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National Science Review 2024年第4期11卷 195-205页

作者： Yanhua Wan Changyao Wang Xingmiao Zhang Yang Yin Mengmeng Liu Bing Ma Linlin Duan Yuzhu Ma Wei Zhang Changlin Zheng Dongliang Chao Fei Wang Yongyao Xia Wei Li department of Chemistry Laboratory of Advanced Materials Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials State Key Laboratory of Molecular Engineering of Polymers College of Chemistry and Materials ScienceFudan University State Key Laboratory of Surface physics and department of physics Fudan University

Due to their uncontrollable assembly and crystallization process,the synthesis of mesoporous metal oxide single crystals remains a formidable ***,we report the synthesis of single-crystal-like mesoporous Li2TiSiO5by using soft micelles as *** key lies in the atomic-scale self-assembly and step-crystallization processes,which ensure the formation of single-crystal-like mesoporous Li2TiSiO5microparticles via an oriented attachment growth mechanism under the confinement of an in-situ formed carbon *** mesoporous Li2TiSiO5anode achieves a superior rate capability(148 mAh g-1at5.0 A g-1) and outstanding long-term cycling stability(138 mAh g-1after 3000 cycles at 2.0 A g-1) for lithium storage as a result of the ultrafast Li+diffusion caused by penetrating mesochannels and nanosized crystal frameworks（5-10 nm）.In comparison,bulk Li2TiSiO5exhibits poor rate capability and cycle performance due to micron-scale diffusion *** method is very simple and reproducible,heralding a new way of designing and synthesizing mesoporous single crystals with controllable frameworks and chemical functionalities.

关键词： mesoporous materials micelles single-crystal-like Li2TiSiO5 lithium-ion batteries

Polyelectrolyte Complexes and Coacervates Formed by De novo-Designed Peptides and Oligonucleotide

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Chinese Journal of Polymer Science 2024年第9期42卷 1333-1340,I0007页

作者： Tian-Hao Ren De-Hai Liang Beijing National Laboratory for Molecular Sciences Department of Polymer Science and Engineering and the Key Laboratory of Polymer Chemistry and Physics of the Ministry of EducationCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing100871China

The liquid-liquid phase separation of biopolymers in living cells contains multiple interactions and occurs in a dynamic *** the regulation mechanism is still a *** this work,we designed a series of peptides(XXLY)_(6)SSSGSS and studied their complexation and coacervation behavior with single-stranded ***“X”and“Y”are varied to combine known amounts of charged and non-charged amino acids,together with the introduction of secondary structures and pH *** show that the electrostatic interaction,which is described as charge density,controls both the strength of complexation and the degree of chain relaxation,and thus determines the growth and size of the *** hydrophobic interaction is prominent when the charges are ***,the secondary structures of peptides exhibit profound effect on the morphology of the phases,such as solid phase to liquid phase *** study gains insight into the phase separation under physiological *** is also helpful to create coacervates with desirable structures and functions.

关键词： Polyelectrolyte complex Coacervate Peptides Secondary structure Electrostatic interaction

High-visibility ghost imaging with phase-controlled discrete classical light sources

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Chinese physics B 2024年第7期33卷 328-334页

作者：仵雪滢赵岳李利明 School of physics and Optoelectronic engineering Shandong University of TechnologyZibo 255049China

We take phase modulation to create discrete phase-controlled sources and realize the super-bunching effect by a phasecorrelated method. From theoretical and numerical simulations, we find the space translation invariance of the bunching effect is a key point for the ghost imaging realization. Experimentally, we create the orderly phase-correlated discrete sources which can realize high-visibility second-order ghost imaging than the result with chaotic sources. Moreover, some factors affecting the visibility of ghost image are discussed in detail.

关键词： ghost imaging high visibility space translation invariance

Programming molecular switches in water and ethanol via thermo-sensitive polymers for phase control in energetic crystals

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Defence Technology（防务技术） 2024年第8期38卷 75-88页

作者： Xinru Yang Yushi Wen Congmei Lin Feiyan Gong Zhijian Yang Fude Nie Institute of Chemical Materials China Academy of Engineering PhysicsMianyang 621900China

The practical application of energetic materials, particularly 2,4,6,8,10,12-hexanitro-2,4,6,8,10,12-hexaazaisowurtzitane(CL-20), is frequently impeded by phase transition challenges. In this study, we propose a novel strategy to enhance the stability of CL-20 by employing a thermo-sensitive polymer,poly(N-isopropylacrylamide)(PNIPAM), to modulate its phase transitions. Our approach involves the use of an in-situ polymerized polydopamine(PDA) shell as a platform for surface grafting through atom transfer radical polymerization, yielding a core-shell structured CL-20@PDA-PNIPAM. Through comprehensive characterization, the successful grafting of PNIPAM is confirmed, significantly enhanced the phase stability of CL-20. Notably, our core-shell structure exhibits a 13℃ increase in phase transition temperature compared to raw CL-20, thereby delaying the ε→a phase transition by over 80 min under combined thermal and solvent conditions. The enhanced stability is attributed to the hydrophobic nature of PNIPAM above its low critical solution temperature in water, which effectively shields the CL-20 crystal. These findings provide new insights into enhancing the stability and safety of energetic materials in complex environments, highlighting the potential of our molecular switch mechanism.

关键词： 2,4,6,8,10,12-Hexanitro-2,4,6,8,10,12-hexaazaisowurtzitane(CL-20) Phase stability Polydopamine(PDA) Poly-N-Isopropylacrylamide(PNIPAM) Thermal and solvent effects

Differences between two methods to derive a nonlinear Schrödinger equation and their application scopes

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Chinese physics B 2024年第2期33卷 421-429页

作者：陈羽西张恒段文山 College of physics and Electronic engineering Northwest Normal UniversityLanzhou 730070China

The present paper chooses a dusty plasma as an example to numerically and analytically study the differences between two different methods of obtaining nonlinear Schrödinger equation(NLSE).The first method is to derive a Korteweg–de Vries(KdV)-type equation and then derive the NLSE from the KdV-type equation,while the second one is to directly derive the NLSE from the original *** is found that the envelope waves from the two methods have different dispersion relations,different group *** results indicate that two envelope wave solutions from two different methods are completely *** results also show that the application scope of the envelope wave obtained from the second method is wider than that of the first one,though both methods are valuable in the range of their corresponding application *** is suggested that,for other systems,both methods to derive NLSE may be correct,but their nonlinear wave solutions are different and their application scopes are also different.

关键词： dusty plasmas nonlinear waves particle-in-cell simulation

Reflection behavior of insensitive explosive detonation propagating around a cylinder

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Acta Mechanica Sinica 2024年第7期40卷 55-65页

作者： Zixuan Zhang Yuan Wang Xiaomian Hu Haitao Chen Institute of Applied physics and Computational Mathematics Beijing 100094China Graduate School of China Academy of engineering physics Beijing 100088China

Insensitive explosive detonation has wide applications in compressing and driving inert materials,and thereby the interaction between detonation and inert materials has received more *** this paper,a two-dimensional numerical simulation based on the Euler multiphase flow framework is used to investigate the reflection behavior of the insensitive explosive detonation propagating around a *** results show that there is a critical incident angle,defined as transition angle for detonation propagating around the cylinder,below which the regular reflection(RR)on the cylinder surface is *** the incident angle is greater than the transition angle,RR changes to Mach *** transition angle is larger than that obtained by polar curve theory and the change of incident angle is used to interpret above *** addition,the influence of cylindrical radius and detonation reaction zone width on the reflection behavior is *** the cylindrical radius increases,the height of Mach stem increases while the transition angle decreases and gradually approaches the value in pole curve *** Neumann reflection is observed when the reaction zone width is relatively *** is because the energy release rate in the reaction zone is high for small reaction zone width,resulting in the formation of a series of compression waves near the cylindrical interface.

关键词： Insensitive explosive detonation Cylindrical inert material Reflection behavior

Coexistence of antiferromagnetism and unconventional superconductivity in a quasi-one-dimensional flat-band system:Creutz lattice

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Chinese physics B 2024年第3期33卷 583-588页

作者：徐峰张磊 School of physics and Telecommunication engineering Shaanxi University of TechnologyHanzhong 723001China

We study the coexistence of antiferromagnetism and unconventional superconductivity on the Creutz lattice which shows strictly flat bands in the noninteracting *** famous renormalized mean-field theory is used to deal with strong electron-electron repulsive Hubbard interaction in the effective low-energy t-J model,the superfluid weight of the unconventional superconducting state has been calculated via the linear response *** unconventional superconducting state with both spin-singlet and staggered spin-triplet pairs emerges beyond a critical antiferromagnetic coupling interaction,while antiferromagnetism accompanies this *** superconducting state with only spin-singlet pairs is dominant with paramagnetic *** A phase is analogous to the pseudogap phase,which shows that electrons go to form pairs but do not cause a *** also show the superfluid behavior of the unconventional superconducting state and its critical *** is proven directly that the flat band can effectively raise the critical temperature of *** is implementable to simulate and control strongly-correlated electrons'behavior on the Creutz lattice in the ultracold atoms experiment or other artificial *** results may help the understanding of the interplay between unconventional superconductivity and magnetism.

关键词： flat-band unconventional superconductivity antiferromagnetism strong electron-electron interaction superfluid weight

A numerical survey of parameters to reach ignition condition for axial compression of a large-sized field reversed configuration

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Plasma Science and Technology 2024年第5期26卷 47-55页

作者：李宜霖廖晖周海洋孙玄 department of Plasma physics and Fusion engineering School of Nuclear Science and TechnologyUniversity of Science and Technology of ChinaHefei 230026People’s Republic of China

Field reversed configuration(FRC)is widely considered as an ideal target plasma for magnetoinertial ***,its confinement and stability,both proportional to the radius,will deteriorate inevitably during radial ***,we propose a new fusion approach based on axial compression of a large-sized *** axial compression can be made by plasma jets or plasmoids converging onto the axial ends of the *** parameter space that can reach the ignition condition while preserving the FRC's overall quality is studied using a numerical model based on different FRC confinement *** is found that ignition is possible for a large FRC that can be achieved with the current FRC formation techniques if compression ratio is greater than 50.A more realistic compression is to combine axial with moderate radial compression,which is also presented and calculated in this work.

关键词： field reversed configuration magnetized target fusion axial compression

Coherence of nonlinear Bloch dynamics of Bose-Einstein condensates in deep optical lattices

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Chinese physics B 2024年第4期33卷 297-303页

作者：张爱霞张薇王杰胡潇文米来来薛具奎 College of physics and Electronics engineering Northwest Normal UniversityLanzhou 730070China

Atomic interaction leads to dephasing and damping of Bloch oscillations(BOs)in optical lattices,which limits observation and applications of *** to obtain persistent BOs is particularly ***,the nonlinear Bloch dynamics of the Bose-Einstein condensate with two-body and three-body interactions in deep optical lattices is *** damping rate induced by interactions is *** damping induced by two-body interaction plays a dominant role,while the damping induced by three-body interaction is ***,when the two-body and three-body interactions satisfy a threshold,long-lived coherent BOs are ***,the Bloch dynamics with periodical modulation of linear force is *** frequencies of linear force corresponding to resonance and pseudoresonance are obtained,and rich dynamical phenomena,i.e.,stable and strong BOs,drifting and dispersion of wave packet,are *** controllable Bloch dynamics is provided with the periodic modulation of the linear force.

关键词： Bose-Einstein condensate atomic interaction Bloch oscillations

Towards sustainable solar cells:unveiling the latest developments in bio-nano materials for enhanced DSSC efficiency

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Clean Energy 2024年第3期8卷 238-257页

作者： Sethu Narayanan Tamilselvan S.Shanmugan Research Centre for Solar Energy Department of Engineering PhysicsCollege of EngineeringKoneru Lakshmaiah Education FoundationGreen FieldsGuntur DistrictVaddeswaramAndhra Pradesh 522502India

Fossil fuels-instrumental in powering the nineteenth-century Industrial Revolution-are now under heightened scrutiny due to environmental concerns and carbon ***,there is a global impetus towards achieving carbon-neutral energy production,with solar energy emerging as a cornerstone in this *** the past three decades,dye-sensitized solar cells(DSSCs)have gained increasing prominence due to their unique *** review elucidates several crucial elements essential to DSSC construction,notably bio-nano materials,prized for their structural flexibility,cost-effectiveness and high molar absorption *** delves into the intricate relationship between molecular structure and DSSC performance,showcasing significant advancements with light-to-power conversion efficiencies reaching 11%.A comprehensive analysis of the photovoltaic performance of DSSCs utilizing bio-nano-based dyes offers invaluable insights into the state of this rapidly evolving *** components under scrutiny include transparent conductive oxide(TCO)layers,physical techniques for metal oxide deposition onto TCO thin films,diverse dye variants and foundational knowledge of components ripe for growth and ***,the review outlines the latest breakthroughs in the field,providing glimpses into the current status of prototype DSSCs.

关键词： DSSC performance TCO thin films environmental solution