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3D bioprinting of in vitro porous hepatoma models:establishment,evaluation,and anticancer drug testing

Bio-Design and Manufacturing 2024年第2期7卷 137-152页

作者： Xiaoyuan Wang Zixian Liu Qianqian Duan Boye Zhang Yanyan Cao Zhizhong Shen Meng Li Yanfeng Xi Jianming Wang Shengbo Sang Shanxi Key Laboratory of Micro Nano Sensors and Artificial Intelligence Perception College of Electronic Information and Optical EngineeringTaiyuan University of TechnologyTaiyuan 030024China Key Lab of Advanced Transducers and Intelligent Control System of the Ministry of Education Taiyuan University of TechnologyTaiyuan 030024China Shanxi Institute of 6D Artificial Intelligence Biomedical Science Taiyuan 030031China Shanxi-Zheda Institute of Advanced Materials and Chemical engineering Taiyuan 030024China department of Pathology Shanxi Provincial Cancer HospitalTaiyuan 030024China General Hospital of taiyuan Iron and Steel Company Taiyuan 030809China

Traditional tumor models do not tend to accurately simulate tumor growth in vitro or enable personalized treatment and are particularly unable to discover more beneficial targeted *** address this,this study describes the use of threedimensional(3D)bioprinting technology to construct a 3D model with human hepatocarcinoma SMMC-7721 cells(3DP-7721)by combining gelatin methacrylate(GelMA)and poly(ethylene oxide)(PEO)as two immiscible aqueous phases to form a bioink and innovatively applying fluorescent carbon quantum dots for long-term tracking of *** GelMA(10%,mass fraction)and PEO(1.6%,mass fraction)hydrogel with 3:1 volume ratio offered distinct pore-forming characteristics,satisfactorymechanical properties,and biocompatibility for the creation of the 3DP-7721 *** analysis and quantitative real-time fluorescence polymerase chain reaction(PCR)were used to evaluate the biological properties of the *** with the two-dimensional culture cell model(2D-7721)and the 3D mixed culture cell model(3DM-7721),3DP-7721 significantly improved the proliferation of cells and expression of tumor-related proteins and ***,we evaluated the differences between the three culture models and the effectiveness of antitumor drugs in the three models and discovered that the efficacy of antitumor drugs varied because of significant differences in resistance proteins and genes between the three *** addition,the comparison of tumor formation in the three models found that the cells cultured by the 3DP-7721 model had strong tumorigenicity in nude *** evaluation of the levels of biochemical indicators related to the formation of solid tumors showed that the 3DP-7721 model group exhibited pathological characteristics of malignant tumors,the generated solid tumors were similar to actual tumors,and the deterioration was *** research therefore acts as a foundation for the application of 3DP-7721 models in drug devel

关键词： 3D bioprinting Hepatoma tumor models Drug screening Antitumor drug development

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Versatile and controlled quantum teleportation network

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Chinese Physics B 2024年第3期33卷 415-423页

作者：周瑶瑶梅鹏娴刘艳红吴量李雁翔闫智辉贾晓军 department of Physics Taiyuan Normal UniversityJinzhong 030619China College of information engineering Shanxi Vocational University of Engineering Science and TechnologyJinzhong 030619China Shanxi North Machinery Manufacturing Co. LtdTaiyuan 030000China State Key Laboratory of Quantum Optics and Quantum Optics Devices Institute of Opto-ElectronicsShanxi UniversityTaiyuan 030006China Collaborative Innovation Center of Extreme Optics Shanxi UniversityTaiyuan 030006China

A quantum teleportation network involving multiple users is essential for future quantum *** far,controlled quantum teleportation has been demonstrated in a three-user ***,versatile and controlled quantum teleportation network involving more users is in demand,which satisfies different combinations of users for practical *** we propose a highly versatile and controlled teleportation network that can switch among various combinations of different *** use a single continuous-variable six-partite Greenberger-Horne-Zeilinger(GHZ)state to realize such a task by choosing the different measurement and feedback *** controlled teleportation network,which includes one sub-network,two sub-networks and three sub-networks,can be realized for different application of user ***,the coherent feedback control(CFC)can manipulate and improve the teleportation *** approach is flexible and scalable,and would provide a versatile platform for demonstrations of complex quantum communication and quantum computing protocols.

关键词： quantum teleportation coherent feedback control versatile controlled transformation

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Immobilizing Triphenylamine with Photoredox Inert Sr^(2+)Forming Sr-MOF with Controlled electron Migration for Photocatalytic Oxidation of Thiols to Disulfides

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Chinese Journal of Chemistry 2024年第10期42卷 1093-1099页

作者： Ying-Xia Wang Fang Zheng Dong-Xia Song Bao-Yue Niu Lu-Qian Deng Xian-Ming Zhang Key Laboratory of Magnetic Molecules and Magnetic information Materials(Ministry of Education) Schoolof Chemistry and Materials ScienceShanxi Normal UniversityTaiyuanShanxi 030006China Key Laboratory of Interface Science and engineering in Advanced Material(Ministry of Education) College of ChemistryTaiyuan University of TechnologyTaiyuanShanxi 030024China

The photocatalytic oxidative coupling of thiols is one of the most popular methods to synthesize the *** and its derivatives(TPAs)are promising for the above reaction,but suffer from the easy polymerization and difficult *** overcome these obstacles while controlling the photogenerated electrons transfer directly to target substrates,herein,we constructed one TPA-based metal-organic framework(MOF),(Me_(2)NH_(2))[Sr(TCBPA)]·DMA·3H_(2)O(1),by direct self-assembly of tris(4′-carboxybiphenyl)amine(H_(3)TCBPA)and photoredox inert strontium ion(Sr^(2+)).DFT calculations revealed that the valence band maximum(VBM)and the conduction band minimum(CBM)are mainly located on TCBPA^(3-),successfully inhibiting the undesirable electron migration to metal *** results indicated that 1 displays superior performance than homogeneous H_(3)TCBPA,which may result from the abundant π…π and C—H…π interactions between the well-arranged TCBPA^(3-)and the build-in electric field between the anionic framework and the Me_(2)NH^(2+).This work highlights that immobilizing TPAs into MOFs is one promising approach to designing heterogeneous photocatalysts for the synthesis of disulfides by oxidative coupling of thiols.

关键词： Triphenylamine Metal-organic frameworks Strontium Photooxidation Thiols Disulfides

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A topology optimization for finite 1D phononic structures with objective function involving tangential derivative quantities using TDBIE

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Acta Mechanica Sinica 2024年第7期40卷 122-136页

作者： Haifeng Gao Jianguo Liang Jianglin Liu Yinhui Li Haojie Lian Toshiro Matsumoto College of Mechanical and Vehicle engineering Taiyuan University of TechnologyTaiyuan 030000China Shanxi-Zheda Institute of Advanced Materials and Chemical engineering Taiyuan 030000China College of electronic information and Optical engineering Taiyuan University of TechnologyTaiyuan 030000China Key Laboratory of In-situ Property-improving Mining of Ministry of Education Taiyuan University of TechnologyTaiyuan 030000China department of Mechanical System Nagoya UniversityNagoya 464-8604Japan

The paper proposes a topology optimization method for 1D phononic structures to minimize the tangential component of particle velocity at the objective *** tangential derivative of the boundary integral equation(TDBIE)is employed for the evaluation of the objective function involves the tangential derivative *** topological derivative is derived through the adjoint method and the Neumann boundary condition of the adjoint field is obtained using the *** average topological derivative which is obtained by calculating the average value of the topological derivative in each layer of design domains,is employed for the updating of the level set *** implementations demonstrate the proposed method is effective for the design of the 1D phononic crystals with the objective function involving tangential derivative quantities.

关键词： Boundary element method Topology optimization Phononic structures Tangential derivative

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Emergent topological ordered phase for the Ising-XY model revealed by cluster-updating Monte Carlo method

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Chinese Physics B 2024年第4期33卷 386-400页

作者：马赫阳张万舟田彦婷丁成祥邓友金 College of Physics Taiyuan University of TechnologyTaiyuan 030024China Hefei National Laboratory for Physical Sciences at the Microscale and department of Modern Physics University of Science and Technology of ChinaHefei 230026China School of Microelectronics&Data Science Anhui University of TechnologyMaanshan 243002China Minjiang Collaborative Center for Theoretical Physics College of Physics and Electronic Information EngineeringMinjiang UniversityFuzhou 350108China Shanghai Research Center for Quantum Sciences Shanghai 201315China

The two-component cold atom systems with anisotropic hopping amplitudes can be phenomenologically described by a two-dimensional Ising-XY coupled model with spatial *** low temperatures,theoretical predictions[***.A 72053604(2005)]and[arXiv:0706.1609]indicate the existence of a topological ordered phase characterized by Ising and XY disorder but with 2XY ***,due to ergodic difficulties faced by Monte Carlo methods at low temperatures,this topological phase has not been numerically *** propose a linear cluster updating Monte Carlo method,which flips spins without rejection in the anisotropy limit but does not change the *** this scheme and conventional Monte Carlo methods,we succeed in revealing the nature of topological phases with half-vortices and domain *** the constructed global phase diagram,Ising and XY-type transitions are very close to each other and differ significantly from the schematic phase diagram reported *** also propose and explore a wide range of quantities,including magnetism,superfluidity,specific heat,susceptibility,and even percolation susceptibility,and obtain consistent and reliable ***,we observed first-order transitions characterized by common intersection points in magnetizations for different system sizes,as opposed to the conventional phase transition where Binder cumulants of various sizes share common *** critical exponents of different types of phase transitions are reasonably *** results are useful to help cold atom experiments explore the half-vortex topological phase.

关键词： topological phase transition Ising-XY model Monte Carlo method half vortex

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An efficient and mild recycling of waste melamine formaldehyde foams by alkaline hydrolysis

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Green Energy & Environment 2024年第5期9卷 919-926页

作者： Shaodi Wu Ning Zhang Chizhou Wang Xianglin Hou Jie Zhao Shiyu Jia Jiancheng Zhao Xiaojing Cui Haibo Jin Tiansheng Deng Shanxi engineering Research Center of Biorefinery Institute of Coal ChemistryChinese Academy of Sciences27 South Taoyuan RoadTaiyuan030001China Center of Materials Science and Optoelectronics engineering University of Chinese Academy of SciencesBeijing100049China department of Chemistry and Chemical engineering Taiyuan Institute of TechnologyTaiyuanShanxi030008China Beijing Key Laboratory of Fuels Cleaning and Advanced Catalytic Emission Reduction technology/College of New Materials and Chemical engineering Beijing Institute of Petrochemical TechnologyBeijing102617China

Melamine formaldehyde foam(MFF)generates many poisonous chemicals through the traditional recycling methods for organic resin ***,a high MFF degradation ratio of ca.97 wt.%was achieved under the mild conditions(160℃)in a NaOH–H2O system with ammelide and ammeline as the main degradation *** alkaline solvent had an obvious corrosion effect for MFF,as indicated by scanning electron microscopy(SEM).The reaction process and products distribution were studied by Fourier-transform infrared spectroscopy(FTIR),X-ray photoelectron spectroscopy(XPS),and ^(13)C nuclear magnetic resonance(NMR).Besides,the MFF degradation products that have the similar chemical structures and bonding performances to those of melamine can be directly used as the raw material for synthesis of melamine urea-formaldehyde resins(MUFs).Moreover,the degradation system demonstrated here showed the high degradation efﬁciency after reusing for 7 *** degradation process generated few harmful pollutants and no pre-or post-treatments were required,which proves its feasibility in the safe removal or recovery of waste MFF.

关键词： Melamine formaldehyde foam Degradation Alkaline hydrolysis Recycling

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Prominent removal of trace lead(Ⅱ)ions from polluted water by terephthalic acid reformed Al/Zn metal organic nanoflakes

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Particuology 2024年第1期84卷 81-88页

作者： Junhua Li Lingshu Gao Junmao Hong Xiaofeng Shi Sifang Kong Jingyu Wang Hassan Algadi Benbin Xu Zhanhu Guo School of Chemistry and Chemical engineering North University of ChinaTaiyuan030051China School of Traffic&Environment Shenzhen Institute of Information TechnologyShenzhen518172China department of Electrical engineering Faculty of EngineeringNajran UniversityNajran11001Saudi Arabia Mechanical and Construction engineering Faculty of Engineering and EnvironmentNorthumbria UniversityNewcastle Upon TyneNE18STUK

Terephthalic acid reformed Al/Zn metal organic nanoflake was prepared and functionalized with trie-thylamine(T-AlZn).Without adding terephthalic acid,there was no product of metal organic nanoflake.T-AlZn has a remarkable performance in removing trace lead(Ⅱ)ions(Pb^(2+)).The adsorption equipoise with the removal rate≥97%was reached within 35 *** removal rates of T-AlZn for Pb^(2+)declined by only 16.73%after four *** adsorption of T-AlZn for Pb^(2+)follows the Langmuir isotherms model and pseudo-second-order dynamics *** utmost adsorption competence was calculated as 215.27 mg g^(-1).The T-AlZn adsorbent exhibits a bright prospect in the adsorption for Pb^(2+)and is a considerable candidate in the disposal of industrial sewage.

关键词： Metal organic complex Nanoflake Trace level Pb^(2+) Adsorption

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Mn-based MXene with high lithium-ion storage capacity

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Nano Research 2024年第5期17卷 4181-4191页

作者： Yanyan Wu Dongqing Liu Xiaonan Wang Usman Ghani Muhammad Asim Mushtaq Jinfeng Yang Huarui Sun Panagiotis Tsiakaras Xingke Cai School of Science and Ministry of Industry and information technology Key Laboratory of Micro-Nano Optoelectronic information System Harbin Institute of Technology ShenzhenShenzhen 5180552 China Collaborative Innovation Center of Extreme Optics Shanxi UniversityTaiyuan 030006China Institute for Advanced Study Shenzhen UniversityShenzhen 518060China College of Mechatronics and Control engineering Shenzhen UniversityShenzhen 518060China Laboratory of Alternative Energy Conversion Systems Department of Mechanical EngineeringSchool of EngineeringUniversity of ThessalyPedion Areos 38834Greece

3d-transition metal(Fe,Co,Ni,and Mn)-based MXene materials have been predicted to demonstrate exceptional electrochemical performance because of their good electrical conductivity and the presence of metallic atoms with multiple charge ***,until now,there have been no reports on MXenes based on Fe,Co,Ni,and Mn,due to the lack of 3d-metal-layered ***,we successfully synthesized the first 3d-transition metal-based MXenes,Mn_(2)CT_(x) by exfoliating a layered precursor derived from the anti-perovskite bulk *** as-prepared Mn_(2)CT_(x) MXene nanosheets were employed as anode materials in lithium-ion batteries,which exhibited stable storage capacity of 764.7 mAh·g^(-1) at 0.5 C,placing its storage capacities at an upper-middle level compared with other reported MXene materials as well as other Mn-based anode ***,this study opens a new avenue for MXene research by synthesizing 3d-transition metal-based MXenes for electrochemical applications.

关键词： Mn_(3)GaC Mn_(2)CT_(x) MXenes lithium-ion battery anode materials negative fading capacity

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Methyl functionalization of trimesic acid in copper-based metal-organic framework for ammonia colorimetric sensing at high relative humidity

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Chinese Chemical Letters 2024年第6期35卷 211-215页

作者： Yuxin Wang Zhengxuan Song Yutao Liu Yang Chen Jinping Li Libo Li Jia Yao College of Chemical engineering and technology Shanxi Key Laboratory of Gas Energy Efficient and Clean UtilizationTaiyuan University of TechnologyTaiyuan 030024China department of Gastroenterology Shanxi Bethune HospitalShanxi Academy of Medical SciencesTongji Shanxi HospitalThird Hospital of Shanxi Medical UniversityTaiyuan 030024China

Exhaled ammonia(NH_(3))can be used as a crucial biomarker of kidney and liver ***,the high humidity in the detection conditions remains a challenge for accurate detection by gas ***,a copper-based metal-organic framework(CH_(3)-Cu-BTC)with methyl(CH_(3)^(-))functionalization of trimesic acid was synthesized for NH_(3) colorimetric *** CH_(3)-Cu-BTC exhibited a strong response for 5 ppm NH_(3) with high selectivity under high relative humidity(75%RH).Density functional theory(DFT)simulations indicated that the NH_(3) molecules interacted more strongly with CH_(3)-Cu-BTC than H_(2)O molecules did,and the corresponding color switching was attributed to the lone-pair electron in NH_(3) changing the coordination environment of Cu^(2+)ions,leading to an obviously visible color switching response from ruby green to *** on the tailor-made pore chemistry,the precise detection of trace amounts of NH_(3) in exhaled air was realized through functionalized MOF *** strategy used in this study not only offers a new pathway for the rapid detection of low concentration NH_(3) under humid conditions,but also shows a method for early respiration diagnosis of kidney and liver diseases.

关键词： Metal-organic framework Ammonia sensing Naked-eye color switching High humidity Respiration diagnosis

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Scalable parallel ultrafast optical random bit generation based on a single chaotic microcomb

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Light(Science & Applications) 2024年第4期13卷 637-644页

作者： Pu Li Qizhi Li Wenye Tang Weiqiang Wang Wenfu Zhang Brent ELittle Sai Tek Chu KAlan Shore Yuwen Qin Yuncai Wang Institute of Advanced Photonics technology School of Information EngineeringGuangdong University of TechnologyGuangzhou 51006China. Key Laboratory of Photonic technology for Integrated Sensing and Communication Ministry of Education of ChinaGuangdong University of TechnologyGuangzhou 51006China. Guangdong Provincial Key Laboratory of information Photonics technology Guangdong University of TechnologyGuangzhou 51006China. Key Laboratory of Advanced Transducers andIntelligent Control System Ministry of EducationTaiyuan University of TechnologyTaiyuan 030024China. State Key Laboratory of Transient Optics and Photonics Xi’an Institute of Optics and Precision MechanicsChinese Academy of SciencesXi’an 710119China. department of Physics and Materials Science City University of Hong KongHong KongChina. School of electronic engineering Bangor UniversityBangorWales LL571UTUK

Random bit generators are critical for information security,cryptography,stochastic modeling,and *** and scalability are key challenges faced by current physical random bit ***,we propose a massively parallel scheme for ultrafast random bit generation towards rates of order 100 terabit per second based on a single micro-ring resonator.A modulation-instability-driven chaotic comb in a micro-ring resonator enables the simultaneous generation of hundreds of independent and unbiased random bit streams.A proof-of-concept experiment demonstrates that using our method,random bit streams beyond 2 terabit per second can be successfully generated with only 7 comb *** bit rate can be easily enhanced by further increasing the number of comb lines *** approach provides a chip-scale solution to random bit generation for secure communication and high-performance computation,and offers superhigh speed and large scalability.

关键词： resonator random chaotic

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