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Magnetron sputtered nickel oxide with suppressed interfacial defect states for efficient inverted perovskite solar cells

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Journal of Energy Chemistry 2025年第1期100卷 348-355页

作者： Guoqiang Ma Qin Tan Zhaoning Li Jingwei Xiu Jiafeng Wang Tianle Cheng Dong He Qiang Sun Xuhang Ma Francesco Lamberti Zhubing He department of Materials Science and engineering Institute of Innovative Materials (I2M) Shenzhen Key Laboratory of Full Spectral Solar Electricity Generation (FSSEG)Southern University of Science and Technology (SUSTech) Core research Facilities Southern University of Science and Technology department of Chemical Sciences Department of Industrial Engineering University of Padova

Widely used spin-coated nickle oxide （NiOx） based perovskite solar cells often suffer from severe interfacial reactions between the NiOxand adjacent perovskite layers due to surface defect states,which inherently impair device performance in a long-term view,even with surface molecule *** this study,we developed high-quality magnetron-sputtered NiOxthin films through detailed process optimization,and compared systematically sputtered and spin-coated NiOxthin film surfaces from materials to *** sputtered NiOxfilms exhibit improved crystallinity,smoother surfaces,and significantly reduced Ni3+or Ni vacancies compared to their spin-coated ***,the interface between the perovskite and sputtered NiOxfilm shows a substantially reduced density of defect *** solar cells （PSCs） fabricated with our optimally sputtered NiOxfilms achieved a high power conversion efficiency （PCE） of up to 19.93%and demonstrated enhanced stability,maintaining 86.2% efficiency during 500 h of maximum power point tracking under one standard sun ***,with the surface modification using (4-(2,7-dibromo-9,9-dimethylacridin-10（9H）-yl)butyl)p hosphonic acid （DMAcPA）,the device PCE was further promoted to 23.07%,which is the highest value reported for sputtered NiOxbased PSCs so far.

关键词： Nickle oxide Magnetron sputter Defect Stability Perovskite solar cell

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A novel solution treatment and aging for powder bed fusion-laser beam Ti-6Al-2Sn-4Zr-6Mo alloy:Microstructural and mechanical characterization

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International Journal of Minerals,Metallurgy and Materials 2025年第2期32卷 414-424页

作者： Gianluca Pirro Alessandra Martucci Alessandro Morri Mariangela Lombardi Lorella Ceschini department of industrial engineering(DIN) Alma Mater Studiorum-University of BolognaBologna 40136Italy department of Applied Science and Technology(DISAT) Politecnico di TorinoTorino TO 10129Italy

Ti-6Al-4Zr-2Sn-6Mo alloy is one of the most recent titanium alloys processed using powder bed fusion-laser beam(PBF-LB)*** alloy has the potential to replace Ti-6Al-4V in automotive and aerospace applications,given its superior mechanical properties,which are approximately 10%higher in terms of ultimate tensile strength(UTS)and yield strength after appropriate heat *** as-built conditions,the alloy is characterized by the presence of soft orthorhombicα″martensite,necessitating a postprocessing heat treatment to decompose this phase and enhance the mechanical properties of the ***,PBFed Ti6246 components undergo an annealing process that transforms theα″martensite into anα-βlamellar *** primary objective of this research was to develop a solution treatment and aging(STA)heat treatment tailored to the unique microstructure produced by the additive manufacturing process to achieve an ultrafine bilamellar microstructure reinforced by precipitation *** study investigated the effects of various solution temperatures in theα-βfield(ranging from 800 to 875℃),cooling media(air and water),and aging time to determine the optimal heat treatment parameters for achieving the desired bilamellar *** each heat treatment condition,differentα-βmicrostructures were found,varying in terms of theα/βratio and the size of the primaryα-phase *** attention was given to how these factors were influenced by increases in solution temperature and how microhardness correlated with the percentage of the metastableβphase present after *** tests were performed on samples subjected to the most promising heat treatment parameters.A comparison with literature data revealed that the optimized STA treatment enhanced hardness and UTS by13%and 23%,respectively,compared with those of the annealed *** surface analyses were conducted to investigate fracture mechanisms.

关键词： powder bed fusion-laser beam titanium alloys heat treatments mechanical properties fractographic analysis

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Maximizing biomass utilization: An integrated strategy for coproducing multiple chemicals

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Journal of Energy Chemistry 2025年第1期100卷 180-191页

作者： Byeongchan Ahn Sua Jo Jonggeol Na J.Jay Liu Young-Ju Kim Wangyun Won department of Chemical and Biological engineering Korea University department of Chemical engineering (Integrated process) Kyung Hee University department of Chemical engineering and Materials Science Ewha Womans University department of Chemical engineering Pukyong National University Resources engineering Plant research department Korea Institute of Geoscience and Mineral Resources

Lignocellulosic biomass is one of the viable solutions to alleviate the global warming. However, the limited utilization of biomass majorly focused on cellulose and hemicellulose restricts the economic and environmental feasibilities. To cope with this issue, we proposed an integrated process of co-producing 1,6-hexanediol（1,6-HDO） with tetrahydrofuran and adipic acid from biomass, referred to as Strategy A. To compare the impacts of lignin upgrading and feedstock, Strategy B, which co-produces tetrahydrofuran alone, and Strategy C, which is the traditional route to produce 1,6-HDO from fossil fuels, were used. Heat networks are also designed to reduce operating costs and indirect carbon emissions due to energy consumption, saving 87% and 83% of the heat and cooling requirements, respectively, in Strategy A. The market competitiveness of Strategy A was evaluated by determining the minimum selling price through techno-economic analysis, and sustainability was thoroughly investigated by quantifying the environmental impacts through both midpoint and endpoint life-cycle assessments（LCAs）.Strategy A was found to be the most favorable both economically（USRDSCHARDOLLAR3,402/ton） and environmentally（-26.9 kg CO2eq.）. This indicates that lignin valorization is not only economically but also environmentally preferred. Finally, changes in economic and environmental feasibilities depending on economic, process, and environmental parameters were investigated using sensitivity and uncertainty analyses. The results of these analyses provide valuable insight into bio-based chemical production.

关键词： Biorefinery Carbon mitigation Climate change Global warming Lignin utilization Bioeconomy

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Ru/NiMnB spherical cluster pillar for highly proficient green hydrogen electrocatalyst at high current density

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Journal of Energy Chemistry 2025年第1期100卷 397-408页

作者： Md Ahasan Habib Shusen Lin Mehedi Hasan Joni Sumiya Akter Dristy Rutuja Mandavkar Jae-Hun Jeong Jihoon Lee department of Electronic engineering College of Electronics and Information Kwangwoon University

Advanced OER/HER electrocatalytic alternatives are crucial for the wide adaptation of green hydrogen ***,Ru/NiMnB spherical cluster pillar （SCP）,denoted as Ru/NiMnB,is synthesized using a combination of electro-deposition and hydrothermal *** investigation of Ru doping in the NiMnB matrix revealed significant improvements in electrocatalytic *** Ru/NiMnB SCPs demonstrate superior OER/HER activity with low overpotentials of 150 and 103 mV at 50mA/cm2in 1 M KOH,making them highly competitive with state-of-the-art ***,the Ru/NiMnB SCPs exhibit a low 2-E cell voltage of 2.80 V at ultra-high current density of 2,000 m A/cm2in 1 M KOH,outperforming the standard benchmark electrodes of RuO2||Pt/C,thereby positioning Ru/NiMnB as one of the best bifunctional *** SCPs exhibit exceptional high-current characteristics,stability and corrosion resistance,as evidenced by continuous operation at 1,000 mA/cm2high-current density for over 150 h in 6 M KOH at elevated temperatures under harsh industrial *** a small amount of Ru incorporation significantly enhances the electrocatalytic performances of NiMnB,attributed to increased active sites and improved intrinsic properties such as conductivity,adsorption/desorption capability and reaction ***,Ru/NiMnB SCPs present a promising bi-functional electrode concept for efficient green H2production.

关键词： Advanced electrocatalyst High current Corrosion resistance industrial requirement

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Developing an engineering-statistical model for estimating aerodynamic coefficients of helicopter fuselage

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Chinese Journal of Aeronautics 2017年第1期30卷 175-185页

作者： Hossein Sheikhi Abas Saghaie department of industrial engineering Science and Research Branch Islamic Azad University

The design of the geometric shape of a helicopter fuselage poses a serious challenge for designers. The most important parameter in determining the shape of the helicopter fuselage is its aerodynamic coefficients. These coefficients are determined using two methods： wind tunnel test and computational fluid dynamics（CFD） simulation. The first method is expensive, time-consuming and limited. In addition, estimates in regions away from data can be poor. The second method,due to the limitations of numerical solution, the number of nodes and the used solution, is often inaccurate. In this paper, with the aim of accelerating the design process and achieving results with reasonable engineering accuracy, an engineering-statistical model which is useful for estimating the aerodynamic coefficients was developed, which mitigated the drawbacks of these two ***, by combining CFD simulation and regression techniques, an engineering model was presented for the estimation of aerodynamic coefficients. Then, by using the data from a wind tunnel test and implementation of statistical adjustment, the engineering model was modified and an engineering-statistical model was obtained. By spending less time and cost, the final model provided the aerodynamic coefficients of a helicopter fuselage at the desired angles of attack with reasonable accuracy. Finally, three numerical examples were provided to illustrate the application of the proposed model. Comparative results demonstrate the effectiveness of the engineering-statistical model in estimating the aerodynamic coefficients of a helicopter fuselage.

关键词： Aerodynamic coefficients Computaticnal fluid dynamics (CFD) engineering-statistical model Helicopter fuselage Wind tunnel test

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Adaptive Pinpoint and Fuel Efficient Mars Landing Using Reinforcement Learning

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IEEE/CAA Journal of Automatica Sinica 2014年第4期1卷 397-411页

作者： Brian Gaudet Roberto Furfaro the research Engineer Department of Systems and Industrial EngineeringUniversity of Arizona department of Systems and industrial engineering Department of Aerospace and Mechanical EngineeringUniversity of Arizona

Future unconstrained and science-driven missions to Mars will require advanced guidance algorithms that are able to adapt to more demanding mission requirements, e.g. landing on selected locales with pinpoint accuracy while autonomously flying fuel-efficient trajectories. In this paper, a novel guidance algorithm designed by applying the principles of reinforcement learning(RL) theory is presented. The goal is to devise an adaptive guidance algorithm that enables robust, fuel efficient,and accurate landing without the need for off line trajectory generation and real-time tracking. Results from a Monte Carlo simulation campaign show that the algorithm is capable of autonomously following trajectories that are close to the optimal minimum-fuel solutions with an accuracy that surpasses that of past and future Mars missions. The proposed RL-based guidance algorithm exhibits a high degree of flexibility and can easily accommodate autonomous retargeting while maintaining accuracy and fuel efficiency. Although reinforcement learning and other similar machine learning techniques have been previously applied to aerospace guidance and control problems(e.g., autonomous helicopter control), this appears, to the best of the authors knowledge, to be the first application of reinforcement learning to the problem of autonomous planetary landing.

关键词： Trajectory Mars Mathematical model Algorithm design and analysis Space missions Atmospheric modeling Learning (artificial intelligence) Space vehicles

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Use of mesophilic and thermophilic bacteria for the improvement of copper extraction from a low-grade ore

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International Journal of Minerals,Metallurgy and Materials 2011年第2期18卷 138-143页

作者： E.Darezereshki M.Schaffie M.Lotfalian S.A.Seiedbaghery M. Ranjbar department of Mineral Processing engineering Bahonar University Energy and Environmental engineering research Center (EERC) Bahonar University department of Chemical engineering Bahonar University industrial Mining research Center (IMRC) Bahonar University Hydrometallurgy research unit R & D Center Sarcheshmeh Copper Complex

Bioleaching was examined for copper extraction from a low grade ore using mesophilic and moderate thermophilic bacteria. Five equal size columns were used for the leaching of the ore. Sulfuric acid solution with a flow rate of 3.12 L·m-2·h-1 and pH 1.5 passed through each column continuously for 90 d. In the first and the second column, bioleaching was performed without agglomeration of the ore and on the agglomerated ore, respectively. 28wt% of the copper was extracted in the first column after 40 d, while this figure was 38wt% in the second column. After 90 d, however, the overall extractions were almost the same for both of them. Bioleaching with mesophilic bacteria was performed in the third column without agglomeration of the ore and in the fourth column on the agglomerated ore. After 40 d, copper extractions in the third and the fourth columns were 62wt% and 70wt%, respectively. Copper extractions were 75wt% for both the columns after 90 d. For the last column, bioleaching was performed with moderate thermophilic bacteria and agglomerated ore. Copper extractions were 80wt% and 85wt% after 40 and 90 d, respectively. It was concluded that crushing and agglomeration of the ore using bacteria could enhance the copper extraction considerably.

关键词： bioleaching mesophilic bacteria thermopilic bacteria copper extraction agglomeration.

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High Conductivity Water Treatment Using Water Surface Discharge with Nonmetallic Electrodes

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Plasma Science and Technology 2013年第6期15卷 528-534页

作者：王小平张兴旺雷乐成 industrial Ecology and Environment research Institute Department of Chemical and Biological EngineeringZhejiang University

Although electrohydraulic discharge is effective for wastewater treatment,its application is restricted by water conductivity and limited to the treatment of low conductivity water. For high conductivity water treatment,water-surface discharge is the preferred ***. the metallic electrodes are easily corroded because of the high temperature and strong oxidative environment caused by gas phase discharge and the electrochemical reaction in *** a result. the efficiency of the water treatment might be affected and the service life of the reactor might be *** order to avoid the corrosion problem,nonmetallic electrode water-surface discharge is introduced into high conductivity water treatment in the present ***-felt and water were used as the high voltage electrode and ground electrode,respectively.A comparison of the electrical and chemical characteristics showed that nonmetallic electrode discharge maintained the discharge characteristics and enhanced the energy efficiency,and furthermore,the corrosion of metal electrodes was avoided.

关键词： high conductivity water-surface discharge nonmetallic electrode

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Ultrathin Wood Laminae–Thermoplastic Starch Biodegradable Composites

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Journal of Renewable Materials 2018年第5期6卷 493-503页

作者： Andrea Dorigato Martino Negri Alessandro Pegoretti University of Trento Department of Industrial Engineering and INSTM Research UnitVia Sommarive 938123 TrentoItaly Trees&Timber Institute CNR IVALSAI-38010 San Michele all’AdigeTrentoItaly

Novel fully biodegradable thermoplastic composite laminates reinforced with ultrathin wood laminae were prepared through a hot-pressing process by using two different thermoplastic starch(TPS)*** microstructure and physical properties of the resulting unidirectional and bidirectional laminates were *** investigated materials presented a complex microstructure,in which the porosity of the wood laminae was almost entirely occluded by the polymer *** mechanical behavior of the laminates was strongly affected by the obtained microstructure,and matrix penetration in wood pores led to biodegradable composites with elastic modulus and tensile strength higher than those of their ***,thermal welding and thermoformability tests proved how these materials possess features typical of thermoplastic materials.

关键词： Starch ultrathin wood laminae composites mechanical properties

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Dynamic Interaction Analysis of Coupled Axial-Torsional-Lateral Mechanical Vibrations in Rotary Drilling Systems

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Structural Durability & Health Monitoring 2025年第1期19卷 77-103页

作者： Sabrina Meddah Sid Ahmed Tadjer Abdelhakim Idir Kong Fah Tee Mohamed Zinelabidine Doghmane Madjid Kidouche Applied Automation Laboratory Faculty of Hydrocarbons and ChemistryUniversity of BoumerdesBoumerdes35000Algeria Institute of Electrical and Electronic engineering(IGEE) University of BoumerdesBoumerdes35000Algeria Laboratory of the Electrification of industrial Enterprises University of BoumerdesBoumerdes35000Algeria Electrical engineering department Mohamed Boudiaf University of M’silaM’sila28000Algeria department of Civil and Environmental engineering King Fahd University of Petroleum&MineralsDhahran31261Saudi Arabia Interdisciplinary research Center for Construction and Building Materials King Fahd University of Petroleum&Minerals(KFUPM)Dhahran31261Saudi Arabia

Maintaining the integrity and longevity of structures is essential in many industries,such as aerospace,nuclear,and *** achieve the cost-effectiveness of large-scale systems in petroleum drilling,a strong emphasis on structural durability and monitoring is *** study focuses on the mechanical vibrations that occur in rotary drilling systems,which have a substantial impact on the structural integrity of drilling *** study speciﬁcally investigates axial,torsional,and lateral vibrations,which might lead to negative consequences such as bit-bounce,chaotic whirling,and high-frequency *** events not only hinder the efﬁciency of drilling but also lead to exhaustion and harm to the system’s components since they are difﬁcult to be detected and controlled in real *** study investigates the dynamic interactions of these vibrations,speciﬁcally in their high-frequency modes,usingﬁeld data obtained from measurement while ***ﬁndings have demonstrated the effect of strong coupling between the high-frequency modes of these vibrations on drilling sys-tem *** obtained results highlight the importance of considering the interconnected impacts of these vibrations when designing and implementing robust control ***,integrating these compo-nents can increase the durability of drill bits and drill strings,as well as improve the ability to monitor and detect ***,by exploiting theseﬁndings,the assessment of structural resilience in rotary drilling systems can be ***,the study demonstrates the capacity of structural health monitoring to improve the quality,dependability,and efﬁciency of rotary drilling systems in the petroleum industry.

关键词： Rotary drilling systems mechanical vibrations structural durability dynamic interaction analysis ﬁeld data analysis

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