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Bimagnetic metal constructed core-shell structure of Fe@Co nanowires for multi-band microwave absorption

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Progress in Natural science:materials International 2024年第02期34卷 354-361页

作者： Ping-an Yang Rui Cai Haibo Ruan Nanqing Zhang Xin Huang Rui Li Yuxin Zhang Yi Lu Zhihao Zhou School of Automation Chongqing University of Posts and Telecommunications Chongqing Key Laboratory of materials Surface & Interface science Chongqing University of Arts and Sciences college of Engineering and Technology Zunyi Normal College college of material science and Engineering Chongqing University

Controlled fabrication of materials by surface modification techniques has been a hot research topic. In this paper,one-dimensional(1D) core-shell structure Fe@Co nanowires(NWs) were successfully prepared by anchoring 0-dimensional(0D) Co nanoparticles on 1D Fe NWs based on the in situ reduction method. The electromagnetic parameters of the specimens at a filler mass fraction of 25 wt% were tested and the microwave loss mechanism was deeply analyzed. Binary magnetic metals in a core-shell structure have excellent multi-band microwave absorption capability(S-band, X-band and Ku-band). This is due to the heterogeneous interface and magnetic coupling effects tuning the dielectric and magnetic loss. This study offers a workable plan for creating effective multi-band magnetic metal-based microwave absorbers.

关键词： Microwave absorption One-dimensional nanowires Core-shell structure Magnetic coupling Interface

Raman signal enhancement for gas detection using a dual near-concentric cavities group

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Chinese Optics Letters 2024年第5期22卷 47-52页

作者：任一凡杨德旺孙颖欣许家旋刘硕芳陈月娥 Key Laboratory for Microstructural material Physics of Hebei Province School of ScienceYanshan UniversityQinhuangdao 066004China college of Ocean science and Engineering Shandong University of Science and TechnologyQingdao 266590China

Effective methods are urgently required to optimize Raman spectroscopy technology to ameliorate its low detection ***,we superposed two near-concentric cavities to develop a dual near-concentric cavities group(DNCCG)to assess its effect on gas Raman signal intensity,signal-to-noise ratio(SNR),and limit of detection(LOD).The results showed that DNCCG generally had higher CO_(2) Raman signal intensity than the sum of two near-concentric ***,the noise intensity of DNCCG was not enhanced by the superposition of near-concentric ***,DNCCG increased the *** LOD for CO_(2) was 24.6 parts per *** could be an effective method to improve the detection capability of trace gases and broaden the dynamic detection range,which might aid the future development of innovative technology for multicomponent gas detection.

关键词： Raman spectroscopy gas detection sensitivity dual near-concentric cavities group

Investigation into the Methodology and Implementation of Life Cycle Engineering under China’s Carbon Reduction Target in the Process Industry

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Engineering 2024年第9期40卷 87-99页

作者： Mingyang Li Feng Gao Zuoren Nie Boxue Sun Yu Liu Xianzheng Gong National Engineering Laboratory for Industrial Big-data Application Technology College of Material Science and EngineeringBeijing University of TechnologyBeijing 100124China

The industrial sector is the primary source of carbon emissions in *** pursuit of meeting its carbon reduction targets,China aims to promote resource consumption sustainability,reduce energy consumption,and achieve carbon neutrality within its processing *** effective strategy to promote energy savings and carbon reduction throughout the life cycle of materials is by applying life cycle engineering *** strategy aims to attain an optimal solution for material performance,resource consumption,and environmental *** this study,five types of technologies were considered:raw material replacement,process reengineering,fuel replacement,energy recycling and reutilization,and material recycling and *** meaning,methodology,and development status of life cycle engineering technology abroad and domestically are discussed in detail.A multidimensional analysis of ecological design was conducted from the perspectives of resource and energy consumption,carbon emissions,product performance,and recycling of secondary resources in a manufacturing *** coupled with an integrated method to analyze carbon emissions in the entire life cycle of a material process industry was applied to the nonferrous industry,as an *** results provide effective ideas and solutions for achieving low or zero carbon emission production in the Chinese industry as recycled aluminum and primary aluminum based on advanced technologies had reduced resource consumption and emissions as compared to primary aluminum production.

关键词： Carbon neutrality Life cycle engineering Process Industry Carbon reduction technology Eco-design

Ultrafast Response and Threshold Adjustable Intelligent Thermoelectric Systems for Next‑Generation Self‑Powered Remote IoT Fire Warning

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Nano-Micro Letters 2024年第11期16卷 413-428页

作者： Zhaofu Ding Gang Li Yejun Wang Chunyu Du Zhenqiang Ye Lirong Liang Long‑Cheng Tang Guangming Chen college of materials science and Engineering&college of Civil and Transportation Engineering Shenzhen UniversityShenzhen 518055People’s Republic of China college of material Chemistry and Chemical EngineeringKey Laboratory of Organosilicon Chemistry and Material Technology of MoEHangzhou Normal UniversityHangzhou 311121People’s Republic of China

Fire warning is vital to human life,economy and ***,the development of effective warning systems faces great challenges of fast response,adjustable threshold and remote ***,we propose an intelligent self-powered remote IoT fire warning system,by employing single-walled carbon nanotube/titanium carbide thermoelectric composite *** flexible films,prepared by a convenient solution mixing,display p-type characteristic with excellent high-temperature stability,flame retardancy and TE(power factor of 239.7±15.8μW m^(-1) K^(-2))*** comprehensive morphology and structural analyses shed light on the underlying *** the assembled TE devices(TEDs)exhibit fast fire warning with adjustable warning threshold voltages(1–10 mV).Excitingly,an ultrafast fire warning response time of~0.1 s at 1 mV threshold voltage is achieved,rivaling many state-of-the-art ***,TE fire warning systems reveal outstanding stability after 50 repeated cycles and desired durability even undergoing 180 days of air ***,a TED-based wireless intelligent fire warning system has been developed by coupling an amplifier,analogto-digital converter and Bluetooth *** combining TE characteristics,high-temperature stability and flame retardancy with wireless IoT signal transmission,TE-based hybrid system developed here is promising for next-generation self-powered remote IoT fire warning applications.

关键词： Thermoelectric Self-powered IoT fire warning Ultrafast response Threshold adjustable

A high-performance electrocatalyst for oxygen reduction derived from copolymer-anchored polyoxometalates

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Nano Research 2024年第6期17卷 5197-5205页

作者： Yue Du Wenxue Chen Zhiyi Zhong Zhixian Shi Yulin Zhang Xuanning Chen Yisi Liu Dongbin Xiong Lina Zhou Zhenhui Liu Mingbo Zheng Hubei Key Laboratory of Photoelectric materials and Devices&college of material science and Engineering Hubei Normal UniversityHuangshi 435002China college of materials science and Technology Nanjing University of Aeronautics and AstronauticsNanjing 210016China

The development and synthesis of cathode electrocatalysts with high activity and durable stability for metal-air batteries is an important challenge in the area of ***,we introduce a novel in-situ nitriding and phosphating strategy for producing W_(3)N_(4)and WP from phosphotungstic acid(HPW)-polyaniline-phytic acid-Fe3+organic-inorganic hybrid *** final material has a three-dimensional porous framework with W_(3)N_(4)-WP heterostructures embedded in the carbon matrix(W_(3)N_(4)-WP@NPC).As-made materials exhibit exceptional electrocatalytic performance for the oxygen reduction reaction(ORR),with a diffusion-limiting current density of 6.9 mA·cm^(−2)and a half-wave potential of 0.82 *** a Zn-air primary cathode,the W_(3)N_(4)-WP@NPC assembled battery can provide a relatively high peak power density(194.2 mW·cm^(−2)).As a Zn-air secondary air-cathode,it has great cycling stability over 500 *** work provides a simple and efficient method for rationally designing high-performance air cathodes from copolymer-anchored polyoxometalates.

关键词： W_(3)N_(4)-WP heterojunctions copolymer-anchored polyoxometalates oxygen reduction reaction Zn-air battery

Preparation,Characterization and Photothermal Study of PVA/Ti_(2)O_(3) Composite Films

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Journal of Wuhan University of Technology(materials science) 2024年第3期39卷 658-663页

作者：尚蒙娅 HE Yanyan YU Jianhui YAN Jiahui XIE Haodi 李金玲 School of material science&Engineering Henan University of TechnologyZhengzhou 450001China college of Advanced Interdis-ciplinary science and Technology Henan University of TechnologyZhengzhou 450001China

In this work,flexible photothermal PVA/Ti_(2)O_(3) composite films with different amount(0 wt%,5 wt%,10 wt%,15 wt%)of Ti_(2)O_(3) particles modified by steric acid were prepared by a simple solution casting *** microstructures,XRD patterns,FTIR spectra,UV-Vis-NIR spectra thermo-conductivity,thermo-stability and photothermal effects of these composite films were all *** results indicated that Ti_(2)O_(3) particles were well dispersed throughout the polyvinyl alcohol(PVA)matrix in the PVA/Ti_(2)O_(3) composite *** Ti_(2)O_(3) particles could also effectively improve the photothermal properties of the composite films which exhibited high light absorption and generated a high temperature(about 57.4℃for film with 15 wt%Ti_(2)O_(3) amount)on the surface when it was irradiated by a simulated sunlight source(1 kW/m^(2)).

关键词： Ti_(2)O_(3)particles solution casting method composite film photothermal conversion

Kinetic-boosted CO_(2) electroreduction to formate via synergistic electric-thermal field on hierarchical bismuth with amorphous layer

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Journal of Energy Chemistry 2024年第3期90卷 233-243,I0007页

作者： Bing Yang Junyi Zeng Zhenlin Zhang Lin Meng Donglin Shi Liang Chen Youju Huang college of material Chemistry and Chemical EngineeringKey Laboratory of Organosilicon Chemistry and Material TechnologyMinistry of EducationHangzhou Normal UniversityHangzhou 311121ZhejiangChina State Key Laboratory of Metastable materials science and Technology College of Materials Science and EngineeringYanshan UniversityQinhuangdao 066004HebeiChina

Electrocatalytic converting CO_(2) into chemical products has emerged as a promising approach to achieving carbon ***,we report a bismuth-based catalyst with high curvature terminal and amorphous layer which fabricated via two-step electrodeposition achieves stable formate output in a wide voltage window of 600 *** Faraday efficiency(FE) of formate reached up to 99.4% at-0.8 V *** and it remained constant for more than 92 h at-15 mA cm^(-2).More intriguingly,FE formate of95.4% can be realized at a current density of industrial grade(-667.7 mA cm^(-2)) in flow *** special structure promoted CO_(2) adsorption and reduced its activation energy and enhanced the electric-thermal field and K^(+) enrichment which accelerated the reaction *** situ spectroscopy and theoretical calculation further confirmed that the introduction of amorphous structure is beneficial to adsorpting CO_(2)and stabling*OCHO *** work provides special insights to fabricate efficient electrocatalysts by means of structural and crystal engineering and makes efforts to realize the industrialization of bismuth-based catalysts.

关键词： CO_(2) electroreduction Hierarchical bismuth Amorphous layer Electric-thermal field Kinetic-boosting

Degradation and biocompatibility of one-step electrodeposited magnesium thioctic acid/magnesium hydroxide hybrid coatings on ZE21B alloys for cardiovascular stents

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Journal of Magnesium and Alloys 2024年第1期12卷 120-138页

作者： Zhao-Qi Zhang Bing-Zhi Li Pei-Duo Tong Shao-Kang Guan Li Wang Zheng-Hui Qiu Cun-Guo Lin Rong-Chang Zeng School of material science and Engineering&Henan Key Laboratory of Advanced Magnesium Alloy&Key Laboratory of materials Processing and Mold Technology(Ministry of Education) Zhengzhou University100 Science RoadZhengzhou 450001China State Key Laboratory for Marine Corrosion and Protection Luoyang Ship Material Research InstituteQingdao 266101China Corrosion Laboratory for Light Metals College of Material Science and EngineeringShandong University of Science and TechnologyQingdao 266590China

Constructing a functional hybrid coating appears to be a promising strategy for addressing the poor corrosion resistance and insufficient endothelialization of Mg-based ***,the steps for preparing composite coatings are usually complicated and ***,a novel composite coating,composed of bioactive magnesium thioctic acid(MTA)layer formed by deposition and corrosion-resistant magnesium hydroxide(Mg(OH)_(2))layer grown in situ,is simply fabricated on ZE21B alloys via one-step *** electron microscopy(SEM)shows that the electrodeposited coating has a compact and uniform *** the high adhesion of the MTA/Mg(OH)_(2)hybrid coating is also confirmed by the micro-scratch *** test,scanning kelvin probe(SKP),and hydrogen evolution measurement indicate that the hybrid coating effectively reduces the degradation rate of Mg *** experiment and cell culture trial detect that the composite coating is of fine ***,the preparation mechanism of MTA/Mg(OH)_(2)hybrid coatings is discussed and *** coating shows a great potential application for cardiovascular stents.

关键词： Magnesium alloy Corrosion resistance Hybrid coating Endothelialization Biocompatibility

Biochar alleviates apple replant disease by reducing the growth of Fusarium oxysporum and regulating microbial communities

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Horticultural Plant Journal 2024年第3期10卷 657-671页

作者： Yinghao Liu Can Wang Ran Chen Weitao Jiang Yun Li Chengmiao Yin Yanfang Wang Zhiquan Mao college of Chemistry and material science Shandong Agricultural UniversityTaianShandong 271018China State Key Laboratory of Crop Biology/college of Horticultural science and Engineering Shandong Agricultural UniversityTaianShandong 271018China

Apple replant disease(ARD)negatively affects plant growth and reduces yields in replanted *** this study,biochar was applied to apple replant soil with Fusarium *** aim was to investigate whether biochar could promote plant growth and alleviate apple replant disease by reducing the growth of harmful soil microorganisms,changing soil microbial community structure and improving the soil *** experiment included five treatments:apple replant soil(CK),methyl bromide fumigation apple replant soil(FM),replant soil with biochar addition(2%),replant soil with *** spore solution(8×10^(7)spores·mL^(-1)),and replant soil with biochar and *** spore solution *** biomass,the activity of antioxidant enzymes in the leaves and roots,and soil environmental variables were *** community composition and community structure were analyzed using 16SrDNA and ITS2 gene *** significantly reduced the abundance of *** and increased soil microbial diversity and *** also increased the soil enzyme activities(urease,invertase,neutral phosphatase,and catalase),the biomass(plant height,fresh weight,dry weight)and the activity of antioxidant enzymes(superoxide dismutase,peroxidase,and catalase).The root indexes of apple seedlings was also increased in replant soil by *** sum,biochar promoted the growth of plants,improved the replant soil environment,and alleviated apple replant disease.

关键词： Biochar Fusarium oxysporum Apple replant disease Soil environment