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environmental geochemistry:Introduction

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Geoscience Frontiers 2022年第1期13卷 374-375页

作者： Luis F.O.Silva Marcos L.S.Oliveira department of civil and environmental.universidad de la costa CUCCalle 58#55-66BarranquillaAtlánticoColombia departamento de Ingeniería civil y Arquitectura Universidad de LimaAvenida Javier Prado Este 4600Santiago de Surco 1503Peru

Assessing the physical,geographic,chemical,and geological aspects are important to understand environmental impacts as well as health concerns in view of building a more sustainable planet with circular economies that would last for the foreseeable *** the recent years,the significance of incorporating ecosystem,anthropogenic activities,and climate has fortified from being an academic concern(e.g.,WEF,2011)into a broadly societal concern as the forecasted realities of environmental deterioration and global climate change come to pass.

关键词： geochemistry climate planet

Hazardous elements and amorphous nanoparticles in historical estuary coal mining area

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Geoscience Frontiers 2019年第3期10卷 927-939页

作者： Ana L.Duarte Kátia DaBoit Marcos L.S.Oliveira Elba C.Teixeira Ismael L.Schneider Luis F.O.Silva department of civil and environmental Universidad de la Costa Faculdade Meridional IMED FEPAM-Funda■o Estadual de Prote■o Ambiental Henrique Luis Roessler

In Brazil, intense coal exploitation activities have led to environmental deterioration, including soil mortification, water contamination, loss of ecosystem, and atmospheric contamination. In addition,considerable quantities of sulfur-rich residues are left behind in the mining area; these residues pose grave environmental issues as they undergo sulfide oxidation reactions. When sulfur oxides come in contact with water, extreme acid leachate is produced with great proportions of sulfate, and hazardous elements(HEs), which are identified as coal drainage(CMD). CMD is an environmental pollution challenge, particularly in countries with historic or active coal mines. To prevent CMD formation or its migration, the source must be controlled; however, this may not be feasible at many locations. In such scenarios, the mine water should be collected, treated, and discharged. In this study, data from 2005 to2010 was gathered on the geochemistry of 11 CMD discharges from ten different mines. There are several concerns and questions on the formation of nanominerals in mine acid drainage and on their reactions and interfaces. The detailed mineralogical and geochemical data presented in this paper were derived from previous studies on the coal mine areas in Brazil. Oxyhydroxides, sulfates, and nanoparticles in these areas possibly go through structural transformations depending on their size and formation conditions. The geochemistry of Fe-precipitates(such as jarosite, goethite, and hematite) existent in the CMD-generating coal areas and those that could be considered as a potential source of hazardous elements(HEs)(e.g., Cr) were also studied because these precipitates are relatively stable in extremely low pH conditions. To simplify and improve poorly ordered iron, strontium, and aluminum phase characterization, field emission scanning electron microscopy(FE-SEM), high-resolution transmission electron microscopy(HR-TEM), micro-Raman spectroscopy, and X-ray diffraction(XRD) a

关键词： Brazilian coal mining environmental impacts Minerals

Comparative carbon emission assessments of recycled and natural aggregate concrete: environmental influence of cement content

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Geoscience Frontiers 2021年第6期12卷 66-75页

作者： Marian Sabǎu Dan V.Bompa Luis F.O.Silva department of civil and environmental Engineering Universidad de la Costa080020 BarranquillaColombia department of civil and environmental Engineering University of SurreyGuildford GU27XHUK departamento de Ingeniería civil y Arquitectura Universidad de LimaAvenida Javier Prado Este 4600Santiago de Surco 1503Peru

This work examines the environmental and geochemical impact of recycled aggregate concrete production with properties representative for structural *** environmental influence of cement content,aggregate production,transportation,and waste landfilling is analysed by undertaking a life cycle assessment and considering a life cycle inventory largely specific for the *** obtain a detailed insight into the optimum life cycle parameters,a sensitivity study is carried out in which supplementary cementitious materials,different values of natural-to-recycled aggregate content ratio and case-specific transportation distances were *** results show that carbon emissions were between 323 and 332 kgCO_(2)e per cubic metre of cement only natural aggregate *** values can be reduced by up to 17%by replacing 25%of the cement with fly *** contrast,carbon emissions can increase when natural coarse aggregates are replaced by recycled aggregates in proportions of 50%and 100%,and transportation is not included in ***,the concrete with 50%recycled aggregate presented lower increase,only 0.3%and 3.4%for normal and high strength concrete,*** some cases,the relative contribution of transportation to the total carbon emissions increased when cement was replaced by fly ash in proportions of 25%,and case-specific transportation distances were *** absolute values,the concrete mixes with 100%recycled aggregates and 25%fly ash had lower carbon emissions than concrete with cement and natural aggregates *** environmental benefits can be obtained when the transportation distances of fly ash are relatively short(15–25 km)and the cement replacement by fly ash is equal or higher than 25%,considering that the mechanical properties are adequate for practical *** observations from this paper show that recycled aggregate concrete with strength characteristics representative for structural members can have lowe

关键词： Life cycle assessment Recycled aggregate Natural aggregate Transportation distance OpenLCA

Comparative carbon emission assessments of recycled and natural aggregate concrete: environmental influence of cement content

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Geoscience Frontiers 2021年第6期12卷 72-81页

作者： Marian Sab?u Dan V.Bompa Luis F.O.Silva department of civil and environmental Engineering Universidad de la Costa department of civil and environmental Engineering University of Surrey departamento de Ingeniería civil y Arquitectura Universidad de Lima

This work examines the environmental and geochemical impact of recycled aggregate concrete production with properties representative for structural applications. The environmental influence of cement content, aggregate production, transportation, and waste landfilling is analysed by undertaking a life cycle assessment and considering a life cycle inventory largely specific for the region. To obtain a detailed insight into the optimum life cycle parameters, a sensitivity study is carried out in which supplementary cementitious materials, different values of natural-to-recycled aggregate content ratio and case-specific transportation distances were considered. The results show that carbon emissions were between 323 and 332 kg CO2e per cubic metre of cement only natural aggregate concrete. These values can be reduced by up to 17% by replacing 25% of the cement with fly ash. By contrast, carbon emissions can increase when natural coarse aggregates are replaced by recycled aggregates in proportions of 50% and 100%, and transportation is not included in analysis. However, the concrete with 50% recycled aggregate presented lower increase, only 0.3% and 3.4% for normal and high strength concrete, respectively. In some cases, the relative contribution of transportation to the total carbon emissions increased when cement was replaced by fly ash in proportions of 25%, and case-specific transportation distances were considered. In absolute values, the concrete mixes with 100% recycled aggregates and 25% fly ash had lower carbon emissions than concrete with cement and natural aggregates only. Higher environmental benefits can be obtained when the transportation distances of fly ash are relatively short(15–25 km) and the cement replacement by fly ash is equal or higher than 25%, considering that the mechanical properties are adequate for practical application. The observations from this paper show that recycled aggregate concrete with strength characteristics representative for s

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Introduction to the special issue on “COVID-19”

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Geoscience Frontiers 2022年第6期13卷 208-209页

作者： Luis F.O.Silva Weijun Li Teresa Moreno department of civil and environmental Universidad de la CostaCUC department of Atmospheric Sciences School of Earth SciencesZhejiang University Institute for environmental Assessment and Water Research Consejo Superior de Investigaciones Científicas

COVID-19 pandemic is wreaking havoc and bringing the whole world into a standstill in an unprecedented fashion. Joint efforts from multiple sectors to address the various aspects of environment and public health through usage of green technologies have become essential. The application of cleaner and effective technologies can be expanded to management and control, pollution mitigation and valorization of waste. In this Special Issue of Geoscience Frontiers, we present contributions addressing the interactions of COVID-19 in relation to environment and human health.

关键词： bringing expanded COV

Source identification and global implications of black carbon

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Geoscience Frontiers 2022年第1期13卷 404-416页

作者： Erika P.Blanco-Donado Ismael L.Schneider Paulo Artaxo Jesus Lozano-Osorio Luana Portz Marcos L.S.Oliveira department of civil and environmental Universidad de la CostaCUCBarranquilla080002Colombia department of Applied Physics Institute of PhysicsUniversity of São PauloSP 05508-220Brazil universidad de Lima Avenida Javier Prado Este 4600Santiago de Surco 1503Peru

Black carbon(BC)is one of the short-lived air pollutants that contributes significantly to aerosol radiative forcing and global climate *** is emitted by the incomplete combustion of fossil fuels,biofuels,and *** environments are quite complex and thus,the use of mobile jointly with fixed monitoring provides a better understanding of the dynamics of BC distribution in such *** present study addresses the measurement of BC concentration using real-time mobile and ambient monitoring in Barranquilla,an industrialized urban area of the Colombian Caribbean.A microaethalometer(MA200)and an aethalometer(AE33)were used for measuring the BC *** absorption Ångström exponent(AAE)values were determined for the study area,for identifying the BC emission *** results of the ambient sampling show that vehicle traffic emissions prevail;however,the influence of biomass burning was also *** mean ambient BC concentration was found to be 1.04±1.03μg/m^(3) and varied between 0.5 and 4.0μg/m^(3).From the mobile measurements obtained in real traffic conditions on the road,a much higher average value of 16.1±16.5μg/m^(3) was *** parts of the city showed BC concentrations higher than 20μg/m^(3).The spatial distribution of BC concentration shows that vehicle emissions and traffic jams,a consequence of road and transport infrastructure,are the factors that most affect the BC concentration.A comparison of results obtained from two aethalometers indicates that the concentrations measured by MA200 are 9%lower than those measured by *** AAE obtained was found to vary between 1.1 and 1.6,indicating vehicular emissions as the most crucial *** addition,it was observed that the BC concentration on working days was 2.5 times higher than on the weekends in the case of mobile monitoring and 1.5 times higher in the case of ambient monitoring.

关键词： Air pollution Black carbon Spatial distribution Source apportionment AbsorptionÅngström exponent

Estimation of the impact of biomass burning based on regional transport of PM_(2.5) in the Colombian Caribbean

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Geoscience Frontiers 2022年第1期13卷 430-436页

作者： Jehison Bolaño-Truyol Ismael L.Schneider Heidis Cano Cuadro Jorge D.Bolaño-Truyol Marcos L.S.Oliveira department of civil and environmental Universidad de la CostaCUCCalle 58#55–66BarranquillaAtlánticoColombia department of Productivity and Innovation Universidad de la CostaCUCCalle 58#55–66BarranquillaAtlánticoColombia Faculdade Meridional IMED 304 Passo FundoRS 99070–220Brazil universidad de Lima Avenida Javier Prado Este 4600Santiago de Surco 1503Peru

deterioration of air quality due to the increase in atmospheric emissions from biomass burning(BB)is one of the major environmental problems *** this study,we estimated the contributions of BB to PM_(2.5) concentrations in the municipalities of Soledad and Malambo located in the Colombian *** evaluation period ranged from February 24 to March 30,2018,a period with a high number of BB events recorded in the surroundings of the evaluated *** contribution of BB to the two sampling sites was estimated using the Hybrid Single-Particle lagrangian Integrated Trajectory(HYSPLIT)dispersion model with forwarding trajectories from each of the burning points identified by satellite images(n=1089).The PM_(2.5) emissions were determined using the fire radiative power(FRP),obtained by remote-sensing data,and corresponded to the radiant energy released per time unit by burning *** average PM_(2.5) concentrations during the evaluation period were 19.91μg/m^(3) for Soledad and 22.44μg/m^(3) for *** average contribution of BB to these municipalities was 22.8%and 28.8%,*** methodology used in this study allowed to estimate the contribution of this important source without knowledge of a previous tracer of BB,thereby increasing the use of the proposed procedure *** information would enable the implementation of effective mitigation,thereby diminishing the adverse impact of PM_(2.5) on the health of the population.

关键词： Biomass burning Particulate matter HYSPLIT Dispersion model Remote sensing

Nanomineralogy of evaporative precipitation of efflorescent compounds from coal mine drainage

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Geoscience Frontiers 2021年第6期12卷 404-410页

作者： Luis F.O.Silva Diana Pinto Guilherme L.Dotto James C.Hower department of civil and environmental.universidad de la costa CUCCalle 58#55–66BarranquillaAtlanticoColombia universidade Federal de Santa Maria–UFSM 1000Roraima Avenue97105–900Santa MariaRSBrazil University of Kentucky Department of Earth&Environmental SciencesLexingtonKY40506USA University of Kentucky Center for Applied Energy Research2540 Research Park DriveLexingtonKY40511USA

Efflorescent nanophases(NPs) are found as a transitory accumulation of potentially hazardous elements(PHEs),particularly in tropical climates. The central objective of this study was to investigate the distribution of PHEs with NPs through the evaporative formation structures(EFS) of enormously PHEs-rich coal-mine drainages(CMD). The EFS were studied in natural coal mine drainage for five months in order to determine their geochemical and ecological structures and to assess their position in the reduction of PHEs in nature. The largest coal-fired power plant in South America, located in south Brazil, is used as an example of such a problem. In this work, a novel methodology for the analysis of PHEs in CMD precipitates is proposed for this affected coal *** analytical method, combining X-Ray Diffraction(XRD) and advanced electron microscopies, shows the importance of nanomineralogy in understanding different circumstances of coal contamination. Several ultrafinenanoparticles(UNPs) were identified in the sampled soils and river sediments together with the PHEs. A decrease in PHEs was identified in association with UNPs. However, further investigations are required with regard to the mobility of PHEs in water, atmosphere, soils, and sediments. The EPS was thoroughly studied, acquiring suitable understanding with investigational facts for Ca and Fe-sulphates, pickeringite, and several amorphous phases.

关键词： Coal mine drainage Evaporative precipitation Sediments Water and soil pollution

Coal energy and environmental impacts:Introduction

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Energy Geoscience 2021年第2期2卷 87-89页

作者： Luis F.O.Silva Amy L.Wolfe department of civil and environmental.universidad de la costa CUCCalle 58#55e66BarranquillaAtlanticoColombia Kentucky Geological Survey University of Kentucky216 Mining and Mineral Resources Building504 Rose StreetLexingtonKY40506-0107USA

Within the last decade,the importance of integrating the envi-ronment,people,and climate has transitioned from being an aca-demic concern(e.g..WEF,2011)into a broadly societal concern asthe forecasted realities of environmental deterioration and globalclimate change come to pass,creating urgent public and environ-mental health issues.

关键词： has integrating environ