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Magnetron sputtered nickel oxide with suppressed interfacial defect states for efficient inverted perovskite solar cells

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Journal of Energy Chemistry 2025年第1期100卷 348-355页

作者： Guoqiang Ma Qin Tan Zhaoning Li Jingwei Xiu Jiafeng Wang Tianle Cheng Dong He Qiang Sun Xuhang Ma Francesco Lamberti Zhubing He department of Materials Science and Engineering Institute of Innovative Materials (I2M) Shenzhen Key Laboratory of Full Spectral Solar Electricity Generation (FSSEG)Southern University of Science and Technology (SUSTech) Core Research Facilities Southern University of Science and Technology department of Chemical Sciences Department of Industrial Engineering University of Padova

Widely used spin-coated nickle oxide （NiOx） based perovskite solar cells often suffer from severe interfacial reactions between the NiOxand adjacent perovskite layers due to surface defect states,which inherently impair device performance in a long-term view,even with surface molecule *** this study,we developed high-quality magnetron-sputtered NiOxthin films through detailed process optimization,and compared systematically sputtered and spin-coated NiOxthin film surfaces from materials to *** sputtered NiOxfilms exhibit improved crystallinity,smoother surfaces,and significantly reduced Ni3+or Ni vacancies compared to their spin-coated ***,the interface between the perovskite and sputtered NiOxfilm shows a substantially reduced density of defect *** solar cells （PSCs） fabricated with our optimally sputtered NiOxfilms achieved a high power conversion efficiency （PCE） of up to 19.93%and demonstrated enhanced stability,maintaining 86.2% efficiency during 500 h of maximum power point tracking under one standard sun ***,with the surface modification using (4-(2,7-dibromo-9,9-dimethylacridin-10（9H）-yl)butyl)p hosphonic acid （DMAcPA）,the device PCE was further promoted to 23.07%,which is the highest value reported for sputtered NiOxbased PSCs so far.

关键词： Nickle oxide Magnetron sputter Defect Stability Perovskite solar cell

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A novel solution treatment and aging for powder bed fusion-laser beam Ti-6Al-2Sn-4Zr-6Mo alloy:Microstructural and mechanical characterization

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International Journal of Minerals,Metallurgy and Materials 2025年第2期32卷 414-424页

作者： Gianluca Pirro Alessandra Martucci Alessandro Morri Mariangela Lombardi Lorella Ceschini department of industrial Engineering(DIN) Alma Mater Studiorum-University of BolognaBologna 40136Italy department of Applied Science and Technology(DISAT) Politecnico di TorinoTorino TO 10129Italy

Ti-6Al-4Zr-2Sn-6Mo alloy is one of the most recent titanium alloys processed using powder bed fusion-laser beam(PBF-LB)*** alloy has the potential to replace Ti-6Al-4V in automotive and aerospace applications,given its superior mechanical properties,which are approximately 10%higher in terms of ultimate tensile strength(UTS)and yield strength after appropriate heat *** as-built conditions,the alloy is characterized by the presence of soft orthorhombicα″martensite,necessitating a postprocessing heat treatment to decompose this phase and enhance the mechanical properties of the ***,PBFed Ti6246 components undergo an annealing process that transforms theα″martensite into anα-βlamellar *** primary objective of this research was to develop a solution treatment and aging(STA)heat treatment tailored to the unique microstructure produced by the additive manufacturing process to achieve an ultrafine bilamellar microstructure reinforced by precipitation *** study investigated the effects of various solution temperatures in theα-βfield(ranging from 800 to 875℃),cooling media(air and water),and aging time to determine the optimal heat treatment parameters for achieving the desired bilamellar *** each heat treatment condition,differentα-βmicrostructures were found,varying in terms of theα/βratio and the size of the primaryα-phase *** attention was given to how these factors were influenced by increases in solution temperature and how microhardness correlated with the percentage of the metastableβphase present after *** tests were performed on samples subjected to the most promising heat treatment parameters.A comparison with literature data revealed that the optimized STA treatment enhanced hardness and UTS by13%and 23%,respectively,compared with those of the annealed *** surface analyses were conducted to investigate fracture mechanisms.

关键词： powder bed fusion-laser beam titanium alloys heat treatments mechanical properties fractographic analysis

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Occupational health and safety performance evaluation of countries based on MAIRCA

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International Journal of Intelligent Computing and Cybernetics 2020年第1期13卷 1-24页

作者： Gülin Feryal Can Muzaffer Bertan Kıran industrial Engineering Baskent UniversitesiAnkaraTurkey Occupational health and safety Science department Baskent UniversitesiAnkaraTurkey

Purpose-The purpose of this paper is to develop an approach to compare occupational health and safety(OHS)performances of ***,another aim is to debate the impacts of using recorded data and ratios for OHS performance ***/methodology/approach-The number of fatal accidents(NFAs),fatal accident rates(FARs),numbers of lost days(NLDs)and accident severity rates(ASRs)are determined as main criteria and six economic activity areas(EAAs)are considered as *** different initial decision matrices are used as the initial decision matrix,the first of which consists of recorded data of countries related to NFAs and NLDs,and the second consists of FAR and ASR values as *** weights of main and sub-criteria regarding the recorded data and ratios are determined using four different weighting *** are ranked via utilizing Multi-Attributive Ideal-Real Comparative Analysis considering two different initial decision ***-It can be stated that an evaluation based on ratios for comparison of OHS performance provides more realistic ***,increasing the effect of the FAR values using the 6,000 equivalent lost days factor is also important in terms of differentiating the data of the countries in ***/value-To the best of the authors’knowledge,there is no study in literature that discusses the ranking of countries by means of recorded data and ratios considering different ***,this study is a first in terms of the number of countries evaluated and the comparison of these countries according to their respective EAAs.

关键词： MAIRCA Criteria weighting Multi-criteria decision making OHS performance

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Dynamic Forecasting of Traffic Event Duration in Istanbul:A Classification Approach with Real-Time Data Integration

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Computers, Materials & Continua 2024年第8期80卷 2259-2281页

作者： Mesut Ulu Yusuf Sait Türkan Kenan Menguc Ersin Namlı Tarık Kucukdeniz Occupational health and safety department Bandirma Onyedi Eylul UniversityBalikesir10200Türkiye department of industrial Engineering Istanbul University-CerrahpasaIstanbul34320Türkiye department of industrial Engineering Istanbul Technical UniversityIstanbul34467Türkiye

Today,urban traffic,growing populations,and dense transportation networks are contributing to an increase in traffic *** incidents include traffic accidents,vehicle breakdowns,fires,and traffic disputes,resulting in long waiting times,high carbon emissions,and other undesirable *** is vital to estimate incident response times quickly and accurately after traffic incidents occur for the success of incident-related planning and response *** study presents a model for forecasting the traffic incident duration of traffic events with high *** proposed model goes through a 4-stage process using various features to predict the duration of four different traffic events and presents a feature reduction approach to enable real-time data collection and *** the first stage,the dataset consisting of 24,431 data points and 75 variables is prepared by data collection,merging,missing data processing and data *** the second stage,models such as Decision Trees(DT),K-Nearest Neighbour(KNN),Random Forest(RF)and Support Vector Machines(SVM)are used and hyperparameter optimisation is performed with *** the third stage,feature selection and reduction are performed and real-time data are *** the last stage,model performance with 14 variables is evaluated with metrics such as accuracy,precision,recall,F1-score,MCC,confusion matrix and *** RF model outperforms other models with an accuracy of 98.5%.The study’s prediction results demonstrate that the proposed dynamic prediction model can achieve a high level of success.

关键词： Traffic event duration forecasting machine learning feature reduction shapley additive explanations(SHAP)

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Numerical assessment of the influence of former mining activities and plasticity of rock mass on deformations of terrain surface

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International Journal of Mining Science and Technology 2021年第2期31卷 209-214页

作者： PawełSikora Marek Wesołowski department of Mining Faculty of MiningSafety Engineering and Industrial AutomationSilesian University of Technology44-100 GliwicePoland

This paper presents the results of numerical simulations carried out to confirm the influence of former mining activities on deformation of the mining *** assessment of deformation changes was carried out with the use of FLAC3 D program based on the finite difference *** calculations were carried out for the example of actual mining operations in seams 703/1-2 and 707/2 of‘‘Marcel"Coal *** into account the influence of the model’s plastic features and the so-called activation of a higher occurring seam in conducted simulations enabled obtaining a very good description of the measured *** on the results one may state that numerical model can be used to assess the influence of former mining activities and the direction of conducted exploitation on deformations of the mining *** factors are not recognized by geometric-integral theories commonly used for predicting the influence of mining operations on the *** results presented in this paper confirm that the applied method of simulating the phenomenon of reactivation of post-mining goafs is correct.

关键词： Rock mass Numerical modeling Post-mining Goafs Land surface deformations

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Relating soil moisture and air temperature to evapotranspiration fluxes during inter-storm periods at a Mediterranean experimental site

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Journal of Arid Land 2015年第1期7卷 27-36页

作者： Antonia LONGOBARDI Elina KHAERTDINOVA department of Civil Engineering University of Salerno department of Production safety and industrial Ecology Ufa State Aviation Technical University

The assessment of the water losses by actual evapotranspiration plays a very important role in water resources management, especially in particular environments suffering soil water stresses and water shortages. The rationales of this study are the scarcity of experimental data, the difficulties in the measurement of direct and continuous evapotranspiration fluxes, and the switching between controls by climate and soil water availability. The temporal patterns of observed soil moisture and air temperature of over three years at an experimental site in southern Italy have been analysed to investigate the relation between them and the actual evapotranspiration volume, estimated using the soil water budget method. To this end, an event-based empirical analysis has been performed, exploring the relation between the mentioned variables. One of the major findings of the explorative phase is the qualitative and quantitative identification of the switching between climate and soil water balance as the controls over actual evapotranspiration at the experimental site. This threshold process has then been modelled at the event and sub-event scale, establishing simple empirical equations to predict actual evapotranspiration losses as a function of soil water content. Multilevel-recorded data also allowed the investigation of the importance of soil depth.

关键词： evapotranspiration soil moisture event scale empirical analysis Italy

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Apparent activation energy of mineral in open pit mine based upon the evolution of active functional groups

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International Journal of Coal Science & Technology 2023年第4期10卷 77-91页

作者： Shipng Lu Jingyu Zhao Jiajia Song Jiaming Chang Chi‑Min Shu School of safety Science and Engineering Xi’an University of Science and TechnologyXi’an 710054China Shaanxi industrial Process safety and Emergency Rescue Engineering Technology Research Center Xi’an 710054ShaanxiChina department of safety Healthand Environmental EngineeringNational Yunlin University of Science and TechnologyDouliou 64002YunlinTaiwan

This study aimed to investigate the mechanism of mineral spontaneous combustion in an open pit. On the study of coal and mineral mixture in open pit mines, as well as through the specifc surface area and Search Engine Marketing (SEM) experiments, the specifc surface area and aperture characteristics of distribution of open pit coal sample and pit mineral mixture samples were analyzed. Thermal analysis experiments were used to divide the oxidation process was divided into three stages, and the thermal behavior characteristics of experimental samples were characterized. On the basis of the stage division, we explored the transfer law of the key active functional groups of the experimental samples. The apparent activation energy calculation of the key active groups, performed by combining the Achar diferential method with the Coats–Redfern integral method, microstructural and oxidation kinetic properties were revealed. The resulted showed that the mixed sample had high ash, the fxed carbon content was reduced, the specifc surface area was far lower than the raw coal, the large aperture distribution was slightly higher than the medium hole, the micropore was exceptionally low, the gas adsorption capacity was weaker than the raw coal, the pit coal sample had the exceedingly more active functional groups, easy to react with oxygen, more likely to occur naturally, and its harm was relatively large. The mixed sample contained the highest C–O–C functional group absorbance. The functional groups were mainly infuenced by the self-OH content, alkyl side chain, and fatty hydrocarbon in the sample. The main functional groups of the four-like mixture had the highest apparent activation energy, and the two reactions were higher in the low-temperature oxidation phase.

关键词： Specifc surface area Aperture distribution characteristics Thermal behavior characteristics Oxidation kinetic properties Gas adsorption capacity

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Photobiomodulation:a novel approach to promote trans-differentiation of adipose-derived stem cells into neuronal-like cells

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Neural Regeneration Research 2025年第2期20卷 598-608页

作者： Daniella Da Silva Madeleen Jansen van Rensburg Anine Crous Heidi Abrahamse Laser Research Centre Faculty of Health SciencesUniversity of JohannesburgDoornfonteinJohannesburgSouth Africa

Photobiomodulation,originally used red and near-infrared lasers,can alter cellular *** has been demonstrated that the visible spectrum at 451-540 nm does not necessarily increase cell proliferation,near-infrared light promotes adipose stem cell proliferation and affects adipose stem cell migration,which is necessary for the cells homing to the site of *** this in vitro study,we explored the potential of adipose-derived stem cells to differentiate into neurons for future translational regenerative treatments in neurodegenerative disorders and brain *** investigated the effects of various biological and chemical inducers on trans-differentiation and evaluated the impact of photobiomodulation using 825 nm near-infrared and 525 nm green laser light at 5 J/*** adipose-derived stem cells can be used in autologous grafting and photobiomodulation has been shown to have biostimulatory *** findings reveal that adipose-derived stem cells can indeed trans-differentiate into neuronal cells when exposed to inducers,with pre-induced cells exhibiting higher rates of proliferation and trans-differentiation compared with the control ***,green laser light stimulation led to notable morphological changes indicative of enhanced trans-differentiation,while near-infrared photobiomodulation notably increased the expression of neuronal *** biochemical analysis and enzyme-linked immunosorbent assays,we observed marked improvements in viability,proliferation,membrane permeability,and mitochondrial membrane potential,as well as increased protein levels of neuron-specific enolase and ciliary neurotrophic ***,our results demonstrate the efficacy of photobiomodulation in enhancing the trans-differentiation ability of adipose-derived stem cells,offering promising prospects for their use in regenerative medicine for neurodegenerative disorders and brain injuries.

关键词： differentiation inducers green photobiomodulation immortalized adipose-derived stem cell near-infrared photobiomodulation neurodegenerative disease neurogenesis photobiomodulation trans-differentiation

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Concentrations of disinfection by-products in swimming pool following modifications of the water treatment process:An exploratory study

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Journal of Environmental Sciences 2017年第8期29卷 163-172页

作者： Robert Tardif Manuel Rodriguez Cyril Catto Ginette Charest-Tardif Sabrina Simard department of Environmental and Occupational health School of Public HealthUniversité de Montréal NSERC industrial Research Chair on Drinking Water Université Laval

The formation and concentration of disinfection by-products（DBPs） in pool water and the ambient air vary according to the type of water treatment process used. This exploratory study was aimed at investigating the short-term impact of modifications of the water treatment process on traditional DBP levels（e.g., trihalomethanes（THMs）, chloramines） and emerging DBPs（e.g., Halonitromethanes, Haloketones, NDMA） in swimming pool water and/or air. A sampling program was carried to understand the impact of the following changes made successively to the standard water treatment process： activation of ultraviolet（UV）photoreactor, halt of air stripping with continuation of air extraction from the buffer tank,halt of air stripping and suppression of air extraction from the buffer tank, suppression of the polyaluminium silicate sulfate（PASS） coagulant. UV caused a high increase of Halonitromethanes（8.4 fold）, Haloketones（2.1 fold）, and THMs in the water（1.7 fold） and, of THMs in the air（1.6 fold） and contributed to reducing the level of chloramines in the air（1.6fold） and NDMA in the water（2.1 fold）. The results highlight the positive impact of air stripping in reducing volatile contaminants. The PASS did not change the presence of DBPs, except for the THMs, which decrease slightly with the use of this coagulant. This study shows that modifications affecting the water treatment process can rapidly produce important and variable impacts on DBP levels in water and air and suggests that implementation of any water treatment process to reduce DBP levels should take into account the specific context of each swimming pool.

关键词： Disinfection by-products Swimming pool UV rays Air stripping Chloramines Emerging DBPs NDMA

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Maximizing biomass utilization: An integrated strategy for coproducing multiple chemicals

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Journal of Energy Chemistry 2025年第1期100卷 180-191页

作者： Byeongchan Ahn Sua Jo Jonggeol Na J.Jay Liu Young-Ju Kim Wangyun Won department of Chemical and Biological Engineering Korea University department of Chemical Engineering (Integrated process) Kyung Hee University department of Chemical Engineering and Materials Science Ewha Womans University department of Chemical Engineering Pukyong National University Resources Engineering Plant Research department Korea Institute of Geoscience and Mineral Resources

Lignocellulosic biomass is one of the viable solutions to alleviate the global warming. However, the limited utilization of biomass majorly focused on cellulose and hemicellulose restricts the economic and environmental feasibilities. To cope with this issue, we proposed an integrated process of co-producing 1,6-hexanediol（1,6-HDO） with tetrahydrofuran and adipic acid from biomass, referred to as Strategy A. To compare the impacts of lignin upgrading and feedstock, Strategy B, which co-produces tetrahydrofuran alone, and Strategy C, which is the traditional route to produce 1,6-HDO from fossil fuels, were used. Heat networks are also designed to reduce operating costs and indirect carbon emissions due to energy consumption, saving 87% and 83% of the heat and cooling requirements, respectively, in Strategy A. The market competitiveness of Strategy A was evaluated by determining the minimum selling price through techno-economic analysis, and sustainability was thoroughly investigated by quantifying the environmental impacts through both midpoint and endpoint life-cycle assessments（LCAs）.Strategy A was found to be the most favorable both economically（USRDSCHARDOLLAR3,402/ton） and environmentally（-26.9 kg CO2eq.）. This indicates that lignin valorization is not only economically but also environmentally preferred. Finally, changes in economic and environmental feasibilities depending on economic, process, and environmental parameters were investigated using sensitivity and uncertainty analyses. The results of these analyses provide valuable insight into bio-based chemical production.

关键词： Biorefinery Carbon mitigation Climate change Global warming Lignin utilization Bioeconomy

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