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Excellent energy storage properties in non-stoichiometric Bi_(0.5)Na_(0.5)TiO_(3)-based relaxor ferroelectric ceramics

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Chinese Chemical Letters 2024年第7期35卷 470-472页

作者： Shunshun Jiang Ji Zhang Jing Wang Shan-Tao Zhang School of materials science and Engineering Nanjing University of Science&TechnologyNanjing 210094China State Key Laboratory of mechanics and Control of Mechanical Structures College of Aerospace EngineeringNanjing University of Aeronautics and AstronauticsNanjing 210016China National Laboratory of Solid State Microstructures Department of Materials Science and EngineeringCollege of Engineering and Applied Science&Jiangsu Key Laboratory of Artificial Functional Materials&Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210093China

The rapid development of high-power and pulsed-power techniques inspires extensive investigates on high-performance ceramic-based ***,the low recoverable energy density(Wrec)hampers their wider ***,the non-stoichiometric Bi_(0.5)Na_(0.5)TiO_(3)-based ceramics were designed and *** proper introduction of oxygen vacancies facilitated activating defect dipole,giving rise to reduced remanent ***,the optimal composition exhibited an exceptional high Wrec of 8.3 J/cm^(3),a high efficiency of 85%,and excellent anti-fatigue and thermal *** work provides an efficient approach to explore ceramic capacitors with high capacitive energy storage performances.

关键词： Non-stoichiometric Bi_(0.5)Na_(0.5)TiO_(3) Ceramic capacitor Energy density Thermal stability

Energy band modulation of N-doped rutile/anatase TiO_(2) photoanode promoting charge separation toward prominent photoelectrochemical performance

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Rare Metals 2024年第8期43卷 3784-3797页

作者： Juan Gao Shi-Xuan Wang Jia-Le Deng Ping-Ping Wei Fu-Zhang Chen Ling-Cheng Zheng Yue-Qin Wang Yang Li Yin Liu Gang He School of mechanics and Photoelectric Physics Anhui University of Science and TechnologyHuainan 232001China School of materials science and Engineering Anhui UniversityHefei230039China Tianneng Battery(Wuhu)Co. Ltd.Wuhu 241000China School of materials science and Engineering Anhui University of Science and TechnologyHuainan 232001China

To solve the problem of high photogenerated carrier recombination rate and low photoelectric conversion efficiency of TiO_(2)-based materials,a simple N-doped anatase/rutile TiO_(2) heterophase nanorod film was designed by a low-temperature hydrothermal method in this *** enhanced separation and transport of photogenerated charges were facilitated by the smaller contact barrier and appropriate band matching between anatase TiO_(2)nanoparticles and rutile TiO_(2) *** introduction of N doping in anatase TiO_(2) resulted in an upward shift of the valence band and a narrowing of the band gap,consequently enhancing the efficiency of visible light *** combination of the heterophase junction and N-doping exhibited a synergistic effect,effectively suppressing the recombination of photogenerated charges and enhancing the photoelectric conversion efficiency of the *** AM 1.5G irradiation,the photocurrent density(J)of the A-TO(N)@R-TONR photoanode reached2.19 mA·cm^(-2)(V_(RHE,1.23 eV)).Additionally,the incident photon-electron conversion efficiency(IPCE)and the charge injection efficiency(η)reached 81.4%and 51.6%at320 ***,the J,IPCE,andηvalues of the A-TO(N)@R-TONR photoanode were 2.96,2.1 and 3.2times those of pure R-TONR photoanode,*** work presents a rational strategy for designing efficient TiO_(2)-based photoanodes.

关键词： TiO_(2) Heterophase junction Photoanode

Sub-Homogeneous Peridynamic Model for Fracture and Failure Analysis of Roadway Surrounding Rock

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Computer Modeling in Engineering & sciences 2024年第6期139卷 3167-3187页

作者： Shijun Zhao Qing Zhang Yusong Miao Weizhao Zhang Xinbo Zhao Wei Xu School of science Qingdao University of TechnologyQingdao266520China college of mechanics and materials Hohai UniversityNanjing211100China Xibei Mining Co. Ltd.Shandong Energy GroupXi’an710018China

The surrounding rock of roadways exhibits intricate characteristics of discontinuity and *** address these complexities,this study employs non-local Peridynamics(PD)theory and reconstructs the kernel function to represent accurately the spatial decline of long-range ***,modifications to the traditional bondbased PD model are *** considering the micro-structure of coal-rock materials within a uniform discrete model,heterogeneity characterized by bond random pre-breaking is *** approach facilitates the proposal of a novel model capable of handling the random distribution characteristics of material heterogeneity,rendering the PD model suitable for analyzing the deformation and failure of heterogeneous layered coal-rock mass *** established numerical model and simulation method,termed the sub-homogeneous PD model,not only incorporates the support effect but also captures accurately the random heterogeneous micro-structure of roadway surrounding *** simulation results obtained using this model show good agreement with field measurements from the Fucun coal mine,effectively validating the model’s capability in accurately reproducing the deformation and failure mode of surrounding rock under bolt-supported(anchor cable).The proposed subhomogeneous PD model presents a valuable and effective simulation tool for studying the deformation and failure of roadway surrounding rock in coal mines,offering new insights and potential advancements.

关键词： Roadway surrounding rock peridynamics heterogeneous material fracture analysis numerical simulation

Cr^(3+) activated Na_(3)RESi_(3)O_(9)(RE=Y,Lu,Sc) silicate broadband near-infrared phosphors for luminescence towards NIR-Ⅱ region via a multi-site occupancy strategy

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Journal of Rare Earths 2024年第8期42卷 1447-1457,I0002页

作者： Jiantong Wang Changshuai Gong Sihan Yang Qi Zhu Xuejiao Wang Ji-Guang Li college of Chemistry and materials Engineering Bohai UniversityJinzhou121007China Key Laboratory for Anisotropy and Texture of materials(Ministry of Education) School of Materials Science and EngineeringNortheastern UniversityShenyang110819China Research Center for Electronic and Optical materials National Institute for Materials ScienceTsukubaIbaraki 305-0044Japan

Phosphor-converted near-infrared light-emitting diodes(NIR pc-LEDs) are finding applications in various fields including food quality analysis,biomedical imaging,night vision,and *** crucial factor in the development of NIR pc-LEDs devices lies in the advancement of high-performance broadband NIR phosphors,In this work,novel Cr^(3+)-activated silicate phosphors NaRESi_(3)O_(9)(RE=Y,Lu,Sc) are *** silicate has a special 3D network structure in which RE has four different sites,forming four octahedrons and providing suitable occupation sites for Cr^(3+).The phosphors demonstrate a wide emission spectrum ranging from 750 to 1450 nm when excited by light at 468 *** full width at half maximum(FWHM),which benefits from the presence of Cr^(3+)ions occupying multiple sites,is measured to be 203 ***,the strongest emission peak is observed at a longer wavelength of 984 nm compared to most other systems activated by Cr^(3+).The Na_(3)ScSi_(3)O_(9) lattice provides a weak crystal field(Dq/B=1.97) and weak phonon-photon coupling for Cr^(3+),and the integrated emission intensity of Na_(3)ScSi_(3)O_(9):0,03Cr^(3+)is 4.66 times stronger than that of Na_(3)YSi_(3)O_(9):0.03Cr^(3+).

关键词： Rare earths Broadband near-infrared Silicate Photoluminescence Cr^(3+)

Preparation and magnetic hardening of low Ti content(Sm,Zr)(Fe,Co,Ti)_(12)magnets by rapid solidification non-equilibrium method

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Chinese Physics B 2024年第9期33卷 576-580页

作者： Xing-Feng Zhang Li-Bin Liu Yu-Qing Li Dong-Tao Zhang Wei-Qiang Liu Ming Yue college of materials science and Engineering Key Laboratory of Advanced Functional MaterialsMinistry of Education of ChinaBeijing University of TechnologyBeijing 100124China

The Sm–Zr–Fe–Co–Ti quinary-alloys with ThMn12 structure has attracted wide attention for ultra-high intrinsic magnetic properties,showing potentiality to be developed into rare-earth permanent *** Ti element in alloys is crucial for phase stability and magnetic properties,and lower Ti content can increase intrinsic magnetic properties but reduce phase *** this study,the 1:12 single-phase melt-spun ribbons with low Ti content was successfully prepared using a rapid solidification non-equilibrium method for the Sm1.1Zr_(0.2)Fe_(9.2)Co_(2.3)Ti_(0.5) ***,this non-equilibrium ribbon did not achieve good magnetic hardening due to the uneven microstructure and ***,annealing was carried out to eliminate micro-strain and homogenize microstructure,therefore,remanence and coercivity were significantly improved even the precipitation of a small amount of a-Fe phase which were not conducive to *** remanence of 86.1 emu/g and coercivity of 151 kA/m was achieved when annealing at 850℃ for 45 *** hot pressing,under the action of high temperature and pressure,a small portion of ThMn12 phases in the magnet decompose into Sm-rich phases and a-Fe,while remanence of 4.02 kGs(1 Gs=10^(-4) T),and coercivity of 1.12 kOe(1 Oe=79.5775 A·m^(-1))were still *** findings can provide reference for exploring practical permanent magnets made of 1:12 type quinary-alloys.

关键词： magnetic materials (Sm,Zr)(Fe,Co,Ti)_(12) magnets nanocrystalline magnet microstructure

CORC电缆中超导带材在缠绕、弯曲和扭曲变形下的应变分析

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Acta Mechanica Sinica 2024年第4期40卷 38-48页

作者：彭昱昊苟晓凡 college of mechanics and materials Hohai UniversityNanjing211000China

CORC(conductor on round core)超导电缆是一种基于REBCO(rare-earth barium copper oxide)导体的高温超导电缆,已经成为迄今为止最灵活的高温超导(HTS)导体之一.然而,由于超导REBCO陶瓷材料的脆性,临界电流表现出敏感的应变依赖性,即... 详细信息

CORC(conductor on round core)超导电缆是一种基于REBCO(rare-earth barium copper oxide)导体的高温超导电缆,已经成为迄今为止最灵活的高温超导(HTS)导体之一.然而,由于超导REBCO陶瓷材料的脆性,临界电流表现出敏感的应变依赖性,即临界电流与应变密切相关.该材料的应变一旦超过临界值,就会引发明显的衰减.除此之外,由于带材缠绕和电缆绞合后的复杂变形,切实存在一个实际性的挑战,即如何准确预测电缆超导带材在各种变形下的轴向应变.在本文中,我们建立了分析模型,可以用来准确计算CORC电缆的超导带材在电缆内芯上缠绕、电缆弯曲和扭曲变形等实际条件下的轴向应变.并且通过比较分析结果与有限元数值结果和实验数据,验证了分析模型,即超导带的临界电流随CORC电缆的核心直径而变化.在轴向应变结果的基础上,进一步确定了临界参数,即超导层的轴向应变恰好达到临界应变时的参数,如临界核心直径、临界弯曲直径和临界绞距等.对CORC电缆中REBCO超导带材的应变分析研究将有助于CORC电缆的加工和进一步设计高水平的超导线圈和磁体.

关键词：临界电流高温超导电缆超导带材扭曲变形应变分析轴向应变超导线圈临界参数

Reinforced SnO_(2) tensile-strength and“buffer-spring”interfaces for efficient inorganic perovskite solar cells

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Carbon Energy 2024年第6期6卷 282-291页

作者： Yuanyuan Zhao Lei Gao Qiurui Wang Qiang Zhang Xiya Yang Jingwei Zhu Hao Huang Jialong Duan Qunwei Tang college of Mechanical and Electronic Engineering Shandong University of Science and TechnologyQingdaoChina Institute of New Energy Technology College of Information Science and TechnologyJinan UniversityGuangzhouChina college of materials science and Engineering Sichuan UniversityChengduChina Guangxi Key Laboratory of Processing for Non-Ferrous Metals and Featured materials School of ResourcesEnvironment and MaterialsGuangxi UniversityNanningChina Institute of Carbon Neutrality College of Chemical and Biological EngineeringShandong University of Science and TechnologyQingdaoChina

Suppressing nonradiative recombination and releasing residual strain areprerequisites to improving the efficiency and stability of perovskite solar cells(PSCs).Here,long-chain polyacrylic acid(PAA)is used to reinforce SnO_(2)film and passivate SnO_(2)defects,forming a structure similar to“reinforcedconcrete”with high tensile strength and fewer ***,PAA is also introduced to the SnO_(2)/perovskite interface as a“buffer spring”torelease residual strain,which also acts as a“dual-side passivation interlayer”to passivate the oxygen vacancies of SnO_(2)and Pb dangling bonds in *** a result,the best inorganic CsPbBr_(3)PSC achieves a championpower conversion efficiency of 10.83%with an ultrahigh open-circuit voltageof 1.674 *** unencapsulated PSC shows excellent stability under 80%relative humidity and 80℃over 120 days.

关键词： charge recombination defect passivation inorganic perovskite solar cells interfacial modification strain relaxation

Enhanced corrosion resistance of epoxy resin coating via addition of CeO_(2) and benzotriazole

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Chinese Journal of Chemical Engineering 2024年第3期67卷 89-96页

作者： Xu Han Ruijie Guo Baolong Niu Hong Yan college of materials science and Engineering Taiyuan University of TechnologyTaiyuan 030024China Key Laboratory of Interface science and Engineering in Advanced materials Ministry of EducationTaiyuan University of TechnologyTaiyuan 030024China

The use of fillers to enhance the corrosion protection of epoxy resins has been widely *** this work,cerium dioxide(CeO_(2))and benzotriazole(BTA)were introduced into an epoxy resin to enhance the corrosion resistance of Q235 carbon *** electron microscopy results indicated that the CeO_(2) grains were rod-like and ellipsoidal in shape,and the distribution pattern of BTA was analyzed by energy dispersive *** dynamic potential polarization curve proved the excellent corrosion resistance of the composite epoxy resin with CeO_(2) and BTA co-addition,and electrochemical impedance spectroscopy test analysis indicated the significantly enhanced long-term corrosion protection performance of the composite *** the optimal protective performance was provided by the coating containing 0.3%(mass)CeO_(2) and 20%(mass)BTA,which was attributed to the barrier performance of CeO_(2) particles and the chemical barrier effect of *** formation of corrosion products was analyzed using X-ray *** addition,the corrosion resistance mechanism of the coating was also discussed in detail.

关键词： Benzotriazole Cerium dioxide Corrosion resistance Carbon steel Epoxy resin coating Preparation

Numerical investigation on compressible flow around a cylinder in proximity to the heated wall

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Journal of Hydrodynamics 2024年第3期36卷 519-533页

作者： Yu-lu Liu Jun-wang Qu Yi-zhou Tao Yong-guang Lyu Xiang Qiu Shanghai Institute of Technology School of ScienceShanghai201418China Shanghai Key Laboratory of mechanics in Energy Engineering Shanghai Institute of Applied Mathematics and MechanicsSchool of Mechanics and Engineering ScienceShanghai UniversityShanghai200072China

In this study,direct numerical simulations were conducted to investigate the compressible flow around a circular cylinder near a heated wall at a Reynolds number(Re)of 500 and a Mach number(Ma)of *** heating ratio T^(*)ranging from 1.0 to 1.6 represents the different situations of a heated wall,whereas the gap ratio ranges from 0.3 to *** study analyzed the impact of heating effect and wall proximity on flow characteristics and aerodynamic *** results indicated that the stability of the flow was enhanced as the gap ratio decreased or the heating ratio *** the calculation of enstrophy,it was found that the strength of shedding vortices weakens with a decrease in gap ratio or an increase in heating ***,the mean drag coefficient decreases as the heating ratio increases or the gap ratio *** contrast,the mean lift coefficient initially decreases and then increases as the gap ratio ***,the drag reduction mechanism was analyzed by examining the pressure distribution on the surface of the cylinder.

关键词： Compressible flow wall proximity heating effect stability enstrophy