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Enhanced dynamics of Al3+/H+ ions in aqueous aluminum ion batteries:Construction of metastable structures in vanadium pentoxide upon oxygen vacancies

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Journal of Energy Chemistry 2025年第2期101卷 562-569页

作者： Zhibao Wang Hanqing Gu Tianci Wu Wenming Zhang Zhanyu Li Hebei Key laboratory of Optic-Electronic Information and Materials National & Local Joint Engineering Laboratory of New Energy Photoelectric Devices College of Physics Science and Technology Hebei University

In recent years,aqueous aluminum ion batteries have been widely studied owing to their abundant energy storage and high theo retical *** in-depth study of vanadium oxide materials is necessary to address the precipitation of insoluble products covered cathode surface and the slow reaction ***,a method using a simple one-step hydrothermal preparation and oxalic acid to regulate oxygen vacancies has been reported.A high starting capacity(400 mAh g-1) can be achieved by Ov-V2O5,and it is capable of undergoing 200 cycles at 0.4 A g-1,with a termination discharge capacity of103 mAh *** analysis demonstrated that metastable structures（AlxV2O5and HxV2O5） were constructed through the insertion of Al3+/H+during discharging,which existed in the lattice intercalation with *** incorporation of oxygen vacancies lowers the reaction energy barrier while improving the ion transport *** addition,the metastable structure allows the electrostatic interaction between Al3+and the main backbone to establish protection and optimize the transport *** parallel,this work exploits ex-situ characterization and DFT to obtain a profound insight into the instrumental effect of oxygen vacancies in the construction of metastable structures during in-situ electrochemical activation,with a view to better understanding the mechanism of the synergistic participation of Al3+and H+in the *** work not only reports a method for cathode materials to modulate oxygen vacancies,but also lays the foundation for a deeper understanding of the metastable structure of vanadium oxides.

关键词： Electrochemical activation Metastable structure Oxygen vacancies Vanadium pentoxide

General and Specific Combining Abilities of Pacific Oyster(Crassostrea gigas)and Fujian Oyster(***)for Growth,Survival and Thermal Tolerance of Their Reciprocal Hybrids

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Journal of Ocean University of China 2025年第1期24卷 238-248页

作者： JIANG Gaowei XU Chengxun LI Qi Key laboratory of Mariculture Ministry of EducationOcean University of ChinaQingdao 266003China laboratory for Marine Fisheries Science and Food Production Processes Laoshan LaboratoryQingdao 266237China

A crossbreeding program was established in 2019 to address the declining Crassostrea gigas harvests caused by Pacific Oyster Mortality Syndrome(POMS).As a part of the program,this study was performed to estimate the genetic structure underlying phenotypic *** complete diallel crossings of *** and ***,comprising 60 full-sib families,were used to evaluate the general combining ability(GCA)and specific combining ability(SCA),as well as genotype and environment interactions for shell height(SH),summer survival(SS),and thermal tolerance(TT)of reciprocal hybrids GA(***♀×***♂)and AG(***♀×***♂)grown in Rongcheng and Rushan,Shandong Province,*** results suggested that heterosis of the reciprocal hybrids was evident for SH,SS,and *** hybrid GA had larger heterosis than AG in both testing environments,and can be a potential donor in the breeding *** male *** had better GCA for SH in Rongcheng,whereas male *** was a good general combiner for SS and TT in both Rongcheng and *** estimate of SCA was much higher than GCA for SH and lower than GCA for *** harness both additive and non-additive genetic effects,combination breed-ing could be taken to develop hybrid varieties possessing both thermal tolerance and fast-growing *** positive correlations between SH and TT suggested that these traits could be improved *** significant G×E interactions demonstrated the importance to undertake site-specific breeding programs in different ***,this study can provide essential information for developing crossbreeding strategies for the oyster farming industry.

关键词： crossbreeding combining ability genotype×environment interaction Crassostrea gigas C.angulata

Low-dose exposure to microplastics retards meiotic maturation via HDAC3 insufficiency

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Science China Life Sciences 2025年

作者： Qi Zhao Ming Zong Entong Song Hongye Linghu Xuanwen Li Baicui Wang Songling Xiao Wanchun Guan Jianzhong Su Jiaming Zhang Jingzhang Ji Qingran Kong Zhejiang Provincial Key laboratory of Medical Genetics Key Laboratory of Laboratory Medicine Ministry of Education School of Laboratory Medicine and Life Sciences Wenzhou Medical University Oujiang laboratory Zhejiang Lab for Regenerative Medicine Vision and Brain Health

Microplastics(MPs) are considered one of the main causes of male and female infertility. However, the reproductive toxicity and its related mechanisms are currently understood primarily through animal models with acute exposure to MPs. In this study, we demonstrate that lowdose exposure to polystyrene microplastics(PSMPs) leads to severely abnormal reproduction in females, manifested by oocyte meiotic maturation defect. Mechanistically, PSMPs exposure induce the overactivation of cell metabolism pathways, insufficient HDACs, and H4K16hyperacetylation in oocytes both in vivo and in vitro. When an HDAC3 inhibitor is added, the oocyte maturation defect, overactivation of cell metabolism pathways, and H4K16 hyperacetylation are recapitulated. Conversely, the overexpression of HDAC3 can rescue the defects in meiotic maturation induced by PSMPs. Our observations suggest a direct link between the maturation defects caused by PSMPs and HDAC3insufficiency. Thus, we propose potential treatments to address the meiotic maturation defect of oocytes in women highly exposed to MPs by activating or supplying HDAC3.

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Gradient maturation experiment on hairs implies taphonomic changes in fossil hairs

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Science China Earth Sciences 2025年第1期68卷 62-73页

作者： Xin LI Yibo ZHOU Tao ZHAO Xingjian HE Yanhong PAN State Key laboratory for Mineral Deposits Research Center for Critical Earth Material CyclingCentre for Research and Education on Biological Evolution and Environment and Frontiers ScienceSchool of Earth Sciences and EngineeringNanjing UniversityNanjing210023China Institute of Palaeontology Yunnan Key Laboratory of Earth System ScienceYunnan Key Laboratory for PalaeobiologyYunnan UniversityKunming650500China

Mammalian hair,as a key feature related to endothermy,physical protection,and camouflage,has a long geohistorical record that dates back even to the ***,the limited information on the taphonomy of hair hinders the understanding of its evolutionary significance in deep *** address this,we conducted taphonomic experiments to simulate the transformation process of black *** changes in the morphological structure,microscopic characteristics,and chemical composition of hair during the simulated fossilization process were documented by scanning electron microscopy,Fourier transform infrared(FTIR)spectroscopy,and Raman *** results revealed that damage to the morphology of hair began at a mild temperature(150–175℃),and hair transformed into a fluid-like mass at a relatively high temperature(200℃).In addition,the morphological structure of melanosomes had relatively greater preservation potential than keratins did,and the microscopic features of melanosomes were persistently *** Raman and FTIR spectra indicated that the characteristic melanin and keratin peaks changed as the temperature *** the chemical signals were not lost completely,the variations in the characteristic amide bands in the FTIR spectra indicate that the keratins severely degraded at high temperatures(>200℃),whereas the characteristic melanin bands in the Raman spectra suggested that melanin signals were still recognizable,even at high temperatures(>200℃).These results were confirmed by principal component analysis(PCA)and principal component analysis linear discriminant analysis(PCA–LDA).In addition,the Raman signals of all the samples in the simulated experiments were distinguished from the signals of common geological carbonaceous materials(humic acid),which suggested that Raman spectroscopy can be used to detect melanin in fossils.

关键词： Mammalian hair Melanin Keratin Fossilization Experimental taphonomy

A fast amplitude preserving three-parameter 3D parabolic Radon transform and its application on multiple attenuation

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Petroleum Science 2025年第1期22卷 163-177页

作者： Ji-Tao Ma Kai-Ge Zhao Zhen Liao College of Geophysics China University of Petroleum (Beijing) State Key laboratory of Petroleum Resources and Engineering China University of Petroleum (Beijing) CNPC Key laboratory of Geophysical Prospecting China University of Petroleum (Beijing)

Seismic wavefields propagate through three-dimensional(3D) space, and their precise characterization is crucial for understanding subsurface structures. Traditional 2D algorithms, due to their limitations, are insufficient to fully represent three-dimensional wavefields. The classic 3D Radon transform algorithm assumes that the wavefield's propagation characteristics are consistent in all directions, which often does not hold true in complex underground media. To address this issue, we present an improved 3D threeparameter Radon algorithm that considers the wavefield variation with azimuth and provides a more accurate wavefield description. However, introducing new parameters to describe the azimuthal variation also poses computational challenges. The new Radon transform operator involves five variables and cannot be simply decomposed into small matrices for efficient computation; instead, it requires large matrix multiplication and inversion operations, significantly increasing the computational load. To overcome this challenge, we have integrated the curvature and frequency parameters, simplifying all frequency operators to the same, thereby significantly improving computation efficiency. Furthermore,existing transform algorithms neglect the lateral variation of seismic amplitudes, leading to discrepancies between the estimated multiples and those in the data. To enhance the amplitude preservation of the algorithm, we employ orthogonal polynomial fitting to capture the amplitude spatial variation in 3D seismic data. Combining these improvements, we propose a fast, amplitude-preserving, 3D threeparameter Radon transform algorithm. This algorithm not only enhances computational efficiency while maintaining the original wavefield characteristics, but also improves the representation of seismic data by increasing amplitude fidelity. We validated the algorithm in multiple attenuation using both synthetic and real seismic data. The results demonstrate that the new algor

关键词： Three-parameter 3D Radon Orthogonal polynomial Amplitude-preserving Multiple attenuation

Unraveling brain aging through the lens of oral microbiota

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Neural Regeneration Research 2025年第7期20卷 1930-1943页

作者： Qinchao Hu Si Wang Weiqi Zhang Jing Qu Guang-Hui Liu State Key laboratory of Membrane Biology Institute of ZoologyChinese Academy of SciencesBeijingChina Hospital of Stomatology Guanghua School of StomatologyGuangdong Provincial Key Laboratory of StomatologySun Yat-sen UniversityGuangzhouGuangdong ProvinceChina Advanced Innovation Center for Human Brain Protection and National Clinical Research Center for Geriatric Disorders Xuanwu HospitalCapital Medical UniversityBeijingChina Aging Translational Medicine Center International Center for Aging and CancerBeijing Municipal Geriatric Medical Research CenterXuanwu HospitalCapital Medical UniversityBeijingChina CAS Key laboratory of genomic and Precision Medicine Beijing Institute of GenomicsChinese Academy of Sciences and China National Center for BioinformationBeijingChina University of Chinese Academy of Sciences BeijingChina Institute for Stem Cell and Regeneration Chinese Academy of SciencesBeijingChina Aging Biomarker Consortium BeijingChina State Key laboratory of Stem Cell and Reproductive Biology Institute of ZoologyChinese Academy of SciencesBeijingChina Beijing Institute for Stem Cell and Regenerative Medicine BeijingChina

The oral cavity is a complex physiological community encompassing a wide range of *** of oral microbiota can lead to various oral infectious diseases,such as periodontitis and tooth decay,and even affect systemic health,including brain aging and neurodegenerative *** studies have highlighted how oral microbes might be involved in brain aging and neurodegeneration,indicating potential avenues for intervention *** this review,we summarize clinical evidence demonstrating a link between oral microbes/oral infectious diseases and brain aging/neurodegenerative diseases,and dissect potential mechanisms by which oral microbes contribute to brain aging and *** also highlight advances in therapeutic development grounded in the realm of oral microbes,with the goal of advancing brain health and promoting healthy aging.

关键词： Alzheimer's disease brain aging multiple sclerosis neurodegeneration neurodegenerative diseases oral microbiota Parkinson's disease periodontitis bacteria Porphyromonas gingivalis

Ultralight and superelastic MXene/reduced graphene oxide aerogels for electromagnetic interference shielding

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Nano Research 2025年第1期18卷 1-9页

作者： Xinfeng Zhou Yang Dai Guoyao Yue Yiman Zhang Lulu Li Zhong-Zhen Yu Peng Min Hao-Bin Zhang State Key laboratory of Organic-Inorganic Composites College of Materials Science and EngineeringBeijing University of Chemical TechnologyBeijing 100029China Beijing Key laboratory of Advanced Functional Polymer Composites College of Materials Science and EngineeringBeijing University of Chemical TechnologyBeijing 100029China Present address:BOE Technology Innovation Center BOE Technology Group Co.Ltd.Beijing 100176China Xi’an Modern Chemistry Research Institute Xi’an 710065China

Lightweight aerogels feature multifunctionality and a high porosity,yet accompanied with poor structure recovery under large strain *** this work,we develop an air bubble-ice crystal dual template and annealing strategy to integrate low density and high resilience for the conductive transition metal carbides/nitrides(MXene)composite *** air bubbles and ice crystals synergistically exclude the nanosheets to the gas-liquid interfaces,thereby constructing unique Y-shaped junctions and robust *** annealing process greatly enhances the interlayer *** external load,the Yshaped structures prevent the stress concentration at the junctions by transferring the forces to the skeleton for maintaining structural *** addition,the wrinkled and thick cell walls,together with the enhanced interlayer interactions,endow the aerogel with exceptional structural stability and *** a result,the MXene/reduced graphene oxide(RGO)composite aerogels exhibit superelasticity with reversible compressive strains of up to 95%.In addition,the electron bridging effect of the RGO sheets affords the aerogel to deliver excellent electromagnetic interference shielding performance,as high as 46.3 dB at 2.5 ***,the remarkable reshapeability of the aerogels allows for precise regulation of structure and performance(33.5-75.1 dB)by a simple wetting compression *** summary,this work offers helpful inspirations for developing lightweight and superelasticity aerogels for extensive applications.

关键词： lightweight superelasticity MXene aerogel electromagnetic interference shielding reshapeability

Sulfur atom occupying surface oxygen vacancy to boost the charge transfer and stability for aqueous Bi2O3 electrode

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Journal of Energy Chemistry 2025年第2期101卷 751-759页

作者： Guangmin Yang Jianyan Lin Guanwu Li Tian Li Dong Wang Weitao Zheng College of Physics Changchun Normal University School of Materials Science and Engineering Northwestern Polytechnical University Key laboratory of Automobile Materials of MOE School of Materials Science and Engineering and Jilin Provincial International Cooperation Key Laboratory of High-Efficiency Clean Energy Materials Jilin University

Oxygen vacancies（Ov） within metal oxide electrodes can enhance mass/charge transfer dynamics in energy storage ***,construction of surface Ovoften leads to instability in electrode structure and irreversible electrochemical reactions,posing a significant *** overcome these challenges,atomic heterostructures are employed to address the structural instability and enhance the mass/charge transfer dynamics associated with phase conversion mechanism in aqueous electrodes,Herein,we introduce an atomic S-Bi2O3heterostructure(sulfur（S） anchoring on the surface Ovof Bi2O3).The integration of S within Bi2O3lattice matrix triggers a charge imbala nce at the heterointerfaces,ultimately resulting in the creation of a built-in electric field（BEF）.Thus,the BEF attracts OH-ions to be adsorbed onto Bi within the regions of high electron cloud overlap in S-Bi2O3,facilitating highly efficient charge ***,the anchored S plays a pivotal role in preserving structural integrity,thus effectively stabilizing the phase conversion reaction of *** a result,the S-Bi2O3electrode achieves72.3 mA h g-1at 10 A g-1as well as high-capacity retention of 81.9% after 1600 *** innovative SBi2O3design presents a groundbreaking approach for fabricating electrodes that exhibit efficient and stable mass and charge transfer ***,it enhances our understanding of the underlying reaction mechanism within energy storage electrodes.

关键词： Anchoring effect Atomic heterostructure Charge/mass transfer Oxygen vavancy Structural integrity

Unifying Fixed Time and Prescribed Time Control for Strict-Feedback Nonlinear Systems

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IEEE/CAA Journal of Automatica Sinica 2025年第2期12卷 347-355页

作者： Xiang Chen Yujuan Wang Yongduan Song the State Key laboratory of Power Transmission Equipment & System Security and New Technology and School of Automation Chongqing University IEEE

This paper investigates the prescribed-time tracking control problem for a class of multi-input multi-output(MIMO)nonlinear strict-feedback systems subject to non-vanishing uncertainties. The inherent unmatched and non-vanishing uncertainties make the prescribed-time control problem become much more nontrivial. The solution to address the challenges mentioned above involves incorporating a prescribed-time filter, as opposed to a finite-time filter, and formulating a prescribed-time Lyapunov stability lemma(Lemma 5). The prescribed-time Lyapunov stability lemma is based on time axis shifting time-varying yet bounded gain, which establishes a novel link between the fixed-time and prescribed-time control method. This allows the restriction condition that the time-varying gain function must satisfy as imposed in most exist prescribed-time control works to be removed. Under the proposed control method, the desire trajectory is ensured to closely track the output of the system in prescribed time. The effectiveness of the theoretical results are verified through numerical simulation.

关键词： Prescribed-time control prescribed-time filter robust control state feedback strict-feedback systems