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Cotransport of nanoplastics with nZnO in saturated porous media:From brackish water to seawater

Journal of environmental Sciences 2025年第2期148卷 541-552页

作者： Yuanzhang Hou Yange Wang Yidi Zhang Zhibo Lu Zhenbo Zhang Zhiqiang Dong Yuping Qiu Department of environmental Science College of Environmental Science and EngineeringTongji UniversityState Key Laboratory of Pollution Control and Resources ReuseShanghai Institute of Pollution Control and Ecological SecurityShanghai 200092China School of Medicine Tongji UniversityShanghai 200065China Municipal environmental Protection engineering Co. Ltd of CERC Shanghai GroupShanghai 201906China China Railway engineering Group Co. Beijing 100039China

The ocean serves as a repository for various types of artificial ***(NPs)and nano zinc oxide(nZnO),which are frequently employed in personal care products and food packaging materials,are likely simultaneously released and eventually into the ocean with surface ***,their mutual influence and shared destiny in marine environment cannot be *** study examined how nanomaterials interacted and transported through sea sand in various salinity *** showed that NPs remained dispersed in brine,while nZnO formed *** seawater of 35 practical salinity units(PSU),nZnO formed heteroaggregates with NPs,inhibiting NPs mobility and decreasing the recovered mass percentage(Meff)from 24.52%to 12.65%.In 3.5 PSU brackish water,nZnO did not significantly aggregate with NPs,and thus barely affected their ***,NPs greatly enhanced nZnO transport with Meff increasing from 14.20%to 25.08%,attributed to the carrier effect of higher mobility *** from brackishwater to seawater was simulated in salinity change experiments and revealed a critical salinity threshold of 10.4 PSU,below which the mobility of NPs was not affected by coexisting nZnO and above which nZnO strongly inhibited NP *** study highlights the importance of considering the mutual influence and shared destiny of artificial nanoparticles in the marine environment and how their interaction and cotransport are dependent on changes in seawater salinity.

关键词： Homoaggregate Heteroaggregate Transport Sea sand Salinity threshold

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The photo-based treatment technology simultaneously removes resistant bacteria and resistant genes from wastewater

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Journal of environmental Sciences 2025年第2期148卷 243-262页

作者： Zicong Guo Xiang Tang Wenjun Wang Zhangxiong Luo Yuxi Zeng Nan Zhou Zhigang Yu Dongbo Wang Biao Song Chengyun Zhou Weiping Xiong college of environmental Science and engineering and Key Laboratory of environmental Biology and Pollution Control(Ministry of Education) Hunan UniversityChangsha 410082China Fujian Provincial Key Laboratory of Soil environmental Health and Regulation College of Resources and EnvironmentFujian Agriculture and Forestry UniversityFuzhou 350002China School of Resources and Environment Hunan University of Technology and BusinessChangsha 410205China Australian Centre for Water and environmental Biotechnology The University of QueenslandBrisbaneQLD 4072Australia

Because of the recent widespread usage of antibiotics,the acquisition and dissemination of antibiotic-resistance genes(ARGs)were prevalent in the majority of ***,the biological wastewater treatment processes used in wastewater treatment plants have a limited efficiencies of antibiotics resistant bacteria(ARB)disinfection and ARGs degradation and even promote the proliferation of ***,ARB and ARGs in effluent pose potential risks if they are not further *** oxidation is considered a promising disinfection technology,where the photocatalytic process generates many free radicals that enhance the interaction between light and deoxyribonucleic acid(DNA)for ARB elimination and subsequent degradation of *** reviewaims to illustrate the progress of photocatalytic oxidation technology for removing antibiotics resistant(AR)from wastewater in recent *** discuss the sources and transfer of ARGs in *** overall removal efficiencies of ultraviolet radiation(UV)/chlorination,UV/ozone,UV/H_(2)O_(2),and UV/sulfate-radical based system for ARB and ARGs,as well as the experimental parameters and removal mechanisms,are systematically *** contribution of photocatalytic materials based on TiO_(2) and g-C_(3)N_(4) to the inactivation of ARB and degradation of ARGs is highlighted,producingmany free radicals to attack ARB and ARGs while effectively limiting the horizontal gene transfer(HGT)in ***,based on the reviewed studies,future research directions are proposed to realize specific photocatalytic oxidation technology applications and overcome current challenges.

关键词： Antibiotics resistant genes Antibiotics resistant bacteria Photocatalytic oxidation

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Efficient activation of peroxymonosulfate for catalytic degradation of organic pollutants by simultaneously using low-level cobalt ions and calcium carbonate micro-particles

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Journal of environmental Sciences 2025年第5期151卷 113-124页

作者： Yu Zhou Xiaobo Wang Nan Wang Shuangshuang Huang Lihua Zhu college of Chemistry and Chemical engineering Huazhong University of Science and TechnologyWuhan 430074China college of Chemistry and Chemical engineering Hubei Polytechnic UniversityHuangshi 435003China college of Chemistry and environmental engineering Wuhan Polytechnic UniversityWuhan 430023China School of Physics and Technology Center for Electron MicroscopyWuhan UniversityWuhan 430072China

An efficient catalytic system was developed to remove various organic pollutants by simultaneously using low-level cobalt ions,calcium carbonate micro-particles and peroxymonosulfate(PMS).A simple base-induced precipitation was used to successfully loaded Co-centered reactive sites onto the surface of CaCO_(3)*** optimal conditions at 25°C,10 mg/L methylene blue(MB)could be completely degraded within 10 min with 480μg/L Co^(2+),0.4 g/L CaCO_(3)microparticles(or 0.4 g/L Co@CaCO_(3))and 0.1 g/L *** MB degradation followed the pseudo first order kinetics with a rate constant of 0.583 min^(−1),being 8.3,11.5 and 53.0 times that by using Co-OH(0.07 min^(−1)),Co^(2+)(0.044 min^(−1))and CaCO_(3)(0.011 min^(−1))as the catalyst,*** was confirmed that there was a synergistic effect in the catalytic activity between Co species and the CaCO_(3)particles but the major contributor was the highly dispersed Co *** Co^(2+)-containing simulated electroplating wastewater was used as the Co^(2+)source,not only the added MB was also completely degraded within 5 min in this catalytic system,but also the coexisting heavy metal ions were substantially *** presently developed method was applied to simultaneously treat organic wastewater and heavy metals *** present method was also successfully used to efficiently degrade other organic pollutants including bisphenol A,sulfamethoxazole,rhodamine B,tetrabromobisphenol A,ofloxacin and benzoic acid.A catalytic mechanism was proposed for the PMS activation by Co@CaCO_(3).The surface of CaCO_(3)particles favors the adsorption of Co^(2+).More importantly,the surface of CaCO_(3)particles provides plentiful surface-OH and-CO_(3)^(2+),and these surface groups complex with Co^(2+)to producemore catalytically active species such as surface[CoOH]^(−),resulting in rapid Co^(2+)/Co^(3+)cycling and electron *** interactions cause the observed synergistic effect between Co species and Ca

关键词： CaCO3 Low-level cobalt Peroxymonosulfate Oxidative degradation

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Bioenergy recovery and carbon emissions benefits of short-term bio-thermophilic pretreatment on low organic sewage sludge anaerobic digestion:A pilot-scale study

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Journal of environmental Sciences 2025年第2期148卷 321-335页

作者： Hui Wang Xiang Fu Haozhe Huang Danni Shen Dongdong Fan Liming Zhu Xiaohu Dai Bin Dong college of environmental Science and engineering Tongji UniversityShanghai 200092China Yangtze Eco-Environment engineering Research Center China Three Gorges CorporationBeijing 100038China Yangtze River Eco-environmental engineering Research Center Shanghai InvestigationDesign and Research Institute Co.LTDShanghai 200092China China Construction Third engineering Bureau First engineering Co. Ltd.Wuhan 430000China

Sewage sludge in cities of Yangzi River Belt,China,generally exhibits a lower organic content and higher silt contentdue to leakage of drainage system,which caused low bioenergy recovery and carbon emission benefits in conventional anaerobic digestion(CAD).Therefore,this paper is on a pilot scale,a bio-thermophilic pretreatment anaerobic digestion(BTPAD)for low organic sludge(volatile solids(VS)of 4%)was operated with a long-term continuous flow of 200 *** VS degradation rate and CH_(4) yield of BTPAD increased by 19.93%and 53.33%,respectively,compared to those of *** analysis of organic compositions in sludge revealed that BTPAD mainly improved the hydrolysis of proteins in *** analysis of microbial community proportions by high-throughput sequencing revealed that the short-term bio-thermophilic pretreatment was enriched in Clostridiales,Coprothermobacter and Gelria,was capable of hydrolyzing acidified proteins,and provided more volatile fatty acid(VFA)for the subsequent *** combined with fluorescence quantitative polymerase chain reaction(PCR)analysis showed that the number of bacteria with high methanogenic capacity in BTPAD was much higher than that in CAD during the medium temperature digestion stage,indicating that short-term bio-thermophilic pretreatment could provide better methanogenic conditions for ***,the greenhouse gas emission footprint analysis showed that short-term bio-thermophilic pretreatment could reduce the carbon emission of sludge anaerobic digestion system by 19.18%.

关键词： Sludge Anaerobic digestion Bio-thermophilic pretreatment Pilot scale Molecular microbiology Carbon emissions

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Enhancing microbial superoxide generation and conversion to hydroxyl radicals for enhanced bioremediation using iron-binding ligands

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Journal of environmental Sciences 2025年第1期147卷 597-606页

作者： Yuhan Wang Xue Ning Jinsong Liang Aijie Wang Jiuhui Qu School of Civil and environmental engineering Harbin Institute of TechnologyShenzhen 518055China SFI MaREI Centre for Energy Climate and MarineEnvironmental Research InstituteUniversity College CorkCorkIreland Center for Water and Ecology Tsinghua UniversityBeijing 100084China

Harnessing bacteria for superoxide production in bioremediation holds immense promise,yet its practical application is hindered by slow production rates and the relatively weak redox potential of *** study delves into a cost-effective approach to amplify superoxide production using an Arthrobacter strain,a prevalent soil bacterial *** research reveals that introducing a carbon source along with specific iron-binding ligands,including deferoxamine(DFO),diethylenetriamine pentaacetate(DTPA),citrate,and oxalate,robustly augments microbial superoxide ***,our findings suggest that these iron-binding ligands play a pivotal role in converting superoxide into hydroxyl radicals by modulating the electron transfer rate between Fe(Ⅲ)/Fe(Ⅱ)and ***,among the tested ligands,only DTPA emerges as a potent promoter of this conversion process when complexed with Fe(Ⅲ).We identify an optimal Fe(Ⅲ)to DTPA ratio of approximately 1:1 for enhancing hydroxyl radical production within the Arthrobacter *** research underscores the efficacy of simultaneously introducing carbon sources and DTPA in facilitating superoxide production and its subsequent conversion to hydroxyl radicals,significantly elevating bioremediation ***,our study reveals that DTPA augments superoxide production in cultures of diverse soils,with various soil microorganisms beyond Arthrobacter identified as contributors to superoxide *** emphasizes the universal applicability of DTPA across multiple bacterial *** conclusion,our study introduces a promising methodology for enhancing microbial superoxide production and its conversion into hydroxyl *** findings hold substantial implications for the deployment of microbial reactive oxygen species in bioremediation,offering innovative solutions for addressing environmental contamination challenges.

关键词： Superoxide Hydroxyl radical Iron-binding ligand Bioremediation DTPA

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In situ formed fluorescent gold nanoclusters inhibit hair follicle regeneration in oxidative stress microenvironment via suppressing NFκB signal pathway

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Chinese Chemical Letters 2025年第2期36卷 284-288页

作者： Xiangdong Lai Tengfei Liu Zengchao Guo Yihan Wang Jiang Xiao Qingxiu Xia Xiaohui Liu Hui Jiang Xuemei Wang State Key Laboratory of Digital Medical engineering School of Biological Science and Medical Engineering Southeast University

Skins expose to kinds of risk factors for damage, such as the hormone drugs, skin care products and ultraviolet radiation, which is accompanied by the production of excessive reactive oxygen species(ROS)and eventually leads to hypertrichosis. This skin disease is not aesthetically pleasing and even causes psychological and spiritual problems such as inferiority, anxiety and irritability. Current therapies are limited and often unsatisfactory, such as pharmacological and physical therapies, which have adverse effects and cause the irreversible destruction of hair follicles. Gold nanoclusters have good biocompatibility and their biosynthesis in vivo is responsive to oxidative stress microenvironment(OSM), which could be a safe and effective drug for ROS-induced skin injury. In our study, we demonstrated that zero valence fluorescent gold nanoclusters(FGNCs) were in situ biosynthesized in the plucking-induced damaged skin but not in the normal skin after the administration of gold precursors(+3), while FGNCs inhibited hair follicle regeneration by negatively regulating nuclear transcription factor kappa B(NFκB)-mediated inflammatory response signaling pathway(NFκB/tumor necrosis factor-α(TNF-α) axis). This OSM-responsive in situ biosynthesis method is facile and safe and holds great promise for curing hypertrichosis associated with skin dermatitis and injury.

关键词： Fluorescent gold nanoclusters Hair follicle regeneration Oxidative stress microenvironment Reactive oxygen species Skin injury

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Tremendously enhanced catalytic performance of Fe(Ⅲ)/peroxymonosulfate process by trace Cu(Ⅱ):A high-valent metals domination in organics removal

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Journal of environmental Sciences 2025年第1期147卷 487-497页

作者： Jieli Ou Yiqing Liu Linyue Zhang Zhenran Wang Yuqi Tang Yongsheng Fu Dandan Zhao Faculty of Geosciences and environmental engineering Southwest Jiaotong UniversityChengdu 611756China

Dissolved copper and iron ions are regarded as friendly and economic catalysts for peroxymonosulfate(PMS)activation,however,neither Cu(Ⅱ)nor Fe(Ⅲ)shows efficient catalytic performance because of the slow rates of Cu(Ⅱ)/Cu(Ⅰ)and Fe(Ⅲ)/Fe(Ⅱ)***,we observed a significant enhancement on the degradation of organic contaminants when Cu(Ⅱ)and Fe(Ⅲ)were coupled to activate PMS in borate(BA)*** degradation efficiency of Rhodamine B(RhB,20μmol/L)reached up to 96.3%within 10 min,which was higher than the sum of individual Cu(Ⅱ)-and Fe(Ⅲ)-activated PMS *** radical,hydroxyl radical and high-valent metal ions(i.e.,Cu(Ⅲ)and Fe(IV))were identified as the working reactive species for RhB removal in Cu(Ⅱ)/Fe(Ⅲ)/PMS/BA system,while the last played a predominated *** presence of BA dramatically facilitated the reduction of Cu(Ⅱ)to Cu(Ⅰ)via chelating with Cu(Ⅱ)followed by Fe(Ⅲ)reduction by Cu(Ⅰ),resulting in enhanced PMS activation by Cu(Ⅰ)and Fe(Ⅱ)as well as accelerated generation of reactive ***,the strong buffering capacity of BA to stabilize the solution pH was satisfying for the pollutants degradation since a slightly alkaline environment favored the PMS activation by coupling Cu(Ⅱ)and Fe(Ⅲ).In a word,this work provides a brand-new insight into the outstanding PMS activation by homogeneous bimetals and an expanded application of iron-based advanced oxidation processes in alkaline conditions.

关键词： Peroxymonosulfate Bimetallic catalyst Borate High-valent metals Complexation

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Effect of chlorination and ultraviolet on the adsorption of pefloxacin on polystyrene and polyvinyl chloride

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Journal of environmental Sciences 2025年第3期149卷 21-34页

作者： Yanan Li Yaning Wu Kai Guo Weiqin Wu Meijing Yao School of environmental Science and engineering Taiyuan University of TechnologyShanxi 030600China

During thewater treatment process,chlorination and ultraviolet(UV)sterilization can modify microplastics(MPs)and alter their physicochemical properties,causing various changes between MPs and other *** this study,the impact of chlorination and UV modification on the physicochemical properties of polystyrene(PS)and polyvinyl chloride(PVC)were investigated,and the adsorption behavior of pefloxacin(PEF)before and after modificationwas *** effect of pH,ionic strength,dissolved organicmatter,heavymetal ions and other water environmental conditions on adsorption behavior was *** results showed that PS had a higher adsorption capacity of PEF than PVC,and the modification increased the presence of O-containing functional groups in the MPs,thereby enhancing the adsorption capacity of both *** had a more significant impact on the physicochemical properties of MPs compared to UV irradiation within the same time period,leading to better adsorption performance of *** optimal pH for adsorption was found to be 6,and NaCl,sodium alginate and Cu2+would inhibit adsorption to varying degrees,among which the inhibition caused by pH was the *** and UV modification would weaken the inhibitory effect of environmental factors on the adsorption of PEF by *** main mechanisms of adsorption involved electrostatic interaction and hydrogen *** study clarified the effects of modification on the physicochemical properties of MPs,providing reference for subsequent biotoxicity analysis and environmental protection studies.

关键词： Microplastics Chlorination Ultraviolet Pefloxacin Adsorption mechanism

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Efficient remediation of different concentrations of Cr-contaminated soils by nano zero-valent iron modified with carboxymethyl cellulose and biochar

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Journal of environmental Sciences 2025年第1期147卷 474-486页

作者： Lihong Xie Qiyan Ma Qingjun Chen Yiyang Liu Pengfei Guo Jinlan Zhang Guilan Duan Aijun Lin Tingting Zhang Shangyi Li Department of environmental Science and engineering College of Chemical EngineeringBeijing University of Chemical TechnologyBeijing 100029China China National Petroleum and Chemical Planning Institute Beijing 100013China State Key Laboratory of Urban and Regional Ecology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China

Nano zero-valent iron(nZVI)is widely used in soil remediation due to its high ***,the easy agglomeration,poor antioxidant ability and passivation layer of Fe-Cr coprecipitates of nZVI have limited its application scale in Cr-contaminated soil remediation,especially in high concentration of Cr-contaminated ***,we found that the carboxymethyl cellulose on nZVI particles could increase the zeta potential value of soil and change the phase of *** with the presence of biochar,97.0%and 96.6%Cr immobilization efficiency through CMC-nZVI/BC were respectively achieved in high and low concentrations of Cr-contaminated soils after 90-days *** addition,the immobilization efficiency of Cr(VI)only decreased by 5.1%through CMC-nZVI/BC treatment after 10 weeks aging in air,attributing to the strong antioxidation *** for the surrounding Crcontaminated groundwater,the Cr(VI)removal capacity of CMC-nZVI/BC was evaluated under different reaction conditions through column experiments and COMSOL ***-nZVI/BC could efficiently remove 85%of Cr(VI)in about 400 hr when the initial Cr(VI)concentration was 40 mg/L and the flow rate was 0.5 mL/*** study demonstrates that uniformly dispersed CMC-nZVI/BC has an excellent remediation effect on different concentrations of Cr-contaminated soils.

关键词： Carboxymethyl cellulose Nanoscale zero-valent iron Biochar Cr-contaminated soils

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Civil aviation emissions in China in 2019:Characteristics and abatement potential

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Journal of environmental Sciences 2025年第5期151卷 225-237页

作者： Haowen An Yu Wang Yaxin Wang Jun Liu Xiaolong Tang Honghong Yi Department of environmental engineering School of Energy and Environmental EngineeringUniversity of Science and Technology BeijingBeijing 100083China Key Laboratory of Beijing Municipal Industry Pollutant Resources Processing Beijing 100083China

Civil aviation is one of the industries facing the greatest challenge in reaching carbon neutrality by the middle of this century,and this sector also contributes to adverse impacts on the regional air quality and human *** exhibits the second highest air passenger turnover *** understanding of civil aviation emissionsmust be urgently enhanced,and themitigation potential should be *** this study,on the basis of real domestic flight information for 2019,we built a greenhouse gas and air pollution emission inventory for the civil aviation sector in China with the fuel flowmethod based on the cruise and other *** thoroughly analyzed emissions by region,aircraft and engine types,and aircraft age,based on which we designed four measures to evaluate the abatement *** found that the hydrocarbon(HC),CO,NO_(x),SO_(2),particulate matter(PM)and CO_(2)emissions in 2019 reached 79.9 kt(95%CI[51.6–114.5]),176.3 kt(95%CI[114.5–248.2]),304.2 kt(95%CI[203.4–420.7]),23.2 kt(95%CI[14.2–33.7]),1.0 kt(95%CI[0.61–1.44])and 87.0 Mt(95%CI[57.4–119.6]),*** cruise phase was the major emission phase,accounting for 67%-87%of the total pollutant *** four measures were jointly implemented,the HC,CO,NO_(x),SO_(2),PM and CO_(2)emissions could be reduced by 61%,54%,55%,45%,32%and 38%,*** lower-emission aircraft and switching travel modes could substantially reduce civil aviation emissions in China.

关键词： Emission inventory Fuel flow method Cruise emission Age structure Reduction measures

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