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Locally Enhanced Flow and Electric Fields Through a Tip Effect for Efficient Flow‑Electrode Capacitive Deionization

Nano-Micro Letters 2025年第2期17卷 1-17页

作者： Ziquan Wang Xiangfeng Chen Yuan Zhang Jie Ma Zhiqun Lin Amor Abdelkader Maria‑Magdalena Titirici Libo Deng College of Chemistry and environmental engineering Shenzhen UniversityShenzhen 518060People’s Republic of China Research Center for environmental Functional Materials College of Environmental Science and EngineeringTongji University1239 Siping RoadShanghai 200092People’s Republic of China department of Chemical and Biomolecular engineering National University of SingaporeSingapore 117585Singapore department of engineering Faculty of Science and TechnologyBournemouth UniversityTalbot CampusFern BarrowPooleEngland BH125BBUK Institut de Chimie de Nice UniversitéCôte d’AzurUMR CNRS 727228 Av.Valrose06108 NiceFrance department of Chemical engineering Imperial College LondonSouth Kensington CampusExhibition RdLondon SW72AZUK

Low-electrode capacitive deionization(FCDI)is an emerging desalination technology with great potential for removal and/or recycling ions from a range of ***,it still suffers from inefficient charge transfer and ion transport kinetics due to weak turbulence and low electric intensity in flow electrodes,both restricted by the current ***,a new tip-array current collector(designated as T-CC)was developed to replace the conventional planar current collectors,which intensifies both the charge transfer and ion transport *** effects of tip arrays on flow and electric fields were studied by both computational simulations and electrochemical impedance spectroscopy,which revealed the reduction of ion transport barrier,charge transport barrier and internal *** the voltage increased from 1.0 to 1.5 and 2.0 V,the T-CC-based FCDI system(T-FCDI)exhibited average salt removal rates(ASRR)of 0.18,0.50,and 0.89μmol cm^(-2) min^(-1),respectively,which are 1.82,2.65,and 2.48 folds higher than that of the conventional serpentine current collectors,and 1.48,1.67,and 1.49 folds higher than that of the planar current ***,with the solid content in flow electrodes increased from 1 to 5 wt%,the ASRR for T-FCDI increased from 0.29 to 0.50μmol cm^(-2) min^(-1),which are 1.70 and 1.67 folds higher than that of the planar current ***,a salt removal efficiency of 99.89%was achieved with T-FCDI and the charge efficiency remained above 95%after 24 h of operation,thus showing its superior long-term stability.

关键词： Flow-electrode Capacitive deionization Current collector Tip effect Desalination

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Aligned Ion Conduction Pathway of Polyrotaxane‑Based Electrolyte with Dispersed Hydrophobic Chains for Solid‑State Lithium–Oxygen Batteries

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Nano-Micro Letters 2025年第2期17卷 169-186页

作者： Bitgaram Kim Myeong‑Chang Sung Gwang‑Hee Lee Byoungjoon Hwang Sojung Seo Ji‑Hun Seo Dong‑Wan Kim department of Materials Science and engineering Korea University145 Anam‑RoSeongbuk‑GuSeoul 02841Republic of Korea School of Civil Environmental and Architectural EngineeringKorea University145 Anam‑RoSeongbuk‑GuSeoul 02841Republic of Korea Materials Science and Chemical engineering Center Institute for Advanced Engineering(IAE)Yongin 17180Republic of Korea

A critical challenge hindering the practical application of lithium–oxygen batteries(LOBs)is the inevitable problems associated with liquid electrolytes,such as evaporation and safety *** study addresses these problems by proposing a modified polyrotaxane(mPR)-based solid polymer electrolyte(SPE)design that simultaneously mitigates solvent-related problems and improves ***-SPE exhibits high ion conductivity(2.8×10^(−3)S cm^(−1)at 25℃)through aligned ion conduction pathways and provides electrode protection ability through hydrophobic chain *** this mPR-SPE into solid-state LOBs resulted in stable potentials over 300 *** situ Raman spectroscopy reveals the presence of an LiO_(2)intermediate alongside Li_(2)O_(2)during oxygen *** situ X-ray diffraction confirm the ability of the SPE to hinder the permeation of oxygen and moisture,as demonstrated by the air permeability *** present study suggests that maintaining a low residual solvent while achieving high ionic conductivity is crucial for restricting the sub-reactions of solid-state LOBs.

关键词： Solid polymer electrolyte Lithium-oxygen batteries Polyrotaxane ion conductivity Hydrophobic chain

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Distribution and contamination status of chromium in surface sediments of northern Kaohsiung Harbor, Taiwan

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Journal of environmental Sciences 2013年第7期25卷 1450-1457页

作者： Cheng-Di Dong Chiu-Wen Chen Chih-Feng Chen department of marine environmental engineering "National" Kaohsiung Marine University

Thedistribution, enrichment, accumulation, and potential ecological risk of chromium （Cr） in the surface sediments of northern Kaohsiung Harbor, Taiwan, Chinawere investigated. Sediment samples from ten locations located between the river mouths and harbor entrance of northern Kaohsiung Harborwere collected quarterly in 2011 and characterized for Cr, aluminum,water content, organic matter, total nitrogen, total phosphorous, total grease, and grain size. Results showed that the Cr concentrations varied from 27.0 to361.9 mg/kgwith an average of （113.5 ± 87.0） mg/kg. High Cr concentrationwas observed near the Jen-Gen River mouth. The mean Cr concentrationwas high at 255.5 mg/kg,whichwas at least 2 to 7 times than that of other sites. This might imply significant Cr contribution from upstream receiving tannerieswastewater into the Jen-Gen River. The spatialdistribution of Cr reveals relatively high in the river mouth region, especially in Jen-Gen River, and graduallydiminishes toward the harbor entrance region. This indicates that the major sources of Cr pollution from upstream industrial and municipalwastewatersdischarged along the river bank; and Cr maydriftwith sea current and bedispersed into open sea. Moreover, Cr concentrations correlated closely to the physical-chemical properties of the sediments,which suggested the influence of industrial and municipalwastewatersdischarged from the neighboring industrial parks and river basins. Results from the enrichment factor andgeo-accumulation index analyses imply that the Jen-Gen River sediments can be characterized as moderate enrichment and none to medium accumulation of Cr, respectively. However, results of potential ecological risk index indicate that the sediment has low ecological potential risk. The results can provide valuable information todeveloping future strategies for the management of river mouth and harbor.

关键词： accumulation chromium ecological risk enrichment sediment

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An experimental study on thermal characteristics of nanofluid with graphene and multi-wall carbon nanotubes

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Journal of Central South University 2015年第8期22卷 3202-3210页

作者： A.K.M Mahmudul Haque Sunghyun Kwon Junhyo Kim Jungpil Noh Sunchul Huh Hanshik Chung Hyomin Jeong department of Ocean System engineering Gyeongsang National University department of marine environmental engineering Gyeongsang National University department of marine engineering Mokpo National Maritime University department of Energy and Mechanical engineering Gyeongsang National UniversityInstitute of Marine Industry

High-thermal conductivity enhancement of nanofluid is one of the promising topics of the nanoscience research field. This work reports the experimental study on the preparation of graphene(GN) and multi-walled carbon nanotubes(MWCNTs) based nanofluids with the assistance of sodium dodecyl benzene sulfonate(SDBS) and sodium dodecyl sulfate(SDS) surfactants, and their thermal behaviors. The present work suggests not a solution, but a solution approach and deduces a new conclusion by trying to resolve the agglomeration problem and improve the dispersibility of nanoparticles in the base fluid. The analysis results of FESEM, thermal conductivity, diffusivity, effusivity and heat transfer coefficient enhancement ratio of nanofluid with surfactants SDS and SDBS expose strong evidence of the dispersing effect of surfactant on the making of nanofluid.

关键词： graphene carbon nanotube surfactant dispersibility thermal conductivity

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Impact of Pollutant Concentration and Particle Deposition on the Radiative Flow of Casson-Micropolar Fluid between Parallel Plates

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Computer Modeling in engineering & Sciences 2025年第1期142卷 665-690页

作者： Ghaliah Alhamzi Badr Saad T.Alkahtani Ravi Shanker Dubey Vinutha Kalleshachar Neelima Nizampatnam department of Mathematics and Statistics College of ScienceImam Mohammad Ibn Saud Islamic University(IMSIU)Riyadh11564Saudi Arabia department of Mathematics College of ScienceKing Saud UniversityRiyadh11989Saudi Arabia department of Mathematics Amity School of Applied SciencesAmity University RajasthanJaipur302002RajasthanIndia department of Studies in Mathematics Davangere UniversityDavangere577002India department of Electronics and Communication engineering Amrita School of EngineeringAmrita Vishwa VidyapeethamBengaluru560035India

Assessing the behaviour and concentration of waste pollutants deposited between two parallel plates is essential for effective environmental *** the effectiveness of treatment methods in reducing pollution scales is made easier by analysing waste discharge *** waste discharge concentration analysis is useful for assessing how effectively wastewater treatment techniques reduce pollution *** study aims to explore the Casson micropolar fluid flow through two parallel plates with the influence of pollutant concentration and thermophoretic particle *** explore the mass and heat transport features,thermophoretic particle deposition and thermal radiation are *** governing equations are transformed into ordinary differential equations with the help of suitable similarity *** Runge-Kutta-Fehlberg’s fourthfifth order technique and shooting procedure are used to solve the reduced set of equations and boundary *** integration of a neural network model based on the Levenberg-Marquardt algorithm serves to improve the accuracy of predictions and optimize the analysis of *** outcomes are displayed to analyze the characteristics of the relevant dimensionless parameters in the current *** reveal that concentration upsurges as the micropolar parameter *** concentration reduces with an upsurge in the thermophoretic *** upsurge in the external pollutant source variation and the local pollutant external source parameters enhances mass *** surface drag force declines for improved values of porosity and micropolar parameters.

关键词： Micropolar fluid thermal radiation porous medium thermophoretic particle deposition waste discharge concentration

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Numerical study on tidal currents and seawater exchange in the Benoa Bay, Bali, Indonesia

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Acta Oceanologica Sinica 2014年第3期33卷 90-100页

作者： HENDRAWAN I Gede ASAI Koji department of marine Sciences Faculty of Marine Sciences and Fisheries Udayana University department of Civil and environmental engineering Yamaguchi University

A three-dimensional （3-D） finite volume coastal ocean model （FVCOM） was used for the study of water cir culation and seawater exchange in the Benoa Bay, Bali Island. The M2 tidal component was forced in open boundary and discharge from six rivers was included in the numerical calculation. The M2 tidal elevation produced by the FVCOM has a good agreement with the observation data. The M2 tidal current is also suc cessfully calculated under the ebb tide and flood tide conditions. The non-linear M2 tidal residual current was produced by the coastline geometry, especially surrounding the narrow strait between the Serangan Is- land and the Benoa Peninsula. The tidal residual current also generated two small eddies within the bay and one small eddy in the bay mouth. The salinity distribution influenced by river discharge could be success- fully calculated, where the numerical calculation and the observation results have a good correlation （r2） of 0.75. Finally in order to examine the seawater exchange in the Benoa Bay, the Lagrangian particle tracking method and calculation of residence time are applied. The mechanism of particle transport to the flushing of seawater is depicted clearly by both methods.

关键词： FVCOM M2 tidal current M2 residual current salinity seawater exchange

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Discrete state space method and modal extension method based impact sound synthesis model

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Chinese Physics B 2018年第11期27卷 270-277页

作者： Xu-Hua Tian Ke-An Chen Yan-Ni Zhang Han Li Jian Xu department of environmental engineering School of Marine Science and Technology Northwestern Polytechnical University Xi＇an 710072 China

The efficient and accurate synthesis of physical parameter-controllable impact sounds is essential for sound source identification. In this study, an impact sound synthesis model of a cylinder is proposed based on discrete state space（DSS） method and modal extension method（MEM）. This model is comprised of the whole three processes of the physical interaction, i.e., the Hertz contact process, the transient structural response process, and the sound radiation process. Firstly,the modal expanded DSS equations of the contact system are constructed and the transient structural response of the cylinder is obtained. Then the impact sound of the cylinder is acquired using improved discrete Raleigh integral. Finally, the proposed model is verified by comparing with existing models. The results show that the proposed impact sound synthesis model is more accurate and efficient than the existing methods and easy to be extended to the impact sound synthesis of other structures.

关键词： impact sound synthesis discrete state space contact force

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Immobilization of nitrite oxidizing bacteria using biopolymeric chitosan media

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Journal of environmental Sciences 2013年第2期25卷 262-267页

作者： Pranee Lertsutthiwong Duangcheewan Boonpuak Wiboonluk Pungrasmi Sorawit Powtongsook Metallurgy and Materials Science Research Institute Chulalongkorn University department of environmental engineering Faculty of EngineeringChulalongkorn University National Center for Genetic engineering and Biotechnology Center of Excellence for marine Biotechnology Department of Marine ScienceChulalongkorn University

The effects of chitosan characteristics including the degree of deacetylation, molecular weight, particle size, pH pretreatment and immobilization time on the immobilization of nitrite-oxidizing bacteria （NOB） on biopolymeric chitosan were investigated. Nitrite removal efficiency of immobilized NOB depended on the degree of deacetylation, particle size, pH pretreatment on the surface of chitosan and immobilization time. Scanning electron microscope characterization illustrated that the number of NOB cells attached to the surface of chitosan increased with an increment of immobilization time. The optimal condition for NOB immobilization on chitosan was achieved during a 24-hr immobilization period using chitosan with the degree of deacetylation larger than 80% and various particle size ranges between 1-5 mm at pH 6.5. In general, the NOB immobilized on chitosan flakes has a high potential to remove excess nitrite from wastewater and aquaculture systems.

关键词： chitosan immobilization nitrite-oxidizing bacteria pH adjustment

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Thorium isotopes ((228)Th,(230)Th,(232)Th) and applications in reconstructing the Yangtze and Yellow River floods

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International Journal of Sediment Research 2013年第4期28卷 588-595页

作者： Wei-feng YANG Min CHEN Xin-xing ZHANG Zhi-gang GUO Guang-xue LI Qiang MA Jun-hong YANG Yi-pu Huang State Key Laboratory of marine environmental Science Xiamen University department of environmental Science and engineering Fudan University College of marine Geo-Science Ocean University of China

In the past decades,the Hoods of the Yangtze and Yellow River introduced unexpected changes of the ecological community and sedimentary dynamics in the Fast China Sea(KCS).To reconstruct the flood events in the ECS,228Th,230Th and232Th have been examined in a sediment *** specific activities of three thorium isotopes have good positive relations with line fractions(<63 urn),indicating that Th activity concentrations heavily depend upon the sediment grain *** size-normalized activities of228Th,230Th and232Th showed significant *** between the higher Th activities and historical Hoods of the Yangtze and Yellow River demonstrated that size-normalized Th recorded the two rivers’ flood *** activity ratios of thorium isotopes,i.e.230Th/232Th and228Th/232Th,also showed similar patterns to the historical river *** three periods(1740s,[840—1860s and1930- 1960s),characterized by frequent Hoods,the thorium activity ratios were fairly low and close to the Yangtze and Yellow River estuary sediments,coinciding with the less oceanic228Th and230Th contributions during the flooding ***,these results support the size-normalized Th activity and thorium ratios as proxies of the river floods in coastal seas.

关键词： Thorium Yellow River Yangtze River Flood East China Sea

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Optimization and evaluation of a bottom substrate denitrification tank for nitrate removal from a recirculating aquaculture system

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Journal of environmental Sciences 2013年第8期25卷 1557-1564页

作者： Wiboonluk Pungrasmi Cholticha Playchoom Sorawit Powtongsook department of environmental engineering Faculty of Engineering Chulalongkorn University Center of Excellence for marine Biotechnology Department of Marine Science Faculty of Science Chulalongkorn University National Center for Genetic engineering and Biotechnology National Science and Technology Development Agency

A bottom substrate denitrification tank for a recirculating aquaculture system was developed. The laboratory scale denitrification tank was an 8 L tank （0.04 m2 tank surface area）, packed to a depth of 5 cm with a bottom substrate for natural denitrifying bacteria. An aquarium pump was used for gentle water mixing in the tank; the dissolved oxygen in the water was maintained in aerobic conditions （e.g. 〉 2 mg/L） while anoxic conditions predominated only at the bottom substrate layer. The results showed that, among the four substrates tested （soil, sand, pumice stone and vermiculite）, pumice was the most preferable material. Comparing carbon supplementation using methanol and molasses, methanol was chosen as the carbon source because it provided a higher denitrification rate than molasses. When methanol was applied at the optimal COD：N ratio of 5：1, a nitrate removal rate of 4591 ± 133 mg-N/m2 tank bottom area/day was achieved. Finally, nitrate removal using an 80 L denitrification tank was evaluated with a 610 L recirculating tilapia culture system. Nitrate treatment was performed by batch transferring high nitrate water from the nitrification tank into the denitrification tank and mixing with methanol at a COD：N ratio of 5：1. The results from five batches of nitrate treatment revealed that nitrate was successfully removed from water without the accumulation of nitrite and ammonia. The average nitrate removal efficiency was 85.17% and the average denitrification rate of the denitrification tank was 6311 ± 945 mg-N/m2 tank bottom area/day or 126 ± 18 mg-N/L of pumice packing volume/day.

关键词： denitrification nitrate removal methanol pumice stone recirculating aquaculture system

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