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Maximizing biomass utilization: An integrated strategy for coproducing multiple chemicals

Journal of Energy Chemistry 2025年第1期100卷 180-191页

作者： Byeongchan Ahn Sua Jo Jonggeol Na J.Jay Liu Young-Ju Kim Wangyun Won department of Chemical and Biological Engineering Korea University department of Chemical Engineering (Integrated process) Kyung Hee University department of Chemical Engineering and Materials Science Ewha Womans University department of Chemical Engineering Pukyong National University resources Engineering Plant Research department Korea Institute of Geoscience and Mineral Resources

Lignocellulosic biomass is one of the viable solutions to alleviate the global warming. However, the limited utilization of biomass majorly focused on cellulose and hemicellulose restricts the economic and environmental feasibilities. To cope with this issue, we proposed an integrated process of co-producing 1,6-hexanediol（1,6-HDO） with tetrahydrofuran and adipic acid from biomass, referred to as Strategy A. To compare the impacts of lignin upgrading and feedstock, Strategy B, which co-produces tetrahydrofuran alone, and Strategy C, which is the traditional route to produce 1,6-HDO from fossil fuels, were used. Heat networks are also designed to reduce operating costs and indirect carbon emissions due to energy consumption, saving 87% and 83% of the heat and cooling requirements, respectively, in Strategy A. The market competitiveness of Strategy A was evaluated by determining the minimum selling price through techno-economic analysis, and sustainability was thoroughly investigated by quantifying the environmental impacts through both midpoint and endpoint life-cycle assessments（LCAs）.Strategy A was found to be the most favorable both economically（USRDSCHARDOLLAR3,402/ton） and environmentally（-26.9 kg CO2eq.）. This indicates that lignin valorization is not only economically but also environmentally preferred. Finally, changes in economic and environmental feasibilities depending on economic, process, and environmental parameters were investigated using sensitivity and uncertainty analyses. The results of these analyses provide valuable insight into bio-based chemical production.

关键词： Carbon capture and utilization

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Atmospheric reductive catalytic fractionation of lignocellulose integrated with one-pot catalytic conversion of carbohydrate yielding valuable lignin monomers and platform chemicals from corn straw

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Green Energy & Environment 2025年第1期10卷 161-172页

作者： Meng-Ying Liu Zhe-Hui Zhang Xue-Qi Wang Qian Sun Chen Zhang Yu Li Zhuohua Sun Katalin Barta Feng Peng Tong-Qi Yuan State Key Laboratory of Efficient Production of forest resources Beijing Forestry UniversityBeijing100083China Beijing Key Laboratory of Lignocellulosic Chemistry Beijing Forestry UniversityBeijing100083China department of Chemistry Organic and Bioorganic ChemistryUniversity of GrazHeinrichstrasse 28/II8010 GrazAustria

Developing a cost-effective and environmentally friendly process for the production of valuable chemicals from abundant herbal biomass receives great attentions in recent ***,taking advantage of the“lignin first”strategy,corn straw is converted to valuable chemicals including lignin monomers,furfural and 5-methoxymethylfurfural via a two steps *** key of this research lies in the development of a green and low-cost catalytic process utilizing magnetic Raney Ni catalyst and high boiling point ethylene *** utilization of neat ethylene glycol as the sole slovent under atmospheric conditions obviates the need for additional additives,thereby facilitating the entire process to be conducted in glass flasks and rendering it highly convenient for scaling *** the initial step,depolymerization of corn straw lignin resulted in a monomer yield of 18.1 wt%.Subsequently,in a dimethyl carbonate system,the carbohydrate component underwent complete conversion in a one-pot process,yielding furfural and 5-methoxymethylfurfural as the primary products with an impressive yield of 47.7%.

关键词： Atmospheric reductive catalytic fractionation Corn straw Ethylene glycol Raney Ni 5-Methoxymethylfurfural

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Wetland and habitat dynamics in the evolving landscape of the Middle Yangtze River Basin

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Journal of Geographical Sciences 2025年第1期35卷 88-111页

作者： YANG Peng SUN Kaiya ZHU Yanchao XIA Jun HUANG Heqing SONG Jingxia SHI Xiaorui LU Xixi Hubei Key Laboratory of Regional Ecology and environmental Change School of Geography and Information Engineering China University of Geosciences department of Geography National University of Singapore State Key Laboratory of Water resources and Hydropower Engineering Science Wuhan University

Wetlands play a critical role in the global environment. The Middle Yangtze River Basin(MYRB), known for its abundant wetland resources, has experienced notable changes resulting from the complex interplay of environmental factors. Therefore, we investigated the spatiotemporal characteristics of wetland ecological quality in the MYRB from 2001 to *** the random forest(RF) regression algorithm and patch-generated land-use simulation(PLUS) model, we forecasted variations in wetland habitat quality and their determinants under the Shared Socioeconomic Pathway-Representative Concentration Pathway(SSPRCP) framework from 2035 to 2095. The main findings are as follows:(1) The RF algorithm was optimal for land-use and land-cover(LULC) classification in the MYRB from 2001 to 2020,when notable changes were observed in water bodies and buildings. However, the forested area exhibited an increase and decrease of 3.9% and 1.2% under the SSP1-2.6 and SSP5-8.5 scenarios, respectively, whereas farmland exhibited a diminishing trend.(2) Wetlands were primarily concentrated in the central and eastern MYRB, with counties in the southwest exhibiting superior ecological-environmental quality from 2001 to 2020. Notably,wetland coverage revealed significantly high level, significant changes, frequent but relatively minor changes under the SSP1-2.6, SSP2-4.5, and SSP 5-8.5 scenarios, respectively.(3)Regions with lower habitat quality were primarily concentrated in urbanized areas characterized by frequent human activities, indicating a clear degradation in habitat quality across different scenarios. In conclusion, we established a foundational framework for future investigations into the eco-hydrological processes and ecosystem quality of watersheds.

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Smart Cellulose‑Based Janus Fabrics with Switchable Liquid Transportation for Personal Moisture and Thermal Management

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Nano-Micro Letters 2025年第1期17卷 333-347页

作者： Jianfeng Xi Yanling Lou Liucheng Meng Chao Deng Youlu Chu Zhaoyang Xu Huining Xiao Weibing Wu Jiangsu Co‑Innovation Center of Efficient Processing and Utilization of forest resources International Innovation Center for Forest Chemicals and MaterialsJiangsu Provincial Key Lab of Sustainable Pulp and Paper Technology and Biomass MaterialsNanjing Forestry UniversityNanjing 210037People’s Republic of China College of Materials Science and Engineering Nanjing Forestry UniversityNanjing 210037People’s Republic of China department of Chemical Engineering University of New BrunswickFrederictonNB E3B 5A3Canada Macromolecular Chemistry and Bavarian Polymer Institute University of BayreuthBayreuth 95440Germany

The Janus fabrics designed for personal moisture/thermal regulation have garnered significant attention for their potential to enhance human ***,the development of smart and dynamic fabrics capable of managing personal moisture/thermal comfort in response to changing external environments remains a ***,a smart cellulose-based Janus fabric was designed to dynamically manage personal moisture/*** cotton fabric was grafted with N-isopropylacrylamide to construct a temperature-stimulated transport ***,hydrophobic ethyl cellulose and hydrophilic cellulose nanofiber were sprayed on the bottom and top sides of the fabric to obtain wettability *** fabric exhibits anti-gravity directional liquid transportation from hydrophobic side to hydrophilic side,and can dynamically and continuously control the transportation time in a wide range of 3–66 s as the temperature increases from 10 to 40℃.This smart fabric can quickly dissipate heat at high temperatures,while at low temperatures,it can slow down the heat dissipation rate and prevent the human from becoming too *** addition,the fabric has UV shielding and photodynamic antibacterial properties through depositing graphitic carbon nitride nanosheets on the hydrophilic *** smart fabric offers an innovative approach to maximizing personal comfort in environments with significant temperature variations.

关键词： Directional water transport Cotton fabric Anti-gravity directional liquid transportation Janus wettability

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Nature Experience, Recreation Activity and Health Benefits of Visitors in Mountain and Urban forests in Vienna, Zurich and Freiburg

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Journal of Mountain Science 2015年第6期12卷 1551-1561页

作者： Ju-hyoung LEE Duk-jae LEE department of forest resources Faculty of Natural Resources Yeungnam University department of forest resources College of Life & Environmental Science Daegu University

Mountain forests are managed for various purposes. Of these, recreation, leisure, and ecotourism are increasingly gaining prominence. Yet, with the development of new techniques for creating and managing urban forests, the perception of the public with regard to mountain forests and such urban forests is narrowing. For the purpose of this study, eight mountain forests and urban forests located in Zurich(Switzerland), Vienna(Austria) and Freiburg(Germany) were shortlisted. These places are renowned for their well-functioning management of mountain forests and creation of urban forests. As the study was to focus on the comparison of the perceptions of visitors in terms of their satisfaction in urban and mountain forests, the interview covered the following questions:(i) how satisfactory was the nature experience;(ii) how satisfactory were the outdoor recreational activities;(iii) whether the nature experiences influenced the mental and physical health of visitors. Responses thus received for each of the mountain forests and urban forests were assessed, with the total number of respondents being 247. Tourists visiting the selected areas were randomly chosen for a one-on-one interview survey. Results of the survey show that there is a clear perceptions of visitors differed between urban and mountain forests. However, the gap is insignificant or almost nonexistent with respect to satisfaction level of outdoor recreational activities and health benefits. These results are contrary to the findings of previous studies, which argued that the natural landscape of mountain areas is superior to other artificially built green spaces. Visitors did not perceive significant differences in outdoor recreational activities and health effects between the two spaces.

关键词： Europe Satisfaction Outdoor recreation Interview survey Preference

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Small modifications of endo-functionalized cavities lead to large changes in molecular interaction in water

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Science China Chemistry 2025年第1期68卷 369-376页

作者： Song-Meng Wang Hao Nian Yan-Fang Wang Li-Shuo Zheng Yu-Tao Zheng Yi-Wei Dong Liping Huang Xiaoping Wang Wei Jiang Liu-Pan Yang department of Chemistry Southern University of Science and Technology School of Chemistry and Pharmaceutical Sciences State Key Laboratory for Chemistry and Molecular Engineering of Medicinal ResourcesGuangxi Normal University School of Pharmaceutical Science Hengyang Medical School University of South China

Studying molecular recognition in aqueous environments is crucial for understanding biological processes. Herein, we present a series of N-doped endo-functionalized anthracene-based cavities by introducing inward-directed pyridine units. The subtle modifications can significantly affect the binding properties of these receptors, which is similar to the mutations in biological systems. Combining theoretical calculations and molecular recognition experiments demonstrated that these “mutations” have an impact on the hydrophobicity and charge distribution of the hosts, consequently significantly influencing molecular *** is crucial for understanding the intricate mechanisms of molecular-level interactions in biological receptors.

关键词： host-guest interaction hydrophobic effect endo-functionalized cavity mutation pyridine

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Effects of Trichoderma harzianum YC_(459) and soil types on seed germination and seedling growth in rock slope restoration

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Journal of Mountain Science 2018年第4期15卷 730-737页

作者： MA Hoseop ETTAGBOR Hans Enukwa KIM Choonsig department of forest environmental resources Institute of Agriculture and Life Science Gyeongsang National University department of forest resources Gyeongnam National University of Science and Technology

We carried out experiments with various concentrations of Trichoderma harzianum YC459 in different soil types(forest soil, mixed soil,merchantable soil, and leaf mold soil) to evaluate its effect on seed germination and seedling establishment of four species(Festuca arundinacea Schreb., Dianthus barbatus var. asiaticus Nakai,Lespedeza cyrtobotrya Miq., and Parthenocissus tricuspidata Planch) for rock slope restoration. We also investigated the use of drilled slanted holes on the rock slopes for seedling establishment. The results showed that T. harzianum concentration had significant effects on seed germination, seedling growth, and seedling survival for all the species with different soil types. Seed germination and survival rates peaked at 5% T. harzianum concentration with leaf mold soil and decreased as T. harzianum concentration increased from 5% to 10%. Seedling survival rates of all four species were generally lowest at 0% T. harzianum concentration in all soil *** height of F. arundinacea and L. cyrtobotrya peaked at 5% T. harzianum concentration whereas that of D. barbatus and P. tricuspidata peaked at 10%T. harzianum concentration. We concluded that 5% T. harzianum concentration with leaf mold soil is appropriate for seed germination and seedling survival rates of most species, thus enhancing seedling establishment. Practical application of the findings of this study will contribute in the vegetation restoration of steep rocks in mountain environments.

关键词： Dianthus barbatus Drilled holes Festuca arundinacea Lespedeza cyrtobotrya Seedling establishment Seedling survival

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Changes and development plans in the mountain villages of South Korea:Comparison of the first and second national surveys

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Journal of Mountain Science 2017年第8期14卷 1473-1489页

作者： Hag Mo KANG Hyun KIM Chang Heon LEE Chong Kyu LEE Soo Im CHOI department of forest environmental Science Chonbuk National University Jeollabuk-do forest Environment Research Institute department of forest resources Gyeongnam National University of Science and Technology department of forest resources Sunchon National University

Owing to the geographic disadvantages of mountain villages, the social, cultural, and economic conditions of mountain villagers are inferior to those of urban dwellers in South Korea. Thus, in 1995, the The government of South Korea launched a mountain village development support program to promote agriculture and forestry, balance national land development, and preserve cultural heritage. The program was effectively implemented, improving the income, population size, and living conditions of villagers in addition to setting up a system for stable project implementation. However, concerns were raised about long-term development planning, the creation and marketing of specialty brands, facility management/operation, and follow-up support. The government conducted surveys of mountain villagers in 2003 and 2014, obtaining basic data to address these issues. This study evaluates the outcomes of these two surveys, suggesting areas requiring focusedaction, concentrating on village development projects, forest resource distribution and use, demographic trends, the economy, exchange with urban areas, green tourism, and master planning. We find that despite growth in the forest labor force, forest ownership is diminishing in terms of the number and scale of holdings. Consequently, it is necessary to commercialize forest resources, establish favorable settlement conditions, and expand government support for village-run projects. In addition, systematic forest management for older tree age classes would benefit the public and provide assets for future mountain village development. Our results are expected to provide baseline information for the establishment and efficient implementation of mountain village development policy.

关键词： forest resources management Mountain village changes Mountain village economy Support for mountain villages Urban-rural exchange

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A structural relationship between place attachment and intention to conserve landscapes–a case study of Harz National Park in Germany

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Journal of Mountain Science 2017年第5期14卷 998-1007页

作者： Dukjae LEE Ju-Hyoung LEE department of forest resources University of Daegu department of forest resources Yeungnam University

Place attachment is an important motivation for people to spend more time outdoors and to protect *** study explores visitors' intention to conserve natural landscapes based on the relationship with their place attachment to National Park landscape. Structural equation modelling(SEM) was used to determine the relationship between landscape conservation and place attachment. A survey with a structured questionnaire was administered to visitors to the seven designated hiking courses of Harz National Park in Germany. The path coefficient of 0.77 revealed that place dependence positively and significantly affected place attachment, whereas place identity did not. Place attachment had a significant effect on both affective appraisals and visiting satisfaction. Higher place attachment led to higher emotional reaction to landscapes on site and higher satisfaction of visiting the park. Among the variables, visiting satisfaction, but not affective appraisals, played a statistically significant mediating role between place attachment and conservation intention. With a path coefficient of 0.86, conservation intention was highly affected by visiting satisfaction. These results suggest that the managers of National Parks should focus on increasing visiting satisfaction based on how visitors are emotionally bonded with their visiting places, in order to enhance the intentions to conserve the landscape of the visitors to National Parks.

关键词： Place attachment Sense of place Mountain forests Structural Equation Model Landscape preference

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Below-ground growth characteristics of 13-year-old Pinus densiflora on different contour conditions in a post-fire plantation in Samcheuk,Korea

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Journal of forestry Research 2017年第5期28卷 1007-1018页

作者： Do-Hyun Kim Sung-Jun Na Sea-Hyun Kim Ewane Basil Ewane Dae-Bong Kang Do-Hyung Lee department of forest resources Yeungnam University department of forest Genetic resources National Institute of Forest Science

We estimated the growth volume of artificially reforested Pinus densiflora in a post-fire area on three different contour conditions by comparing and analyzing the vertical and horizontal distributions of below-ground roots on each contour. The main roots at the south-facing slope (SS) developed in a long and straight form, and those on the north-facing slope (NS) in a twisted form. The side roots developed more than the main roots on the Ridge. The depth of taproots decreased in the following order: SS > NS > Ridge. The roots on the SS developed in a pile-form root structure whereas those in the Ridge and NS developed concentrically near the root collar. The amount of root development decreased in the following order: SS > NS > Ridge. The ratio of fine roots from the whole-root development decreased in the following order: Ridge > SS > NS. These results can guide considerations of growth differences according to the planting contour conditions for future establishment of P. densiflora artificial plantations.

关键词： Pinus densiflora Growth characteristics Contour conditions Post-fire plantation Wildfire Restoration Soil depth

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