检索结果-南通市图书馆

Multifunctional Film Assembled from N‑Doped Carbon Nanofiber with Co–N_(4)–O Single Atoms for Highly Efficient Electromagnetic Energy Attenuation

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Nano-Micro Letters 2024年第11期16卷 359-376页

作者： Jia Xu Bei Li Zheng Ma Xiao Zhang Chunling Zhu Feng Yan Piaoping Yang Yujin Chen college of Materials science and Chemical engineering Harbin Engineering UniversityHarbin 150001People’s Republic of China Key Laboratory of In‑Fiber Integrated Optics College of Physics and Optoelectronic EngineeringHarbin Engineering UniversityHarbin 150001People’s Republic of China

Single-atom materials have demonstrated attractive physicochemical ***,understanding the relationships between the coordination environment of single atoms and their properties at the atomic level remains a considerable ***,a facile waterassisted carbonization approach is developed to fabricate well-defined asymmetrically coordinated Co–N_(4)–O sites on biomass-derived carbon nanofiber(Co–N_(4)–O/NCF)for electromagnetic wave(EMW)*** such nanofiber,one atomically dispersed Co site is coordinated with four N atoms in the graphene basal plane and one oxygen atom in the axial ***-depth experimental and theoretical studies reveal that the axial Co–O coordination breaks the charge distribution symmetry in the planar porphyrin-like Co–N_(4) structure,leading to significantly enhanced dielectric polarization loss relevant to the planar Co–N_(4) ***,the film based on Co–N_(4)–O/NCF exhibits light weight,flexibility,excellent mechanical properties,great thermal insulating feature,and excellent EMW absorption with a reflection loss of−45.82 dB along with an effective absorption bandwidth of 4.8 *** findings of this work offer insight into the relationships between the single-atom coordination environment and the dielectric performance,and the proposed strategy can be extended toward the engineering of asymmetrically coordinated single atoms for various applications.

关键词： Co single atoms Asymmetric coordination structure Axial oxygen coordination Electromagnetic wave absorption Multifunctional film

In vivo label-free measurement of blood flow velocity symmetry based on dual line scanning third-harmonic generation microscopy excited at the 1700 nm window

在线全文

学校读者我要写书评

暂无评论

Journal of Innovative Optical Health sciences 2024年第1期17卷 61-68页

作者： Hui Cheng Jincheng Zhong Ping Qiu Ke Wang Key Laboratory of optoelectronic Devices and Systems of Ministry of Education and Guangdong Province college of Physics and optoelectronic engineering Shenzhen University Shenzhen 518060 P.R.China

Measurement of bloodflow velocity is key to understanding physiology and pathology in *** most measurements are performed at the middle of the blood vessel,little research has been done on characterizing the instantaneous bloodflow velocity *** is mainly due to the lack of measurement technology with high spatial and temporal ***,we tackle this problem with our recently developed dual-wavelength line-scan third-harmonic generation(THG)imaging *** acquisition of dual-wavelength THG line-scanning signals enables measurement of bloodflow velocities at two radially symmetric positions in both venules and arterioles in mouse brain in *** results clearly show that the instantaneous bloodflow velocity is not symmetric under general conditions.

关键词： 1700 nm-Window third-harmonic generation imaging blood flow velocity

Chlorofullerene C_(60)Cl_(6) Enables Efficient and Stable Tin-Based Perovskite Solar Cells

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Energy & Environmental Materials 2024年第1期7卷 176-183页

作者： Jingfu Chen Chengbo Tian Chao Sun Panpan Yang Wenjing Feng Lingfang Zheng Liu Yang Enlong Hou Jiefeng Luo Liqiang Xie Zhanhua Wei Xiamen Key Laboratory of optoelectronic Materials and Advanced Manufacturing Institute of Luminescent Materials and Information DisplaysCollege of Materials Science and EngineeringHuaqiao UniversityXiamen 361021China

Tin-based perovskite solar cells(TPSCs)have received great attention due to their eco-friendly properties and high theoretical ***,the fast crystallization feature of tin-based perovskites leads to poor film quality and limits the corresponding device ***,a chlorofullerene,C_(60)Cl_(6),with six chlorine attached to the C_(60)cage,is applied to modulate the crystallization process and passivate grain boundary defects of the perovskite *** chemical interactions between C_(60)Cl_(6)and perovskite components retard the transforming process of precursors to perovskite crystals and obtain a high-quality tin-based perovskite *** is also revealed that the C_(60)Cl_(6)located at the surfaces and grain boundaries can not only passivate the defects but also offer a role in suturing grain boundaries to suppress the detrimental effects of water and oxygen on perovskite films,especially the oxidation of Sn^(2+)to Sn^(4+).As a result,the C_(60)Cl_(6)-based device yields a remarkably improved device efficiency from 10.03%to 13.30%with enhanced *** work provides a new strategy to regulate the film quality and stability of TPSCs using functional fullerene materials.

关键词： crystallization regulation defect passivation fullerene derivative perovskites solar cell tin-based perovskite

Stabilizing semi-transparent perovskite solar cells with a polymer composite hole transport layer

在线全文

学校读者我要写书评

暂无评论

Nano Research 2024年第3期17卷 1500-1507页

作者： Yongbin Jin Huiping Feng Zheng Fang Liu Yang Kaikai Liu Bingru Deng Jingfu Chen Xueling Chen Yawen Zhong Jinxin Yang Chengbo Tian Liqiang Xie Zhanhua Wei Xiamen Key Laboratory of optoelectronic Materials and Advanced Manufacturing Institute of Luminescent Materials and Information DisplaysCollege of Materials Science and EngineeringHuaqiao UniversityXiamen 361021China

Semi-transparent perovskite solar cells(ST-PSCs)have broad applications in building integrated ***,the stability of ST-PSCs needs to be improved,especially in n-i-p ST-PSCs since the doped 2,2',7,7'-tetrakis(N,N-di-p-methoxyphenyl-amine)-9,9'-spirobifluorene(Spiro-OMeTAD)is unstable at elevated temperatures and high *** this work,aπ-conjugated polymer poly[(2,6-(4,8-bis(5-(2-ethylhexyl)thiophene-2-yl)-benzo[1,2-b:4,5-b']dithiophene))-alt-(5,5-(1',3'-di-2-thienyl-5',7'-bis(2-ethylhexyl)benzo[1',2'-c:4',5'-c']dithiophene-4,8-dione)](PBDB-T)is selected to form a polymer composite hole transport layer(HTL)with *** sulfur atom of the thiophene unit and the carbonyl group of the polymer interact with the undercoordinated Pb2+at the perovskite surface,which stabilizes the perovskite/HTL interface and passivates the interfacial *** incorporation of the polymer also increases the glass transition temperature and the moisture resistance of *** a result,we obtain ST-PSCs with a champion efficiency of 13.71%and an average visible light transmittance of 36.04%.Therefore,a high light utilization efficiency of 4.94%can be ***,the encapsulated device can maintain 84%of the initial efficiency after 751 h under continuous one-sun illumination(at 30%relative humidity)at the open circuit and the unencapsulated device can maintain 80%of the initial efficiency after maximum power tracking for more than 1250 h under continuous one-sun illumination.

关键词： semi-transparent solar cells π-conjugated polymer composite hole transport layer building integrated photovoltaics

Ultra-homogeneous dense Ag nano layer enables long lifespan solid-state lithium metal batteries

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Journal of Energy Chemistry 2024年第9期96卷 110-119页

作者： Yaning Liu Tianqi Yang Ruyi Fang Chengwei Lu Ruojian Ma Ke Yue Zhen Xiao Xiaozheng Zhou Wenkui Zhang Xinping He Yongping Gan Jun Zhang Xinhui Xia Hui Huang Xinyong Tao Yang Xia college of Materials science and engineering Zhejiang University of TechnologyHangzhou 310014ZhejiangChina Key Laboratory of Rare Earth optoelectronic Materials and Devices of Zhejiang Province Institute of Optoelectronic Materials and DevicesChina Jiliang UniversityHangzhou 310018ZhejiangChina

The unstable electrolyte/lithium(Li)anode interface has been one of the key challenges in realizing high energy density solid-state lithium metal batteries(LMBs)***,a dense and uniform silver(Ag)nano interlayer with a thickness of∼35 nm is designed accurately by magnetron sputtering technology to optimize the electrolyte/Li anode *** Ag nano layer reacts with Li metal anode to in-situ form Li-Ag alloy,thus enhancing the physical interfacial contact,and further improving the interfacial wettability and *** particular,the Li-Ag alloy is inclined to form AgLi phase proved by cryo-TEM and DFT,effectively preventing SN from continuously“attacking”the Li metal anode due to the lower adsorption of succinonitrile(SN)molecules on AgLi than that of pure Li metal,thereby significantly reinforcing the interfacial ***,the enhanced physical and chemical stability of electrolyte/Li anode interface promotes the homogeneous deposition of Li^(+)and inhibits the dendrite *** Li-symmetric cell maintains stable operation for up to 1700 h and the cycling stability of LiFePO_(4)|SPE|Li full cell is remarkably improved at room temperature(capacity retention rate of 91.9%for 200 cycles).This work opens an effective way for accurate and controllable interface design of long lifespan solid-state LMBs.

关键词： Silvernano layer Poly(ethylene oxide) Solid polymer electrolyte Succinonitrile Lithium metal battery

Highly transparent anti-reflection coating enhances the underwater efficiency and stability of perovskite solar modules

在线全文

学校读者我要写书评

暂无评论

Nano Research 2024年第9期17卷 8126-8133页

作者： Feng Qian Shihao Yuan Ting Zhang Lei Wang Xiaobo Li Hualin Zheng Qien Xu Zhi David Chen Shibin Li School of optoelectronic science and engineering University of Electronic Science and Technology of ChinaChengdu 610054China Department of Electrical and Computer engineering and Center for Nanoscale science and engineering University of KentuckyLexingtonKentucky 40506USA

Perovskite solar cells have shown great potential in the field of underwater solar cells due to their excellent optoelectronic properties;however,their underwater performance and stability still hinder their practical *** this research,a 1H,1H,2H,2H-heptadecafluorodecyl acrylate(HFDA)anti-reflection coating(ARC)was introduced as a high-transparent material for encapsulating perovskite solar modules(PSMs).Optical characterization results revealed that HFDA can effectively reduce reflection of light below 800 nm,aiding in the absorption of light within this wavelength range by underwater solar ***,a remarkable efficiency of 14.65%was achieved even at a water depth of 50 ***,the concentration of Pb^(2+)for HFDA-encapsulated film is significantly reduced from 186 to 16.5 ppb after being immersed in water for 347 ***,the encapsulated PSMs still remained above 80%of their initial efficiency after continuous underwater illumination for 400 ***,being exposed to air,the encapsulated PSMs maintained 94%of their original efficiency after 1000 h light *** highly transparent ARC shows great potentials in enhancing the stability of perovskite devices,applicable not only to underwater cells but also extendable to land-based photovoltaic devices.

关键词： underwater photovoltaics perovskite solar modules anti-reflection coating underwater stability

Ultrafast pulse-dilation framing camera and its application for time-resolved X-ray diagnostic

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Nuclear science and Techniques 2024年第7期35卷 101-114页

作者： Hou-Zhi Cai Qiu-Yan Luo Kai-Xuan Lin Xuan Deng Jun-Kai Liu Kai-Zhi Yang Dong Wang Jia-Jie Chen Jia-Heng Wang Jing-Hua Long Li-Hong Niu Yun-Fei Lei Jin-Yuan Liu Key Laboratory of optoelectronic Devices and Systems of Ministry of Education and Guangdong Province Shenzhen Key Laboratory of Photonics and BiophotonicsCollege of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen518060China

An ultrafast framing camera with a pulse-dilation device,a microchannel plate(MCP)imager,and an electronic imaging system were *** camera achieved a temporal resolution of 10 ps by using a pulse-dilation device and gated MCP imager,and a spatial resolution of 100μm by using an electronic imaging system comprising combined magnetic *** spatial resolution characteristics of the camera were studied both theoretically and *** results showed that the camera with combined magnetic lenses reduced the field curvature and acquired a larger working area.A working area with a diameter of 53 mm was created by applying four magnetic lenses to the ***,the camera was used to detect the X-rays produced by the laser-targeting *** diagnostic results indicated that the width of the X-ray pulse was approximately 18 ps.

关键词： Inertial confinement fusion Plasma diagnostics Framing camera Combined lenses Pulse-dilation

Mechanoluminescent Materials Enable Mechanochemically Controlled Atom Transfer Radical Polymerization and Polymer Mechanotransduction

在线全文

学校读者我要写书评

暂无评论

Research 2024年第3期2023卷 97-104页

作者： Zexuan Li Zhenhua Wang Chen Wang Wenxi Li Wenru Fan Ruoqing Zhao Haoyang Feng Dengfeng Peng Wei Huang Frontiers science Center for Flexible Electronics Institute of Flexible ElectronicsNorthwestern Polytechnical UniversityXi’an 710072China. School of Materials science and engineering Northwestern Polytechnical UniversityXi’an 710072China Key Laboratory of optoelectronic Devices and Systems of Ministry of Education and Guangdong Province College of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen 518060China.

Organic mechanophores have been widely adopted for polymer ***,most examples of polymer mechanotransduction inevitably experience macromolecular chain rupture,and few of them mimic mussel’s mechanochemical regeneration,a mechanically mediated process from functional units to functional materials in a controlled *** this paper,inorganic mechanoluminescent(ML)materials composed of CaZnOS-ZnS-SrZnOS:Mn2+were used as a mechanotransducer since it features both piezoelectricity and *** utilization of ML materials in polymerization enables both mechanochemically controlled radical polymerization and the synthesis of ML polymer *** procedure features a mechanochemically controlled manner for the design and synthesis of diverse mechanoresponsive polymer composites.

关键词： chemically polymerization luminescent

Effects of vacancy and external electric field on the electronic properties of the MoSi_(2)N_(4)/graphene heterostructure

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Chinese Physics B 2024年第3期33卷 542-550页

作者：梁前罗祥燕钱国林王远帆梁永超谢泉 college of Big Data and Information engineering Institute of New Optoelectronic Materials and TechnologyGuizhou UniversityGuiyang 550025China

Recently,the newly synthesized septuple-atomic layer two-dimensional(2D)material MoSi_(2)N_(4)(MSN)has attracted attention *** work delves into the effect of vacancies and external electric fields on the electronic properties of the MSN/graphene(Gr)heterostructure using first-principles *** find that four types of defective structures,N-in,N-out,Si and Mo vacancy defects of monolayer MSN and MSN/Gr heterostructure are stable in ***,vacancy defects can effectively modulate the charge transfer at the interface of the MSN/Gr heterostructure as well as the work function of the pristine monolayer MSN and MSN/Gr ***,the application of an external electric field enables the dynamic switching between n-type and p-type Schottky *** work may offer the possibility of exceeding the capabilities of conventional Schottky diodes based on MSN/Gr heterostructures.

关键词： MoSi_(2)N_(4) vacancy defects external electric field Schottky contacts