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Four-birds-with-one-stone:A multifunctional Ti-based material for solar-driven water evaporation

Nano Research 2024年第5期17卷 4498-4506页

作者： Yannan Li Yaning Sun Dan Zhang Yu Xue Jie Wang Nan Zhang Jun Wang Jiangwei Zhang Yan Zhao Jun-Jie Liu School of Physical Science and Technology College of Energy Materials and ChemistryInner Mongolia UniversityHohhot 010021China

Sustainable,environmentally friendly and low-energy desalination materials have important research value for the increasing demand of freshwater year by ***,it is a huge challenge to maintain high heat energy transfer efficiency without reducing the heat conversion capacity of specific solar photothermal conversion ***,their efficiency and durability are greatly limited by the problems of seawater corrosion,oil,and bacteria *** now,no related work has been reported to solve all the aforementioned problems via a simple four-birds-with-one-stone ***,a class of multifunctional porous photothermal silver(Ag)modified Ti foams(Tf-TA/Ag series materials)is prepared for the development of advanced solar water evaporation devices,and provides alternative materials for alleviating freshwater crisis and treating *** oil contact angle(OCA)changes from 41°to 180°,which significantly reduces the adhesion of *** addition,Tf-TA2/Ag sample also shows an excellent and sustained antibacterial effect,which maintains above 99.9%of antibacterial rate after repeated 5 *** surface temperature of the Tf-TA2/Ag sample reaches 52.5℃ after simulated sun irradiation for 20 min,which is significantly higher than that of the contact groups(water:36.4℃,Ti foam:38.2℃ and Tf-TA2:40.9℃).The capacity of seawater evaporation and salt removal is enhanced due to the excellent photothermal properties,low reflectance,and uniform heat dissipation *** water production efficiency of Tf-TA2/Ag sample is 1.41 kg·m^(-2)·h^(-1) in artificial seawater and 0.76 kg·m^(-2)·h^(-1) in oily sewage under simulated sun ***,the hydrophilic and oleophobic properties of Tf-TA2/Ag are critical to extracting water from oil/water mixture in diverse water ***,this four-birds-with-one-stone approach provides a new perspective for the improvement of solar seawater desalination performance.

关键词： four-birds-with-one-stone photothermal material antibacterial material antifouling property

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Seasonal response of nitrogen exchange fluxes to crab disturbance at sediment-water interface in coastal tidal wetlands

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Water Science and Engineering 2024年第2期17卷 129-138页

作者： Guo-fen Hua Shang-qing Liu Xiang-dong Liu Jin-li Li Yue Fang Wen-ting Xie Xiang Xu college of Water Conservancy and Hydroelectric Power Hohai UniversityNanjing 210098China college of Renewable energy Hohai UniversityNanjing 210098China

Coastal wetlands are hotspots for nitrogen(N)cycling,and crab burrowing is known to transform N in intertidal marsh ***,the underlying mechanisms remain *** study conducted field experiments and used indoor control test devices to investigate the seasonal response of nitrogen to crab disturbance at the sediment-water interface in coastal tidal flat *** results showed that crab disturbance exhibited significant seasonality with large seasonal differences in cave density and *** to crab disturbance,nitrogen fuxes at the sediment-water interface were much greater in the box with crabs than in the box without *** summer,NH-N showed a positive flux from the sediment to the overlying water,but NO2-N and NOg-N showed positive fluxes from the sediment to the overlying water only in early *** winter,NH-N showed a positive flux from the sediment to the overlying water,but NO-N and NO,-N both exhibited positive and negative *** results indicated that the presence of crab burrows can cause the aerobic layer to move downward by approximately 8-15 cm in summer and directly promote nitrification at the sediment surface.

关键词： Coastal tidal flat wetland Crab disturbance Nitrogen flux Nitrification Denitrification Sediment-water interface

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Pyrolysis technologies for biochar production in waste management:a review

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Clean energy 2024年第4期8卷 61-78页

作者： Kavan Kumar V NLPanwar Department of Renewable energy Engineering College of Technology and EngineeringMPUATUdaipurRajasthan 313001India

Pyrolysis is a thermal conversion process in the absence of air to derive energy components from the ***-energy technologies will play a major role in addressing future challenges related to environmental safety and energy *** of the many easily available renewable energy sources is biomass-an organic material that is thought to be *** technology is a thermochemical process that can be used to produce useful products from biomass,such as biochar,bio-oil and combustible pyrolysis *** structure and relative product yield are impacted by the pyrolysis method *** article evaluates different approaches for biomass ***,slow and advanced pyrolysis methods using various pyrolyser reactors have been studied in the literature and are provided to increase the variety and use of these methods in upcoming studies and re*** pyrolysis can lead to increased ecological well-being,as it increases the amount of biochar produced using auger and rotary-kiln *** pyrolysis,mainly in fluidized-bed reactors with bubbling and rotating circulation,can be used to obtain *** pyrolysis methods offer a good probability of yielding great prosperity for specific *** selection of a pyrolysis process is based on the required output in terms of solid,liquid and gaseous fuels,and the parameter plays a crucial role in the pyrolysis performance.

关键词： biomass thermochemical process slow pyrolysis fast pyrolysis and advanced pyrolysis

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Achieving a superior Na storage performance of Fe-based Prussian blue cathode by coating perylene tetracarboxylic dianhydride amine

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Carbon energy 2024年第5期6卷 53-64页

作者： Xin-Yuan Fu Lu-Lu Zhang Zhao-Yao Chen Yunkai Xu Junxiu Wu Cheng-Cheng Wang Xiao-Kai Ding Xue-Lin Yang Jun Lu Hubei Provincial Collaborative Innovation Center for New energy Microgrid College of Electrical Engineering&New EnergyChina Three Gorges UniversityYichangHubeiChina college of Materials and Chemical Engineering China Three Gorges UniversityYichangHubeiChina college of Chemical and Biological Engineering Zhejiang UniversityHangzhouChina

Fe-based Prussian blue(Fe-PB)cathode material shows great application potential in sodium(Na)-ion batteries due to its high theoretical capacity,long cycle life,low cost,and simple preparation ***,the crystalline water and vacancies of Fe-PB lattice,the low electrical conductivity,and the dissolution of metal ions lead to limited capacity and poor cycling *** this work,a perylene tetracarboxylic dianhydride amine(PTCDA)coating layer is successfully fabricated on the surface of Fe-PB by a liquid-phase *** aminated PTCDA(PTCA)coating not only increases the specific surface area and electronic conductivity but also effectively reduces the crystalline water and vacancies,which avoids the erosion of Fe-PB by ***,the PTCA layer reduces the charge transfer resistance,enhances the Na-ion diffusion coefficient,and improves the structure *** PTCA-coated Fe-PB exhibits superior Na storage performance with a first discharge capacity of 145.2 mAh g^(−1) at 100 mA g^(−1).Long cycling tests exhibit minimal capacity decay of 0.027%per cycle over 1000 cycles at 1 A g^(−1).Therefore,this PTCA coating strategy has shown promising competence in enhancing the electrochemical performance of Fe-PB,which can potentially serve as a universal electrode coating strategy for Na-ion batteries.

关键词： cathode material coating Fe-based Prussian blue Na-ion batteries perylene tetracarboxylic dianhydride amine

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Novel high-safety aeroengine performance predictive control method based on adaptive tracking weight

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Chinese Journal of Aeronautics 2024年第7期37卷 352-374页

作者： Qian CHEN Hanlin SHENG Jie ZHANG Jiacheng LI college of energy and Power Engineering Nanjing University of Aeronautics and AstronauticsNanjing 210016China college of Automation Engineering Nanjing University of Aeronautics and AstronauticsNanjing 210016China

Increasing attention has been attracted to the dynamic performance and safety of advanced performance predictive control systems of the next-generation *** latest research demonstrates that Subspace-based Improved Model Predictive Control(SIMPC)can overcome the difficulty in solving the predictive model in MPC/NMPC ***,applying constant design parameters cannot maintain consistent control effects in all ***,the designed system relies too much on sensor-measured data,and thus it is difficult to thoroughly validate the safety of the system because of its high *** means that any potential hardware/software faults will endanger the ***,this paper first presents a novel nonlinear mapping relationship to adaptively tune the tracking weight online with the change of Power Lever Angle(PLA)and real-time relative tracking ***,without introducing additional design parameters,an Adaptive Tracking Weight-based SIMPC(ATW-SIMPC)controller is designed to improve the control performance in all operating states ***,a Primary/Backup Hybrid Control(PBHC)strategy with the ATW-SIMPC controller as the primary system and the traditional speed(Nf)controller as the backup system is proposed to ensure *** designed affiliated switching controller and the real-time monitor therein can be used to realize reasonable and smooth switching between primary/backup systems,so as to avoid bump *** PBHC system switches to the Nf controller when the ATW-SIMPC controller is wrong because of potential hardware/software faults;otherwise,the ATW-SIMPC controller keeps acting on the *** main results prove that the ATW-SIMPC controller with the optimal nonlinear mapping relationship,compared with the existing SIMPC controller,uplifts the dynamic control performance by 32%and reduces overshoots to an allowable limit,resulting in a better control effect in full *** comparison results consistently i

关键词： Aeroengine Model predictive control Hybrid system Adaptive weight safety

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Bimetallic In_(2)O_(3)/Bi_(2)O_(3) Catalysts Enable Highly Selective CO_(2) Electroreduction to Formate within Ultra-Broad Potential Windows

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energy & Environmental Materials 2024年第1期7卷 257-264页

作者： Zhongxue Yang Hongzhi Wang Xinze Bi Xiaojie Tan Yuezhu Zhao Wenhang Wang Yecheng Zou Huai ping Wang Hui Ning Mingbo Wu State Key Laboratory of Heavy Oil Processing College of Chemical EngineeringCollege of New EnergyChina University of Petroleum(East China)Qingdao 266580China Shandong Dongyue Future Hydrogen energy Material Co. Ltd.Zibo 255000China

CO_(2)electrochemical reduction reaction(CO_(2)RR)to formate is a hopeful pathway for reducing CO_(2)and producing high-value chemicals,which needs highly selective catalysts with ultra-broad potential windows to meet the industrial ***,the nanorod-like bimetallic ln_(2)O_(3)/Bi_(2)O_(3)catalysts were successfully synthesized by pyrolysis of bimetallic InBi-MOF *** abundant oxygen vacancies generated from the lattice mismatch of Bi_(2)O_(3)and ln_(2)O_(3)reduced the activation energy of CO_(2)to*CO_(2)·^(-)and improved the selectivity of*CO_(2)·^(-)to formate ***,the carbon skeleton derived from the pyrolysis of organic framework of InBi-MOF provided a conductive network to accelerate the electrons *** catalyst exhibited an ultra-broad applied potential window of 1200 mV(from-0.4 to-1.6 V vs RHE),relativistic high Faradaic efficiency of formate(99.92%)and satisfactory stability after 30 *** in situ FT-IR experiment and DFT calculation verified that the abundant oxygen vacancies on the surface of catalysts can easily absorb CO_(2)molecules,and oxygen vacancy path is dominant *** work provides a convenient method to construct high-performance bimetallic catalysts for the industrial application of CO_(2)RR.

关键词： bimetallic catalyst CO_(2)electrochemical reduction reaction formate oxygen vacancy wide potential window

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Thermal Property Enhancement of a Novel Shape-Stabilized Sodium Acetate Trihydrate-Acetamide/Expanded Graphite-Based Composite Phase Change Material

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Journal of Thermal Science 2024年第4期33卷 1564-1576页

作者： AN Zhoujian HOU Wenjie DU Xiaoze HUANG Zhongzheng MOMBEKI PEA Hamir Johan ZHANG Dong LIU Xiaomin college of energy and Power Engineering Lanzhou University of TechnologyLanzhou730050China Key Laboratory of Multi-supply System with Solar energy and Biomass of Gansu Province Lanzhou730050China Gansu Natural energy Research Institute Lanzhou730046China

Phase change materials(PCMs)are a kind of highly efficient thermal storage materials which have a bright application prospect in many fields such as energy conservation in buildings,waste heat recovery,battery thermal management and so *** inorganic hydrated salt PCMs have received increasing attention from researchers due to their advantages of being inexpensive and ***,inorganic hydrated salt PCMs are still limited by the aspects of inappropriate phase change temperature,liquid phase leakage,large supercooling and severe phase separation in the application *** this work,sodium acetate trihydrate was selected as the basic inorganic PCM,and a novel shape-stabilized composite phase change material(CPCM)with good thermal properties was prepared by adding various functional *** first,the sodium acetate trihydrate-acetamide binary mixture was prepared and the melting point was adjusted using *** the binary mixture was incorporated into expanded graphite to synthesize a novel shape-stabilized *** thermophysical properties of the resultant shape-stabilized CPCM were systematically *** microscopic morphology and chemical structure of the obtained shape-stabilized CPCM were characterized and *** experiment results pointed out that acetamide could effectively lower the melting point of sodium acetate *** obtained shape-stabilized CPCM modified with additional 18%(mass fraction)acetamide and 12%(mass fraction)expanded graphite exhibited good shape stability and thermophysical characteristics:a low supercooling degree of 1.75℃and an appropriate melting temperature of 40.77℃were obtained;the latent heat of 151.64 kJ/kg and thermal conductivity of 1.411 W/(m·K)were also ***,after 50accelerated melting-freezing cycles,the obtained shape-stabilized CPCM represented good thermal reliability.

关键词： sodium acetate trihydrate melting point modification agent expanded graphite shape stability thermal conductivity enhancement

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Influence of Surface Ice Roughness on the Aerodynamic Performance of Wind Turbines

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Fluid Dynamics & Materials Processing 2024年第9期20卷 2029-2043页

作者： Xin Guan Mingyang Li Shiwei Wu Yuqi Xie Yongpeng Sun School of New energy Shenyang Engineering CollegeShenyang110136China Shenyang Key Laboratory Clean energy Fine Comprehensive Utilization and Scheduling energy Storage Shenyang110136China

The focus of this research was on the equivalent particle roughness height correction required to account for the presence of ice when determining the performances of wind *** particular,two icing processes(frost ice and clear ice)were examined by combining the FENSAP-ICE and FLUENT analysis *** ice type on the blade surfaces was predicted by using a multi-time step ***,the influence of variations in icing shape and ice surface roughness on the aerodynamic performance of blades during frost ice formation or clear ice formation was *** results indicate that differences in blade surface roughness and heat flux lead to disparities in both ice formation rate and shape between frost ice and clear *** ice has a greater impact on aerodynamics compared to frost ice,while frost ice is significantly influenced by the roughness of its icy surface.

关键词： Wind turbine icing blade surface roughness aerodynamic characteristics airfoil

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Balanced Fracturing and Cold-welding of Magnesium during Ball Milling Assisted by Carbon Coating:Experimental and Molecular Dynamic Simulation

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Journal of Wuhan University of Technology(Materials Science) 2024年第4期39卷 895-903页

作者：韩宗盈 DONG Hui DING Guoyang ZHANG Jiale SONG Xiufang college of energy Storage Technology Shandong University of Science and TechnologyQingdao 266590China college of Chemical and Biological Engineering Shandong University of Science and TechnologyQingdao 266590China

The lignite-derived carbon from self-protection pyrolysis was employed to balance the fracturing and cold-welding of magnesium during ball *** size analysis indicates that the introduction of lignite-derived carbon can effectively reduce the particle size of Mg while the introduction of graphite does no ***,the effect of lignite-derived carbon on crystallite size reduction of Mg is also better than graphite.A moderate cold-welding phenomenon was observed after ball-milling Mg with the lignite-derived carbon,suggesting less Mg is wasted on the milling vials and *** dynamic simulations reveal that the balanced fracturing and cold-welding of magnesium during ball milling is mainly attributed to the special structure of the lignite-derived carbon:graphitized short-range ordered stacking function as dry lubricant and irregular shape/sharp edge function as milling *** preliminary findings in current study are expected to offer implications for designing efficient Mg-based hydrogen storage materials.

关键词： magnesium lignite-derived carbon cold-welding ball milling molecular dynamic

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Effect of preload forces on multidimensional signal dynamic behaviours for battery early safety warning

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Journal of energy Chemistry 2024年第5期92卷 484-498页

作者： Kuijie Li Jiahua Li Xinlei Gao Yao Lu Depeng Wang Weixin Zhang Weixiong Wu Xuebing Han Yuan-cheng Cao Languang Lu Jinyu Wen Shijie Cheng Minggao Ouyang School of Electrical and Electronic Engineering Huazhong University of Science and TechnologyWuhan 430074HubeiChina State Key Laboratory of Automotive safety and energy Tsinghua UniversityBeijing 100084China energy and Electricity Research Center Jinan UniversityZhuhai 519070GuangdongChina Department of Mechanical Engineering Imperial College LondonLondon.SW7:2AZ.UK

Providing early safety warning for batteries in real-world applications is *** this study,comprehensive thermal abuse experiments are conducted to clarify the multidimensional signal evolution of battery failure under various preload *** time-sequence relationship among expansion force,voltage,and temperature during thermal abuse under five categorised stages is *** characteristic peaks are identified for the expansion force,which correspond to venting,internal short-circuiting,and thermal *** particular,an abnormal expansion force signal can be detected at temperatures as low as 42.4°C,followed by battery thermal runaway in approximately 6.5 ***,reducing the preload force can improve the effectiveness of the early-warning method via the expansion ***,reducing the preload force from 6000 to 1000 N prolongs the warning time(i.e.,227 to 398 s)before thermal runaway is *** on the results,a notable expansion force early-warning method is proposed that can successfully enable early safety warning approximately 375 s ahead of battery thermal runaway and effectively prevent failure propagation with module *** study provides a practical reference for the development of timely and accurate early-warning strategies as well as guidance for the design of safer battery systems.

关键词： Lithium-ion battery Thermal runaway Preload force Expansionforce Early warning Multidimensional signal

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