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Multifunctional Film Assembled from N‑Doped Carbon Nanofiber with Co–N_(4)–O Single Atoms for Highly Efficient Electromagnetic Energy Attenuation

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Nano-Micro Letters 2024年第11期16卷 359-376页

作者： Jia Xu Bei Li Zheng Ma Xiao Zhang Chunling Zhu Feng Yan Piaoping Yang Yujin Chen College of Materials Science and chemical engineering Harbin Engineering UniversityHarbin 150001People’s Republic of China Key Laboratory of In‑Fiber Integrated Optics College of Physics and Optoelectronic EngineeringHarbin Engineering UniversityHarbin 150001People’s Republic of China

Single-atom materials have demonstrated attractive physicochemical ***,understanding the relationships between the coordination environment of single atoms and their properties at the atomic level remains a considerable ***,a facile waterassisted carbonization approach is developed to fabricate well-defined asymmetrically coordinated Co–N_(4)–O sites on biomass-derived carbon nanofiber(Co–N_(4)–O/NCF)for electromagnetic wave(EMW)*** such nanofiber,one atomically dispersed Co site is coordinated with four N atoms in the graphene basal plane and one oxygen atom in the axial ***-depth experimental and theoretical studies reveal that the axial Co–O coordination breaks the charge distribution symmetry in the planar porphyrin-like Co–N_(4) structure,leading to significantly enhanced dielectric polarization loss relevant to the planar Co–N_(4) ***,the film based on Co–N_(4)–O/NCF exhibits light weight,flexibility,excellent mechanical properties,great thermal insulating feature,and excellent EMW absorption with a reflection loss of−45.82 dB along with an effective absorption bandwidth of 4.8 *** findings of this work offer insight into the relationships between the single-atom coordination environment and the dielectric performance,and the proposed strategy can be extended toward the engineering of asymmetrically coordinated single atoms for various applications.

关键词： Co single atoms Asymmetric coordination structure Axial oxygen coordination Electromagnetic wave absorption Multifunctional film

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A contrasting analysis of CO_(2) and N_(2) foam flood for enhanced oil recovery and geological storage of CO_(2)

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Petroleum Research 2024年第1期9卷 55-60页

作者： Alireza Roozbahani Farshad Soofivan Ali Sagban Hassoon Al-Tameemi Hadi Abdollahi Sogand Saatchi Abdolhamid Ansari Petroleum engineering department Faculty of Chemical EngineeringTarbiat Modares UniversityTehranIran School of chemical and Petroleum engineering Shiraz UniversityShirazIran School of chemical and Petroleum engineering Shiraz BranchIslamic Azad UniversityShirazIran department of Petroleum engineering Science and Research BranchAzad UniversityTehranIran department of Chemistry and chemical engineering Rasht BranchIslamic Azad UniversityRashtIran department of Petroleum engineering Lamerd BranchIslamic Azad UniversityLamerdIran

Foam flooding using CO_(2)has emerged as a promising method for both enhanced oil recovery(EOR)and the storage of CO_(2)in geological *** study conducts a thorough analysis of the behavior of CO_(2)and N_(2)foams in bulk and porous media,utilizing bubble-scale analyses and foam flooding *** study compares the foamability and longevity of CO_(2)and N_(2)foams,with findings indicating that N_(2)foam bubbles tend to be smaller and less varied in size than CO_(2)foam bubbles,leading to increased foam ***,the study compares the half-lives of CO_(2)and N_(2)foams generated through sparging and winding methods,showing that N_(2)foam has half-lives 22 and 10 times greater than CO_(2)foam when produced using the sparging and winding methods,***,CO_(2)foam generated through the sparging method had a lower foaming volume than N_(2)foam due to CO_(2)'s *** the foam flooding experiments,N_(2)foam proved more effective in recovering oil from porous media than CO_(2)foam,thus demonstrating the effectiveness of the foam injection *** results offer valuable insights into the differing performance of N_(2)and CO_(2)foam floods for EOR and CO_(2)geological storage.

关键词： CO_(2) storage Foam flood Enhanced oil recovery N_(2) foam CO_(2) foam

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“Buckets effect”in the kinetics of electrocatalytic reactions

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Journal of Energy Chemistry 2024年第2期89卷 388-396,I0010页

作者： Haowen Cui Yan-Xia Chen Hefei National Laboratory for Physical Sciences at Microscale Department of Chemical PhysicsUniversity of Science and Technology of ChinaHefei 230026AnhuiChina

In this study,we systematically investigated the effect of proton concentration on the kinetics of the oxygen reduction reaction(ORR)on Pt(111)in acidic *** results demonstrate a rectangular hyperbolic relationship,i.e.,the ORR current excluding the effect of other variables increases with proton concentration and then tends to a constant *** consider that this is caused by the limitation of ORR kinetics by the trace oxygen concentration in the solution,which determines the upper limit of ORR kinetics.A model of effective concentration is further proposed for rectangular hyperbolic relationships:when the reactant concentration is high enough to reach a critical saturation concentration,the effective reactant concentration will become a constant *** could be due to the limited concentration of a certain reactant for reactions involving more than one reactant or the limited number of active sites available on the *** study provides new insights into the kinetics of electrocatalytic reactions,and it is important for the proper evaluation of catalyst activity and the study of structureperformance relationships.

关键词： Oxygen reduction reaction Kinetics Zero order Rectangular hyperbolic relationship pH effect

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12.6μm-Thick Asymmetric Composite Electrolyte with Superior Interfacial Stability for Solid-State Lithium-Metal Batteries

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Nano-Micro Letters 2024年第9期16卷 397-409页

作者： Zheng Zhang Jingren Gou Kaixuan Cui Xin Zhang Yujian Yao Suqing Wang Haihui Wang Beijing Key Laboratory for Membrane Materials and engineering Department of Chemical EngineeringTsinghua UniversityBeijing 100084People’s Republic of China School of Chemistry and chemical engineering South China University of TechnologyGuangzhou 510000People’s Republic of China

Solid-state lithium metal batteries(SSLMBs)show great promise in terms of high-energy-density and high-safety ***,there is an urgent need to address the compatibility of electrolytes with high-voltage cathodes/Li anodes,and to minimize the electrolyte thickness to achieve highenergy-density of ***,we develop an ultrathin(12.6μm)asymmetric composite solid-state electrolyte with ultralight areal density(1.69 mg cm^(−2))for *** electrolyte combining a garnet(LLZO)layer and a metal organic framework(MOF)layer,which are fabricated on both sides of the polyethylene(PE)separator separately by tape *** PE separator endows the electrolyte with flexibility and excellent mechanical *** LLZO layer on the cathode side ensures high chemical stability at high *** MOF layer on the anode side achieves a stable electric field and uniform Li flux,thus promoting uniform Li^(+)*** to the well-designed structure,the Li symmetric battery exhibits an ultralong cycle life(5000 h),and high-voltage SSLMBs achieve stable cycle *** assembled pouch cells provided a gravimetric/volume energy density of 344.0 Wh kg^(−1)/773.1 Wh L^(−1).This simple operation allows for large-scale preparation,and the design concept of ultrathin asymmetric structure also reveals the future development direction of SSLMBs.

关键词： Solid-state lithium metal batteries Composite solid-state electrolyte Ultrathin asymmetric structure Pouch cells

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Sustainable ammonia synthesis:An in-depth review of non-thermal plasma technologies

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Journal of Energy Chemistry 2024年第9期96卷 1-38页

作者： Vahid Shahed Gharahshiran Ying Zheng department of chemical and Biochemical engineering Thompson Engineering BuildingWestern UniversityLondonON N6A 5B9Canada

Ammonia serves both as a widely used fertilizer and environmentally friendly energy source due to its high energy density,rich hydrogen content,and emissions-free ***,it offers convenient transportation and storage as a hydrogen *** dominant method used for large-scale ammonia production is the Haber-Bosch process,which requires high temperatures and pressures and is ***,non-thermal plasma offers an eco-friendly alternative for ammonia synthesis,gaining significant *** enables ammonia production at lower temperatures and pressures using plasma *** review provides insights into the catalyst and reactor developments,which are pivotal for promoting ammonia efficiency and addressing existing *** first,the reaction kinetics and mechanisms are introduced to gain a comprehensive understanding of the reaction pathways involved in plasma-assisted ammonia ***,the enhancement of ammonia synthesis efficiency is discussed by developing and optimizing plasma reactors and effective *** effect of other feeding sources,such as water and methane,instead of hydrogen is also ***,the challenges and possible solutions are outlined to facilitate energy-saving and enhance ammonia efficiency in the future.

关键词： Nitrogen fixation Ammonia synthesis NH_(3) Non-thermal plasma Ni Ru catalyst

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Advances in laser-plasma interactions using intense vortex laser beams

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Science China(physics,Mechanics & Astronomy) 2024年第9期67卷 14-42页

作者： Yin Shi Xiaomei Zhang Alexey Arefiev Baifei Shen department of Plasma physics and Fusion engineering University of Science and Technology of ChinaHefei 230026China department of physics Shanghai Normal UniversityShanghai 200234China department of Mechanical and Aerospace engineering University of California at San DiegoLa JollaCA 92093USA

Low-intensity light beams carrying orbital angular momentum(OAM),commonly known as vortex beams,have garnered significant attention due to promising applications in areas ranging from optical trapping to *** recent years,there has been a surge in global research exploring the potential of high-intensity vortex laser beams and specifically their interactions with *** paper provides a comprehensive review of recent advances in this *** with conventional laser beams,intense vortex beams exhibit unique properties such as twisted phase fronts,OAM delivery,hollow intensity distribution,and spatially isolated longitudinal *** distinct characteristics give rise to a multitude of rich phenomena,profoundly influencing laser-plasma interactions and offering diverse *** paper also discusses future prospects and identifies promising general research areas involving vortex *** areas include low-divergence particle acceleration,instability suppression,high-energy photon delivery with OAM,and the generation of strong magnetic *** growing scientific interest and application potential,the study of intense vortex lasers is poised for rapid development in the coming years.

关键词： intense vortex laser orbital angular momentum laser plasma interactions high power laser high energy density science

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Detailed characterization of kHz-rate laser-driven fusion at a thin liquid sheet with a neutron detection suite

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High Power Laser Science and engineering 2024年第1期12卷 13-23页

作者： Benjamin M.Knight Connor M.Gautam Colton R.Stoner Bryan V.Egner Joseph R.Smith Chris M.Orban Juan J.Manfredi Kyle D.Frische Michael L.Dexter Enam A.Chowdhury Anil K.Patnaik department of engineering physics Air Force Institute of TechnologyWPAFBOHUSA physics department Marietta CollegeMariettaOHUSA department of physics The Ohio State UniversityColumbusOHUSA department of Materials Science and engineering and Department of Electrical and Computer ScienceThe Ohio State UniversityColumbusOHUSA Intense Energy Solutions LLCPlain CityOHUSA

We present detailed characterization of laser-driven fusion and neutron production(-10^(5)/second) using 8 mJ, 40 fs laser pulses on a thin(<1 μm) D_2O liquid sheet employing a measurement suite. At relativistic intensity(~ 5 × 10^(18)W/cm^(2))and high repetition rate(1 kHz), the system produces deuterium±deuterium(D-D) fusion, allowing for consistent neutron generation. Evidence of D-D fusion neutron production is verified by a measurement suite with three independent detection systems: an EJ-309 organic scintillator with pulse-shape discrimination, a ~3He proportional counter and a set of 36 bubble detectors. Time-of-flight analysis of the scintillator data shows the energy of the produced neutrons to be consistent with 2.45 MeV. Particle-in-cell simulations using the WarpX code support significant neutron production from D-D fusion events in the laser±target interaction region. This high-repetition-rate laser-driven neutron source could provide a low-cost, on-demand test bed for radiation hardening and imaging applications.

关键词： high-repetition-rate laser-driven fusion laser-plasma interaction liquid target neutron detectors

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Sustainable bio-energy generation via the conversion of spent wash using dual chamber microbial fuel cell

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Waste Disposal and Sustainable Energy 2024年第2期6卷 219-231页

作者： Abdul Sattar Jatoi Jawad Ahmed Afaque Ahmed Bhutto Muhammad Shuaib Shaikh department of chemical engineering Dawood University of Engineering and Technology KarachiSindhPakistan Changzhou DUBO Polymer Co. Ltd.Changzhou 213002China department of Basic Science and Related Studies The University of LarkanoSindhPakistan department of chemical engineering Mehran University of Engineering and Technology JamshoroSindhPakistan

Microbial fuel cells(MFCs)are innovative devices that combine microbial processes with electrochemical reactions to convert organic matter in wastewater into electricity while simultaneously treating the *** such application is the treatment of spent wash,a highly polluting effluent generated from the distillery industry after crude mesh is separated into ethanol and spent *** wash,also known as distillery effluent or stillage,is a highly challenging wastewater treatment method due to its high chemical oxygen demand(COD),biological oxygen demand(BOD),and total dissolved solids(TDS).These characteristics make it a complex and polluting industrial effluent that requires specialized treatment processes to reduce its environmental impact ***,MFCs have shown promise in treating spent wash,as they can utilize the organic matter in wastewater as a fuel source for microbial growth as well as for electricity *** the treatment of spent wash,Saccharomyces cerevisiae *** used as a biocatalyst along with 340 mol/L potassium ferricyanide in the cathode chamber and 170 mol/L methylene blue in the anode as a *** tests were conducted by balancing a one-liter volume for power production from spent wash in MFC with the optimal conditions of 10%agarose,pH 8.5,300 mL/min of aeration in the cathode chamber,and 40%(in weight)substrate *** an ideal concentration,the maximum current and power density are roughly 53.41 mA/m^(2)and 72.22 mW/m^(2),*** each litre of processed spent wash,a maximum voltage of 850 mV(4.5 mA)was ***,91%of COD and BOD were removed from the effluent *** findings show that MFCs are capable of producing electricity and efficiently removing COD from wasted wash at the same time.

关键词： Microbial fuel cell chemical oxygen demand Biological oxygen demand-Current density Power density Spent wash

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Nanofluidic memristor based on the elastic deformation of nanopores with nanoparticle adsorption

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National Science Review 2024年第04期11卷 46-54页

作者： Xi Zhou Yuanyuan Zong Yongchang Wang Miao Sun Deli Shi Wei Wang Guanghua Du Yanbo Xie department of Chemistry and chemical engineering Northwestern Polytechnical University School of Physical Science and Technology Northwestern Polytechnical University School of Aeronautics and Institute of Extreme Mechanics Northwestern Polytechnical University Institute of Modern physics Chinese Academy of Sciences

The memristor is the building block of neuromorphic computing. We report a new type of nanofluidic memristor based on the principle of elastic strain on polymer nanopores. With nanoparticles absorbed at the wall of a single conical polymer nanopore, we find a pinched hysteresis of the current within a scanning frequency range of 0.01–0.1 Hz, switching to a diode below 0.01 Hz and a resistor above 0.1 Hz. We attribute the current hysteresis to the elastic strain at the tip side of the nanopore, caused by electrical force on the particles adsorbed at the inner wall surface. Our simulation and analytical equations match well with experimental results, with a phase diagram for predicting the system transitions. We demonstrate the plasticity of our nanofluidic memristor to be similar to a biological synapse. Our findings pave a new way for ionic neuromorphic computing using nanofluidic memristors.

关键词： nanofluidics memristor neurocomputing elastic deformation

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Direct microwave leaching conditions of rare earth elements in fluorescent wastes

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Journal of Rare Earths 2024年第6期42卷 1165-1174,I0007页

作者： A.Bilen B.Birol M.N.Saridede S.S.Kaplan M.S.Sonmez department of Metallurgical and Materials engineering Yildiz Technical UniversityIstanbulTurkey department of chemical engineering and Materials Science Stevens Institute of TechnologyNew JereyUSA department of Metallurgical and Materials engineering Istanbul Technical UniversityIstanbulTurkey

The luminescent phosphor powder in the fluorescent lamp constitutes 2%of the lamp’s *** can be mentioned that fluorescent wastes are a crucial raw material to produce rare earth *** the present study,microwave leaching process was conducted to dissolve rare earth elements yttrium(Y),europium(Eu),and remaining rare earth elements(REEs)present in the phosphor powder of the fluorescent *** the yields were *** the microwave leaching process,the effects of the temperature(80-160℃),acid type(hydrochloric acid(HCl),nitric acid(HNO_(3)),sulphuric acid(H_(2)SO_(4))),acid concentration(0.5-6 mol/L),solid to liquid ratio(0.1:10-0.5:10)and reaction time(5-90 min)parameters on leaching efficiencies of varying rare earth elements and calcium were *** highest yield was obtained in the direct microwave leaching of fluorescent waste with the experimental conditions of 6 mol/L HCl,160℃,0.1:10 solid-to-liquid ratio(S:L),and 90 *** energy calculations were made,and kinetic models of the reactions were obtained,and it is observed that Y and Eu dissolution is diffusion-controlled,on the other hand,lanthanum(La),cerium(Ce),and terbium(Tb)were examined to be chemical reaction ***,calcium(Ca)and gadolinium(Gd)seem coherent with the mixed ***,mathematical models of all experimental studies are created with the response surface Box-Behnken method and the correlation coefficients of all the models are over 90%.

关键词： Rare earth elements(REEs) Direct microwave leaching Fluorescent waste Kinetic models Response surface method

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