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Catalyst–Support Interaction in Polyaniline‑Supported Ni_(3)Fe Oxide to Boost Oxygen Evolution Activities for Rechargeable Zn‑Air Batteries

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Nano-Micro Letters 2025年第1期17卷 176-190页

作者： Xiaohong Zou Qian Lu Mingcong Tang Jie Wu Kouer Zhang Wenzhi Li Yunxia Hu Xiaomin Xu Xiao Zhang Zongping Shao Liang An department of mechanical engineering The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong SARPeople’s Republic of China Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and TechnologyNanjing University of Information Science and TechnologyNanjing 210044People’s Republic of China department of Chemistry The Chinese University of Hong KongMa Lin BuildingShatinHong Kong SAR 999077People’s Republic of China WA School of Mines:Minerals Energy and Chemical Engineering(WASM‑MECE)Curtin UniversityPerthWA 6102Australia Research Institute for Advanced Manufacturing The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong SARPeople’s Republic of China Research Institute for Smart Energy The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong SARPeople’s Republic of China

Catalyst–support interaction plays a crucial role in improving the catalytic activity of oxygen evolution reaction(OER).Here we modulate the catalyst–support interaction in polyaniline-supported Ni_(3)Fe oxide(Ni_(3)Fe oxide/PANI)with a robust hetero-interface,which significantly improves oxygen evolution activities with an overpotential of 270 mV at 10 mA cm^(-2)and specific activity of 2.08 mA cm_(ECSA)^(-2)at overpotential of 300 mV,3.84-fold that of Ni_(3)Fe *** is revealed that the catalyst–support interaction between Ni_(3)Fe oxide and PANI support enhances the Ni–O covalency via the interfacial Ni–N bond,thus promoting the charge and mass transfer on Ni_(3)Fe *** the excellent activity and stability,rechargeable Zn-air batteries with optimum Ni_(3)Fe oxide/PANI are assembled,delivering a low charge voltage of 1.95 V to cycle for 400 h at 10 mA cm^(-2).The regulation of the effect of catalyst–support interaction on catalytic activity provides new possibilities for the future design of highly efficient OER catalysts.

关键词： Catalyst-support interaction Supported catalysts Heterointerface Oxygen evolution reaction Zn-air batteries

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Machine learning driven rational design of dual atom catalysts on graphene for carbon dioxide electroreduction

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Nano Research 2025年第1期18卷 186-194页

作者： Dongxu Jiao Xinyi Li Mingzi Sun Lin Liu Jinchang Fan Jingxiang Zhao Bolong Huang Xiaoqiang Cui State Key Laboratory of Automotive Simulation and Control School of Materials Science and Engineeringand Key Laboratory of Automobile Materials of MOEJilin UniversityChangchun 130012China department of Applied Biology and Chemical Technology The Hong Kong Polytechnic UniversityHung HomKowloonHong KongChina College of Chemistry and Chemical engineering and Key Laboratory of Photonic and Electronic Bandgap MaterialsMinistry of EducationHarbin Normal UniversityHarbin 150025China

The development of high-performance atomiccatalysts for the carbon dioxide reduction reaction(CO_(2)RR)is atime-consuming process due to the complexity of the reactionmechanism and the uncertainty of the active ***,wehave proposed combining density functional theory(DFT)andmachine learning(ML)to investigate the potential of topologicalgraphene-based dual-atom catalysts(DACs)as CO_(2)*** analyzing the ML results,we identify thenumber of d-orbital electrons in the active site as a key factorinfluencing the CO_(2)RR catalytic ***,wepropose a simple descriptor to measure the CO_(2)RR activity ofthese *** findings provide plausible explanations for thesynergistic interactions between bimetallic atoms in CO_(2)RR andallow us to screen the homogeneous Ni-Ni pair as the mostpromising dual-atom *** work offers a fast MLapproach based on limited DFT calculations to predict the mostelectroactive and stable DACs on carbon support for CO_(2)RR,facilitating rapid screening of high-performance dual-atomcatalysts.

关键词： CO_(2)reaction reduction dual-atom catalysts density functional theory machine learning

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Spontaneous Orientation Polarization of Anisotropic Equivalent Dipoles Harnessed by Entropy engineering for Ultra‑Thin Electromagnetic Wave Absorber

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Nano-Micro Letters 2025年第1期17卷 424-438页

作者： honghan Wang Xinyu Xiao Shangru Zhai Chuang Xue Guangping Zheng Deqing Zhang Renchao Che Junye Cheng Liaoning Key Lab of Lignocellulose Chemistry and BioMaterials Liaoning Collaborative Innovation Center for Lignocellulosic BiorefinerySchool of Light Industry and Chemical EngineeringDalian Polytechnic UniversityDalian 116034People’s Republic of China School of Life Science and Biotechnology Dalian University of TechnologyDalian 116024People’s Republic of China department of mechanical engineering Hong Kong Polytechnic UniversityHung HomKowloonHong Kong 999077People’s Republic of China School of Materials Science and engineering Qiqihar UniversityQiqihar 161006People’s Republic of China Laboratory of Advanced Materials Shanghai Key Lab of Molecular Catalysis and Innovative MaterialsAcademy for Engineering&TechnologyFudan UniversityShanghai 200438People’s Republic of China department of Materials Science Shenzhen MSU-BIT UniversityShenzhen 517182People’s Republic of China

The synthesis of carbon supporter/nanoscale high-entropy alloys(HEAs)electromagnetic response composites by carbothermal shock method has been identified as an advanced strategy for the collaborative competition engineering of conductive/dielectric *** migration modes within HEAs as manipulated by the electronegativity,valence electron configurations and molar proportions of constituent elements determine the steady state and efficiency of equivalent ***,enlightened by skin-like effect,a reformative carbothermal shock method using carbonized cellulose paper(CCP)as carbon supporter is used to preserve the oxygencontaining functional groups(O·)of carbonized cellulose fibers(CCF).Nucleation of HEAs and construction of emblematic shell-core CCF/HEAs heterointerfaces are inextricably linked to carbon metabolism induced by O·.Meanwhile,the electron migration mode of switchable electronrich sites promotes the orientation polarization of anisotropic equivalent *** virtue of the reinforcement strategy,CCP/HEAs composite prepared by 35%molar ratio of Mn element(CCP/HEAs-Mn_(2.15))achieves efficient electromagnetic wave(EMW)absorption of−51.35 dB at an ultra-thin thickness of 1.03 *** mechanisms of the resulting dielectric properties of HEAs-based EMW absorbing materials are elucidated by combining theoretical calculations with experimental characterizations,which provide theoretical bases and feasible strategies for the simulation and practical application of electromagnetic functional devices(e.g.,ultra-wideband bandpass filter).

关键词： High-entropy alloys Carbothermal shock Switchable electron migration modes Emblematic shell-core heterointerfaces Ultra-thin thickness

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Compositionally complex coherent precipitation-strengthened high-entropy alloys:a critical review

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Rare Metals 2022年第6期41卷 2002-2015页

作者： Jin-Xiong Hou Bo-Xuan Cao Bo Xiao Zeng-Bao Jiao Tao Yang department of Materials Science and engineering City University of Hong KongHong Kong 999077China hong kong Institute for Advanced Study City University of Hong KongHong Kong 999077China department of mechanical engineering.the hong kong polytechnic university Hong Kong 999077China

The coherent precipitation-strengthened high-entropy alloys(CPS-HEAs)as a new type of structural materials are expected to possess many unique mechanical properties,such as the outstanding strength-ductility com-bination at cryogenic and room *** from this,most of their strengths can even be well retained at elevated *** compositionally complex matrix and nanoprecipitation phases,as well as the coherent interfaces between them,can potentially bring novel merits of these CPS-HEAs,including sluggish dif-fusion,excellent thermal stability,and controlled magnetic *** that the ductile coherent L1_(2)-nanoparticles can improve the strength of alloys without too much reduction of plasticity,while the coherent B2-nanoparticles strengthened HEAs display completely brittle failure upon tensile test at room *** overview of the alloy design,microstructure evolution,oxidation resistance,mechanical and magnetic properties of CPS-HEAs are briefly discussed *** advantages of multicomponent coherent precipitation-strengthened HEAs as well as the limitations in this field are also *** addition,this review also points out the future research directions and prospects.

关键词： High-entropy alloys Coherent precipitation strengthening Multicomponent intermetallic mechanical properties Magnetic properties

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Numerical simulation of particle formation and evolution in a vehicle exhaust plume using the bimodal Taylor expansion method of moments

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Particuology 2019年第2期17卷 46-55页

作者： Shuyuan Liu Tat Leung Chan Huijie Liu department of mechanical engineering The Hong Kong Polytechnic University Kowloon Hong Kong China

The bimodal Taylor expa nsion method of moments (B-TEMOM) model scheme was developed to simulate the formation and evolution of vehicle exhaust particles. Two independent types of log-normal particle size distributions were selected in the B-TEMOM model scheme, comprising large and small particles to represent background (i.e., the surrounding environment) and vehicle exhaust particles, respectively. Concentration distributions of exhaust and background particles derived using this model scheme were verified against results from a moving secti onal method and the bimodal quadrature method of moments, showing excellent agreement. The effects of vehicle tailpipe ex 让 cond 让 ions (e.g., exhaust particle concentrations and velocity), sulfurcontent, and relative humidity on the evoluti on of particles were investigated numerically. Both two-dimensional and three-dimensional numerical simulations showed that tailpipe exit velocity and relative humid让y did not greatly affect the steady-state concentrations or the diameters of particles in urban atmospheres. Although an increase in sulfur content had little effect on the particle concentration, it led to background particles with larger geometric average diameter entering the environment. This coupled CFD-B-TEMOM numerical model provides a simple but accurate and efficient method for studying bimodal aerosol dynamics.

关键词： Vehicle exhaust particles Bimodal Taylor expansi on method of moments Homogeneous nucleation Coagulation Tailpipe exit velocity Sulfur content and ambient relative humidity

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Differentially weighted operator splitting Monte Carlo method for simulating complex aerosol dynamic processes

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Particuology 2018年第1期16卷 114-126页

作者： hongmei Liu Tat Leung Chan department of mechanical engineering.the hong kong polytechnic university Kowloon Hong Kong China

A differentially weighted operator splitting Monte Carlo （DWOSMC） method is developed to solve com- plex aerosol dynamic processes by coupling the differentially weighted Monte Carlo method and the operator splitting technique. This method is validated by analytical solutions and a sectional method in different aerosol dynamic processes. It is first validated in coagulation and condensation processes, and nucleation and coagulation processes, and then validated through simultaneous nucleation, coagulation, and condensation processes. The results show that the DWOSMC method is a computationally efficient and quantitatively accurate method for simulating complex aerosol dynamic processes.

关键词： Differentially weighted Monte Carlo Operator splitting Aerosol dynamics Particle size distribution

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In situ Reduction of Silver Nanoparticles on Chitosan Hybrid Copper Phosphate Nanoflowers for Highly Efficient Plasmonic Solar-driven Interfacial Water Evaporation

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Journal of Bionic engineering 2021年第1期18卷 30-39页

作者： Mei Zhang Wanghuai Xu Minfei Li Jiaqian Li Peng Wang Zuankai Wang department of mechanical engineering City University of Hong KongHong Kong999077China department of Civil and Environmental engineering the Hong Kong Polytechnic UniversityHong Kong999077China

The development of water purification device using solar energy has received tremendous *** extensive progress,traditional photothermal conversion usually has a high cost and high environmental *** overcome this problem,we develop a low cost,durable and environmentally friendly solar *** bilayered evaporator is constructed with a thermal insulating polyvinylidene fluoride(PVDF)membrane as a bottom supporting layer and plasmonic silver nanoparticles decorated miero-sized hybrid flower(Ag/MF)as a top light-to-heat conversion *** with the sample with a flat silver film,the two-tier Ag/MF has a plasmonic enrichment property and high efficiency in converting the solar light to hcat as cach flower can gencrate a microscale hotspot by enriching the absorbed solar *** the other hand,the PVDF membrane on the bottom with porous structure not only improves the mechanicalstability of the entire structure,but also maintains a stable water supply from the bulk water to the evaporation interface by capillarity and minimizes the thermal *** combination of excellent water evaporation ability simple operation,and low cost of the production process imparts this type of plasmonic enhanced solar-driven interfacial water evaporator with promising prospects for potable water purification for point-of-use applications.

关键词： bionic plasmonic water evaporation synergistic effect Ag NPs hybrid flower

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Effectiveness of air cleaner on mitigating the transmission of respiratory disease in a dental clinic environment

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Building Simulation 2024年第10期17卷 1789-1803页

作者： Gang Yang Yifan Wang Ka Chung Chan Kwok Wai Mui Thomas F.Flemmig SThomas Ng Christopher Y.H.Chao Sau Chung Fu department of Building Environment and Energy engineering The Hong Kong Polytechnic UniversityHong KongChina Faculty of Dentistry The University of Hong KongHong KongChina department of Architecture&Civil engineering City University of Hong KongHong KongChina department of mechanical engineering The Hong Kong Polytechnic UniversityHong KongChina

In dental clinics with an open floor plan,the risk of patient-to-patient transmission of respiratory disease is a *** dental procedures large amounts of bioaerosol are produced and patients cannot wear personal protective *** paper examines how to effectively deploy air cleaner to reduce the infection risk in dental clinics with an open floor *** locations of air cleaners at various clean air delivery rates(CADRs)were *** dispersion of bioaerosol was studied through numerical simulations,and risk assessment was performed by a dose-response *** findings indicated that dental patients downstream of the background ventilation have a higher infection risk than those to the left and right of an infected patient(i.e.,the source).The lowest infection risks for the adjacent patients were found when the air cleaner was place opposite to the dentists,i.e.,on the floor at low CADR levels of 2.2 m^(3)/min or on the bench at CADR levels of 4.4 m^(3)/min or *** results of this study indicated that air cleaner can mitigate the risk of patient-to-patient transmission of SARS-CoV-2 in dental clinics with an open floor *** CADR levels determine the optimal placement of air cleaners.

关键词： infection risk air cleaner location dental clinic CFD simulation respiratory disease

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Adaptive state-constrained/model-free iterative sliding mode control for aerial robot trajectory tracking

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Applied Mathematics and Mechanics(English Edition) 2024年第4期45卷 603-618页

作者： Chen AN Jiaxi ZHOU Kai WANG College of mechanical and Vehicle engineering Hunan UniversityChangsha 410082China department of mechanical engineering The Hong Kong Polytechnic UniversityHong KongChina

This paper develops a novel hierarchical control strategy for improving the trajectory tracking capability of aerial robots under parameter *** hierarchical control strategy is composed of an adaptive sliding mode controller and a model-free iterative sliding mode controller(MFISMC).A position controller is designed based on adaptive sliding mode control(SMC)to safely drive the aerial robot and ensure fast state convergence under external ***,the MFISMC acts as an attitude controller to estimate the unmodeled dynamics without detailed knowledge of aerial ***,the adaption laws are derived with the Lyapunov theory to guarantee the asymptotic tracking of the system ***,to demonstrate the performance and robustness of the proposed control strategy,numerical simulations are carried out,which are also compared with other conventional strategies,such as proportional-integralderivative(PID),backstepping(BS),and *** simulation results indicate that the proposed hierarchical control strategy can fulfill zero steady-state error and achieve faster convergence compared with conventional strategies.

关键词： aerial robot hierarchical control strategy model-free iterative sliding mode controller(MFISMC) trajectory tracking reinforcement learning

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Characterization and Analysis of Inconel 718 Alloy Ground at Different Speeds

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Chinese Journal of mechanical engineering 2024年第2期37卷 137-149页

作者： Hao Liu Huili Han Qinghong Jiang Minglin He Bi Zhang department of mechanical and Energy engineering Southern University of Science and TechnologyShenzhen 518055China department of mechanical engineering Hong Kong Polytechnic UniversityHong KongChina

Inconel 718(IN718)alloy is widely applied to fabricate high temperature resistant or corrosion resistant parts due to its excellent mechanical ***,the machining of IN718 alloy is difficult as it may cause serious tool wear and poor surface quality(SQ)of the *** this work,grinding experiments on IN718 alloy at different speeds were conducted by using a CBN grinding *** relationship between grinding speed,SQ and subsurface damage(SSD)was well *** increasing grinding speed,surface roughness decreased,and SQ was greatly ***,the microhardness of the grinding surface declined as the grinding speed *** SSD depth was almost unchanged when the grinding speed was lower than 15 m/s,then it decreased with higher grinding *** was attributed to the mechanical-thermal synergistic effect in the grinding *** results indicated that increasing grinding speed can effectively improve the SQ and reduce the SSD of IN718 *** conclusion in the work may also provide insight into processing other hard-to-machining materials.

关键词： Surface integrity Grinding speed IN718 alloy Precision machining CBN grinding wheel

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