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High performance wide bandgap perovskite solar cell with low V_(OC) deficit less than 0.4 V

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Journal of Energy Chemistry 2024年第4期91卷 313-322页

作者： Haikuo Guo Fuhua Hou Xuli Ning Xiaoqi Ren Haoran Yang Rui Liu Tiantian Li Chengjun Zhu Ying Zhao Wei Li Xiaodan Zhang School of Physical Science and Technology Key Laboratory of Semiconductor Photovoltaic Technology and Energy Materials at Universities of Inner Mongolia Autonomous RegionInner Mongolia UniversityHohhot 010021Inner MongoliaChina Institute of Photoelectronic thin film Devices and Technology of Nankai University Key Laboratory of Photoelectronic Thin Film Devices and Technology of TianjinSolar Energy Research Center of Nankai UniversityTianjin 300350China State Key laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430000HubeiChina

Wide bandgap perovskite solar cells(PSCs)have attracted significant attention because they can be applied to the top cells of tandem solar ***,high open-circuit voltage(V_(OC))deficit(>0.4 V)result from poor crystallization and high non-radiative recombination losses become a serious limitation in the pursuit of high ***,the relevance between different Pbl_(2)proportions and performance parameters are revealed through analysis of surface morphology,residual stress,and *** increase of Pbl_(2)proportion promotes crystal growth and reduces the work function of the perovskite film surface and promotes the energy level alignment with the carrier transport layer,which decreased the V_(OC)***,residual PbI_(2)exacerbated the stress level of perovskite film,and the resulting lattice disorder deteriorated the photostability of the ***,after the synergistic passivation of residual PbI_(2)and PEAI,the V_(OC)achieves 1.266 V and V_(OC)deficit is less than 0.4 V,the record value in wide bandgap PSCs.

关键词： Pb management Perovskite solar cell Strain Wide bandgap Stability

Advancing mid-infrared microdisk laser emission with Tm:YAG

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Science China(Physics,Mechanics & Astronomy) 2024年第7期67卷 91-96页

作者： Zhaocong Wang Huiqi Li Lei Wang Yang Tan Feng Chen School of Physics State Key Laboratory of Crystal MaterialsShandong UniversityJinan 250100China

Mid-infrared microcavity lasers have important applications in biosensing,mid-infrared spectroscopy,and environmental ***,the low output power of existing mid-infrared microcavity lasers hinders their practical *** drawback is attributed to the insufficient laser gain medium,which limits the development of mid-infrared whispering-gallerymode(WGM)*** address this issue,we have employed ion implantation-enhanced etching to fabricate Tm:YAG thin films as effective gain media for mid-infrared WGM *** Tm:YAG thin film,with a thickness of 2μm,exhibits excellent fluorescence ***,the Tm:YAG thin film is processed using focused ion beam to form microdisks with a diameter of 30μ*** 785 nm laser pumping,the maximum output power of the Tm:YAG microdisk at 2023.1 nm is229μW,with a slope efficiency of 2.9%.This work demonstrates the outstanding potential of Tm:YAG as a mid-infrared laser gain medium,providing a new option for the development of mid-infrared lasers.

关键词： microdisk microlaser ultrathin film

Textured Perovskite/Silicon Tandem Solar Cells Achieving Over 30% Efficiency Promoted by 4-Fluorobenzylamine Hydroiodide

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Nano-Micro Letters 2024年第9期16卷 557-570页

作者： Jingjing Liu Biao Shi Qiaojing Xu Yucheng Li Yuxiang Li Pengfei Liu Zetong SunLi Xuejiao Wang Cong Sun Wei Han Diannan Li Sanlong Wang Dekun Zhang Guangwu Li Xiaona Du Ying Zhao Xiaodan Zhang Renewable Energy Conversion and Storage Center Solar Energy Conversion CenterInstitute of Photoelectronic Thin Film Devices and TechnologyNankai UniversityTianjin 300350People’s Republic of China Key laboratory of Photoelectronic thin film Devices and Technology of Tianjin Tianjin 300350People’s Republic of China Haihe laboratory of Sustainable Chemical Transformations Tianjin 300192People’s Republic of China Engineering Research Center of thin film Photoelectronic Technology of Ministry of Education Tianjin 300350People’s Republic of China Collaborative Innovation Center of Chemical Science and Engineering(Tianjin) Tianjin 300072People’s Republic of China Center of Single‑Molecule Sciences Institute of Modern OpticsTianjin Key Laboratory of Micro‑Scale Optical Information Science and TechnologyCollege of Electronic Information and Optical EngineeringNankai University38 Tongyan RoadJinnan DistrictTianjin 300350People’s Republic of China Shenzhen Research Institute of Nankai University 16Th FloorYantian Science and Technology BuildingHaishan StreetYantian DistrictShenzhen 518083People’s Republic of China

Monolithic textured perovskite/silicon tandem solar cells(TSCs)are expected to achieve maximum light capture at the lowest cost,potentially exhibiting the best power conversion ***,it is challenging to fabricate high-quality perovskite films and preferred crystal orientation on commercially textured silicon substrates with micrometersize ***,we introduced a bulky organic molecule(4-fluorobenzylamine hydroiodide(F-PMAI))as a perovskite *** is found that F-PMAI can retard the crystallization process of perovskite film through hydrogen bond interaction between F^(−)and FA^(+)and reduce(111)facet surface energy due to enhanced adsorption energy of F-PMAI on the(111)***,the bulky molecular is extruded to the bottom and top of perovskite film after crystal growth,which can passivate interface defects through strong interaction between F-PMA+and undercoordinated Pb^(2+)/I^(−).As a result,the additive facilitates the formation of large perovskite grains and(111)preferred orientation with a reduced trap-state density,thereby promoting charge carrier transportation,and enhancing device performance and *** perovskite/silicon TSCs achieved a champion efficiency of 30.05%based on a silicon thin film tunneling *** addition,the devices exhibit excellent longterm thermal and light stability without *** work provides an effective strategy for achieving efficient and stable TSCs.

关键词： Perovskite crystallization (111)preferred orientation Defect passivation Perovskite/silicon tandem solar cells

Wafer-level substrate-free YIG single crystal film for a broadband tunable terahertz isolator

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Photonics Research 2024年第3期12卷 505-513页

作者： XILAI ZHANG DAN ZHAO DING ZHANG QIANG XUE FEI FAN YULONG LIAO QINGHUI YANG QIYE WEN School of Electronic Science and Engineering State Key Laboratory of Electronic Thin Film and Integrated DevicesUniversity of Electronic Science and Technology of ChinaChengdu 610054China Tianjin Key laboratory of Optoelectronic Sensor and Sensing Network Technology Institute of Modern OpticsNankai UniversityTianjin 300350China Shenzhen Institute for Advanced Study University of Electronic Science and Technology of ChinaShenzhen 518110China

Yttrium iron garnet(YIG)is a promising material for various terahertz applications due to its special optical *** present,a high-quality YIG wafer is the desire of terahertz communities and it is still challenging to prepare substrate-free YIG single crystal *** this work,we prepared wafer-level substrate-free La:YIG single crystal films,for the first time,to our *** optical and magneto-optical properties of La:YIG films were characterized by terahertz time domain spectroscopy(THz-TDS).Results show that the as-prepared La:YIG film has an insertion loss of less than 3 dB and a low absorption coefficient of less than10 cm-1below 1.6 *** from the thickness of the substrate-free YIG films and low insertion loss,their terahertz properties could be further manipulated by simply using a wafer-stacking *** four La:YIG films were stacked,there was an insertion loss of less than 10 dB in the range of 0.1-1.2 *** Faraday rotation angle of the four-layer-stacked La:YIG films reached 19°,and the isolation could reach17 *** further increasing the stacking number to eight pieces,a remarkable Faraday rotation angle of45°was achieved with an isolation of 23 dB,which is important for practical application in the THz *** material may provide a milestone opportunity to make various non-reciprocal devices,such as isolators and phase shifters.

关键词： YIG film insertion

Interfacial DMI in Fe/Pt thin films grown on different buffer layers

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Chinese Physics B 2024年第4期33卷 712-718页

作者：张文君魏菲刘冰周阳康仕寿孙兵 School of Physics and Electronic Information Weifang UniversityWeifang 261061China School of Physics and State Key laboratory of crystal Materials Shandong UniversityJinan 250100China

We study the interfacial Dzyaloshinskii-Moriya interactions(i-DMI)of Fe/Pt bilayers grown on Si substrates with MgO,SiO_(2),or Ta each as a buffer layer on the basis of wave-vector-resolved Brillouin light scattering(BLS)*** obtained i-DMI energy values for Fe/Pt on MgO,Ta,and SiO_(2) buffer layers are 0.359,0.321,and 0.274 mJ/m~2,*** large i-DMI value observed in Fe/Pt system on the MgO buffer layer can be attributed to the good interfacial quality and the Rshaba effect at the MgO/Fe ***,the MgO/Fe/Pt system,benefiting from better sample quality,exhibits a lower damping ***,layer-resolved first-principles calculations are carried out to gain a more in-depth understanding of the origin of the i-DMI in the Fe/Pt *** results indicate that in the Fe(110)/Pt(111)system,the substantial DMI energy between Fe spins at the interface is related to a significant change in spin-orbit coupling(SOC)energy in the neighboring Pt *** contrast,for the MgO(002)/Fe(002)system,both the DMI and its related SOC energy are concentrated at the interfacial Fe *** investigation will provide a valuable insight into the spintronic community in exploring novel devices with chirality dependence.

关键词： Fe/Pt i-DMI BLS ferromagnetic resonance magnetic relaxation

Influence of Nd^(3+) concentration on mid-infrared emission in PbF_(2) crystal co-doped with Ho^(3+) and Nd^(3+) ions

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Journal of Rare Earths 2024年第3期42卷 479-487,I0002页

作者： Yan Chen Juncheng Tan Peixiong Zhang Weibi Zheng Lin Li Lianhan Zhang Zhen Li Yin Hang Zhenqiang Chen Department of Optoelectronic Engineering Jinan UniversityGuangzhou510632China Guangdong Provincial Engineering Research Centerof crystal and Laser Technology.Guangzhou 510632China Research Center of Laser crystal Key Laboratory of High Power Laser MaterialsShanghai Institute of Optics and Fine MechanicsChinese Academy of SciencesShanghai201800China

A promising series of Ho_(y)Nd_(x)Pb_((1-x-y))F_2(x = 0, 0.01, 0.02, 0.03, 0.04;y = 0.02) crystals was grown by the Bridgman method. The influence of the Nd^(3+)ions concentration on mid-infrared(~2.0, ~2.9 and ~3.9 μm)fluorescence emissions of Ho^(3+)ions in the PbF_(2) crystal excited by 808 nm laser diode was investigated in this work. The energy transfer mechanism between Nd^(3+)ions and Ho~(3+)ions under different concentrations of the Nd^(3+)ions was systematically analyzed. The results show that the Nd^(3+)ions have good sensitization and deactivation effect on the Ho^(3+)ions to stimulate the mid-infrared fluorescence emissions. The experimental analysis proves that the sensitization efficiency of the Nd^(3+)ions is relatively stable at around 93.45% with varying Nd^(3+)-doping concentrations. Concentration dependence studies indicate that the concentration of the Nd^(3+)ions has significant influence on mid-infrared *** the doping concentration of the Nd^(3+)ions is up to 2.0 at%, the intensity of ~2.0, ~2.9 and ~3.9 μm emissions all reach the maximum. The output characteristics of a 3.9 μm laser are simulated, and it is found that with the increase of the Nd^(3+)-doping concentration, the peak power, pulse width, and peak energy all meet the trend of first increasing and then decreasing, and Ho_(0.02)Nd_(0.02)Pb_(0.96)F_(2) crystal displays the best performance. All the results show that the Nd^(3+)/Ho^(3+)co-doped PbF_(2) crystals might act as a useful optical medium for mid-infrared laser applications.

关键词： crystal growth Mid-infrared PbF_(2) Rare earth ions

Lithium-Ion Charged Polymer Channels Flattening Lithium Metal Anode

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Nano-Micro Letters 2024年第4期16卷 379-393页

作者： Haofan Duan Yu You Gang Wang Xiangze Ou Jin Wen Qiao Huang Pengbo Lyu Yaru Liang Qingyu Li Jianyu Huang Yun‑Xiao Wang Hua‑Kun Liu Shi Xue Dou Wei‑Hong Lai Hunan Provincial Key laboratory of thin film Materials and Devices School of Material Sciences and EngineeringXiangtan UniversityXiangtan 411105People’s Republic of China Guangxi Key laboratory of Low Carbon Energy Materials School of Chemical and Pharmaceutical ScienceGuangxi Normal UniversityGuilin 541004People’s Republic of China Institute for Superconducting and Electronic Materials Australian Institute of Innovative MaterialsUniversity of WollongongInnovation CampusSquires WayNorth WollongongNSW 2500Australia Institute of Energy Materials Science University of Shanghai for Science and TechnologyShanghai 200093People’s Republic of China

The concentration difference in the near-surface region of lithium metal is the main cause of lithium dendrite *** this issue will be key to achieving high-performance lithium metal batteries(LMBs).Herein,we construct a lithium nitrate(LiNO_(3))-implanted electroactiveβphase polyvinylidene fluoride-co-hexafluoropropylene(PVDF-HFP)crystalline polymorph layer(PHL).The electronegatively charged polymer chains attain lithium ions on the surface to form lithium-ion charged *** channels act as reservoirs to sustainably release Li ions to recompense the ionic flux of electrolytes,decreasing the growth of lithium *** stretched molecular channels can also accelerate the transport of Li *** combined effects enable a high Coulombic efficiency of 97.0%for 250 cycles in lithium(Li)||copper(Cu)cell and a stable symmetric plating/stripping behavior over 2000 h at 3 mA cm^(-2)with ultrahigh Li utilization of 50%.Furthermore,the full cell coupled with PHL-Cu@Li anode and Li Fe PO_(4) cathode exhibits long-term cycle stability with high-capacity retention of 95.9%after 900 ***,the full cell paired with LiNi_(0.87)Co_(0.1)Mn_(0.03)O_(2)maintains a discharge capacity of 170.0 mAh g^(-1)with a capacity retention of 84.3%after 100 cycles even under harsh condition of ultralow N/P ratio of *** facile strategy will widen the potential application of LiNO_(3)in ester-based electrolyte for practical high-voltage LMBs.

关键词： Polymer ionic channel Li metal batteries Artificial protective layer Uniform Li deposition Electrochemical performances

Stable photocurrent-voltage characteristics of perovskite single crystal detectors obtained by pulsed bias

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Chinese Physics B 2024年第4期33卷 209-214页

作者：刘新陈之龙王虎张雯清董昊王鹏祥邵宇川 laboratory of thin film Optics Shanghai Institute of Optics and Fine MechanicsChinese Academy of SciencesShanghai 201800China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Key laboratory of Materials for High-Power Laser Shanghai Institute of Optics and Fine MechanicsChinese Academy of SciencesShanghai 201800China Key laboratory for Ultrafine Materials of Ministry of Education Shanghai Engineering Research Center of Hierarchical NanomaterialsSchool of Materials Science and EngineeringEast China University of Science and TechnologyShanghai 200237China School of Microelectronics Shanghai UniversityShanghai 201899China Hangzhou Institute for Advanced Study University of Chinese Academy of SciencesHangzhou 310024China

Photocurrent-voltage characterization is a crucial method for assessing key parameters in x-ray or y-ray semiconductor detectors,especially the carrier mobility lifetime ***,the high biases during photocurrent measurements tend to cause severe ion migration,which can lead to the instability and inaccuracy of the test *** the mixed electronic-ionic charac teristics,it is imperative to devise novel methods capable of precisely measuring photocurrentvoltage characteristics under high bias conditions,free from interference caused by ion *** this paper,pulsed bias is employed to explore the photocurrent-voltage characteristics of MAPbBr_(3) single *** method yields stable photocurrent-voltage characteristics at a pulsed bias of up to 30 V,proving to be effective in mitigating ion *** fitting the modified Hecht equation,we determined the mobility lifetime products of 1.0×10^(2) cm^(2)·V^(-1)for hole and 2.78×10~(-3)cm^(2)·V^(-1)for *** approach offers a promising solution for accurately measuring the transport properties of carriers in perovskite.

关键词： perovskites ion migration pulsed bias mobility lifetime product

Optical secret sharing by multi-step liquid crystal planar doublet panning and coupling

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Chinese Optics Letters 2024年第8期 26-33页

作者：莫之畅陈壹朱翔宇张洲豪李大伟邵建达赵元安王建国 laboratory of thin film Optics Shanghai Institute of Optics and Fine Mechanics Chinese Academy of Sciences Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of Sciences Key laboratory of Materials for High Power Laser Chinese Academy of Sciences Henan Key laboratory of Infrared Materials & Spectrum Measures and Applications School of Physics Henan Normal University Hangzhou Institute for Advanced Study University of Chinese Academy of Sciences

The hologram, which is formed by phases coupled through cascade devices for secret information sharing, still carries a cracking risk. We propose a liquid crystal planar doublet as the information carrier, and new holograms generated by the new coupled phases when the relative displacements of the different liquid crystal layers change. The designed geometrical phases are generated by an optimized iterative restoration algorithm, and each holographic image formed by these phases is readable. This scheme achieves an increase in the capacity of the stored secret information and provides more misdirection, which is expected to have potential value in optical steganography and storage.

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