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Investigation of multi-step fast charging protocol and aging mechanism for commercial NMC/graphite lithium-ion batteries

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Journal of Energy Chemistry 2023年第5期80卷 237-246,I0006页

作者： Yaqi Li Jia Guo Kjeld Pedersen Leonid Gurevich Daniel-Ioan Stroe department of materials and Production Aalborg UniversityAalborg 9220Denmark department of Energy Aalborg UniversityAalborg 9220Denmark

Fast charging is considered a promising protocol for raising the charging efficiency of electric ***,high currents applied to Lithium-ion(Li-ion)batteries inevitably accelerate the degradation and shorten their *** work designs a multi-step fast-charging method to extend the lifetime of LiNi0.5Co0.2Mn0.3O2(NMC)/graphite Li-ion batteries based on the studies of half cells and investigates the aging mechanisms for different charging *** degradation has been studied from both full cell behaviour and materials perspectives through a combination of non-destructive diagnostic methods and post-mortem *** the proposed multi-step charging protocol,the state-of-charge(SOC)profile is subdivided into five ranges,and the charging current is set differently for different SOC *** of the designed multi-step fast charging protocols is shown to allow for a 200 full equivalent cycles longer lifetime as compared to the standard charging method,while the charging time is reduced by 20%.From the incremental capacity analysis and electrical impedance spectroscopy,the loss of active materials and lithium inventory on the electrodes,as well as an increase in internal resistance for the designed multistep constant-current-constant-voltage(MCCCV)protocol have been found to be significantly lower than for the standard charging ***-mortem analysis shows that cells aged by the designed MCCCV fast charging protocol exhibit less graphite exfoliation and crystallization damage,as well as a reduced solid electrolyte interphase(SEI)layer growth on the anode,leading to a lower Rseiresistance and extended lifetime.

关键词： Fast-charging Lithium-ion battery Aging mechanism Electrode

A comprehensive review on microchannel heat sinks for electronics cooling

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International Journal of Extreme Manufacturing 2024年第2期6卷 133-162页

作者： Zhi-Qiang Yu Mo-Tong Li Bing-Yang Cao Key Laboratory for Thermal Science and Power Engineering of Ministry of Education Department of Engineering MechanicsTsinghua UniversityBeijing 100084People’s Republic of China

The heat generation of electronic devices is increasing dramatically,which causes a serious bottleneck in the thermal management of electronics,and overheating will result in performance deterioration and even device *** the development of micro-machining technologies,the microchannel heat sink(MCHS)has become one of the best ways to remove the considerable amount of heat generated by high-power *** has the advantages of large specific surface area,small size,coolant saving and high heat transfer *** paper comprehensively takes an overview of the research progress in MCHSs and generalizes the hotspots and bottlenecks of this *** heat transfer mechanisms and performances of different channel structures,coolants,channel materials and some other influencing factors are ***,this paper classifies the heat transfer enhancement technology and reviews the related studies on both the single-phase and phase-change flow and heat *** comprehensive review is expected to provide a theoretical reference and technical guidance for further research and application of MCHSs in the future.

关键词： microchannel heat sink thermal management of electronics microscale heat transfer heat transfer enhancement

Experimental demonstration of deterministic quantum search algorithms on a programmable silicon photonic chip

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中国科学:物理学、力学、天文学英文版 2023年第9期66卷 1-7页

作者： Zhi-Hao Li Gui-Fang Yu Ya-Xin Wang Ze-Yu Xing Ling-Wen Kong Xiao-Qi Zhou State Key Laboratory of Optoelectronic materials and Technologies School of PhysicsSun Yat-sen UniversityGuangzhou 510000China Hefei National Laboratory Hefei 230088China

The Grover quantum search algorithm is a landmark quantum computing application, which has a speed advantage over classical algorithms for searching an unsorted database. For an√ unsorted database of N items, the classical algorithm needs to search O(N) times, while the Grover algorithm only needs O(√N) times. However, except for the special case of N = 4, the traditional Grover algorithm always has some probability of failure. To solve this problem, several schemes for deterministically performing quantum search have been proposed, but they all impose additional requirements on the query Oracle and cannot be implemented in many practical scenarios. Recently, Roy et al. [Phys. Rev. Res. 4, L022013(2022)] proposed a new deterministic quantum search scheme with no additional requirements on the query Oracle, which has the potential to perfectly replace the traditional Grover algorithm. In this study, we experimentally implement on a programmable silicon quantum photonic chip four deterministic quantum search algorithms, including the Roy algorithm, all of which obtained an average search success rate of over0.93, exceeding the theoretical maximum of 0.9074 that the traditional Grover algorithm can achieve. Our results demonstrate the feasibility and superiority of the deterministic quantum search algorithms and are expected to facilitate the wider application of these algorithms in future quantum information processing.

关键词： integrated photonics quantum information technology deterministic quantum search

Electrochemical scanning probe microscopies for artificial photosynthesis

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Nano Research 2023年第3期16卷 4013-4028页

作者： Chunlei Yang Tianhui Su Yanbo Hua Liming Zhang department of Chemistry iChEM(Collaborative Innovation Center of Chemistry for Energy Materials)and Shanghai Key Laboratory of Molecular Catalysis and Innovative MaterialsFudan UniversityShanghai 200438China

The rational design of efficient artificial photosynthetic components requires thorough understandings towards(photo)electrochemical properties and kinetic processes at the solid/liquid *** scanning probe microscopy(EC-SPM),which enables the high-spatial resolution imaging in an electrolyte environment,becomes an indispensable experimental technique for operando studies of(photo)*** review summarizes the latest results of relevant ECSPM techniques to study the interfacial properties of electrocatalysts and *** methods include atomic force microscopy,Kelvin probe force microscopy,conductive atomic force microscopy,scanning tunneling microscopy,scanning electrochemical microscopy,and other advanced SPM-based operando ***,we offer some perspectives on the future outlook in this fascinating research area.

关键词： (photo)electrocatalysis scanning probe microscopies scanning tunneling microscopy atomic force microscopy in-situ

Structural characterization of Nd-doped in silica host matrix prepared by wet chemical process

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Journal of Rare Earths 2009年第1期27卷 83-86页

作者： Surender Duhan Sunita Devi M.Singh materials Science Lab Department of Applied Physics Guru Jambheshwar University of Science & Technology materials Science Lab Department of Physics department of Chemistry Lajpat Rai College department of physics Amity School of Engineering and TechnologyAmity University Sec-125

Silica host matrix containing neodymium which is potentially important for the formation of nanocrystalline metal oxides was prepared by solgel method, using tetra-ethoxysilane and Nd（NO3）3 as precursor *** prepared samples were changed from amorphous to nanocrystallites phase at sintered temperature 550 °C（4 h）, 750 °C（8 h） and 950 °C（12 h）.The thermally treated sample microstructures were investigated using X-ray diffraction（XRD）, Fourier transformation infrared spectroscopy（FTIR）, and scanning electron mi-croscopy（SEM）.While a further increase of the temperature at 750 °C and annealing time（8 h） resulted in the formation of cubic and hexagonal Nd2O3 *** constant sintering temperature 950 °C for 12 h, the samples showed sharper and intense *** sizes of Nd2O3 nanocrystallites were characterized by XRD with average size ～46 nm.

关键词： rare earth oxide silica annealing/calcination nanocrystallites

A review on WO_(3)-based composite photocatalysts:synthesis,catalytic mechanism and diversified applications

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Rare Metals 2024年第8期43卷 3441-3459页

作者： Xue Zhang Zi-Qi Zhang Yan-Dong Sun Xiao-Jia Ma Feng-Xian Jin Fang-Yuan Zhang Wei-Guang Han Bo-Xiong Shen Sheng-Qi Guo College of Energy and Environmental Engineering Hebei University of TechnologyTianjin 300401China department of Food and Chemical Engineering Liuzhou Institute of TechnologyLiuzhou 545616China

Photocatalysis as an emerging "green" energy conversion technology has attracted domestic and international *** technology uses semiconductor photocatalysts to convert solar energy into directly usable chemical energy,showing great potential for application in environmental pollutant purification and clean energy production,with broad development *** many semiconductor materials,tungsten trioxide(WO_(3)) is favored by researchers in the field of photocatalysis because of its good visible light response and excellent valence band hole oxidation ***,a large number of photocatalysts based on WO_(3),in particular W03-based composite photocatalysts,have been reported,and their applications cover a wide range of *** order to promote the development of WO_(3)-based photocatalysts and provide a reference for colleagues,we present a systematic summary of the applications and research progress of W03-based composites in the field of photocatalysis in recent *** from the structural properties of WO_(3)itself,this article summarizes the preparation methods and structure-activity relationships of WO_(3)-based composite ***,it introduces the current application status of existing WO_(3)-based composite photocatalysts in CO_(2) reduction,hydrogen production,nitrogen fixation,and pollutant ***,the development prospects were analyzed.

关键词： WO_(3)-based composite photocatalysts Intrinsic characteristic Preparation method Reaction mechanism Applications

Ag-integrated mixed metallic Co-Fe-Ni-Mn hydroxide composite as advanced electrode for high-performance hybrid supercapacitors

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Journal of Energy Chemistry 2024年第1期88卷 579-591,I0013页

作者： Anki Reddy Mule Bhimanaboina Ramulu Shaik Junied Arbaz Anand Kurakula Jae Su Yu department of Electronics and Information Convergence Engineering Institute for Wearable Convergence ElectronicsKyung Hee UniversityYongin-siGyeonggi-do 17104Republic of Korea

Direct growth of redox-active noble metals and rational design of multifunctional electrochemical active materials play crucial roles in developing novel electrode materials for energy storage *** this regard,silver(Ag)has attracted great attention in the design of efficient *** by the house/building process,which means electing the right land,it lays a strong foundation and building essential columns for a complex ***,we report the construction of multifaceted heterostructure cobalt-iron hydroxide(CFOH)nanowires(NWs)@nickel cobalt manganese hydroxides and/or hydrate(NCMOH)nanosheets(NSs)on the Ag-deposited nickel foam and carbon cloth(i.e.,Ag/NF and Ag/CC)***,the formation and charge storage mechanism of Ag are described,and these contribute to good conductive and redox chemistry *** switching architectural integrity of metal and redox materials on metallic frames may significantly boost charge storage and rate performance with noticeable drop in *** as-fabricated Ag@CFOH@NCMOH/NF electrode delivered superior areal capacity value of 2081.9μA h cm^(-2)at 5 mA cm^(-2).Moreover,as-assembled hybrid cell based on NF(HC/NF)device exhibited remarkable areal capacity value of 1.82 mA h cm^(-2)at 5 mA cm^(-2)with excellent rate capability of 74.77%even at 70 mA cm^(-2)Furthermore,HC/NF device achieved maximum energy and power densities of 1.39 mW h cm^(-2)and 42.35 mW cm^(-2),*** verify practical applicability,both devices were also tested to serve as a self-charging station for various portable electronic devices.

关键词： Current collectors Redox-active silver Transition metal-hydroxides Electrochemical performance Hybrid supercapacitor

Transport in electron–photon systems

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Frontiers of physics 2023年第4期18卷 129-175页

作者： Jian-Sheng Wang Jiebin Peng Zu-Quan Zhang Yong-Mei Zhang Tao Zhu department of physics National University of SingaporeSingapore 117551Republic of Singapore Center for Phononics and Thermal Energy Science China-EU Joint Center for NanophononicsShanghai Key Laboratory of Special Artificial Microstructure Materials and TechnologySchool of Physics Science and EngineeringTongji UniversityShanghai 200092China department of physics Zhejiang Normal UniversityJinhua 321004China College of physics Nanjing University of Aeronautics and AstronauticsNanjing 210016China School of Electronic and Information Engineering Tiangong UniversityTianjin 300387China Beijing National Laboratory for Condensed Matter physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China

We review the description and modeling of transport phenomena among the electron systems coupled via scalar or vector *** consists of three *** first part is about scalar photons,i.e.,Coulomb *** second part is with transverse photons described by vector *** third part is onϕ=0 or temporal gauge,which is a full theory of the *** use the nonequilibrium Green’s function(NEGF)formalism as a basic tool to study steady-state *** with local equilibrium it is equivalent to the fluctuational electrodynamics(FE),the advantage of NEGF is that it can go beyond FE due to its *** have given a few examples in the review,such as transfer of heat between graphene sheets driven by potential bias,emission of light by a double quantum dot,and emission of energy,momentum,and angular momentum from a graphene *** of these calculations are based on a generalization of the Meir–Wingreen formula commonly used in electronic transport in mesoscopic systems,with materials properties represented by photon self-energy,coupled with the Keldysh equation and the solution to the Dyson equation.

关键词： quantum transport thermal radiation scalar and vector photons nonequilibrium Green's function

Designing electrodes and electrolytes for batteries by leveraging deep learning

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Nano Research Energy 2024年第2期3卷 83-99页

作者： Chenxi Sui Ziyang Jiang Genesis Higueros David Carlson Po-Chun Hsu Pritzker School of Molecular Engineering University of ChicagoChicagoIL 60637USA Civil and Environmental Engineering Duke UniversityDurhamNC 27708USA Thomas Lord department of Mechanical Engineering and materials Science Duke UniversityDurhamNC 27708USA

High-performance batteries are poised for electrification of vehicles and therefore mitigate greenhouse gas emissions,which,in turn,promote a sustainable ***,the design of optimized batteries is challenging due to the nonlinear governing physics and *** advancements have demonstrated the potential of deep learning techniques in efficiently designing batteries,particularly in optimizing electrodes and *** review provides comprehensive concepts and principles of deep learning and its application in solving battery-related electrochemical problems,which bridges the gap between artificial intelligence and *** also examine the potential challenges and opportunities associated with different deep learning approaches,tailoring them to specific battery ***,we aim to inspire future advancements in both fundamental scientific understanding and practical engineering in the field of battery ***,we highlight the potential challenges and opportunities for different deep learning methods according to the specific battery demand to inspire future advancement in fundamental science and practical engineering.

关键词： battery design fast-charging battery three-dimensional(3D)structure deep learning optimization