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Journal of Geographical sciences 2025年第2期35卷 293-314页

作者： LIU Chao XU Yueqing JI Zhengxin college of land science and technology China Agricultural University Faculty of Political science College of Public Administration Central China Normal University

Changes in production-living-ecological spaces(PLES) profoundly affect the global carbon cycle, further challenging socio-ecological system sustainability. However, the impacts of PLES changes on carbon balance have been insufficiently discussed under a spatial heterogeneity perspective, resulting in an inadequate understanding of green development. This paper quantified the dynamics of PLES using the transfer matrix method and assessed the carbon balance computed by the ecological support coefficient of carbon emissions(ESC) in Shandong province from 2000 to 2020. The impacts of PLES changes on ESC were further investigated using a geographically weighted regression model. On this basis, carbon balance zones were delineated through cluster analysis. The results indicated that both production and ecological spaces decreased while the living space increased during 2000–2020. Carbon emissions increased and its sequestration decreased. As a result, ESC initially increased and then decreased, exhibiting apparent spatial clustering. The impact of different PLES transfer changes on ESC varies across county sites, with production→living space having the most significant impact on regional ESC and ecology→living space having the most negligible impact. Finally, six types of carbon balance zones were established to reduce carbon emissions. The findings are expected to support policy implementations for reducing carbon emissions and optimizing territorial development through low-carbon land use.

关键词： carbon emission carbon sequestration land use spatial heterogeneity Shandong province

Research on Stock Price Prediction Method Based on the GAN-LSTM-Attention Model

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Computers, Materials & Continua 2025年第1期82卷 609-625页

作者： Peng Li Yanrui Wei Lili Yin college of Computer science and technology Harbin University of Science and TechnologyHarbin150006China

Stock price prediction is a typical complex time series prediction problem characterized by dynamics,nonlinearity,and *** paper introduces a generative adversarial network model that incorporates an attention mechanism(GAN-LSTM-Attention)to improve the accuracy of stock price ***,the generator of this model combines the Long and Short-Term Memory Network(LSTM),the Attention Mechanism and,the Fully-Connected Layer,focusing on generating the predicted stock *** discriminator combines the Convolutional Neural Network(CNN)and the Fully-Connected Layer to discriminate between real stock prices and generated stock ***,to evaluate the practical application ability and generalization ability of the GAN-LSTM-Attention model,four representative stocks in the United States of America(USA)stock market,namely,Standard&Poor’s 500 Index stock,Apple Incorporatedstock,AdvancedMicroDevices Incorporatedstock,and Google Incorporated stock were selected for prediction experiments,and the prediction performance was comprehensively evaluated by using the three evaluation metrics,namely,mean absolute error(MAE),root mean square error(RMSE),and coefficient of determination(R2).Finally,the specific effects of the attention mechanism,convolutional layer,and fully-connected layer on the prediction performance of the model are systematically analyzed through ablation *** results of experiment show that the GAN-LSTM-Attention model exhibits excellent performance and robustness in stock price prediction.

关键词： Stock price prediction generative adversarial network attention mechanism time-series prediction

Mechanical properties and flow stress constitutive relationship of Ti–6Al–4V alloy with equiaxed microstructure at cryogenic temperatures

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Chinese Journal of Aeronautics 2025年第1期38卷 365-379页

作者： Jingwen HU Xun CHEN Yashun WANG Chen YANG college of Intelligence science and technology National University of Defense TechnologyChangsha 410073China Laboratory of science and technology on Integrated Logistics Support National University of Defense TechnologyChangsha 410073China

This paper investigates the uniaxial tensile mechanical properties and flow behavior of Ti-6Al-4V alloys with equiaxed microstructure at cryogenic temperatures ranging from 77 K to298 K and strain rates from 10^(-4)/s to 10^(-2)/*** electron microscopy is utilized to analyze the fracture morphology,aiming to reveal the fracture behavior at various *** applicability of the Zener-Hollomon parameter and the Johnson-Cook model in describing the flow stress of Ti-6Al-4V at cryogenic temperatures is ***,a constitutive relationship modeling method based on the variational recurrent networks is *** test results show a significant increase in the strength of equiaxed Ti-6Al-4V alloy under cryogenic conditions while the plastic deformation process is ***,the fracture analysis indicates that even at 77 K,the fracture process is still dominated by ductile fracture,and brittle fracture does not occur within the range of 77 K to 298 *** fitting results validate the performance of the Zener-Hollomon parameter and the Johnson-Cook model in describing the deformation flow stress of Ti-6Al-4V alloy at cryogenic *** results also indicate that the proposed constitutive relationship modeling method based on the variational recurrent network performs better,making it a potential method for widespread applications.

关键词： Titanium alloys Mechanical properties Cryogenics Fracture testing Flow behavior

Anchoring thiol-rich traps in 1D channel wall of metal-organic framework for efficient removal of mercury ions

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Chinese Chemical Letters 2025年第2期36卷 432-435页

作者： Xudong Zhao Yuxuan Wang Xinxin Gao Xinli Gao Meihua Wang Hongliang Huang Baosheng Liu college of Chemical Engineering and technology Taiyuan University of Science and Technology Instrumental Analysis Center Taiyuan University of Science and Technology State Key Laboratory of Separation Membranes and Membrane Processes School of Chemical Engineering and TechnologyTiangong University college of Materials science and Engineering Taiyuan University of Science and Technology

Metal-organic frameworks （MOFs） attract broad interests in mercury （Hg） ion adsorption field,while unreasonable distribution of active groups commonly restricts their utilization *** this work,we constructed a new MOF （TYUST-6） with dense thiol-rich traps in the 1D pore *** accessible channel and rational distribution of thiols allow the smooth diffusion of Hg ions and thereby result in a high Langmuir adsorption capacity of 1347.6 mg/g,almost reaching the theoretical maximum （1444.3 mg/g）.Adsorption equilibrium needs 10 and 30 min at the initial concentrations of 10 and 100 mg/L,*** co-existing ions and solution pH show almost negligible interferences on the adsorption,and adsorbent regeneration can be well *** experimental characterizations and theoretical calculations,the thiol groups in the pore wall are proved to be the dominant interaction ***,this work reports a novel high-capacity adsorbent for Hg2+,and proposes a feasible guideline for designing effective adsorbents.

关键词： Adsorption Mercury ion Metal-organic frameworks Thiol groups Waste water treatment

Realizing interfacial coupled electron/ion transport through reducing the interfacial oxygen density of carbon skeletons for high-performance lithium metal anodes

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Journal of Energy Chemistry 2025年第2期101卷 744-750页

作者： Yao-Lu Ye Yan Zhou Huan Ye Fei-Fei Cao college of Chemistry Huazhong Agricultural University Institute of Applied Mycology College of Plant Science and Technology Huazhong Agricultural University

Lithium plating/stripping occurs at the a node/electrolyte interface which involves the flow of electrons from the current collector and the migration of lithium ions from the solid-electrolyte interphase（SEI）.The dual continuous rapid transport of interfacial electron/ion is required for homogeneous Li ***,we propose a strategy to improve the Li metal anode performance by rationally regulating the interfacial electron density and Li ion transport through the SEI *** key technique involves decreasing the interfacial oxygen density of biomass-derived carbon host by regulating the arrangement of the celluloses precursor *** higher specific surface area and lower interfacial oxygen density decrease the local current density and ensure the formation of thin and even SEI film,which stabilized Li+transfer through the Li/electrolyte ***,the improved graphitization and the interconnected conducting network enhance the surface electronegativity of carbon and enable uninterruptible electron *** result is continuous and rapid coupled interfacial electron/ion transport at the anode/electrolyte reaction interface,which facilitates uniform Li deposition and improves Li anode *** Li/C anode shows a high initial Coulombic efficiency of 98% and a long-term lifespan of over 150cycles at a practical low N/P（negative-to-positive） ratio of 1.44 in full cells.

关键词： Cellulose Electron/ion conducting Interfacial oxygen density Lithium metal batteries Lithium-lean metal anodes

Theoretical and experimental study on high-entropy flotation of micro-fine cassiterite

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International Journal of Mining science and technology 2025年第1期35卷 19-39页

作者： Shuming Wen Yongchao Miao Yanyu Tang Zhengyong Song Qicheng Feng State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization Faculty of Land Resource EngineeringKunming University of Science and TechnologyKunming 650093China

Tin is a critical metal for various industries,making its recovery from low-grade cassiterite ores *** study aimed to optimize the flotation recovery of cassiterite using multi-component collector *** collectors were initially selected through micro-flotation tests,leading to the identification of optimal proportions for a four-component collector system(SHA-OHA-SPA-DBIA in a 4:3:2:1 ratio).Molecular dynamics simulations and surface tension tests were used to investigate the micellar behavior of these collectors in aqueous *** adsorption characteristics were quantified using microcalorimetry,enabling the determination of collection entropy and changes in Gibbs free *** four-component collector system showed the highest entropy change and the most favorable Gibbs free energy,leading to a cassiterite recovery of above 90%at a concentration of 8.0×10^(5)mol/*** analytical techniques were employed to systematically characterize the adsorption *** findings revealed a positive correlation between the adsorption products formed by the multicomponent collectors on the cassiterite surface and the entropy ***-scale testing of the high-entropy collector system produced a tin concentrate with an Sn grade of 6.17%and an Sn recovery of 82.43%,demonstrating its substantial potential for practical applications in cassiterite flotation.

关键词： High-entropy Flotation Cassiterite Adsorption Molecular dynamics QCM-D

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Integrating Cu+/Cu0 sites on porous nitrogen-doped carbon nanofibers for stable and efficient CO2 electroreduction to multicarbon products

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Journal of Energy Chemistry 2025年第2期101卷 453-462页

作者： Yicheng Chao Jiahao Zhang Qinyue Wu Xinfei Fan Xie Quan Yanming Liu Key Laboratory of Industrial Ecology and Environmental Engineering (MOE) School of Environmental Science and Technology Dalian University of Technology college of Environmental science and Engineering Dalian Maritime University Frontier science Center for Smart Materials Dalian University of Technology

The Cu+/Cu0sites of copper-based catalysts are crucial for enhancing the production of multicarbon(C2+)products from electrochemical CO2reduction reaction（eCO2RR）.However,the unstable Cu+and insufficient Cu+/Cu0active sites lead to their limited selectivity and stability for C2+***,we embedded copper oxide（CuOx） particles into porous nitrogen-doped carbon nanofibers（CuOx@PCNF）by pyrolysis of the electrospun fiber film containing ZIF-8 and Cu2O *** porous nitrogendoped carbon nanofibers protected and dispersed Cu+species,and its micro porous structure enhanced the interaction between CuOxand reactants during *** obtained CuOx@PCNF created more effective and stable Cu+/Cu0active *** showed a high Faradaic efficiency of 62.5% for C2+products in Hcell,which was 2 times higher than that of bare CuOx（～31.1%）.Furthermore,it achieved a maximum Faradaic efficiency of 80.7% for C2+products in flow *** situ characterization and density functional theory（DFT） calculation confirmed that the N-doped carbon layer protected Cu+from electrochemical reduction and lowered the energy barrier for the dimerization of**** and exposed Cu+/Cu0active sites enhanced the enrichment of*CO and promoted the C-C coupling reaction on the catalyst surface,which facilitated the formation of C2+products.

关键词： Carbon nanofibers Cu+/Cu0 sites C–C coupling Electrocatalytic CO2 reduction Multicarbon products

Intricate interplay between shear stress and extrusion temperature in Mg−Al composite rods

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Transactions of Nonferrous Metals Society of China 2025年第1期35卷 105-125页

作者： Jian-xing ZHAO Chao-wei ZENG Ting YUAN Wei PENG Zhen-wei SUN Ou ZHANG Hong-jun HU college of Materials science and Engineering Chongqing University of TechnologyChongqing 400054China

The Mg−Al composite rods of aluminum core-reinforced magnesium alloy were prepared by the extrusion−shear(ES)process,and the microstructure,deformation mechanism,and mechanical properties of the Mg−Al composite rods were investigated at different extrusion temperatures and shear *** experimental results show that the proportion of dynamic recrystallization(DRX)and texture for Al and Mg alloys are controlled by the combination of temperature and shear *** texture type of the Al alloys exhibits slight variations at different *** the increase of temperature,the DRX behavior of Mg alloy shifts from discontinuous DRX(DDRX),continuous DRX(CDRX),and twin-induced DRX(TDRX)dominant to CDRX,the dislocation density in Mg alloy grains decreases significantly,and the average value of Schmid factor(SF)of the basalslip system *** particular,partial grains exhibit a distinct dominant slip system at 390℃.The hardness and thickness of the bonding layer,as well as the yield strength and elongation of the Mg alloy,reach their maximum at 360℃as a result of the intricate influence of the combined temperature and shear stress.

关键词： Mg−Al composite rod texture evolution deformation mechanism intermetallic compound extrusion−shear process

The influence mechanism of environmental factors on DGT adsorbing sulfonamides and the migration between water and sediment

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Journal of Environmental sciences 2025年第5期151卷 347-359页

作者： Peng Zhang Jingfeng Yan Hao Ji Linke Ge Yanying Li School of Environmental science and technology Shaanxi University of Science&TechnologyXi’an 710021China college of Environmental sciences and Engineering Dalian Maritime UniversityDalian 116026China

Obtaining the sulfonamides(SAs)concentrations in the water body and sediment bulk was a prerequisite to reveal their transport and partitioning behavior in sediment-water environments and accurately assess their ecological *** the present study,the influences of multifactor interactions on the performance of o-DGTs with XAD-18 binding gels were analyzed by central combination experiments and response surfaces analysis,in which the target compounds were 9 *** results indicated that dissolved organic matter(DOM),pH,and suspended particulate matter(SS)had significant effects on the o-DGT sampling,whereas this o-DGT was independent of the ionic strength(IS).Concentning the composite influence of the four factors,the interaction between DOM and SS posed the most significant effect on all 9 SAs ***,an o-DGT and DIFSmodel was applied to explore the SAs migration between the water-sediments *** difference between desorption rate(k_(b))and adsorption rates(k_(f))values suggested that the kinetics of SAs was dominated by ***,the short-term sediment-water partitioning of SAs was clarified on the basis of distribution coefficient(K_(dl))for the labile SAs,among which the sulfadiazine(SDZ)had the largest labile *** ability of sediments to release SAs to the liquid phase as a sink was determined by response time(T_(c)).Among the 9 SAs,the longterm release of soseulfamethoxypyridazine(SMP)from the solid phase of sediments would have a potential risk to the aquatic environment,to which more attention should be paid in the future.

关键词： Sulfonamides O-DGT Water-sediments interface DIFS Distribution

New results on finite-time stability and instability theorems for stochastic nonlinear time-varying systems

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science China(Information sciences) 2025年第2期68卷 186-199页

作者： Weihai ZHANG Liqiang YAO college of Electrical Engineering and Automation Shandong University of Science and Technology School of Mathematics and Information science Yantai University

This paper studies finite-time stability and instability theorems in the probability sense for stochastic nonlinear timevarying systems. Firstly, a new sufficient condition is proposed to guarantee that the considered system has a global ***, we propose new finite-time stability and instability criteria that relax the constraints on LV(the infinitesimal operator of Lyapunov function V) by the uniformly asymptotically stable function. On the one hand, these obtained results make up for the shortcomings of the existing results. On the other hand, the new finite-time stability theorems can be viewed as natural extensions of the existing results and also allow LV to be indefinite(negative or positive) rather than just only allow LV < ***, some simulation examples verify the validity of the theoretical results.

关键词： stochastic nonlinear systems finite-time stability finite-timeinstability uniformly asymptotically stable function