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Ultrahigh Energy and Power Density in Ni-Zn Aqueous Battery via Superoxide-Activated Three-Electron Transfer

Nano-Micro Letters 2025年第4期17卷 63-76页

作者： Yixue Duan Bolong Li Kai Yang Zheng Gong Xuqiao Peng Liang He Derek Ho School of mechanical engineering State Key Laboratory of Intelligent Construction and Healthy Operation and Maintenance of Deep Underground EngineeringSichuan UniversityChengdu 610065People’s Republic of China department of Materials Science and engineering City University of Hong KongKowloonHong Kong 999077People’s Republic of China hong kong Centre for Cerebro-Cardiovascular Health engineering Hong Kong Science ParkHong Kong 999077People’s Republic of China School of mechanical engineering Sichuan UniversityChengdu 610065People’s Republic of China

Aqueous Ni-Zn microbatteries are safe,reliable and inexpensive but notoriously suffer from inadequate energy and power ***,we present a novel mechanism of superoxide-activated Ni substrate that realizes the redox reaction featuring three-electron transfers(Ni↔Ni3+).The superoxide activates the direct redox reaction between Ni substrate and KNiO_(2)by lowering the reaction Gibbs free energy,supported by in-situ Raman and density functional theory *** prepared chronopotentiostatic superoxidation-activated Ni(CPS-Ni)electrodes exhibit an ultrahigh capacity of 3.21 mAh cm^(-2)at the current density of 5 mA cm^(-2),nearly 8 times that of traditional one-electron processes *** under the ultrahigh 200 mA cm^(-2)current density,the CPS-Ni electrodes show 86.4%capacity retention with a Columbic efficiency of 99.2%after 10,000 *** CPS-Ni||Zn microbattery achieves an exceptional energy density of 6.88 mWh cm^(-2)and power density of 339.56 mW cm^(-2).Device demonstration shows that the power source can continuously operate for more than 7 days in powering the sensing and computation intensive practical application of photoplethysmographic waveform *** work paves the way to the development of multi-electron transfer mechanisms for advanced aqueous Ni-Zn batteries with high capacity and long lifetime.

关键词： Superoxide Multiple electron transfer Ni aqueous battery AIoT power source Wearable health monitoring

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Enhanced battery life prediction with reduced data demand via semi-supervised representation learning

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Journal of Energy Chemistry 2025年第2期101卷 524-534页

作者： Liang Ma Jinpeng Tian Tieling Zhang Qinghua Guo Chi Yung Chung School of mechanical Materials Mechatronic and Biomedical Engineering University of Wollongong department of Electrical and Electronic engineering and Research Centre for Grid Modernisation The Hong Kong Polytechnic University Photonics Research Institute The Hong Kong Polytechnic University School of Electrical Computer and Telecommunications Engineering University of Wollongong

Accurate prediction of the remaining useful life(RUL) is crucial for the design and management of lithium-ion *** various machine learning models offer promising predictions,one critical but often overlooked challenge is their demand for considerable run-to-failure data for *** of such training data leads to prohibitive testing efforts as the run-to-failure tests can last for ***,we propose a semi-supervised representation learning method to enhance prediction accuracy by learning from data without RUL *** approach builds on a sophisticated deep neural network that comprises an encoder and three decoder heads to extract time-dependent representation features from short-term battery operating data regardless of the existence of RUL *** approach is validated using three datasets collected from 34 batteries operating under various conditions,encompassing over 19,900 charge and discharge *** method achieves a root mean squared error(RMSE)within 25 cycles,even when only 1/50 of the training dataset is labelled,representing a reduction of 48%compared to the conventional *** also demonstrate the method's robustness with varying numbers of labelled data and different weights assigned to the three decoder *** projection of extracted features in low space reveals that our method effectively learns degradation features from unlabelled *** approach highlights the promise of utilising semi-supervised learning to reduce the data demand for reliability monitoring of energy devices.

关键词： Lithium-ion batteries Battery degradation Remaining useful life Semi-supervised learning

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Towards high-performance,efficient and sustainable material processing technologies for aerospace applications

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Chinese Journal of Aeronautics 2025年第1期38卷 1-2页

作者： Jun MA M.W.FU Stefania BRUSCHI Heng LI State Key Laboratory of Solidification Processing Northwestern Polytechnical UniversityXi’an 710072China department of mechanical and Industrial engineering Norwegian University of Science and TechnologyTrondheim 7491Norway department of mechanical engineering The Hong Kong Polytechnic UniversityHung HomKowloonHong KongChina department of Industrial engineering University of PadovaPadova 35131Italy

The aerospace and aviation industry has long been at the forefront of materials and processing technologies,driven by its ongoing demand for lightweight,highly reliable,and durable *** manufacturing is a critical discipline that directly affects the performance,functionality,and safety of aircraft and aerospace *** meet the above-mentioned stringent requirements,advanced materials and cutting-edge processing technologies have evolved alongside aerospace innovations.

关键词： performance aviation mentioned

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Ultrasonic vibration-assisted cutting of titanium alloys:A state-of-the-art review

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Chinese Journal of Aeronautics 2025年第1期38卷 3-42页

作者： Ahmar KHAN Xin WANG Biao ZHAO Wenfeng DING Muhammad JAMIL Aqib Mashood KHAN Syed Hammad ALI Sadam HUSSAIN Jiong ZHANG Raj DAS National Key Laboratory of Science and Technology on Helicopter Transmission Nanjing University of Aeronautics and AstronauticsNanjing 210016China department of mechanical engineering College of EngineeringCity University of Hong KongHong Kong 999077China Centre for Additive Manufacturing School of EngineeringAerospace Engineering and AviationRMIT UniversityVictoria 3083Australia

The remarkable ability of titanium alloys to preserve their superior physical and chemical characteristics when subjected to extreme conditions significantly enhances their importance in the aerospace,military,and medical ***,conventional machining of titanium alloys leads to elevated tool wear,development of surface defects,and reduced machining efficiency due to their low heat conductivity,and chemical *** issues can be somewhat counteracted by integrating ultrasonic vibration in the conventional machining of titanium alloys and also enhance *** review article offers a holistic evaluation of the influence of ultrasonic vibration-assisted milling and turning on cutting forces,temperature,tool wear,and surface integrity,encompassing surface morphology,surface roughness,surface residual stress,surface hardness,and surface tribological properties during titanium alloys ***,it investigates the sustainability aspect that has not been previously *** on the performance of ultrasonic-assisted cutting revealed several advantages,including decreased cutting forces and cutting temperature,improved tool life,and a better-machined surface during ***,the sustainability factor is improved due to minimized energy consumption and residual *** conclusion,the key challenges and future prospects in the ultrasonic-assisted cutting of titanium alloys are also *** review article provides beneficial knowledge for manufactur-ers and researchers regarding ultrasonic vibration-assisted cutting of titanium alloy and will play an important role in achieving sustainability in the industry.

关键词： Ultrasonic vibration-assisted cutting Titanium alloys Material removal mechanism Machinability Sustainability

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Distributed Nash Equilibrium Seeking with Disturbances of Unknown Frequencies for High-Order Integrators over Jointly Strongly Connected Switching Networks

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Journal of Systems Science & Complexity 2025年第01期 369-389页

作者： HE Xiongnan HUANG Jie department of mechanical and Automation engineering The Chinese University of Hong Kong

In this paper, the authors study the problem of distributed Nash equilibrium seeking of N-player games with high-order integrator dynamics subject to disturbances generated by an uncertain exosystem. Similar problems have been studied for disturbances with an exactly known *** with the existing results of high-order integrator dynamics, which can only handle sinusoidal disturbances with known frequencies, this paper aims to handle multi-tone disturbances with unknown frequencies by introducing an adaptive control technique to estimate the unknown frequencies. Technically, when the exosystem is known, the disturbance can be dealt with by the Luenburger observer. In contrast, the Luenburger observer cannot deal with an uncertain exosystem. The authors combine the internal model design and some adaptive control technique to solve the proposed problem. Further, the authors also establish the sufficient condition to guarantee the convergence of the estimated unknown frequencies to the actual values of these frequencies. Two examples are given to verify the proposed algorithm.

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Efficient photocatalytic reduction of CO_(2)to formate by a molecular noble metal-free system

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Science China Chemistry 2025年第1期68卷 152-156页

作者： Lihua Zhang Lingjing Chen Huatian Shi Yue Wei Gui Chen Tai-Chu Lau School of Environment and Civil engineering Research Center for Eco-environmental EngineeringDongguan University of TechnologyDongguan 523808China department of Chemistry and Institute of Molecular Functional Materials City University of Hong KongHong Kong 999077China

Reducing CO_(2)to carbon-neutral solar fuels can not only alleviate the energy demand but also mitigate the greenhouse *** present,developing an efficient non-noble metal photo/electrocatalytic system for converting CO_(2)to a specific product beyond CO is still a big ***,we report a new cobalt complex bearing 2,2′-bi-1,10-phenanthroline ligand that can photocatalytically reduce CO_(2)to formate(HCOO^(-)).Turnover number(TON)for HCOO^(-)up to 677 with 99%selectivity can be achieved using organic dyes purpurin as photosensitizer and 1,3-dimethyl-2-phenyl-2,3-dihydro-1H-benzo[d]imidazole(BIH)as sacrificial reductant in a CO_(2)-saturated NMP/TEA(v/v,3:1)solution under visible light *** potential electrolysis at-1.41 V(***/Ag Cl)in the presence of 12 mM Et_(3)NHBF_(4)also produced HCOO^(-)with Faradaic efficiency of 39%.Spectroscopic and electrochemical studies suggest that a[CoI-H]species is the key intermediate for CO_(2)reduction.

关键词： photocatalysis noble metal-free CO_(2)reduction formate cobalt hydride

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Daytime radiative freezing

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Science Bulletin 2025年第1期70卷 29-32页

作者： Yi Zhang Chenglong She Jingjing Chen Kui Lai Keqiao Li Fan Yang Chenxi Wang Baoling Huang Lihua Shen Xiaobo Yin department of mechanical engineering The University of Hong KongHong Kong 999077China MOE Key Laboratory for Nonequilibrium Synthesis and Modulation of Condensed Matter School of PhysicsXi’an Jiaotong UniversityXi’an 710000China department of mechanical and Aerospace engineering The Hong Kong University of Science and TechnologyHong Kong 999077China department of Physics The University of Hong KongHong Kong 999077China

While modern refrigerators can easily produce ice at any time,Ancient Persians were known to harvest ice from shallow pools without such *** ice would form on clear nights even when the ambient temperature remained above freezing[1].The nocturnal ice formation occurs because the water,facing the sky,radiates heat to the cold expanse of space through the transparent atmospheric window between 8 to 13μm[2,3].As a result,the temperature of the water could drop below the ambient ***,achieving daytime ice-making under the sunshine remains a captivating and challenging pursuit.

关键词： temperature. freezing ambient

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Power synchronization: taming massive diversified serverless functions under power constraints

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Science China(Information Sciences) 2025年第03期68卷 47-65页

作者： Du LIU Lu ZHANG Yechen XU Xinkai WANG Lingyu SUN Yifei PU Xiaofeng HOU Chao LI Minyi GUO department of Computer Science and engineering Shanghai Jiao Tong University AI Chip Center for Emerging Smart Systems The Hong Kong University of Science and Technology

Carbon neutrality has become an important design objective worldwide. However, the on-going shift to cloud-naive era does not necessarily mean energy efficiency. From the perspective of power management, co-hosted serverless functions are difficult to tame. They are lightweight, short-lived applications sensitive to power capping activities. In addition, they exhibit great individual and temporal variability, presenting idiosyncratic performance/power scaling goals that are often at odds with one another. To date, very few proposals exist in terms of tailored power management for serverless platforms. In this work, we introduce power synchronization, a novel yet generic mechanism for managing serverless functions in a power-efficient way. Our insight with power synchronization is that uniform application power behavior enables consistent and uncompromised function operation on shared host machines. We also propose PowerSync, a synchronization-based power management framework that ensures optimal efficiency based on a clear understanding of functions. Our evaluation shows that PowerSync can improve the energy efficiency of functions by up to 16% without performance loss compared to conventional power management strategies.

关键词： serverless computing variability energy efficiency power management power synchronization

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Recent progress on elemental tellurium and its devices

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Journal of Semiconductors 2025年第1期46卷 91-106页

作者： Jiachi Liao Zhengxun Lai You Meng Johnny C.Ho department of Materials Science and engineering City University of Hong KongKowloonHong Kong 999077China Changsha Semiconductor Technology and Application Innovation Research Institute College of Semiconductors(College of IntegratedC ircuits)Hunan UniversityChangsha 410082China Institute for Materials Chemistry and engineering Kyushu UniversityFukuoka 8168580Japan State Key Laboratory of Terahertz and Millimeter Waves City University of Hong KongKowloonHong Kong 999077China

The rapid advancement of information technology has heightened interest in complementary devices and *** p-type semiconductors often lack sufficient electrical performance,thus prompting the search for new materials with high hole mobility and long-term *** tellurium(Te),featuring a one-dimensional chiral atomic structure,has emerged as a promising candidate due to its narrow bandgap,high hole mobility,and versatility in industrial applications,particularly in electronics and renewable *** review highlights recent progress in Te nanostructures and related devices,focusing on synthesis methods,including vapor deposition and hydrothermal synthesis,which produce Te nanowires,nanorods,and other *** applications in photodetectors,gas sensors,and energy harvesting devices are discussed,with a special emphasis on their role within the internet of things(IoT)framework,a rapidly growing field that is reshaping our technological *** prospects and potential applications of Te-based technologies are also highlighted.

关键词： elemental tellurium photodetector field-effect transistor gas sensor energy harvesting device

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Bioaccessibility and health risk assessment of hydrophobic organic pollutants in soils from four typical industrial contaminated sites in China

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Journal of Environmental Sciences 2025年第1期147卷 282-293页

作者： Shi-Ping Ou Xiao-Liang Liao Zi-Tao Huang Yan-Cong Hu Zongwei Cai Zhi-Feng Chen Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control Guangdong-Hong Kong-Macao Joint Laboratory for Contaminants Exposure and HealthSchool of Environmental Science and EngineeringGuangdong University of TechnologyGuangzhou 510006China State Key Laboratory of Environmental and Biological Analysis Department of ChemistryHong Kong Baptist UniversityHong Kong 999077China

There have been reports of potential health risks for people from hydrophobic organic pollutants,such as polycyclic aromatic hydrocarbons(PAHs),polychlorinated hydrocarbons(PCHs),and organophosphate flame retardants(OPFRs).When a contaminated site is used for residential housing or public utility and recreation areas,the soil-bound organic pollutantsmight pose a threat to human *** this study,we investigated the contamination profiles and potential risks to human health of 15 PAHs,6 PCHs,and 12 OPFRs in soils from four contaminated sites in *** used an in vitro method to determine the oral bioaccessibility of soil *** PAHswere found at concentrations ranging from26.4 ng/g to 987 ng/***(0.27-14.3 ng/g)and OPFRs(6.30-310 ng/g)were detected,but at low levels compared to earlier *** levels of PAHs,PCHs,and OPFRs released from contaminated soils into simulated gastrointestinal fluids ranged from 1.74%to 91.0%,2.51%to 39.6%,and 1.37%to 96.9%,*** on both spiked and unspiked samples,we found that the oral bioaccessibility of pollutantswas correlated with their logKow andmolecularweight,and the total organic carbon content and pH of *** in 13 out of 38 contaminated soil samples posed potential high risks to *** considering oral bioaccessibility,nine soils still posed potential risks,while the risks in the remaining soils became *** contribution of this paper is that it corrects the health risk of soil-bound organic pollutants by detecting bioaccessibility in actual soils from different contaminated sites.

关键词： Contaminated soil Hydrophobic organic pollutant Polycyclic aromatic hydrocarbon Oral bioaccessibility Risk assessment

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