

In traditional digital twin communication system testing,we can apply test cases as completely as possible in order to ensure the correctness of the system implementation,and even then,there is no guarantee that the digital twin communication system implementation is completely *** verification is currently recognized as a method to ensure the correctness of software system for communication in digital twins because it uses rigorous mathematical methods to verify the correctness of systems for communication in digital twins and can effectively help system designers determine whether the system is designed and implemented *** this paper,we use the interactive theorem proving tool Isabelle/HOL to construct the formal model of the X86 architecture,and to model the related assembly *** verification result shows that the system states obtained after the operations of relevant assembly instructions is consistent with the expected states,indicating that the system meets the design expectations.

关键词： Theorem proving Isabelle/HOL Formal verification System modeling Correctness verification

Effects of Ta content on microstructure and oxidation behavior of AlCoCrFeNiYTax high entropy alloy

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Rare Metals 2024年第9期43卷 4462-4475页

作者： Cang Gu Jun-Hao Hu Jian-Bo Song Cheng Xu Ming-Yu Hu Yu-Xuan Zhang Jiang Tian Chao Li Jing Feng Faculty of Materials science and engineering Kunming University of Science and Technology department of Physics Hong Kong Baptist University

The oxidation behavior of the Al Co Cr Fe Ni YTaxhigh entropy alloy（HEA） doped with different Ta contents at 1100 °C is investigated. In this study, different reasons for the spallation of the oxide scales of HEAs without/with excessive Ta addition after 1000 h of oxidation are discussed, and the most suitable Ta doping content for this HEA is explored, in which the HEA exhibits both an exceptionally low oxidation rate, and the formation of oxide scales composed of intact a-Al2O3. Meanwhile, it is found that the addition of Ta can effectively inhibit the phase transition of β phase, which makes the surface of the oxide scale smoother. By combining our experimental results with Wagner–Hauffe theory, the influence of Ta drag effect on oxide scale growth is explained, which provides some theoretical guidance for the subsequent design of Al Co Cr Fe Ni HEAs, and can lead to the development of thermal barrier coatings at higher service temperature.

关键词： Al2O3 scales Elements diffusion High-entropy alloy Oxidation

Converting an O-vacancy-rich oxide into a multifunctional separator modifier for long-lifespan lithium metal batteries

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Journal of Energy Chemistry 2024年第10期97卷 371-378页

作者： Juntao Si Xiaoying Li Yixuan Li Kuo Cao Yiran Zhu Chunhua Chen CAS Key Laboratory of Precision and Intelligent Chemistry Department of Materials Science and Engineering University of Science and Technology of China

The lithium metal anode is hailed as the desired "holy grail" for the forthcoming generation of highenergy-density batteries,given its astounding theoretical capacity and low ***,the formation and growth of dendrites seriously compromise battery life and ***,an yttriastabilized bismuth oxide（YSB） layer is fabricated on the polypropylene（PP） separator,where YSB reacts with Li anode in-situ in the cell to form a multi-component composite interlayer consisting of Li3Bi,Li2O,and *** interlayer can function not only as a redistributor to regulate Li+distribution but also as an anion adsorber to increase the Li+transference number from 0.37 to 0.79 for suppressing dendrite nucleation and ***,compared with the cell with a baseline separator,those with modified separators exhibit prolonged lifespan in both Li/Li symmetrical cells and Li/Cu ***,the full cells coupled with ultrahigh-loading LiFePO4display an excellent cycling performance of 1700 cycles with a high capacity retention of ～80% at 1 C,exhibiting great potential for practical *** work provides a feasible and effective new strategy for separator modification towards building a much-anticipated dendrite-free Li anode and realizing long-lifespan lithium metal batteries.

关键词： Conversion-alloying reaction Dendrite-free Lithium metal battery Multifunctional interlayer Separator

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Design and evaluation of the traveling wave piezoelectric beam actuators

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Acta Mechanica Sinica 2024年第7期40卷 152-163页

作者： Yuanshuai Ding Zengyao Lv Hangyu Li Yuyang Lin Yongmao Pei department of Mechanics and engineering science College of EngineeringPeking UniversityBeijing100871China department of Civil and Environmental engineering Northwestern UniversityEvanstonIL60208USA

Traveling wave piezoelectric beam actuators(TWPBAs)present an advantageous structural configuration for self-moving actuators and hold significant promise for operation in confined ***,current research on TWPBAs faces several limitations,including deficient design methods of excitation and structural parameters,inadequate evaluation metrics,and lack of a quantitative relationship between these parameters and evaluation *** study presents a systematic approach to determining TWPBAs'structure and excitation parameters,proposes criteria for determining the excitation parameters through an established analytical model,and introduces an effective evaluation method for TWPBAs'*** the analytical model and evaluation metrics,we reveal:(1)the coupling relationship between excitation parameters and structural parameters,(2)the influence of participating mode pairs on vibration response,(3)the quantitative relationship between the evaluation metrics and excitation parameters is also *** conclusions are substantiated by the results of finite element analysis,laser vibration measurements,and motion test ***,the practical application of TWPBAs in pipeline operations underscores their potential for use in endoscopy and precision instruments.

关键词： Piezoelectric actuator Exciter-Exciter method Wave propagation Vibration control

Spherical Bi_(2)O_(3)/ATO catalyst with N_(2)pre-reduction electrocatalytic reduction of CO_(2)to formic acid

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Journal of Environmental sciences 2024年第6期140卷 331-340页

作者： Junying Yi Yuli Chen Dongze Lai Bihong Lv Xiaomin Wu Guohua Jing department of Environmental science&engineering College of Chemical EngineeringHuaqiao UniversityXiamenFujian 361021China

To achieve carbon neutrality,the Chinese government needs to gain a comprehensive understanding of the sources and drivers of greenhouse gas(GHG)emissions,particularly at the county *** County in eastern China is a typical example of an industrial transformation from quarrying to a low-carbon *** study analyzed the decoupling types and structural characteristics of GHG emissions and the driving factors of carbon dioxide(CO_(2))emissions in the Anji from 2006 to 2019,and explored the differences between countylevel and provincial-level or city-level *** was observed that energy-related activities are the main source of GHG emissions in Anji and that economic development is the driving factor behind the increasing CO_(2)***,industrial transformation and upgradation coupled with the alternative use of clean energy limit the growth of GHG *** study details the GHG emissions of county during the industrial transformation stage and provides corresponding policy recommendations for county governments.

关键词： N_(2)prereduction CO_(2)electroreduction Bi_(2)O_(3)/ATO catalyst Formate

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Synergistic enhancement of photocatalytic and antimicrobial efficacy of nitrogen and erbium co-doped ZnO nanoparticles

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Journal of Rare Earths 2024年第5期42卷 859-868,I0002页

作者： Sudipta Mondal Moniruzzaman Jamal Sikder Ashikuzzaman Ayon Md Jannatul Ferdous Anik Md Muktadir Billah department of Materials and Metallurgical engineering Bangladesh University of Engineering and TechnologyDhaka1000Bangladesh School of Materials engineering Purdue UniversityWest LafayetteIN47907USA department of Materials science and engineering University of CaliforniaBerkeleyCA94720USA department of Materials science and engineering Northwestern UniversityEvanstonI28USA

Using the chemical co-precipitation approach,a series of nitrogen(N) and erbium(Er) co-doped ZnO nanoparticles(NPs) was effectively synthesized to enhance the photocatalytic and antibacterial *** characterization techniques,including X-ray diffraction(XRD),X-ray photoelectron spectro scopy(XPS),scanning electron microscopy(SEM),UV-vis,and photoluminescence(PL) spectroscopy,were carried out to validate the evaluated photocatalytic and antibacterial *** analysis confirms the pure wurtzite ZnO phase without the presence of any secondary *** analysis confirms the succe ssful incorporation of nitrogen and erbium into the ZnO *** optical bandgap of ZnO calculated from UV-vis spectroscopy shows a redshift after Er-N co-doping,with the lowest bandgap of 3.215 eV calculated for Zn_(0.97)Er_(0.03)N_(0.01)O_(0.99) *** images demonstrate the formation of nanorods after N-Er co-doping,followed by gradually increase d rod diameter and length after N-Er ***,the photocatalytic activities of ZnO samples we re measured by their ability to facilitate the photodegradation of Rhodamine B under UV *** with 1 mol% N doping exhibits 88% photodegradation of RhB under UV light within 360 min,and the photodegradation and antibacterial activity are greatly improved with Er *** fact,3 mol% Er-1 mol% N doped ZnO NPs demonstrate the highest photocatalytic activity,with approximately 96% degradation after 360 min,as well as superior antibacterial activity against Staphylococcus aureus(Gram-positive bacteria) and Pseudomonas aeruginosa(Gram-negative bacteria) with the highest zone of inhibition(ZOI) of 16 nm,due to nanorod formation,increased reactive oxygen species(ROS),and decreased electron-hole recombination,as validated by SEM,XPS,and PL spectroscopy.

关键词： Chemical co-precipitation Co-doping Bandgap Photocatalysis Rare earths Antimicrobial

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Efficient Communication in Wireless Sensor Networks Using Optimized Energy Efficient Engroove Leach Clustering Protocol

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Tsinghua science and Technology 2024年第4期29卷 985-1001页

作者： N.Meenakshi Sultan Ahmad A.V.Prabu J.Nageswara Rao Nashwan Adnan Othman Hikmat A.M.Abdeljaber R.Sekar Jabeen Nazeer SRM Institute of science and Technology KattankulathurChennai 603203India department of Computer science College of Computer Engineering and SciencesPrince Sattam Bin Abdulaziz UniversityAlkharj 11942Saudi Arabia University Center for Research and Development(UCRD) Department of Computer Science and EngineeringChandigarh UniversityGharuanMohali 140413India department of ECE Koneru Lakshmaiah Education FoundationVaddeswaramGuntur 522502India department of Computer science and engineering Lakireddy Balireddy College of Engineering(A)NTR District 521230India department of Computer engineering College of EngineeringKnowledge UniversityErbil 44001Iraq department of Computer science Faculty of Information TechnologyApplied Science Private UniversityAmman 11937Jordan department of Electronics and Communication engineering(ECE) School of EngineeringPresidency UniversityBangalore 834001India

The Wireless Sensor Network(WSN)is a network that is constructed in regions that are inaccessible to human *** widespread deployment of wireless micro sensors will make it possible to conduct accurate environmental monitoring for a use in both civil and military *** make use of these data to monitor and keep track of the physical data of the surrounding environment in order to ensure the sustainability of the *** data have to be picked up by the sensor,and then sent to the sink node where they may be *** nodes of the WSNs are powered by batteries,therefore they eventually run out of *** energy restriction has an effect on the network life span and environmental *** objective of this study is to further improve the Engroove Leach(EL)protocol’s energy efficiency so that the network can operate for a very long time while consuming the least amount of *** lifespan of WSNs is being extended often using clustering and routing *** Meta Inspired Hawks Fragment Optimization(MIHFO)system,which is based on passive clustering,is used in this study to do *** cluster head is chosen based on the nodes’residual energy,distance to neighbors,distance to base station,node degree,and node *** on distance,residual energy,and node degree,an algorithm known as Heuristic Wing Antfly Optimization(HWAFO)selects the optimum path between the cluster head and Base Station(BS).They examine the number of nodes that are active,their energy consumption,and the number of data packets that the BS *** overall experimentation is carried out under the MATLAB *** the analysis,it has been discovered that the suggested approach yields noticeably superior outcomes in terms of throughput,packet delivery and drop ratio,and average energy consumption.

关键词： wireless sensor networks energy efficient engroove leach protocol meta inspired Hawks fragment optimization heuristic wing antfly optimization