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Ru/NiMnB spherical cluster pillar for highly proficient green hydrogen electrocatalyst at high current density

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Journal of Energy Chemistry 2025年第1期100卷 397-408页

作者： Md Ahasan Habib Shusen Lin Mehedi Hasan Joni Sumiya Akter Dristy Rutuja Mandavkar Jae-Hun Jeong Jihoon Lee Department of electronic engineering College of Electronics and InformationKwangwoon UniversityNowon-guSeoul 01897Republic of Korea

Advanced OER/HER electrocatalytic alternatives are crucial for the wide adaptation of green hydrogen ***,Ru/NiMnB spherical cluster pillar(SCP),denoted as Ru/NiMnB,is synthesized using a combination of electro-deposition and hydrothermal *** investigation of Ru doping in the NiMnB matrix revealed significant improvements in electrocatalytic *** Ru/NiMnB SCPs demonstrate superior OER/HER activity with low overpotentials of 150 and 103 mV at 50mA/cm^(2)in 1 M KOH,making them highly competitive with state-of-the-art ***,the Ru/NiMnB SCPs exhibit a low 2-E cell voltage of 2.80 V at ultra-high current density of 2,000 m A/cm^(2)in 1 M KOH,outperforming the standard benchmark electrodes of RuO_(2)||Pt/C,thereby positioning Ru/NiMnB as one of the best bifunctional *** SCPs exhibit exceptional high-current characteristics,stability and corrosion resistance,as evidenced by continuous operation at 1,000 mA/cm^(2)high-current density for over 150 h in 6 M KOH at elevated temperatures under harsh industrial *** a small amount of Ru incorporation significantly enhances the electrocatalytic performances of NiMnB,attributed to increased active sites and improved intrinsic properties such as conductivity,adsorption/desorption capability and reaction ***,Ru/NiMnB SCPs present a promising bi-functional electrode concept for efficient green H_(2)production.

关键词： Advanced electrocatalyst High current Corrosion resistance Industrial requirement

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An Improved Practical Byzantine Fault-Tolerant Algorithm Based on XGBoost Grouping for Consortium Chains

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Computers, Materials & Continua 2025年第1期82卷 1295-1311页

作者： Xiaowei Wang Haiyang Zhang Jiasheng Zhang Yingkai Ge Kexin Cui Zifu Peng Zhengyi Li Lihua Wang college of electronic and information engineering Shandong University of Science and TechnologyQingdao266590China

In response to the challenges presented by the unreliable identity of the master node,high communication overhead,and limited network support size within the Practical Byzantine Fault-Tolerant(PBFT)algorithm for consortium chains,we propose an improved PBFT algorithm based on XGBoost grouping called XG-PBFT in this ***-PBFT constructs a dataset by training important parameters that affect node performance,which are used as classification indexes for *** XGBoost algorithm then is employed to train the dataset,and nodes joining the system will be grouped according to the trained grouping *** them,the nodes with higher parameter indexes will be assigned to the consensus group to participate in the consensus,and the rest of the nodes will be assigned to the general group to receive the consensus *** order to reduce the resource waste of the system,XG-PBFT optimizes the consensus protocol for the problem of high complexity of PBFT ***,we evaluate the performance of *** experimental results show that XG-PBFT can significantly improve the performance of throughput,consensus delay and communication complexity compared to the original PBFT algorithm,and the performance enhancement is significant compared to other algorithms in the case of a larger number of *** results demonstrate that the XG-PBFT algorithm is more suitable for large-scale consortium chains.

关键词： Consortium chain PBFT grouping reputation XGBoost

Phase-matching enhanced quantum phase and amplitude estimation of a two-level system in a squeezed reservoir

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Chinese Physics B 2025年第1期34卷 257-263页

作者： Yan-Ling Li Cai-Hong Liao Xing Xiao School of information engineering Jiangxi University of Science and TechnologyGanzhou 341000China college of Physics and electronic information Gannan Normal UniversityGanzhou 341000China

Squeezed reservoir engineering is a powerful technique in quantum information that combines the features of squeezing and reservoir engineering to create and stabilize non-classical quantum states. In this paper, we focus on the previously neglected aspect of the impact of the squeezing phase on the precision of quantum phase and amplitude estimation based on a simple model of a two-level system(TLS) interacting with a squeezed reservoir. We derive the optimal squeezed phase-matching conditions for phase φ and amplitude θ parameters, which are crucial for enhancing the precision of quantum parameter estimation. The robustness of the squeezing-enhanced quantum Fisher information against departures from these conditions is examined, demonstrating that minor deviations from phase-matching can still result in remarkable precision of estimation. Additionally, we provide a geometric interpretation of the squeezed phase-matching conditions from the classical motion of a TLS on the Bloch sphere. Our research contributes to a deeper understanding of the operational requirements for employing squeezed reservoir engineering to advance quantum parameter estimation.

关键词： quantum parameter estimation squeezed reservoir phase-matching conditions quantum Fisher information

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PltcRB:a practical distributed randomness beacon with optimal amortized communication complexity

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Science China(information Sciences) 2025年第2期68卷 269-284页

作者： Zheyi WU Haolin LIU Lei WANG School of electronic information and Electrical engineering Shanghai Jiao Tong University

The distributed randomness beacon(DRB) is a crucial tool for continuously generating unpredictable, bias-resistant,and publicly verifiable random numbers on a regular basis. This is particularly useful for applications such as lotteries, electronic voting, and cryptographic parameter generation. However, existing studies either require complex communication or rely on a public bulletin board to meet security requirements. This brings a performance bottleneck when dealing with a large number of participants. This paper introduces a novel DRB protocol PltcRB based on timed commitments, eliminating the need for a public bulletin board. Our approach achieves optimal communication complexity of O(n) while maintaining the desired properties of a DRB protocol. The computation complexity is also O(n) when n is larger than the security parameter κ. These results demonstrate the practicality and performance of PltcRB, supported by our experimental analysis under various configurations.

关键词： timed commitment randomness beacon random number optimal communication complexity permissionlessłinebreak setting

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Low dielectric loss in vanadium-based zircon ceramics via high-entropy strategy

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Journal of Advanced Ceramics 2025年第1期14卷 151-161页

作者： Yuheng Zhang Huaicheng Xiang Xiaoyu Wu Yang Zhou Ying Tang Liang Fang college of Physics and electronic information engineering Guilin University of TechnologyGuilin 541004China Guangxi Universities Key Laboratory of Non-Ferrous Metal Oxide electronic Functional Materials and Devices Guangxi Key Laboratory of Optical and Electronic Materials and DevicesCollege of Materials Science and EngineeringGuilin University of TechnologyGuilin 541004China

Zircon ceramics have potential applications in next-generation wireless communication because of their low permittivity and adjustable temperature coefficient at microwave ***,the vast challenge of realizing ultralow dielectric loss still ***,we propose a high-entropy strategy to enhance the bonding of the A-site dodecahedron in zircon and design(Nd0.2Eu0.2Y0.2Ho0.2Yb0.2)VO4 ceramics with a high quality factor(high Q×f,that is,low dielectric loss).The(Nd0.2Eu0.2Y0.2Ho0.2Yb0.2)VO4 high-entropy ceramics,which belong to the tetragonal zircon structure with the I41/amd space group,exhibit a low relative permittivity(εr=11.55),a negative temperature coefficient of resonant frequency(τf=−37.3 ppm/℃),and a high Q×f of 76,400 GHz(at 12.31 GHz).The high Q×f value can be attributed to the high chemical bond strength and structural ***,the relationship between the crystal structure and the microwave dielectric properties of(Nd0.2Eu0.2Y0.2Ho0.2Yb0.2)VO4 high-entropy ceramics was analyzed through high resolution transmission electron microscopy(HRTEM),Raman spectroscopy,far-infrared reflection spectroscopy,and chemical bond *** work provides an effective avenue for designing microwave dielectric materials with low loss to meet the demands of passive components.

关键词： high-entropy ceramics vanadium-based zircon microwavedielectric properties low dielectric loss chemical bond characteristics

Enhanced dynamics of Al3+/H+ ions in aqueous aluminum ion batteries:Construction of metastable structures in vanadium pentoxide upon oxygen vacancies

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Journal of Energy Chemistry 2025年第2期101卷 562-569页

作者： Zhibao Wang Hanqing Gu Tianci Wu Wenming Zhang Zhanyu Li Hebei Key Laboratory of Optic-electronic information and Materials National & Local Joint Engineering Laboratory of New Energy Photoelectric Devices College of Physics Science and Technology Hebei University

In recent years,aqueous aluminum ion batteries have been widely studied owing to their abundant energy storage and high theo retical *** in-depth study of vanadium oxide materials is necessary to address the precipitation of insoluble products covered cathode surface and the slow reaction ***,a method using a simple one-step hydrothermal preparation and oxalic acid to regulate oxygen vacancies has been reported.A high starting capacity(400 mAh g-1) can be achieved by Ov-V2O5,and it is capable of undergoing 200 cycles at 0.4 A g-1,with a termination discharge capacity of103 mAh *** analysis demonstrated that metastable structures（AlxV2O5and HxV2O5） were constructed through the insertion of Al3+/H+during discharging,which existed in the lattice intercalation with *** incorporation of oxygen vacancies lowers the reaction energy barrier while improving the ion transport *** addition,the metastable structure allows the electrostatic interaction between Al3+and the main backbone to establish protection and optimize the transport *** parallel,this work exploits ex-situ characterization and DFT to obtain a profound insight into the instrumental effect of oxygen vacancies in the construction of metastable structures during in-situ electrochemical activation,with a view to better understanding the mechanism of the synergistic participation of Al3+and H+in the *** work not only reports a method for cathode materials to modulate oxygen vacancies,but also lays the foundation for a deeper understanding of the metastable structure of vanadium oxides.

关键词： Electrochemical activation Metastable structure Oxygen vacancies Vanadium pentoxide

A robust multi-VSGs coordinated control strategy for distributed secondary frequency regulation in islanded microgrids

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Science China Technological Sciences 2025年第3期68卷 335-352页

作者： Jing ZHANG Yong LI Jinjie LIN Sijia HU Yijia CAO Fang LIU Mingmin ZHANG Li HE college of Electrical and information engineering Hunan University Greater Bay Area Institute for Innovation Hunan University college of information Science and engineering Central South University college of electronic information and Electrical engineering Changsha University college of information and Electrical engineering Hunan University of Science and Technology

Islanded microgrids(IMGs) offer a viable and efficient energy self-sustaining solution for distributed resources in remote areas. While without utility grid support, the frequency of IMG is susceptible to mismatches between demand and generation. Moreover, IMGs encounter uncertain and nonlinear load disturbances together with system parameter perturbation,which further compromises frequency stability. To this aim, this paper proposes a robust multi-virtual synchronous generators(multi-VSGs) coordinated control strategy for distributed secondary frequency regulation(DSFR) in IMGs, which exhibits minimal model dependency and avoids reliance on global information. Two critical methods are developed:(1) a robust VSG control framework that incorporates the linear active disturbance rejection control(LADRC) technique, which enables the estimation and effective elimination of uncertain load disturbances and system's parameter perturbations;(2) a novel secondorder consensus algorithm-based control law for robust secondary frequency regulation, which is featured with proper power sharing among different participants, suppressed power oscillation caused by response disparities, and reduced reliance on complex communication system. Building on methods(1) and(2), a novel multi-VSGs coordinated control strategy is proposed, providing a robust solution for IMG's frequency restoration, and its dynamic characteristics are explored in detail. The correctness and effectiveness of the proposal are verified by both simulation and the hardware-in-the-loop(HIL) experiment results across typical scenarios.

关键词： islanded microgrid (IMG) distributed secondary frequency regulation (DSFR) robust multi-VSGs coordinated control linear active disturbance rejection control (LADRC)

Intelligent integrated sensing and communication:a survey

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Science China(information Sciences) 2025年第03期68卷 5-46页

作者： Jifa ZHANG Weidang LU Chengwen XING Nan ZHAO Naofal AL-DHAHIR George K.KARAGIANNIDIS Xiaoniu YANG School of information and Communication engineering Dalian University of Technology college of information engineering Zhejiang University of Technology School of information and electronics Beijing Institute of Technology Department of Electrical and Computer engineering The University of Texas at Dallas Department of Electrical and Computer engineering Aristotle University of Thessaloniki

Integrated sensing and communication (ISAC) is a promising technique to increase spectral efficiency and support various emerging applications by sharing the spectrum and hardware between these functionalities. However, the traditional ISAC schemes are highly dependent on the accurate mathematical model and suffer from the challenges of high complexity and poor performance in practical scenarios. Recently, artificial intelligence (AI) has emerged as a viable technique to address these issues due to its powerful learning capabilities, satisfactory generalization capability, fast inference speed, and high adaptability for dynamic environments, facilitating a system design shift from model-driven to data-driven. Intelligent ISAC, which integrates AI into ISAC, has been a hot topic that has attracted many researchers to investigate. In this paper, we provide a comprehensive overview of intelligent ISAC, including its motivation, typical applications, recent trends, and challenges. In particular, we first introduce the basic principle of ISAC, followed by its key techniques. Then, an overview of AI and a comparison between model-based and AI-based methods for ISAC are provided. Furthermore, the typical applications of AI in ISAC and the recent trends for AI-enabled ISAC are reviewed. Finally, the future research issues and challenges of intelligent ISAC are discussed.

关键词： artificial intelligence deep learning deep reinforcement learning federated learning generative artificial intelligence integrated sensing and communication machine learning transfer learning

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Distributed optimal consensus control for multiagent systems based on event-triggered and prioritized experience replay strategies

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Science China(information Sciences) 2025年第1期68卷 306-321页

作者： Cuijuan ZHANG Lianghao JI Shasha YANG Xing GUO Huaqing LI Chongqing Key Laboratory of Image Cognition Chongqing University of Posts and Telecommunications Key Laboratory of Intelligent Perception and Computing of Anhui Province Anqing Normal University college of electronic and information engineering Southwest University

This study uses event-triggered(ET) and reinforcement learning methods to investigate the optimal consensus control problem for cooperative-competitive multiagent systems. It proposes a novel distributed ET control strategy, which relies on a prioritized experience replay(PER) policy. This strategy not only conserves communication resources but also ensures acceptable system performance. To implement the proposed method, actor-critic(AC) dual-structured neural networks(NNs) are used to approximate the value function and control policy. In the AC NNs, the weight estimates for the NNs are updated at the moment of event triggering, resulting in a nonperiodic weight adjustment pattern. This approach decreases the computational cost in comparison with the traditional ET mechanism. The PER-based ET mechanism makes full use of valid historical data and effectively establishes a balance between system performance and communication resource ***, it does not require the following two conditions in most existing studies:(1) requirement of the system dynamics model to be known, and(2) persistent excitation. In addition, Zeno behavior is excluded from this study. Finally, a simulation is conducted to confirm the validity of the suggested approach.

关键词： multiagent systems event-triggered mechanism prioritized experience replay dual-structured neural networks optimal consensus control