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Machine Learning-Aided Data Analysis in Single-Protein Conductance Measurement with Electron Tunneling Probes

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Chinese Journal of Chemistry 2024年第1期42卷 67-72页

作者： Yuxin Yang Tao Jiang Ye Tian Biaofeng Zeng Longhua Tang State Key Laboratoryof Extreme Photonics and instrumentation College of Optical Science and EngineeringZhejiang University HangzhouZhejiang 310027China Nanhu Brain-computer Interface Institute HangzhouZhejiang 311100China State Key Laboratory of Fluid Power and Mechatronic Systems College of Mechanical EngineeringZhejiang University HangzhouZhejiang 310027China

The electrical tunneling sensors have excellent potential in the next generation of single-molecule measurement and sequencing technologies due to their high sensitivity and spatial resolution *** tunneling signals that have been measured at a high sampling rate may provide detailed molecular *** the extraordinarily large amount of data that has been gathered,it is still difficult to correlate signal transformations with molecular processes,which creates great obstacles for signal *** learning is an effective tool for data analysis that is currently gaining more *** has demonstrated promising results when used to analyze data from single-molecule electrical *** order to extract meaningful information from raw measurement data,we have combined intelligent machine learning with tunneling electrical *** the purpose of analyzing tunneling electrical signals,we investigated the clustering approach,which is a classic algorithm in machine learning.A clustering model was built that combines the advantages of hierarchical clustering and Gaussian mixture model ***,customized statistical algorithms were *** has been proven to efficiently gather molecular information and enhance the effectiveness of data analysis.

关键词： Tunneling sensor Single-molecule measurement Machine learning Single-protein conductance Molecular electrochemistry Nanotechnology Molecular electronics

Cross-layer all-interface defect passivation with pre-buried additive toward efficient all-inorganic perovskite solar cells

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Carbon Energy 2024年第9期6卷 283-291页

作者： Qiurui Wang Jingwei Zhu Yuanyuan Zhao Yijie Chang Nini Hao Zhe Xin Qiang Zhang Cong Chen Hao Huang Qunwei Tang college of Mechanical and electronic engineering Shandong University of Science and TechnologyQingdaoChina college of Materials Science and engineering Sichuan UniversityChengduChina Guangxi Key Laboratory of Processing for Non-Ferrous Metals and Featured Materials School of ResourcesEnvironment and MaterialsGuangxi UniversityNanningChina Institute of Carbon Neutrality College of Chemical and Biological EngineeringShandong University of Science and TechnologyQingdaoChina

The buried interface in the perovskite solar cell(PSC)has been regarded as a breakthrough to boost the power conversion efficiency and ***,a comprehensive manipulation of the buried interface in terms of the transport layer,buried interlayer,and perovskite layer has been largely ***,we propose the use of a volatile heterocyclic compound called 2-thiopheneacetic acid(TPA)as a pre-buried additive in the buried interface to achieve cross-layer all-interface defect passivation through an in situ bottom-up infiltration diffusion *** not only suppresses the serious interfacial nonradiative recombination losses by precisely healing the interfacial and underlying defects but also effectively enhances the quality of perovskite film and releases the residual strain of perovskite *** to this versatility,TPA-tailored CsPbBr3 PSCs deliver a record efficiency of 11.23% with enhanced long-term *** breakthrough in manipulating the buried interface using TPA opens new avenues for further improving the performance and reliability of PSC.

关键词： buried interfaces charge recombination defect passivation inorganic perovskite solar cells strain relaxation

Higher-order properties and extensions for indirect MRAC and APPC of linear systems

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Science China(Information Sciences) 2024年第4期67卷 218-238页

作者： Yanjun ZHANG Zhipeng ZHANG Jian SUN Lei WANG Kangkang ZHANG National Key Lab of Autonomous Intelligent Unmanned Systems Beijing Institute of Technology Beijing Institute of Technology Chongqing Innovation Center college of Control Science and engineering Zhejiang University Department of Electrical and electronic engineering Imperial College London KIOS Research and Innovation Center of Excellence University of Cyprus

Recently, a reference derived some new higher-order output tracking properties for direct model reference adaptive control(MRAC) of linear time-invariant(LTI) systems: limt→∞ e~((i))(t) = 0, i = 1,..., n~*-1, where n~* and e~((i))(t) denote the relative degree of the system and the i-th derivative of the output tracking error, respectively. However, a naturally arising question involves whether indirect adaptive control(including indirect MRAC and indirect adaptive pole placement control) of LTI systems still has higher-order tracking properties. Such properties have not been reported in the literature. Therefore, this paper provides an affirmative answer to this question. Such higher-order tracking properties are new discoveries since they hold without any additional design conditions and, in particular, without the persistent excitation condition. Given the higher-order properties, a new adaptive control system is developed with stronger tracking features.(1) It can track a reference signal with any order derivatives being unknown.(2) It has higher-order exponential or practical output tracking properties.(3) Finally, it is different from the usual MRAC system, whose reference signal’s derivatives up to the n~* order are assumed to be known. Finally, two simulation examples are provided to verify the theoretical results obtained in this paper.

关键词： higher-order tracking indirect adaptive control model reference adaptive control adaptive pole placement control

Ti_(3)C_(2)T_(x)/SnO_(2)P–N heterostructure construction boosts room-temperature detecting formaldehyde

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Rare Metals 2024年第1期43卷 267-279页

作者： Yue Zhang Ming-Yue Wang Xiao-Guang San Yan-Bai Shen Guo-Sheng Wang Lei Zhang Dan Meng college of Chemical engineering Shenyang University of Chemical TechnologyShenyang 110142China Institute for Superconducting and electronic Materials(ISEM) Australian Institute for Innovative Materials(AIIM)University ofWollongongWollongongNSW2500Australia college of Resources and Civil engineering Northeastern UniversityShenyang 110819China

Formaldehyde is a common atmospheric pollutant produced in industrial production and daily ***,the traditional semiconductor formaldehyde gas sensor cannot work at room temperature,which limits its practical ***,developing high-performance gas sensors for rapidly and accurately detecting formaldehyde at room temperature is an important *** this study,Ti_(3)C_(2)Tx/SnO_(2)heterostructures were constructed,which could selectively detect formaldehyde at room temperature with a response value of 29.16%(10×10^(-6)).In addition,the sensor shows a remarkable theoretical detection limit of 5.09×10^(-9)and good longterm *** functional theory(DFT)simulations reveal that SnO_(2)nano spheres provide the majority of adsorption sites that strongly interact with ***,Ti_(3)C_(2)T_(x)acting as a conductive layer facilitates the transfer of charge carriers so that they show a sensing response to formaldehyde at room ***,the formation of p-n heterostructures between SnO_(2)and Ti_(3)C_(2)T_(x)boosts the Schottky barrier at the interface,which is the critical factor in enhancing the sensing properties by turning the Schottky barrier upon introducing formaldehyde *** perspective is expected to provide instructive guidance for utilizing MXene/metal oxide nanocomposites to improve the gas sensing performance at room temperature.

关键词： Ti_(3)C_(2)T_(x)/SnO_(2)nanocomposites p-n heterostructures Formaldehyde sensing Room temperature DFT calculations

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A Practical Study of Intelligent Image-Based Mobile Robot for Tracking Colored Objects

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Computers, Materials & Continua 2024年第8期80卷 2181-2197页

作者： Mofadal Alymani Mohamed Esmail Karar Hazem Ibrahim Shehata college of Computing and Information Technology Shaqra UniversityShaqra11961Saudi Arabia Faculty of electronic engineering Menoufia UniversityMenouf32952Egypt Faculty of engineering Zagazig UniversityZagazig44519Egypt

Object tracking is one of the major tasks for mobile robots in many real-world ***,artificial intelligence and automatic control techniques play an important role in enhancing the performance of mobile robot *** contrast to previous simulation studies,this paper presents a new intelligent mobile robot for accomplishing multi-tasks by tracking red-green-blue(RGB)colored objects in a real experimental ***,a practical smart controller is developed based on adaptive fuzzy logic and custom proportional-integral-derivative(PID)schemes to achieve accurate tracking results,considering robot command delay and tolerance *** design of developed controllers implies some motion rules to mimic the knowledge of experienced *** scenarios of three colored object combinations have been successfully tested and evaluated by using the developed controlled image-based robot *** PID control failed to handle some tracking scenarios in this *** proposed adaptive fuzzy PID control achieved the best accurate results with the minimum average final error of 13.8 cm to reach the colored targets,while our designed custom PID control is efficient in saving both average time and traveling distance of 6.6 s and 14.3 cm,*** promising results demonstrate the feasibility of applying our developed image-based robotic system in a colored object-tracking environment to reduce human workloads.

关键词： Mobile robot autonomous systems fuzzy logic control real-time image processing

A Polarization Control Operator for Polarized Electromagnetic Wave Designing

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Chinese Journal of electronics 2024年第5期33卷 1253-1260页

作者： Shuo CUI Yaoyao LI Shijian ZHANG Ling CHEN Cheng CAO Donglin SU School of electronic and Information engineering Beihang University Shenyuan Honors college Beihang University Research Institute for Frontier Science Beihang University

To describe and control the polarization state of electromagnetic waves, a polarization control operator of the complex vector form is proposed. Distinct from traditional descriptors, the proposed operator employs an angle parameter to configure the polarization state of the polarized wave. By setting the parameter in the proposed operator,the amplitude of the field components can be modified, resulting in changes in the magnitude and direction of the field vector, and thus realizing control of the polarization state of the electromagnetic wave. The physical meaning,orthogonal decomposition, and discrete property of the proposed operator are demonstrated through mathematical derivation. In the simulation examples, the polarization control operator with fixed and time-varying parameters is applied to the circularly polarized wave. The propagation waveform, the trajectory projection and the waveform cross section in different reception directions of the new electromagnetic waves are observed. The simulation results indicate that complex electromagnetic waves with more flexible polarization states can be obtained with the aid of the polarization operator.

关键词： Polarization Simulation Modulation Electromagnetic compatibility Vectors Trajectory Electromagnetics Electromagnetic wave Polarization control operator Polarization descriptor Polarization state MIMO

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Visibility restoration for real-world hazy images via improved physical model and Gaussian total variation

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Frontiers of Computer Science 2024年第1期18卷 267-269页

作者： Chuan LI Enping HU Xinyu ZHANG Hao ZHOU Hailing XIONG Yun LIU college of Computer and Information Science Southwest UniversityChongqing 400715China School of Big Data and Intelligent engineering Chongqing College of International Business and EconomicsChongqing 401520China college of Artificial Intelligence Southwest UniversityChongqing 400715China college of electronic and Information engineering Southwest UniversityChongqing 400715China

1 Introduction Under real-world haze conditions,the existence of haze particles in the atmosphere reduces the visibility of captured ***,the noise is inevitably introduced into the degraded image,which further deteriorates the visual quality of the *** enhance the visibility and quality of outdoor real-world hazy images,numerous algorithms have been proposed to remove haze from a single input *** existing methods are broadly lumped into two categories:prior-based methods[1,2]and learning-based methods[3–6].Unfortunately,the widely used atmospheric scattering model and the corresponding haze removal methods fail to take the noise interference into account,which may result in poor visibility restoration performance.

关键词： visibility remove noise

Magneto-optical Kerr Effect of Mono-layer NiX_(2)(X=Cl,Br,I):A Density Functional Theory Study

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Journal of Wuhan University of Technology(Materials Science) 2024年第5期39卷 1121-1128页

作者： FAN Qingqian DU Chaochao School of Economics and Management Shanghai Institute of TechnologyShanghai 200235China college of Information Science&electronic engineering Zhejiang UniversityHangzhou 310027China

The full-potential linearized augmented plane wave plus local orbital method is utilized for exploring the electronic,magnetic,and magneto-optical properties of the NiX_(2)(X=Cl,Br,and I)single *** first-principles calculation demonstrates that these compounds are ferromagnetic indirect semiconductors,and the energy band gaps of NiX_(2)for X=Cl,Br,and I are 3.888,3.134,and 2.157 eV,*** magnetic moments of Ni atoms in NiX_(2)monolayer are 1.656,1.588,1.449μB,and their magneto-crystalline anisotropy energies are 0.167,0.029,0.090 meV,*** on the macro-linear response theory,we systematically studied the influences of the external magnetic field and out-of-plane strain on the magneto-optical Kerr effect(MOKE)spectrum of the NiX_(2)single *** is found that,when the external magnetic field is perpendicular to the sample plane,the value of the Kerr rotation angle reaches the maximum,and the single-layer NiI_(2)material has a Kerr rotation angle of 1.89°at the photon energy of 1.986 ***,the Kerr rotation spectrum of NiCl_(2)and NiBr_(2)monolayers redshift as the out-of-plane strain increases,while NiI_(2)monolayer *** computation of the MOKE spectrum of NiX_(2)materials provides an opportunity for applications of 2D magnetic material ranging from sensing to data storing.

关键词： magneto-optical Kerr effect(MOKE) first-principles calculations external magnetic field out-of-plane strain

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Event-triggered predefined-time control for full-state constrained nonlinear systems: A novel command filtering error compensation method

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Science China(Technological Sciences) 2024年第9期67卷 2867-2880页

作者： PAN YingNan CHEN YiLin LIANG HongJing college of Control Science and engineering Bohai UniversityJinzhou 121013China School of Automation engineering University of Electronic Science and Technology of ChinaChengdu 611731China Laboratory of Electromagnetic Space Cognition and Intelligent Control Beijing 100089China

In this paper, a command filter-based adaptive fuzzy predefined-time event-triggered tracking control problem is investigated for uncertain nonlinear systems with time-varying full-state constraints. By designing a sliding mode differentiator, the inherent computational complexity problem within the predefined-time backstepping framework is solved. Different from the existing command filter-based finite-time and fixed-time control strategies that the convergence time of the filtering error is adjusted through the system initial value or numerous parameters, a novel command filtering error compensation method is presented,which tunes one control parameter to make the filtering error converge in the predefined time, thereby reducing the complexity of design and analysis of processing the filtering error. Then, an improved event-triggered mechanism(ETM) that builds upon the switching threshold strategy, in which an inverse cotangent function is designed to replace the residual term of the ETM,is proposed to gradually release the controller's dependence on the residual term with increasing time. Furthermore, a tan-type nonlinear mapping technique is applied to tackle the time-varying full-state constraints problem. By the predefined-time stability theory, all signals in the uncertain nonlinear systems exhibit predefined-time stability. Finally, the feasibility of the proposed algorithm is substantiated through two simulation results.

关键词： predefined-time control command filtering error compensation method event-triggered mechanism time-varying full-state constraints uncertain nonlinear systems

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